High Photon Count Rates Research Articles

A digital approach for real time high-rate high-resolution radiation measurements

Modern spectrometers are currently developed by using digital pulse processing (DPP) systems, showing several advantages over traditional analog electronics. The aim of this work is to present digital strategies, in a time domain, for the development of real time high-rate high-resolution spectrometers. We propose a digital method, based on the single delay line (SDL) shaping technique, able to perform multi-parameter analysis with high performance even at high photon counting rates. A robust pulse shape and height analysis (PSHA), applied on single isolated time windows of the detector output waveforms, is presented.The potentialities of the proposed strategy are highlighted through both theoretical and experimental approaches. To strengthen our approach, the implementation of the method on a real-time system together with some experimental results are presented. X-ray spectra measurements with a semiconductor detector are performed both at low and high photon counting rates (up to 1.1Mcps).

High-flux ptychographic imaging using the new 55 µm-pixel detector `Lambda' based on the Medipix3 readout chip

Suitable detection systems that are capable of recording high photon count rates with single-photon detection are instrumental for coherent X-ray imaging. The new single-photon-counting pixel detector `Lambda' has been tested in a ptychographic imaging experiment on solar-cell nanowires using Kirkpatrick–Baez-focused 13.8 keV X-rays. Taking advantage of the high count rate of the Lambda and dynamic range expansion by the semi-transparent central stop, a high-dynamic-range diffraction signal covering more than seven orders of magnitude has been recorded, which corresponds to a photon flux density of about 105 photons nm−2 s−1or a flux of ∼1010 photons s−1on the sample. By comparison with data taken without the semi-transparent central stop, an increase in resolution by a factor of 3–4 is determined: from about 125 nm to about 38 nm for the nanowire and from about 83 nm to about 21 nm for the illuminating wavefield.

Simulating quantum state engineering in spontaneous parametric down-conversion using classical light.

We present a simple method of simulating the effect of the pumping process in spontaneous parametric down-conversion (SPDC) by modulating a classical laser beam with two spatial light modulators through a back projection setup. We simulate a wide range of pump beams for quantum state engineering and confirm that the results are in agreement with theory. Our approach offers high photon count rates, is quick to yield results and can easily be converted back to a SPDC setup. It is likely to be a useful tool before starting more complicated SPDC experiments with custom pump profiles.

Experimental results from Al/p-CdTe/Pt X-ray detectors

Recently, Al/CdTe/Pt detectors have been proposed for the development of high resolution X-ray spectrometers. Due to the low leakage currents, these detectors allow high electric fields and the pixellization of anodes with the possibility to realize single charge carrier sensing detectors. In this work, we report on the results of electrical and spectroscopic investigations on CdTe diode detectors with Al/CdTe/Pt electrode configuration (4.1×4.1×0.75 and 4.1×4.1×2mm3). The detectors are characterized by very low leakage currents in the reverse bias operation: 0.3nA at 25°C and 2.4pA at −25°C under a bias voltage of −1000V. The spectroscopic performance of the detectors at both low and high photon counting rates were also investigated with a focus on the minimization of time instability, generally termed as polarization, looking for the optimum bias voltage and temperature. Good time stability, during a long-term operation of 10h, was observed for both detectors at −25°C and by using an electric field of 5000V/cm. The 2mm thick detector exhibited good energy resolution of 6.1%, 2.5% and 2.0% (FWHM) at 22.1keV, 59.5 and 122.1keV, respectively. Performance enhancements were obtained by using digital pulse processing techniques, especially at high photon counting rates (300kcps). The 2mm thick detector, after a digital pulse shape correction (PSC), is characterized by similar performance to the thin detector ones, opening up to the use of thick CdTe detectors without excessive performance degradations. This work was carried out in the framework of the development of portable X-ray spectrometers for both laboratory research and medical applications.

InGaAs/InP Single-Photon Avalanche Diode With Reduced Afterpulsing and Sharp Timing Response With 30 ps Tail

In this paper, we present the design, fabrication, and experimental characterization of a new Single-Photon Avalanche Diode (SPAD) made in InGaAs/InP for photon-counting operations up to 1700 nm. Working in gated-mode at 225 K with 5 V excess bias, this detector shows very low afterpulsing, hence the hold-off time can be set as low as a few microseconds, thus allowing high photon-counting rates (towards 1 Mcps). The timing response has a full-width at half maximum of less than 90 ps and a full-width at 1/1000 of maximum of less than 450 ps, thanks to a very fast (30 ps) exponential tail, thus allowing extremely wide dynamic ranges in time-correlated single photon counting measurements. Furthermore, such InGaAs/InP SPAD shows good photon detection efficiency ( <formula formulatype="inline" xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink"> <tex Notation="TeX">${&gt;}{25\%}$</tex></formula> at 1550 nm and 40% at 1000 nm) at a moderately low dark count rate, below 100 kcps for a 25 <formula formulatype="inline" xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink"><tex Notation="TeX">$\mu{\rm m}$</tex></formula> active-area diameter detector. These good results are due to design and fabrication optimization.

Direct measurement of mammographic X-ray spectra with a digital CdTe detection system.

In this work we present a detection system, based on a CdTe detector and an innovative digital pulse processing (DPP) system, for high-rate X-ray spectroscopy in mammography (1–30 keV). The DPP system performs a height and shape analysis of the detector pulses, sampled and digitized by a 14-bit, 100 MHz ADC. We show the results of the characterization of the detection system both at low and high photon counting rates by using monoenergetic X-ray sources and a nonclinical X-ray tube. The detection system exhibits excellent performance up to 830 kcps with an energy resolution of 4.5% FWHM at 22.1 keV. Direct measurements of clinical molybdenum X-ray spectra were carried out by using a pinhole collimator and a custom alignment device. A comparison with the attenuation curves and the half value layer values, obtained from the measured and simulated spectra, from an ionization chamber and from a solid state dosimeter, also shows the accuracy of the measurements. These results make the proposed detection system a very attractive tool for both laboratory research, calibration of dosimeters and advanced quality controls in mammography.

Requirements on Photon Counting Detectors for Terahertz Interferometry

Future Terahertz astronomy requires higher angular resolution observations. One possibility is to use photon counting interferometry, which is similar to the intensity interferometry demonstrated by Hanbury Brown and Twiss in 1956. In terahertz frequencies, it will be possible to measure all the photon arrivals and can identify bunched photons from thermal sources to measure correlation amplitude and time delay of the photon arrivals. By obtaining the complex visibility, aperture synthesis images can be obtained. I name this technology as photon counting terahertz interferometry (PCTI). From scientific case study, requirements to the detectors are high photon counting rate and accurate time resolution. I discuss on requirements on possible detector technologies such as superconducting single photon detectors (SSPD), superconducting tunnel junction (STJ) detectors and charge sensitive infrared photo-transistors (CSIP).

High‐rate x‐ray spectroscopy in mammography with a CdTe detector: A digital pulse processing approach

Direct measurement of mammographic x-ray spectra under clinical conditions is a difficult task due to the high fluence rate of the x-ray beams as well as the limits in the development of high resolution detection systems in a high counting rate environment. In this work we present a detection system, based on a CdTe detector and an innovative digital pulse processing (DPP) system, for high-rate x-ray spectroscopy in mammography. The DPP system performs a digital pile-up inspection and a digital pulse height analysis of the detector signals, digitized through a 14-bit, 100 MHz digitizer, for x-ray spectroscopy even at high photon counting rates. We investigated on the response of the digital detection system both at low (150 cps) and at high photon counting rates (up to 500 kcps) by using monoenergetic x-ray sources and a nonclinical molybdenum anode x-ray tube. Clinical molybdenum x-ray spectrum measurements were also performed by using a pinhole collimator and a custom alignment device. The detection system shows excellent performance up to 512 kcps with an energy resolution of 4.08% FWHM at 22.1 keV. Despite the high photon counting rate (up to 453 kcps), the molybdenum x-ray spectra, measured under clinical conditions, are characterized by a low number of pile-up events. The agreement between the attenuation curves and the half value layer values, obtained from the measured spectra, simulated spectra, and from the exposure values directly measured with an ionization chamber, also shows the accuracy of the measurements. These results make the proposed detection system a very attractive tool for both laboratory research and advanced quality controls in mammography.

Performance of a digital CdTe X-ray spectrometer in low and high counting rate environment

The high performances of CdTe detectors for X-ray and gamma ray spectroscopy are already well known. Among the traditional semiconductor spectrometers, CdTe detectors show high detection efficiency and good room temperature performance and are well suited for the development of compact detection systems. In this work, we investigated the performance of a CdTe detector coupled with a custom digital pulse processing (DPP) system for X-ray spectroscopy. The DPP method, implemented on a PC platform, performs a pile-up inspection and a pulse height analysis of the preamplifier output pulses, digitized by a 14-bit, 100MHz ADC. The spectroscopic results point out the excellent performance of the digital spectrometer both at low (150cps) and at high photon counting rate (up to 370kcps), confirming the high potentialities of CdTe detectors coupled with DPP systems. The detector and the DPP system were developed by our collaboration as a spectrometer prototype for direct measurement of diagnostic X-ray spectra in the 1–40keV energy range.

Ultra Storage-Efficient Time Digitizer for Pseudorandom Single Photon Counter Implemented on a Field-Programmable Gate Array

Pseudorandom single photon counting is a novel time-resolved optical measurement method, which is advantageous over convention techniques in terms of data-acquisition speed and system cost. As a critical component of the pseudorandom single photon counter, the photon arriving time digitizer should be storage efficient for a high photon counting rate, while maintaining good time accuracy. We report an ultra storage-efficient time digitizer for a pseudorandom single photon counter in this paper, which is based on the asynchronous serial communication and can store the arriving time of every photon in 1-b memory space. In addition, a novel comb-wave modulator is proposed to achieve the dc balance required for asynchronous serial communication. Our prototype implemented on field-programmable gate arrays provides a time resolution of 400 ps. It can register up to 4.2-Giga photon arriving time tags with 1024 × 32-b memory space.

An Experimental System of X-ray Magnetic Diffraction at the Photon Factory

An experimental system of X-ray magnetic diffraction (XMD) for ferromagents is established at the Photon Factory in KEK to realize high photon-counting rate up to 105 cps and high magnetic-field strength over 20 kOe. These performances have been achieved by upgrading (i) an X-ray detector and photon-counting apparatus and (ii) an electromagnet, respectively. The spin magnetic form factor of ferromagnetic YTiO3 for 30 reciprocal lattice points of hk0 and 0kl series has been measured by using the XMD system in various geometries including magnetic-field direction parallel to the hard axis. The result is in good agreement with that of the neutron diffraction experiment. This fact shows that the system is valuable for measuring magnetic form factor of ferromagnets. In this paper we report the details of the system.

Pseudo-random single photon counting for time-resolved optical measurement

We report a new time-resolved optical measurement method which combines single photon counting and the spread spectrum time-resolved optical measurement method. A laser diode modulated with pseudo-random bit sequences replaces the short pulse laser used in conventional time-resolved optical systems, while a single photon detector records the pulse sequence in response to the modulated excitation. Periodic cross-correlation is used to retrieve the impulse response. Feasibility of our approach is validated experimentally. A rise time around 150 picoseconds has been achieved with our prototype. Besides high temporal resolution, the new method also affords other benefits such as high photon counting rate, fast data acquisition, portability, and low cost.

4H-SiC Visible-Blind Single-Photon Avalanche Diode for Ultraviolet Detection at 280 and 350 nm

This paper reports on a 4H-SiC single-photon avalanche diode (SPAD) operating at UV wavelengths of 280 and 350 nm. The SPAD shows low dark currents of 20 and 57 fA at 80 V and 90% breakdown voltage, respectively. The quantum efficiency (QE) reaches its peak of 43% at 270 nm and is 6100. The 4H-SiC SPAD shows a fast self-quenching and a high photon count rate of 1.44 MHz in the passive-quenching mode. At the wavelength of 280 nm, a single-photon detection efficiency (SPDE) of 2.83 % with a low dark count rate of 22 kHz is achieved at the reverse bias of 116.8 V. The SPDE at 350 nm is lower, which is 0.195%, owing to the correspondingly smaller QE. Optimization measurements were conducted on SPDE as a function of voltage bias and signal output threshold.

Self-suppression of reset induced triggering in picosecond SPAD timing circuits

We present a new photon timing circuit that achieves a time resolution of 35 ps full width at half maximum with single photon avalanche diodes having active area diameters up to 200 microm. The timing circuit is based on a double avalanche current sensing network that makes it particularly suited to operation at high photon counting rates. Thanks to its self-adjusting capabilities, no trimming is needed even when changing the photodetector operating conditions over a wide range.

Spectroscopy With Nanostructured Superconducting Single Photon Detectors

Superconducting single-photon detectors (SSPDs) are nanostructured devices made from ultrathin superconducting films. They are typically operated at liquid helium temperature and exhibit high detection efficiency, in combination with very low dark counts, fast response time, and extremely low timing jitter, within a broad wavelength range from ultraviolet to mid-infrared (up to 6 <i xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink">mu</i> m). SSPDs are very attractive for applications such as fiber-based telecommunication, where single-photon sensitivity and high photon-counting rates are required. We review the current state-of-the-art in the SSPD research and development, and compare the SSPD performance to the best semiconducting avalanche photodiodes and other superconducting photon detectors. Furthermore, we demonstrate that SSPDs can also be successfully implemented in photon-energy-resolving experiments. Our approach is based on the fact that the size of the hotspot, a nonsuperconducting region generated upon photon absorption, is linearly dependent on the photon energy. We introduce a statistical method, where, by measuring the SSPD system detection efficiency at different bias currents, we are able to resolve the wavelength of the incident photons with a resolution of 50 nm.

Probing conformational dynamics in single donor-acceptor synthetic molecules by means of photoinduced reversible electron transfer.

We use single-molecule fluorescence lifetimes to probe dynamics of photoinduced reversible electron transfer occurring between triphenylamine (donor) and perylenediimide (acceptor) in single molecules of a polyphenylenic rigid dendrimer embedded in polystyrene. Here, reversible electron transfer in individual donor-acceptor molecules results in delayed fluorescence that is emitted with a high photon count rate. By monitoring fluorescence decay times on a photon-by-photon basis, we find fluctuations in both forward and reverse electron transfer spanning a broad time range, from milliseconds to seconds. Fluctuations are induced by conformational changes in the dendrimer structure as well by polystyrene chain reorientation. The conformational changes are related to changes in the dihedral angle of adjacent phenyl rings located in the dendritic branch near the donor transferring the charge, a torsional motion that results in millisecond fluctuations in the "through-bond" donor-acceptor electronic coupling. Polymer chain reorientation leads to changes in the local polarity experienced by the donors and to changes in the solvation of the charge-separated state. As a result, switching between different donor moieties within the same single molecule becomes possible and induces fluctuations in decay time on a time scale of seconds.

Multispectral/fluorescence CT using superconducting tunnel junction detector for 3-D material analysis

We have developed superconducting tunnel junctions (STJs) for applications to astrophysics, particle physics, material physics, etc. The spectrum capability of STJs is the wide wavelength/energy range from visible light to X-ray. STJs are applicable to photon detectors with good energy resolution and a high photon-counting rate. STJs also have good efficiency because of their high absorption efficiency below 1keV photon energy. This is advantageous in low photon emission observation like fluorescence from objects. STJs have potentials to open new windows of the Multispectral/fluorescence computed tomography (CT) below 1keV photon energy. As first step, we are starting STJ-CT experiments from the high-energy X-ray region (6–20keV). We report and discuss the CT using STJs.

A pixel detector with large dynamic range for high photon counting rates

In this paper, results obtained from a prototype photon counting detector are presented. The pixel size is 330 µm × 330 µm for a total area of 16 µm × 40 mm. The detector works at room temperature and its dynamic response ranges from 0.01 up to 106photons pixel−1s−1. An energy resolution of about 1.5 keV has been measured. Very encouraging small-angle X-ray scattering (SAXS) and diffraction patterns were obtained, demonstrating the success of the prototype. Plans for future developments based on this study are presented.

DEVELOPMENT OF SUPERCONDUCTING TUNNEL JUNCTIONS FOR EUV DETECTORS

Superconducting tunnel junctions (STJs) are applicable to as photon detectors with an energy resolution and a high photon-counting rate. The absorption of a photon in the superconductor of the STJ generates a number of quasiparticles that is proportional to the photon energy. Especially for soft X-ray and extreme ultraviolet (EUV) applications, STJs have good performance because of their high absorption efficiency below 1 keV. We are developing an energy-dispersive photon detector for EUV radiation using STJs with Al trapping layers. We evaluated the performance of the detector for EUV photons by using the Synchrotron Facility at KEK-PF in Tsukuba, Japan. We achieved an energy resolution of FWHM=18 eV (including the external noise of 17.6 eV) for 55 eV EUV photons with a 100 × 100 μ m 2 STJ. We present details of the junction design and discuss our experiments and the results.

Development of superconducting tunnel junctions for ultra soft X-ray detectors

Nb-based superconducting tunnel junctions (STJs) with Al trapping layers have been developed for X-ray detectors. One applications for STJs is a low energy radiation detector having energy resolution and a high photon counting rate. STJs have good potential in the band of energies from 40 eV up to 1 keV, because STJs materials have good absorbing properties in this region. The energy resolution was measured by using the Photon Factory beamline BL-12A of High Energy Accelerator Research Organization (KEK) in Japan, and for 200 eV photon, 11 eV Full Width Half at Half Maximum (FWHM) with a 20/spl times/20 /spl mu/m/sup 2/ junction were achieved. In this article, the fabrication technique and preliminary results of measuring the response for this band of energies are reported.