High-energy Laser Research Articles

Predictable thermoelectric performance of directly synthesized Bi0.5Sb1.5Te3 using laser powder bed fusion additive manufacturing

Laser powder bed fusion (LPBF) additive manufacturing, as a novel technique provides broad benefits in thermoelectric materials synthesis, such as enhanced printing speed, reduced waste materials, and customized dimension design. The high energy density of laser could potentially balance the synthesis rate and thermoelectric figure-of-merit zT, but the correlations between laser energy and material performance are still vague. Herein, Bi0.5Sb1.5Te3 bulks are directly synthesized by LPBF with a recorded synthesis rate of 254 g h−1. The maximum zT, without any post-processing, reaches 1.1 at 75 °C. Induced nanoscale pores by high laser energy printing, obtain a comparable diameter to phonon mean free path, leading to reduced lattice thermal conductivity and enhanced TE performance. We found that input laser energy critically affected thermoelectric performance and concluded the correlation between volumetric energy density EV and power factor PF, PF = 9.05EV2 – 30.01EV + 48.84. It potentially predicts thermoelectric performance with inputted laser energy density.

High-energy continuous wave laser ablation of alumina ceramic

The development of high-energy continuous wave (CW) laser has enabled the generation of output powers ranging from 300 to 500 kW. Understanding the ablation mechanism of CW lasers at high laser fluence is crucial for the design of effective high-energy laser protection materials. We note that the particle-like impurities present in the protective coating material can induce defects on the ceramic-like target surface during high-energy CW laser ablation, which can alter the laser absorptivity and manifest a completely different ablation mechanism. Here, we systematically investigate the mechanism of high-energy CW laser ablation of alumina ceramic, with a specific focus on the roles of defect induction, energy transfer, and impact sputtering in the dynamic ablation of target. Specifically, the transient processes between high-energy CW laser and ceramic target will be investigated in terms of the evolution results of the ablation region, the microscopic characteristics of the ablated material, the high time-resolved on-line monitoring, and the multiphase hydrodynamics simulation. Finally, the transparent property of molten alumina ceramic to laser is proved to allow for penetrating damage to ceramic-metal composites.

CURRENT TRENDS IN THE DEVELOPMENT OF HIGH-ENERGY LASERS

Current trends in developing high-energy lasers with pulse energies in the tens and hundreds of joules are considered. Active media are analyzed for their use in such lasers. Yb:YAG active crystalline and ceramic elements (AE) of Russian production are experimentally investigated at temperatures from 100 K to 295 K. The data of the AE cryogenic cooling system are presented. A diode pumping system for AE and a homogenizer of its radiation are described. The physical and technical characteristics of the pumping system are given. Fresnel losses, absorption losses, and losses due to amplified spontaneous emission (ASE), which reduce the energy stored in an inverted population, are experimentally measured. The results of measuring the gain in multipass circuits with different sets of AEs are presented.

Rapid photo-bleaching gamma irradiated Yb-doped optical fibers by high-energy ns pulsed laser

A rapid and efficient photo-bleaching process was demonstrated with a high-energy nanosecond pulse to recover existing and/or revealed color centers on 10 kGy Gamma-irradiated Yb-doped optical fiber. Multi-mJ pulsed laser based on an optical parametric amplifier system operating at wavelengths of 532 nm, 680 nm and 793 nm was used. The photo-bleaching performance is investigated as a function of the wavelength and energy of the pulsed light source. It was observed that the photo-bleaching level of the Yb-doped optical fiber increased when the exposure time of the pulsed laser light and the photon energy was increased. The maximum PB occurred in the pulsed laser of 532 nm wavelength in the optical fiber. Also, a drastically increase in the PB was observed due to the increasing laser energy at the wavelength of 532 nm and 680 nm pulsed laser. The results show that the recovery levels of color centers in the Yb-doped optical fibers could be reached up to 96 % in a shorter time (h) by using the pulsed laser compared to that of the studies using continuous laser.

Enhanced laser-induced damage performance ofall-glass metasurfaces for energetic pulsed laserapplications.

To fabricate optical components with surface layers compatible with high-power laser applications that may operate as antireflective coatings, polarization rotators, or harness physical anisotropy for other uses, metasurfaces are becoming an appealing candidate. In this study, large-beam (1.05cm diameter) 351-nm laser-induced damage testing was performed on an all-glass metasurface structure composed of cone-like features with a subwavelength spacing of adjacent features. These structures were fabricated on untreated fused silica glass and damage tested, as were structures that were fabricated on fused silica glass that experienced a preliminary etching process to remove the surface Beilby layer that is characteristic of polished fused silica. The laser-induced damage onset for structures on untreated fused silica glass was 19.3J⋅c m -2, while the sample that saw an initial pretreatment etch exhibited an improved damage onset of 20.4J⋅c m -2, only 6% short of the reference pretreated glass damage onset of 21.7J⋅c m -2. For perspective, the National Ignition Facility operational average fluence at this wavelength and pulse length is about 10J/c m 2. At a fluence of 25.5J⋅c m -2, the reference (pretreated) fused silica initiated 5.2 damage sites per m m 2, while the antireflective metasurface sample with a preliminary etching process treatment initiated 9.8 damage sites per m m 2. These findings demonstrate that substrate-engraved metasurfaces are compatible with high energy and power laser applications, further broadening their application space.

Effect of optical fiber end face scratches on laser-induced damage threshold.

The scratches on the fiber end face can enhance the local electrical field, which lowers the damage threshold. The damage mechanism of a high-energy laser is investigated. The effect of scratches on the electric field is simulated by the finite difference time domain (FDTD) solution. The results show that the depth of the scratch has a greater ability to influence the electric field than the width, and multiple scratches have a stronger modulation than a single scratch. In calculation, the damage threshold of the scratch-free end face is 0.456J/c m 2 when the incident light electric field intensity is 50M V/c m, compared to 0.345J/c m 2 in the presence of the scratch on the end face.

Spectral peak recovery in parametrically amplified THz-repetition-rate bursts.

Multi-photon resonant spectroscopies require tunable narrowband excitation to deliver spectral selectivity and, simultaneously, high temporal intensity to drive a nonlinear-optical process. These contradictory requirements are achievable with bursts of ultrashort pulses, which provides both high intensity and tunable narrowband peaks in the frequency domain arising from spectral interference. However, femtosecond pulse bursts need special attention during their amplification [Optica7, 1758 (2020)10.1364/OPTICA.403184], which requires spectral peak suppression to increase the energy safely extractable from a chirped-pulse amplifier (CPA). Here, we present a method combining safe laser CPA, relying on spectral scrambling, with a parametric frequency converter that automatically restores the desired spectral peak structure and delivers narrow linewidths for bursts of ultrashort pulses at microjoule energies. The shown results pave the way to new high-energy ultrafast laser sources with controllable spectral selectivity.

Investigation on the kinetics of a diode-pumped plasma-jet type metastable argon laser

Diode-pumped rare gas lasers (DPRGLs) have the potential for high-energy laser output with high beam quality. The metastable concentration >1014 cm−3 and pump intensity >10 kW/cm2 are required in developing high-power and efficient DPRGLs. However, the kinetics of 1s and 2p levels (Paschen notation) under these conditions is unclear yet, particularly regarding the adverse effects of interference energy levels (e.g., 1s4 and 2p1–2p8). This study addresses this gap by measuring the number densities of 1s and 2p levels in a diode-pumped plasma jet metastable argon laser. The experiment was conducted with a much higher number density of 1014 cm−3 and a higher pump intensity of 12 kW/cm2 than our previous works. The results indicate that the adverse effect of 1s4 accumulation could be partially compensated, and the relative population distribution of 2p energy levels remained unchanged. However, the high gas temperature (>1000 K) caused a significant negative impact of high 2p levels (2p1–2p8), and the air environment weakened the effect of He collision relaxation.

Research on the core factors affecting the temperature rise of dichroic mirrors in wavelength beam combination system under high-power CW laser

The wavelength beam combination is considered an important method for improving the source power of high-energy laser weapons while maintaining high beam quality. The dichroic mirror is the key component that decisively determines the laser beam quality of the wavelength beam combining system. However, the temperature rise of the dichroic mirror due to continuous high-power laser irradiation can significantly deteriorate the beam quality and decrease the efficiency of the systems. Along these lines, in this work, the factors that influence the temperature rise of the dichroic mirror under high power CW laser were systematically examined. The temperature field equation of the dichroic mirror under transmission and reflection laser was also calculated. The variation of the dichroic mirror temperature by the laser power, laser spot size, diameter, and thickness of substrates, as well as material of substrates and thin-film absorption was simulated. The simulated results were verified by performing experiments on both sapphire and quartz substrates. The transmittance absorption was proved to be the main cause of the temperature rise and the laser power had a linear relationship with the maximum temperature. Interestingly, the temperature decreased with the thermal conductivity and the laser spot size. As a result, the optimization of the substrate size can significantly reduce the temperature of the dichroic mirror. Our work provides valuable insights into the design and increase in performance of dichroic mirrors in the wavelength combination system.

Arrays of glass wedges for multi-dimensional optical diagnostics.

There is a common need in the advancement of optical diagnostic techniques to increase the dimensionality of measurements. For example, point measurements could be improved to multi-point, line, planar, volumetric, or time-resolved volumetric measurements. In this work, a unique optical element is presented to enable multi-dimensional measurements, namely, an array of glass wedges. A light source is passed through the wedges, and different portions of the illumination are refracted by different amounts depending on the glass wedge angle. Subsequent optics can be used to focus the light to multiple points, lines, or planes. Basic characterization of a glass wedge array is presented. Additional wedge-array configurations are discussed, including the use of a periodic intensity mask for multi-planar measurements via structured illumination. The utility of this optical element is briefly demonstrated in (a)multi-planar flame particulate measurements, (b)multi-point femtosecond-laser electronic excitation tagging for flow velocimetry, and (c)multi-line nitric oxide molecular tagging velocimetry in a hypersonic shock-tunnel. One significant advantage of this optical component is its compatibility with high-energy laser sources, which may be a limiting factor with other beam-splitting or beam-forming elements such as some diffractive optics. Additionally, an array of glass wedges is simple and easily customizable compared to other methods for forming multiple closely spaced illumination patterns. Suggestions for further development and applications are discussed.

Investigation of the Multimechanism Laser Cleaning Dynamics for Rough Fused Silica Surfaces with Organic Contaminants: A Computational Simulation and Atomic Analysis.

The detrimental impact of organic contaminants on optical components poses a significant obstacle to high-energy laser systems. However, irregularities or defects on the surface of optical components during manufacturing can affect the process of organic contaminant removal. Thus, a comprehensive understanding of the intricate interplay among surface roughness, contaminant absorption, and ablation is essential to effectively address the challenges of laser-induced damage. In this study, a molecular dynamics approach was employed to investigate the interaction between laser-fused silica and contaminants and to analyze the influence of surface roughness on the removal of contaminants from fused silica. Research findings demonstrate that during laser irradiation, organic contaminants on the surface of mechanical components diffuse into the optical elements. As the laser flux increases, the contaminants gradually decompose into smaller molecular clusters. Additionally, the phenomenon of contaminant ablation is observed to consist of two distinct phases: the "Thermal expansion phase" and the "Thermal ablation phase." The study examines the impact of substrate roughness on the contaminant removal in these two phases. It is found that a higher surface roughness leads to stronger thermal expansion and vaporization of contaminants. With increasing roughness of the fused silica substrate, the corresponding van der Waals energy and pressure decrease under the same laser fluence, making the removal of contaminants easier. These results provide valuable insights into the interaction between laser irradiation and organic contaminants.

Acoustic positioning of closely-flying aircraft for eye safety of space laser applications

In laser-based space technologies where laser beams are transmitted from a ground station, it is required for the ground station to avoid irradiating aircraft with high energy lasers. A simple, inexpensive acoustic positioning technique using four microphones is developed and its performance is evaluated. It is demonstrated to be sensitive to and effective in detecting aircraft flying at short ranges. Aircraft closer than 5 km can easily be detected and the maximum range is about 10 km. The time series of two-dimensional directional position estimates are harmonic with those of ADS-B (Automatic Dependent Surveillance-Broadcast), and the precision reaches 1 degree (standard deviation) in the best case. The processing time for data collection and computation is short enough to establish a realtime feedback mechanism to stop firing laser. With its advantages and disadvantages, effective combinations with existing methods are discussed to avoid injury to the eyes, in which the acoustic approach is found to be useful to enhance safety measures in particular of low-altitude aircraft with a large angular velocity.

Strain-modulated band structure and high harmonic generations in two-dimensional MoS2

Two-dimensional (2D) condensed matter is a material that is restricted in one direction while being periodic in the other. Since the restricted size of 2D materials is comparable to the wavelength of electrons, a quantum confinement effect may occur. Moreover, the absence of periodicity provides weak screening in 2D materials, which brings novel physical properties such as the quantum well, which is widely applied in quantum information, and the fine absorption structures in graphene. Among the 2D materials, the monolayer transition metal chalcogenides represented by MoS2 have attracted wide attention due to the direct band gap in the visible light region (1.8 eV) and valley polarizations, which are prospective for solar cells as well as photoelectric devices. High-harmonic generation (HHG) is a strong non-linear process during which a high-energy laser impulse is applied to materials and high-harmonic radiations are yielded. As a typical ultrafast dynamic, HHG has important applications in laser generation, such as EUV lithographic metrology and high-resolution coherent imaging. According to the Bloch oscillation model, HHG is highly dependent on band structure. Here, we report the strain-dependent HHG dynamics in MoS2. Further investigation reveals that the strain-dependence of HHG is caused by band modulation under different strains, which is dominant during HHG. Our research sheds light on ways to achieve effective modulations in ultrafast dynamics, implying an all-optical measurement band structure in strained materials.

Spot Invalid Point Repair Algorithm of Detector Array Measurement System Based on Image Correlation Coefficient

The detector array method has been widely used in the field of high-energy laser far-field spot parameter measurement due to its ability to directly measure the far-field spot of high-energy lasers, wide dynamic range of the detectors, high system sampling frequency, good real-time performance, and suitability for various testing environment requirements. However, during the measurement process, the irradiation of strong lasers or damage to other hardware systems can result in invalid points in the acquired spot images, thereby reducing the measurement accuracy of the system. In order to achieve accurate measurement of laser far-field spot parameters, this paper establishes an experimental model based on the analysis of the sampling spacing of the detector array target and proposes a laser far-field spot invalid point repair algorithm based on image correlation coefficient. Experimental results demonstrate that the algorithm proposed in this paper effectively reduces the impact of invalid points in the measurement system on the measurement accuracy, and achieves accurate measurement of high-energy laser measurement systems.

Behavior of Zr–1Nb alloy in coarse- and ultrafine-grain states under laser-induced shock wave loading

The work is devoted to the study of the Zr-1Nb alloy in coarse-grained and ultrafine-grained states under laser-induced shock-wave loading. This material is of interest due to the application for the manufacture of shells for fuel elements of nuclear reactors. The properties of this alloy in the ultrafine-grained state is attracted for the reliability improvement of fuel rods in wide range of load intensity. Shock wave loading was carried out using a Beamtech SGR-Extra-10 high-energy nanosecond laser. The free surface velocity profiles were registered by the VISAR system. Mechanical characteristics are obtained using velocity profiles. It is shown that the spall strength and dynamic elastic limit for the coarse-grained state are higher than for the ultrafine-grained state. In general, the Zr-1Nb alloy in the ultrafine-grained state is more susceptible to spall fracture, including laser shock peening. Numerical simulation of the process under study has been carried out using statistically based nonlinear model of solid with defects and finite element method to describe the deformation behavior and fracture of the material under shock-wave loading. Simulation results are qualitatively consistent with experiments in the prediction of the conditions of spall failure.

Simulation Analysis of Dynamic Damage Probability Modelling for Laser Systems

The paper proposes a method that analyses the dynamic damage probability of laser systems to address the shortcomings of the quantitative model for the damage probability of laser systems. Firstly, the far-field energy density distribution model is constructed according to the power spectrum inversion method. Then, the instantaneous on-target spot power density distribution is equivalently portrayed based on the combination of the far-field power density and the missile target characteristics. Next, the instantaneous on-target spot is combined with the tracking and aiming error to obtain the probability distribution of the energy density of the long-period on-target spot. Finally, the temperature probability distribution is obtained by analyzing the relation between the target energy density and the temperature of the inner wall of the warhead. Consequently, the damage probability was calculated. The simulation shows that there is a unique maximum damage probability when the target is flying in a straight line and the laser system strikes the missile sideways. The method can provide support for the shooting timing of high-energy laser systems.

2.2 kW single-mode narrow-linewidth laser delivery through a hollow-core fiber

Antiresonant hollow-core fibers (AR-HCFs) have opened up exciting possibilities for high-energy and high-power laser delivery because of their exceptionally low nonlinearities and high damage thresholds. While these fiber designs offer great potential for handling kilowatt-class powers, it is crucial to investigate their performance at multi-kW power levels. Until now, transmission of narrow-linewidth single-mode lasers at multi-kW power levels through a HCF has not been demonstrated, to our knowledge. Here, we present the delivery of a record 2.2 kW laser power with an input spectral linewidth of 86 GHz, centered at 1080 nm, while maintaining 95% transmission efficiency and beam quality (M2) of 1.03. This was achieved via a 104.5 m single-mode five-tube nested AR-HCF with 0.79 dB/km loss. Furthermore, we show power delivery of 1.7 kW with a spectral linewidth as narrow as 38 GHz through the same fiber. Our results could lead to a new generation of fiber-based laser beam delivery systems with applications in precision machining, nonlinear science, directed energy, and power beaming over fiber.

Ablation properties of SiC-reinforced PBI resin matrix composites under high-energy continuous laser ablation

In this work, poly-p-phenylene benzobisoxazole (PBO) fibers reinforced polybenzimidazole (PBI) resin-based laser ablation composites (thickness = 5 mm) with different SiC contents were prepared. SiC/PBI/PBO composites exhibited good mechanical properties, excellent thermal stability and laser ablation properties. The laser ablation properties and ablation mechanism of the composites were investigated using a high-energy continuous-wave laser (30 MW·m−2). Increasing the SiC content led to increase in composites density, while decreasing the bending performance of the composites. However, it improves the mass and linear ablation rates, resulting in an overall improvement in ablation properties. At a SiC content of 70 %, the composite exhibited a mass loss of 8.2 %, a mass ablation rate of 9.2 mg·s−1, and a linear ablation rate of 0.11 mm·s−1. The ablation process of SiC/PBI/PBO composites was delineated into pre-ablation and post-ablation stages, with the ablated composites divided into the ablation center, transition region, and outer region based on morphological characteristics. After ablation, numerous white hollow SiO2 spheres and SiO2 protective layers were formed in the ablation centers, the transition regions were deformed and cracked, while the outer region remained unscathed.

TiC morphology and corrosion resistance of CrMnFeCoNi+x(TiC) coatings prepared by laser cladding

The corrosion resistance of CrMnFeCoNi coatings with varying TiC contents and the evolution of TiC within these coatings were comprehensively investigated. These CrMnFeCoNi coatings, with different TiC concentrations, were fabricated using laser cladding technology. The behavior of TiC evolution in CrMnFeCoNi coatings was observed to follow a distinct pattern. At a TiC loading of 2 wt%, TiC exhibited a dispersed distribution. Interestingly, in coatings loaded with 4 wt% TiC, TiC was observed in various shapes, including elongated, square, petaled, and circular forms owing to the melting of TiC particles under the influence of a high-energy laser beam. The convection action of the molten pool combined several unmelted, partially melted, and precipitated TiC particles, resulting in diverse shapes. Furthermore, increasing the TiC content to 10 wt% led to the aggregation and fusion of TiC into clusters. Additionally, the electrochemical corrosion resistance behavior of CrMnFeCoNi coatings with varying TiC content displayed a significant correlation with the TiC concentration. As the TiC content increased, the galvanic corrosion resistance also increased. At lower TiC content levels, a higher number of electrochemical cells formed between the CrMnFeCoNi matrix and the dispersed TiC, leading to an elevated corrosion rate. In contrast, as the TiC content increased, the dispersed TiC phase fused together, reducing the likelihood of electrochemical cell formation. Notably, the electrochemical corrosion resistance of the CrMnFeCoNi coating containing 10 wt% TiC resembled that of the TiC-free coating.

Generation of high-energy near-infrared femtosecond laser pulses by optical parametric amplification in YCOB crystals

"The energy of near-infrared femtosecond laser pulses generated by optical parametric amplification (OPA) in β-barium borate (BBO) crystals pumped by femtosecond Ti:sapphire lasers is restricted to few-mJ due to the 20 mm limited diam- eter of available crystals. In a type I collinear OPA with an yttrium calcium oxoborate (YCOB) crystal, pumped with femtosecond Ti:sapphire lasers at 800 nm wavelength, the 1300 nm signal wavelength and 2080 nm idler wavelength are located in the normal and anomalous group velocity dispersion range, respectively. Due to the small group velocity mismatch (GVM) between signal and idler pulses, as broad as 27 THz gain bandwidth can be obtained in a 3-mm YCOB crystal at 100 GW/cm2 pump intensity. A high parametric gain is the result of the increased parametric interaction length due to the different signs of GVM between pump-signal and pump-idler pulses. More than 10-mJ energy femtosecond laser pulses at 1300 nm wavelength can be generated by OPA in YCOB crystals with larger than 50 mm clear aperture."