High Peak Power Laser Research Articles

Bridgman growth and characterizations of nonlinear optical crystal La3Ga5.5Nb0.5O14

La3Ga5.5Nb0.5O14 (LGN) crystal is a promising material for optical parametric chirped-pulse amplification (OPCPA) with high laser damage threshold and wide transmission range which is able to achieve high peak power laser. LGN with a diameter of 25 mm was successfully grown by the vertical Bridgman method for the first time and a series of characterizations were performed. The 1.7 µm absorption peak in transmittance spectra of LGN crystal which was caused by the Czochralski technique can be effectively eliminated by the vertical Bridgman method. LGN crystal possesses a high transmittance of 81.3 % in the range of 0.294 ∼ 7.500 μm. The experimental optical band gap of LGN is 4.16 eV which is positively correlated with laser damage threshold. The experimental laser damage threshold of LGN was determined to 1.416 GW/cm2 by Nd:YAG. The outstanding thermal properties of LGN indicate that it possesses thermal stability in high energy laser field. This work demonstrates that LGN crystal holds great potential for OPCPA applications and the vertical Bridgman method is proved to be a effective and excellent technique to grow high quality LGN crystal.

Multi-mode stable, high peak power Nd:YAG laser device for laser cleaning

High average power and peak power solid-state lasers are of great interest in the field of laser cleaning. In this research, a high peak power laser with over 400 W average power using a multi-mode stable resonator in a diode-pumped Nd:YAG master oscillator power amplifier has been demonstrated. A maximum peak power over 1.08 MW was achieved at a repetition frequency of 5 kHz. Delivery fiber with a 400 µm core diameter was utilized for flexible laser transmission. A prototype of the laser cleaning system was developed and inspiring application effects for paint and mold cleaning were achieved.

Experimental study of injection seeded single-longitudinal-mode Q-switched fiber laser

--The role of injection seeding power on the operation and output characteristics of a single-longitudinal-mode (SLM) injection seeded Q-switched fiber laser is investigated. The mode coupling between seeding laser and the potential longitudinal-modes of the oscillator changes as the injection seeding power increase. So the Q-switched laser may operate at different regimes which can be distinguished by the pulse features. Only with a proper range of injection seeding power that is not too larger or too small, the operation of injection seeded Q-switched fiber laser with narrow-linewidth, high peak power and narrow pulsewidth laser pulses is possible. The Q-switched fiber laser linewidth is narrowed through inserting a dual-OCs oscillator into the laser cavity. 200-ns, 1-W peak power SLM Q-switched laser pulse with nearly transform-limited linewidth is obtained when the pump power is 300 mW.

Sub-Nanosecond, High Peak Power Yb:YAG/Cr4+:YAG/YVO4 Passively Q-Switched Raman Microchip Laser with the Emission of Multiple Pulses

This paper demonstrates the capability of sub-nanosecond, high peak power Yb:YAG/Cr4+:YAG/YVO4 passively Q-switched Raman microchip lasers at 1134 nm operated in multiple pulses mode under quasi-continuous-wave (QCW) pumping. Total pulse energy for the Stokes laser was 1.8 mJ with a 4 mm YVO4 crystal and TOC = 16%. The corresponding pulse repetition rate reached 225 kHz within a single pumping pulse. By employing a compact plane-concave cavity and 5 mm YVO4 crystal, the single pulse energy for the Raman laser was further scaled up to 44 μJ. The corresponding peak power was 95 kW. A highest output pulse repetition rate of 87.8 kHz and shortest pulse duration of 464 ps were found for the Raman laser. The results indicate that the Raman microchip laser configuration under QCW LD pumping is a promising approach for developing high peak power, commercial and portable Raman lasers with a pulse duration of several hundred-picoseconds at a pulse repetition rate of hundred kilohertz.

A novel small-scale self-focusing suppression method for post-compression in high peak power lasers

Abstract A novel method, combining an asymmetric four-grating compressor (AFGC) with pulse post-compression, is numerically demonstrated to improve the spatial uniformity of laser beams and hence to suppress small-scale self-focusing (SSSF) during the beam propagation in nonlinear materials of high peak power lasers. The spatial uniformity of laser beams is an important factor in performing post-compression, due to the spatial intensity modulation, or hot spots will be aggravated during the nonlinear propagation and then seriously damage the subsequent optical components. Three-dimensional numerical simulations of post-compression are implemented based on a femtosecond laser with a standard compressor and an AFGC, respectively. The simulated results indicate that post-compression with the AFGC can efficiently suppress the SSSF and also shorten the laser pulses from 30 fs to sub-10 fs. This work can provide a promising route to overcome the challenge of SSSF and will be meaningful to promote the practical application of the post-compression technique in high peak power lasers.

Dynamic range enhancement of self-referenced spectral interferometry with extended time excursion method by the cascaded Kerr lens process.

Self-referenced spectral interferometry with extended time excursion (SRSI-ETE) is a powerful method for single-shot characterization of the temporal contrast of a high peak power laser, which has high temporal resolution but a low dynamic range. Here, a temporal contrast reduction method is proposed that uses the cascaded Kerr lens process in two thin glass plates. Combined with the SRSI-ETE method, the measurement dynamic range of the method is increased about two orders of magnitude while having a 20fs temporal resolution and a 40ps time window in single shot.

From design to realization of high diffraction efficiency Littrow configuration diffraction gratings based on multilayer dielectric mirrors patterned with electron beam lithography

Diffraction efficiency (DE) and laser-induced damage threshold of Chirped pulse amplification (CPA) system diffraction gratings (DGs) are one of the main limiting factors for the anticipated progress of high peak power lasers. Optimization of a high reflectivity dielectric multilayer ZrO2/SiO2 stack mirror with a DG etched in the top SiO2 layer was carried out employing the Rigorous coupled wave analysis method. Two families of solutions possessing DE > 0.99 over the bandwidth of the 1030 nm wavelength ultrashort laser and withstanding different fabrication margins were identified for the Littrow configuration. DGs were produced and verified experimentally. Structures permitting variation in both the depth of the DG and filling factor without loss in DE were obtained for the 690 nm thick SiO2 layer. While the 770 nm thick layer permitted separation of the two parameters requiring either rigorous control of the DG depth or filling factor. DG realization technology was proposed employing electron beam lithography and inductively coupled plasma reactive ion etching. Measurements of the fabricated structures demonstrated 0.91 DE for the first diffraction order over the 60 nm bandwidth and under a 6° mounting error from the Littrow configuration. Spectral angular reflectance DE simulations and respective measurements indicated quantitative agreement. The work provides an integrated overview of high DE periodic structure numerical optimization and manufacturing roadmap which could be applied for the high-peak-power laser CPA system development.

Fast laser field reconstruction method based on a Gerchberg–Saxton algorithm with mode decomposition

Knowledge of the electric field of femtosecond, high intensity laser pulses is of paramount importance to study the interaction of this class of lasers with matter. A hybrid method to reconstruct the laser field from fluence measurements in the transverse plane at multiple positions along the propagation axis is presented, combining a Hermite–Gauss mode decomposition (MD) and elements of the Gerchberg–Saxton algorithm (GSA). The proposed GSA-MD takes into account the pointing instabilities of high intensity laser systems by tuning the centers of the HG modes. Furthermore, it quickly builds a field description by progressively increasing the number of modes and thus the accuracy of the field reconstruction. The results of field reconstruction using the GSA-MD are shown to be in excellent agreement with experimental measurements from two different high peak power laser facilities.

Nonlinear Imaging Histopathology: A Pipeline to Correlate Gold-Standard Hematoxylin and Eosin Staining With Modern Nonlinear Microscopy.

Hematoxylin and eosin (H&E) staining, the century-old technique, has been the gold standard tool for pathologists to detect anomalies in tissues and diseases such as cancer. H&E staining is a cumbersome, time-consuming process that delays and wastes precious minutes during an intraoperative diagnosis. However, even in the modern era, real-time label-free imaging techniques such as simultaneous label-free autofluorescence multiharmonic (SLAM) microscopy have delivered several more layers of information to characterize a tissue with high precision. Still, they have yet to translate to the clinic. The slow translation rate can be attributed to the lack of direct comparisons between the old and new techniques. Our approach to solving this problem is to: 1) reduce dimensions by pre-sectioning the tissue in 500 μm slices, and 2) produce fiducial laser markings which appear in both SLAM and histological imaging. High peak-power femtosecond laser pulses enable ablation in a controlled and contained manner. We perform laser marking on a grid of points encompassing the SLAM region of interest. We optimize laser power, numerical aperture, and timing to produce axially extended marking, hence multilayered fiducial markers, with minimal damage to the surrounding tissues. We performed this co-registration over an area of 3 × 3 mm2 of freshly excised mouse kidney and intestine, followed by standard H&E staining. Reduced dimensionality and the use of laser markings provided a comparison of the old and new techniques, giving a wealth of correlative information and elevating the potential of translating nonlinear microscopy to the clinic for rapid pathological assessment.

Wavefront Correction in Vacuum of SULF-1PW Laser Beamline

The focusing quality of high peak power lasers plays a crucial role in laser wakefield electron acceleration investigations. We report here an improvement in the focusing quality of the SULF-1PW laser beamline, planning to drive and generate 5~10 GeV electron beams. After the wavefront correction in vacuum with an adaptive optical system and the focusing with an f/56 off-axis parabolic mirror, near-diffraction-limited focal spots with a size of 52 × 54 μm2 at full width at half maximum are achieved, and the enclosed energy inside this size is ~36.6%. Consequently, the focused intensity of ~1.66 × 1019 W/cm2 can be achieved at 1 PW peak power. Moreover, we also examine the wavefront stability in air and vacuum, respectively. From the statistical analysis of 1900 shots of successive laser pulses at 1 Hz, we identify the wavefront fluctuation resulting from air turbulence and the better correction capacity in vacuum. This work demonstrates the importance and necessity of wavefront correction in vacuum for high peak power lasers.

Large dispersion-managed broadband high-energy fiber femtosecond laser system with sub 300 fs pulses and high beam quality output

We experimentally demonstrate a high-energy sub 300 fs polarization maintaining fiber chirped pulse amplification (CPA) system. The preamplifier is a monolithic fiberized system that uses two cascaded temperature-assisted dispersion-tuning broadband chirped fiber Bragg gratings (CFBGs) with a reflected bandwidth of 20 nm as stretchers. To make full use of the stretcher to lower the system’s nonlinearity accumulation, a homemade mode locked fiber laser with a spectral width of 14.8 nm (full width at half maximum) is selected as the seeder to offer a stretched pulse width of 1.69 ns. The main amplifier is based on a one-stage simple Yb:YAG single crystal fiber amplifier with an amplified output power of 40.6 W at a repetition rate of 200 kHz, and the beam quality is conserved in a single mode beam profile with beam quality of 1.246 and 1.142 in the horizontal direction and vertical direction, respectively. During amplification, the spectral gain narrowing effect is observed. To achieve the high-speed switch of the laser, an acoustical optical modulator (AOM) is inserted before the compressor to achieve high-speed turn-on/off control. The compressor is based on a diffraction grating pair with a groove density of 1600 line/mm to offer a dispersion match with the stretcher of the CFBGs. With the CFBG’s fine-tuned capacity of second-order dispersion and higher-order dispersion, the compressed average power of 29.6 W and pulse duration of 278 fs, corresponding to a pulse energy of 148 µJ and a peak power of 532 MW with ignoring the wings of the pulse, is obtained. The beam quality is well conserved after compression, and the beam quality is 1.250 and 1.196 in the horizontal direction and vertical direction, respectively. A power fluctuation of 0.1% (root mean square) and a beam pointing drift of 8.47 µrad/°C over 8 h are realized. This high peak power and high beam quality femtosecond laser is promising in science and industrial applications.

Multicell accelerating structure driven by a lens-focused THz pulse

Recently, gradients on the order of $1\text{ }\text{ }\mathrm{GV}/\mathrm{m}$ have been obtained with single-cycle ($\ensuremath{\sim}1\text{ }\text{ }\mathrm{ps}$) THz pulses produced by the conversion of high peak power laser radiation, in nonlinear crystals ($\ensuremath{\sim}1\text{ }\text{ }\mathrm{mJ}$, 1 ps, up to 3% conversion efficiency). Such high intensity radiation can be utilized for charged particle acceleration. For efficient acceleration, a large number of accelerating cells have to be stacked together with delay lines in order to provide proper timing between accelerating fields and moving electrons. Additionally, THz pulses in individual cells need to be focused transversely to maximize the accelerating gradient. This focusing is currently done by the tapering of the waveguide. In this paper, we propose instead to use dielectric lenses for the robust focusing of THz pulses in accelerating cells. Each lens is made from the same material as the delay line in a monolithic unit. We have fabricated prototype units from quartz and silicon. Such an approach simplifies the fabrication and alignment of the multicell accelerating structure. We present a design in which a 100 microJoule THz pulse produces a 600 keV energy gain in a 5-mm long 10-cell accelerating structure for an ultrarelativistic electron. This approach can be extended to nonrelativistic particles.

Probability density function estimation for filament creation in lossy, turbulent, nonlinear media.

Optical Kerr effects induced by the propagation of high peak-power laser beams through real atmospheres have been a topic of interest to the nonlinear optics community for several decades. Previous work has focused on estimating the Filamentation Onset Distance (FOD) in real atmospheres but not its statistical variance. This paper describes two ad hoc engineering models for predicting the FOD Probability Density Function (PDF) for lossy, turbulent, nonlinear media. Specifically, these models characterize the FOD variation with turbulence. One model uses a log-normal PDF with mean and variance proportional to the Rytov Variance. The other uses a gamma PDF employing the same mean and variance equations. These two PDFs will be compared to previous computer simulation results. Both show reasonable agreement between PDF predictions and computer simulation results for long-range filamentation. In fact, both give similar results, and there is no preference given to the data comparisons presented.

A novel focal spot positioning method for high peak power lasers

A novel focal spot positioning method for high peak power lasers

Femtosecond damage experiments and modeling of broadband mid-infrared dielectric diffraction gratings

High peak and average power lasers with high wall-plug efficiency, like the Big Aperture Thulium (BAT) laser, have garnered tremendous attention in laser technology. To meet the requirements of the BAT laser, we have developed low-dispersion reflection multilayer dielectric (MLD) gratings suitable for compression of high-energy pulses for operations at 2 micron wavelength. We carried out 10000-on-1 damage tests to investigate the fluence damage thresholds of the designed MLD gratings and mirrors, which were found between 100-230 mJ/cm2. An ultrashort pulsed laser (FWHM = 53 fs, λ = 1.9 μm) operating at 500 Hz was used in the serpentine raster scans. The atomic force microscope images of the damage sites show blister formation of the underlying layers at lower fluences but ablation of the grating pillars at higher fluences. We simulated the dynamic electronic excitation in the MLD optics with a finite-difference in the time domain approach in 2D. The simulation results agree well with the LIDT measurements and the observed blister formation. This model is able to evaluate the absolute LIDT of MLD gratings.

Multimodal nonlinear endomicroscopic imaging probe using a double-core double-clad fiber and focus-combining micro-optical concept

Multimodal non-linear microscopy combining coherent anti-Stokes Raman scattering, second harmonic generation, and two-photon excited fluorescence has proved to be a versatile and powerful tool enabling the label-free investigation of tissue structure, molecular composition, and correlation with function and disease status. For a routine medical application, the implementation of this approach into an in vivo imaging endoscope is required. However, this is a difficult task due to the requirements of a multicolour ultrashort laser delivery from a compact and robust laser source through a fiber with low losses and temporal synchronization, the efficient signal collection in epi-direction, the need for small-diameter but highly corrected endomicroobjectives of high numerical aperture and compact scanners. Here, we introduce an ultra-compact fiber-scanning endoscope platform for multimodal non-linear endomicroscopy in combination with a compact four-wave mixing based fiber laser. The heart of this fiber-scanning endoscope is an in-house custom-designed, single mode, double clad, double core pure silica fiber in combination with a 2.4 mm diameter NIR-dual-waveband corrected endomicroscopic objective of 0.55 numerical aperture and 180 µm field of view for non-linear imaging, allowing a background free, low-loss, high peak power laser delivery, and an efficient signal collection in backward direction. A linear diffractive optical grating overlays pump and Stokes laser foci across the full field of view, such that diffraction-limited performance is demonstrated for tissue imaging at one frame per second with sub-micron spatial resolution and at a high transmission of 65% from the laser to the specimen using a distal resonant fiber scanner.

Damage morphologies of Al2O3 and Fe particles attached on the input surface of fused silica after irradiation by a 355 nm laser.

Particulate contamination on the optical surface can seriously degrade the performance of optics working in the high peak power laser system. In this study, we show that the nature of optical damages on the input surface induced by particles depends on the optical property of the particles. Ceramic Al2O3 particles tend to cause micro-fractures to the optical surface, but metallic Fe particles mainly undergo ablation on the substrate. Different microscopes are used to characterize their damage morphologies, and the light distribution and thermal evolution of two different particles are simulated, focusing on better understanding their special damage morphologies.

Optical Kerr effect field measurements and ad hoc engineering model comparisons.

Optical Kerr effects induced by the propagation of high peak-power laser beams through real atmospheres have been a topic of interest to the nonlinear optics community for several decades. This paper proposes a new analytical model for predicting the filamentation/light channel onset distance in real atmospheres based on modulation instability model considerations. The normalized intensity increases exponentially as the beam propagates through the medium. It is hypothesized that this growth can be modeled as a weighted ratio of the Gaussian beam diameter at range to the lateral coherence radius and can be used to set the power ratio for an absorbing, turbulent, nonlinear media to estimate the beam collapse distance. Comparison of onset distance predictions with those found from computer simulation and deduced from field experiments will be presented. In addition, this model will be used with an analytical approach to quantify the expected radius of light channels resulting from self-focusing both with and without the production of a plasma filament. Finally, this paper will describe a set of 1.5-micron, variable focal length USPL field experiments. Comparisons of theoretical radius calculations to measurements from field experiments will be presented.

Real-time monitoring of airborne molecular contamination on antireflection silica coatings using surface acoustic wave technology

Real time monitoring of contamination on antireflection (AR) silica coatings in high peak power laser systems (HPLs) is critically needed in order to avoid reductions of transmission and laser damage to optical surfaces. Herein we proposed to apply a surface acoustic wave (SAW) sensor to real-time monitor trace amounts of airborne molecular contaminants (AMCs) adsorbed on the AR silica coatings. The silica coating is found to be susceptible to AMCs because of its mesoporous structure, huge surface area and polar nature. The adsorbed AMCs caused the increased mass on the silica coating of the SAW sensor, which resulted in a significant increase of its frequency shift. The fabricated sensor showed a high sensitivity of ∼-490 mm2 ng−1Hz and an excellent linearity vs. the areal density of adsorbed AMCs since the frequency shift of the sensor is linearly related to the change of mass of the silica coating.

Diode-pumped master oscillator power amplifier system based on cryogenically cooled Tm:Y2O3 transparent ceramics

We demonstrated a master oscillator power amplifier system using cryogenically cooled Tm:Y2O3 transparent ceramics. The electro-optically switched master oscillator acted as a seed source and could be tuned from 1 to 100 Hz. A maximum pulse energy of 1.35 mJ with a pulse duration of 30 ns amounting to a peak power of 45 kW was obtained at 10 Hz. The power amplification via double-pass geometry achieved maximum single pulse energy of 2.94 mJ at 10 Hz with a pulse duration of 32 ns. The results showed the pulsed lasing potential of Tm:Y2O3 transparent ceramics at cryogenic temperatures. This gain material can be considered as an alternative gain medium for high average and peak power laser development around 2 µm in nano-second regime.