Highest Dust Fluxes Research Articles

A detailed quartz and feldspar luminescence chronology for the Khonako II loess section (Southern Tajikistan)

Parts of Central Asia have been dominated by high dust flux since the start of the Quaternary. The resulting loess-palaeosol deposits are important archives for landscape and climate changes, but there is a lack of chronological data for the subaerial deposits of Southern Tajikistan. Our study presents a high-resolution luminescence chronology for the Khonako II section in the Khovaling region. Thirty-seven samples were collected from the first ∼8 m of the section, corresponding to the Holocene soil and the upper part of the Loess 1 (L1) unit. We applied quartz OSL dating to the coarse-silt fraction (40–63 μm) and polymineral pIRIR200,290 dating to the very fine sand fraction (63–90 μm). The polymineral pIRIR200,290 signal has satisfactory characteristics. The quartz dose response curve displays a non-single exponential growth above ∼100 Gy, thus, the De values were estimated by fitting a single exponential function plus linear component to the dose response data. To assess the pIRIR200,290 residual dose at deposition, we used the offset between our quartz and polymineral chronologies from Khonako II and equivalent doses measured on modern dust samples from Tajikistan and Uzbekistan. The resulting 9.2 ± 0.4 Gy dose was then subtracted from the pIRIR200,290 doses for final age calculation. The quartz OSL and pIRIR ages are then generally consistent. The obtained high-resolution luminescence chronology shows that the upper part of the L1 unit accumulated during the end of marine isotope stage (MIS) 3 and through MIS 2 (39–20 ka). The average dust accumulation rates (DAR) increased from ∼31 cm ka−1 to 41 cm ka−1 between MIS 3 and MIS 2. The DAR reached a peak of ∼71 cm ka−1 at 21 ka. A hiatus of ∼7–9 ka was then identified between the end of the last glacial maximum (LGM) and the beginning of the Holocene, and the average DAR decreased during the Holocene. Our results indicate a continuous high dust flux in the Khovaling plateau over the last 39 ka, but reworking processes and potential deflation events mark the LGM-Holocene transition. High-resolution luminescence dating studies in Tajikistan are therefore important to detect potential discontinuities in the sequences and provide an independent timescale for interpreting the climate proxies and calculating dust accumulation rates.

Characterizing the response of Timepix solid state detectors to dust impacts

Timepix Solid State Detectors (TSSDs) are used in a range of applications, including high energy particle physics, x-ray imaging spectroscopy, medical imaging, radiation monitors and compact dosimeters. In space sciences, such detectors have been used for characterizing the radiation environments of the Earth and lunar surface. This study is a pilot investigation of the response of TSSDs to high-velocity dust impacts. The setup used for the measurements is a silicon slab with 500μm thickness combined with the Timepix 2 read-out chip with a pixel size of 55×55 μm2. The outer surface of the SSD is coated with a 150 nm thick layer of aluminum to eliminate the sensitivity to light. The dust accelerator facility operated at the University of Colorado is used to expose the TSSD to micron- and sub-micron sized iron particles in a velocity range of 1–10 km/s. A fraction (5%) of the impacting dust particles were detected by the TSSD. The primary mechanism of the detection is through the light generated upon the impact and the charge signal spreads over multiple pixels. The fraction of dust particles kinetic energy that is converted to detectable charge on the TSSD is small, in the range of 10−3−10−6. The largest craters generated by the dust impacts were examined using a scanning electron microscope (SEM). The SEM images confirm that the particles penetrated the aluminum layer and the craters contain iron residue from the dust material. Over the investigated impact parameter range, the TSSD does not suffer a permanent damage from the dust impacts. Due to their small size and relatively low sensitivity to dust impacts, TSSDs could be used as dust detectors only in environments with high dust fluxes (e.g., in cometary trails), or where the precision measurements of the impact location are desired.

Dust correlation and oxygen isotope stratigraphy in the Southern Ocean over the last 450 kyrs: An Indian sector perspective

The chronology of Southern Ocean (SO) marine sediment cores forms the basis of understanding the SO paleoceanography, with significant implications for global climate. Because tuning of the oxygen isotope (δ18O) record of a marine sediment core to a δ18O stack (δ18O stratigraphy) is difficult in the SO because of a general paucity of calcareous foraminifera, tuning of the dust proxy signal of a marine sediment core to the dust record of an ice core (dust correlation) is a promising way to construct an age–depth model. However, the reliability of dust correlation has not been established, especially beyond the last ∼300 kyrs, and such work has been performed more in the Atlantic and Pacific sectors of the SO than in the Indian sector. Here we present a new dust correlation using the rock magnetic record, together with continuous δ18O stratigraphy, for a marine sediment core in the Indian sector of the SO over the last ∼410 kyrs. The δ18O stratigraphy is consistent with the dust correlation within their chronological uncertainties, supporting the reliability of the latter chronology for glacial–interglacial timescales. However, the dust correlation often produces older ages than the δ18O stratigraphy by up to 3 kyrs (410–126 ka and 84–50 ka). We additionally compiled, based on dust correlation, available dust proxy records in the circum-Antarctic SO for the last 450 kyrs to discuss variations in the dust proxy record within the Indian sector and between all three sectors. For the Indian sector, there is a marked difference in dust proxy signals for Marine Isotope Stage (MIS) 6 between two cores that have markedly different latitudinal positions relative to the oceanic fronts. Increased biogenic magnetite production by iron fertilization in the Subantarctic Zone during MIS 6 may partly explain the difference between the two cores. For the circum-Antarctic SO, moving correlation coefficients were computed between the marine sediment-core dust proxy signals and the dust flux of an Antarctic ice core. Strong correlation was recognized for intervals of high dust flux in the ice core, except for MIS 6. Although minor, the slightly lower correlation in the Indian sector than in the other sectors indicates a contribution from local dust source and volcanic materials and thus suggests the necessity for caution when performing dust correlation in the Indian sector of the SO.

Geochemistry and granulometry as indicators of paleoclimate, weathering, and provenance of sediments for the past 1,00,000 years in the eastern Arabian Sea

• Climate during MIS1, 3, 5a & 5c was hot and humid with intense SWM than YD, LGM, MIS2, 4, 5b. • Source area has experienced moderate to intense chemical weathering. • Provenance of sediments was felsic rocks during warm periods and mafic rocks and dust during cold periods. • Sources of sediments are ∼50% basalt , 40–80% gneiss and 10–20% dust. • Climate of lower and higher latitudes suggests inter-regional teleconnections . Geochemical and granulometric investigation of a 408 cm long sediment core raised from the Eastern Arabian Sea was carried out to decipher the climate, weathering, dust flux and provenance of sediments during the past 100 ka. The diagnostic ratio of Cr/Ni (0.99 to 1.77), Rb/Al (6.01 to 17.14), Ti/Al (0.02 to 0.03), Fe/Al (0.94 to 1.61), Mg/Al (0.31 to 0.59) and silt% (38.68 to 66.37) indicate hot and humid climate with the intensification of south-west monsoon during marine isotope stage (MIS) 1, 3, 5a and 5c and cold and dry climate with the intensification of the northeast monsoon and high dust flux during Younger Dryas cooling, last glacial maximum, MIS 2, 4 and 5b. The clay% (20.42 to 53.92), Silica–Titanium Index (71.88 to 86.28), Ruxton Ratio (2.89 to 7.22), and Th/U ratio (0.98 to 4.11) indicate moderate to intense chemical weathering in the source area during warmer climate. Th(ppm) versus Sc(ppm), La/Th versus Th/Yb, Al 2 O 3 % versus Fe 2 O 3 %, Th/Sc versus Sc(ppm), La/Sc versus Sc/Th ratios and La-Th-Sc plot indicate intermediate/mixed sources for sediment provenance. Sand% (2.82 to 25.3), Si/Al (2.74 to 7.43), ΣLREE/ΣHREE (7.65 to 10.40), La/Sc (2.24 to 3.55) indicate felsic sources from Peninsular India during warm climates and ΣREE (103.98–201.17), Rb/Ga (1.36–4.33), Ni (70.42–137.3 ppm), Rb (55.39–138.90 ppm) indicate mafic sources from Deccan Traps and Arabian desert during cold climates. The synchronous relationship between the climate of lower and higher latitudes was observed, suggesting the global teleconnections of climate during the Late Quaternary.

Contemporary and future dust sources and emission fluxes from gypsum- and quartz-dominated eolian systems, New Mexico and Texas, USA

AbstractRecent research on dust emissions from eolian dunes seeks to improve regional and global emissions estimates and knowledge of dust sources, particularly with a changing climate. Dust emissions from dune fields can be more accurately estimated when considering the whole eolian system composed of active to stabilized dunes, interdunes, sand sheets, and playas. Each landform can emit different concentrations of dust depending on the supply of silt and clay, soil surface characteristics, and the degree to which the landforms are dynamic and interact. We used the Portable In Situ Wind Erosion Laboratory (PI-SWERL) to measure PM10 (particulate matter <10 μm) dust emission potential from landforms in two end-member eolian systems: the White Sands dune field in New Mexico (USA), composed of gypsum, and the Monahans dune field in west Texas, composed of quartz. White Sands is a hotspot of dust emissions where dunes and the adjacent playa yield high dust fluxes up to 8.3 mg/m2/s. In contrast, the active Monahans dunes contain 100% sand and produce low dust fluxes up to 0.5 mg/m2/s, whereas adjacent stabilized sand sheets and dunes that contain silt and clay could produce up to 17.7 mg/m2/s if reactivated by climate change or anthropogenic disturbance. These findings have implications for present and future dust emission potential of eolian systems from the Great Plains to the southwestern United States, with unrealized emissions of >300 t/km2/yr.

Atmospheric dust flux in northeastern Gondwana during the peak of the late Paleozoic ice age

The silicate mineral fraction of shallow marine carbonates archives dust contributions to the Central Persian Terranes along the northeastern margin of Gondwana (∼30ºS paleolatitude), enabling reconstruction of atmospheric dust loading and circulation for intervals of the late Paleozoic ice age. The Central Persian Terranes hosted cyclic deposition of warm water carbonates from middle Pennsylvanian to earliest Permian time, and our data set includes two ∼28 m sections from the Moscovian and Asselian sampled at 20 cm intervals. Bounding surfaces between successive cycles (high-frequency sequences) are recognized by either abrupt basinward shifts in facies or subtle exposure features; these high-frequency sequences range from 1 m to 5 m thick and are interpreted to record glacioeustatic variations. Time series analysis of the dust fraction through the studied interval supports the hypothesis of orbital forcing for the dust signal. The stratigraphic pattern of the dust flux indicates minimal flux during interglacial highstands (0.19−0.27 g/cm2/kyr) and peak flux during glacial lowstands (3.77−4.57 g/cm2/kyr) after accounting for hiatal time at sequence boundaries. Grain size analysis of the dust for all samples (n = 230) reveals modal sizes (volume-based) of 1−15 µm through the Moscovian interval and 10−75 µm through the Asselian interval. Dust deposition increased during glacial times relative to interglacial times by a factor of 16 to 19. Additionally, the Asselian interval exhibits higher dust flux overall relative to the Moscovian interval, which is interpreted to reflect the more extreme icehouse conditions of the Asselian. Variation in the dust content through the studied sections provides an indicator of temporal changes in atmospheric loading that varied at both glacial−interglacial and higher-frequency (<104 yr) scales. Geochemical data reveal that the Arabian−Nubian Shield and southwestern Pangaea (South America) are the most likely sources of dust deposition in the Central Persian Terranes, with sources shifting during different phases. Increased dust flux during glacials likely reflects multiple factors, including enhanced aridity in the source region, exposure of shelf regions, and potential changes in winds. However, the discrepancy in model reconstructions of the amplitude of glacial−interglacial dust variations indicates that increased production of dust sourced by dynamic glaciation played a large role in enhancing dust flux during glacial phases.

Quartz OSL chronology of the loess deposits in the Western Qinling Mountains, China, and their palaeoenvironmental implications since the Last Glacial period

Extensive loess deposits exist in the Western Qinling Mountains (WQM), which constitute the transition zone between the Tibetan Plateau and the Chinese Loess Plateau (CLP). These deposits are one of the most important terrestrial archives regarding past dust activity and environmental changes in East Asia; however, they remain insufficiently known and poorly understood. Herein, we conducted detailed quartz optically stimulated luminescence dating and multi‐proxy analysis on the Zhouqu loess sequence. Our results show that the loess on the high terrace of the Bailong River started to accumulate by at least ~60 ka. The mass accumulation rate (MAR) in Zhouqu significantly varied during the Last Glacial period. The Marine Isotope Stage (MIS) 3 MARs were relatively high and stable. The highest MAR occurred in MIS 2, with peak MARs during 25–19 ka, and it decreased with rapid changes during the Holocene. The discrepancy in the MARs of the WQM loess since the Last Glacial period compared with the rates in the CLP may imply different dust deposition processes in the WQM. The reconstructed palaeoenvironmental records indicate climate changes with warm‐moist climate patterns and low dust flux in interglacial periods and cold‐dry conditions with high dust flux in glacial periods, consistent with those on the CLP. The results contribute to better understanding of the linkages between dust accumulation and climate change in the WQM area.

Insight Into Provenance and Variability of Atmospheric Dust in Antarctic Ice Cores During the Late Pleistocene From Magnetic Measurements

We measured saturation isothermal remanent magnetization (SIRM), coercivity of remanence (Hcr) and insoluble dust concentration (IDC) of 52 ice samples from Vostok and EPICA Dome-C ice cores (Antarctica) as a measure of magnetic properties of the aerosol dust entrapped in the ice. Samples range in age from marine isotopic stage (MIS) 7 to 19 in EPICA Dome-C ice core and from MIS 1 to 11 in Vostok ice core. Data from ice samples were compared with 86 samples from possible source areas (PSA) from East Antarctica, and 10 samples from South America and New Zealand. Previous results from MIS 1 to MIS 6 found that magnetic properties of aerosol dust could be divided in two distinct groups characterized by high-Hcr and low-SIRMdust for glacial samples, and low-Hcr and high-SIRMdust, for interglacial samples. The new data from older ice samples highlighted several discrepancies from this expectation with significant differences between Vostok and Dome-C sites. Magnetic properties of Antarctic PSA sample show a large variability, however PSA samples from Victoria Land and few other, have magnetic properties compatible with that of the glacial dust, or more precisely with samples characterized by high dust flux. The new data from Pleistocene ice and from PSA samples confirm the South American and Antarctic provenance of the largest atmospheric dust load typical of glacial stages. On the other hand, we did not found any PSA sample with properties compatible with the highly magnetic samples (mostly from interglacial stages), which are characterized by low IDC. These samples from the oldest and deepest part of the cores revealed a more complex picture than previously outlined from the analysis of MIS 1–6, and show unusual magnetic properties which can be tentatively attributed to chemical.

Hints of a Population of Solar System Analog Planets from ALMA

Abstract The recent Atacama Large Millimeter/submillimeter Array (ALMA) Disk Substructures at High Angular Resolution Project (DSHARP) survey provided illuminating results on the diversity of substructures in planet-forming disks. These substructures trace pebble-sized grains accumulated at local pressure maxima, possibly due to planet–disk interactions or other planet formation processes. DSHARP sources are heavily biased to large and massive disks that only represent the high (dust flux) tail end of the disk population. Thus it is unclear whether similar substructures and corresponding physical processes also occur in the majority of disks that are fainter and more compact. Here we explore the presence and characteristics of features in a compact disk around GQ Lup A, the effective radius of which is 1.5–10 times smaller than those of DSHARP disks. We present our analysis of ALMA 1.3 mm continuum observations of the GQ Lup system. By fitting visibility profiles of the continuum emission, we find substructures including a gap at ∼10 au. The compact disk around GQ Lup exhibits similar substructures to those in the DSHARP sample, suggesting that mechanisms of trapping pebble-sized grains are at work in small disks as well. Characteristics of the feature at ∼10 au, if due to a hidden planet, are evidence of planet formation at Saturnian distances. Our results hint at a rich world of substructures to be identified within the common population of compact disks, and subsequently a population of solar system analogs within these disks. Such study is critical to understanding the formation mechanisms and planet populations in the majority of protoplanetary disks.

Dust deposition tracks late-Holocene shifts in monsoon activity and the increasing role of human disturbance in the Puna-Altiplano, northwest Argentina

The Puna-Altiplano plateau represents a regionally significant dust source, which is critically located at the nexus between the tropical and sub-polar synoptic systems that dominate the South American climate. Dust emissions in this region would therefore be expected to be sensitive to changes in these systems, in particular the strength and position of the South American Summer Monsoon (SASM). Here, we present a late-Holocene multi-proxy study where changes in dust flux, reconstructed from a high-altitude peat mire, are examined in light of climate variability and human impacts. Results show that for most the 4300 cal. yr BP record, dust flux sensitively tracked changes in SASM activity. Prior to 2600 cal. yr BP relatively high dust flux implies dry conditions prevailed across the Puna-Altiplao in association with reduced SASM activity. The chemistry of dust deposited at this time matched the large endorheic basins on the Puna, which host ephemeral lakes and terminal fans, indicating these were actively supplying dust to the airstream. After 2600 cal. yr BP, SASM activity increased while dust flux decreased and the dust chemistry changed, collectively implying the shutting down of the Puna-Altiplano as a significant dust source. Dust flux increased after 1000 cal. yr BP during the ‘Medieval Warm Period’, associated with a return to drier conditions and reactivation of dust sources across the endorheic basins of the Puna. Natural variability in dust flux was dwarfed, however, by the very significant increase in flux after 400 cal. yr BP following Spanish Colonisation and associated changing landuse practices. This finding attests to the globally significant role of humans on dust emissions.

An Observational Overview of Dusty Deep Convection in Martian Dust Storms.

Deep convection, as used in meteorology, refers to the rapid ascent of air parcels in the Earth's troposphere driven by the buoyancy generated by phase change in water. Deep convection undergirds some of the Earth's most important and violent weather phenomena and is responsible for many aspects of the observed distribution of energy, momentum, and constituents (particularly water) in the Earth's atmosphere. Deep convection driven by buoyancy generated by the radiative heating of atmospheric dust may be similarly important in the atmosphere of Mars but lacks a systematic description. Here we propose a comprehensive framework for this phenomenon of dusty deep convection (DDC) that is supported by energetic calculations and observations of the vertical dust distribution and exemplary dusty deep convective structures within local, regional, and global dust storm activity. In this framework, DDC is distinct from a spectrum of weaker dusty convective activity because DDC originates from pre-existing or concurrently forming mesoscale circulations that generate high surface dust fluxes, oppose large-scale horizontal advective-diffusive processes, and are thus able to maintain higher dust concentrations than typically simulated. DDC takes two distinctive forms. Mesoscale circulations that form near Mars's highest volcanoes in dust storms of all scales can transport dust to the base of the upper atmosphere in as little as two hours. In the second distinctive form, mesoscale circulations at low elevations within regional and global dust storm activity generate freely convecting streamers of dust that are sheared into the middle atmosphere over the diurnal cycle.

Constraints on aragonite precipitation in the Dead Sea from geochemical measurements of flood plumes

The laminated sequences of the Holocene Dead Sea (DS) and its late Pleistocene precursor Lake Lisan comprise primary aragonite and fine detritus that record the hydro-climate conditions of the late Quaternary Levant. Several studies suggested that the primary aragonite precipitated due to mixing between runoff that brought bicarbonate to the lake and the lake's Ca-chloride brine. However, the factors controlling the aragonite precipitation were not robustly established. Here, we addressed this issue by measuring the chemical composition (pH, Na+, K+, Ca2+, Mg2+, Sr2+, Cl−, Br−, B, alkalinity) of flood plumes where the mixing occurs. The results indicate that: (a) Na+, Mg2+, K+ and Cl− are conservative during the floodwater-brine mixing whereas Ca2+ and Sr2+ adsorb on flood's suspended sediments; (b) Boron (an important alkalinity species in the DS) adsorption on flood's suspended load enabled the bicarbonate that entered the lake via runoff to react with the Ca2+ thus facilitating aragonite precipitation (c) Dissolution of calcite dust blown from the Sahara during winter storm is the source of bicarbonate which is required for aragonite precipitation. These observations explain the occurrence of aragonite laminae both during the wet last glacial period and during the dry last 3000yr. Although the water input during these two periods was completely different, they both were characterized by high dust fluxes and a stratified lake configuration in which the boron concentrations in the epilimnion were low enough to enable the bicarbonate that entered the lake via runoff to react with the lake brine Ca2+ and precipitate aragonite.

Late Quaternary Soil Development Enhances Aeolian Landform Stability, Moenkopi Plateau, Southern Colorado Plateau, USA

The Moenkopi dune field in northeastern Arizona covers roughly 1250 km2, but most of the field is inactive. Dune deposits on the Moenkopi Plateau (MP) have remained inactive throughout the Holocene despite periods of elevated aridity or historical reductions of vegetation cover by livestock grazing. We argue that this inactivity is not because of any diminishment of driving forces in the aeolian system (e.g., insufficient winds), but rather because of increased cohesion due to soil development that enhances resistance to wind erosion. Abundant aeolian sediments were supplied to the Black Mesa region by the Little Colorado River and its tributaries during the late Pleistocene (MIS 2 and 3), which enabled the development of climbing dunes and transport of sand over the Adeii Eechii Cliffs and onto the MP. These deposits (Qe1) stabilized during the Pleistocene/Holocene climatic transition (~12–7.5 ka) because of reduced sediment supply and high dust flux which resulted in rapid soil formation. Erosion of climbing dunes/sand ramps from the Adeii Eechii Cliffs eliminated delivery of large quantities of new sand to the MP during the mid to late Holocene. Soil development within the Qe1 mantle increased sediment cohesion and prevented widespread aeolian reactivation during the Holocene, despite the occurrence of conditions (wind speed, climate, etc.) under which dune reactivation would be expected. Drylands comprise roughly 40% of the land cover of earth and climate models predict their expansion. Pedogenic stability is not commonly considered in climate-based models used to predict aeolian activity. To improve predictions of future dune activity in drylands, the degree of soil development in aeolian deposits should be considered when evaluating sediment availability in aeolian systems.

Atmospheric nutrients in seawater under current and high pCO2 conditions after Saharan dust deposition: Results from three minicosm experiments

The Mediterranean basin receives among the highest dust fluxes in the world ocean, and also appears to be one of the regions the most strongly impacted by ocean acidification. The aim of this study was to assess, on a short time scale (one-week), the effect of ocean acidification on the dissolution of nutrients (inorganic nitrogen, phosphate and iron) from Saharan dust. Three experiments were performed in three distinct seasons: in May, after the spring bloom with low autotrophic biomass, in September, at the end of the oligotrophic period, and in January, during the winter bloom. On each occasion, a dust flux of 10 g m−2 was simulated at the surface of two minicosms (tanks of ∼0.3 m3) filled with filtered (<0.2 µm) seawater collected in the Bay of Villefranche (NW Mediterranean Sea). One minicosm served as a control and the other was acidified to reach a partial pressure of CO2 (pCO2) close to that projected for the end of this century (∼1250 μatm). Following a high-resolution sampling protocol, results showed that whatever the season and in situ biogeochemical conditions (1) all nitrogen from dust was soluble in seawater, allowing a large and stable increase in the stock of NOx (nitrate + nitrite) under the two pCO2 conditions (ambient and future), (2) transient increases in dissolved iron and phosphate concentrations were driven by scavenging processes, with a low dissolution percentage averaging 0.14 ± 0.08 and 4.7 ± 1.2%, respectively. While the absence of pCO2 effects on the release of atmospheric nitrogen was confirmed in the present study, no clear conclusion could be drawn for phosphate and dissolved iron as a consequence of very low concentrations and rapid (within less than 1 h) dissolved-particulate exchanges. Nevertheless, as the lifetime of these elements in solution is limited to a few hours, whatever the pH conditions, our results suggest that ocean acidification would have only a minor impact on their bioavailability for surface phytoplankton communities in such Low Nutrient Low Chlorophyll areas.

Early-Holocene greening of the Afro-Asian dust belt changed sources of mineral dust in West Asia

Production, transport and deposition of mineral dust have significant impacts on different components of the Earth systems through time and space. In modern times, dust plumes are associated with their source region(s) using satellite and land-based measurements and trajectory analysis of air masses through time. Reconstruction of past changes in the sources of mineral dust as related to changes in climate, however, must rely on the knowledge of the geochemical and mineralogical composition of modern and paleo-dust, and that of their potential source origins. In this contribution, we present a 13,000-yr record of variations in radiogenic Sr–Nd–Hf isotopes and Rare Earth Element (REE) anomalies as well as dust grain size from an ombrotrophic (rain fed) peat core in NW Iran as proxies of past changes in the sources of dust over the interior of West Asia. Our data shows that although the grain size of dust varies in a narrow range through the entire record, the geochemical fingerprint of dust particles deposited during the low-flux, early Holocene period (11,700–6,000 yr BP) is distinctly different from aerosols deposited during high dust flux periods of the Younger Dryas and the mid-late Holocene (6,000–present). Our findings indicate that the composition of mineral dust deposited at the study site changed as a function of prevailing atmospheric circulation regimes and land exposure throughout the last deglacial period and the Holocene. Simulations of atmospheric circulation over the region show the Northern Hemisphere Summer Westerly Jet was displaced poleward across the study area during the early Holocene when Northern Hemisphere insolation was higher due to the Earth's orbital configuration. This shift, coupled with lower dust emissions simulated based on greening of the Afro-Asian Dust Belt during the early Holocene likely led to potential sources in Central Asia dominating dust export to West Asia during this period. In contrast, the dominant western and southwest Asian and Eastern African sources have prevailed during the mid-Holocene to modern times.

Increasing dust fluxes on the northeastern Tibetan Plateau linked with the Little Ice Age and recent human activity since the 1950s

Arid and semi-arid areas in inner Asia contribute lots of mineral dust in the northern hemisphere, but dust flux evolution in the past is poorly constrained. Based on particle sizes and elemental compositions of a sediment core from Lake Qinghai on the northeastern Tibetan Plateau, dust fluxes during ∼1518–2011 A.D. were reconstructed based on 18–100 μm fractions of the lake sediment. The dust fluxes during the past ∼500 years ranged between 100 and 300 g/m2/yr, averaging 202 g/m2/yr, experiencing four stages: Stage 1 (∼1518–1590s), the flux was averaged 165 g/m2/yr, much lower than that in the Stage 2 (1590s–1730s, 254 g/m2/yr); similarly, an average flux of 169 g/m2/yr in the Stage 3 (1730s–1950s) was followed by an increased flux of 259 g/m2/yr in the Stage 4 (1950s–2011). During the first three stages the fluxes were dominated by natural dust activities in arid inner Asia, having a positive relation with wind intensity but a poor correlation with effective moisture (or precipitation) and temperature. The high dust flux in Stage 2 was due to relatively strong wind during the maximum Little Ice Age, whereas the remarkably high flux in 1950s–2011 was resulted from recent increasing human activities in northwestern China. The dust record not only documents past dust fluxes on the northeastern Tibetan Plateau but also reflects evolutions and mechanisms of dust activity/emission in inner Asia during the past ∼500 years.

Late-Holocene atmospheric dust deposition in eastern Canada (St. Lawrence North Shore)

Dust deposition in two ombrotrophic peatlands (Baie and Ile du Havre peatland (IDH) bogs) of the Estuary and Gulf of the St. Lawrence in eastern Canada was reconstructed using elemental geochemistry. The rare earth elements (REEs) and other lithogenic element concentrations were measured by ICP-oES and Q-ICP-MS along two peat cores spanning the last 4000 years. Principal component analyses on the geochemical profiles show that REEs display the same behavior as Al, Ti, Sc, and Zr, all conservative elements, which suggests that REEs are immobile in the studied peat bogs and can be used as tracers of dust deposition. Plant macrofossils were also used to infer past environmental and humidity changes. The dust fluxes were reconstructed using the sum of REEs (ΣREE). The range of dust deposition varies from 0.2 to 3.8 g m−2 yr−1 in the Baie bog, while the IDH bog shows lower fluxes ranging between 0.1 and 1.2 g m−2 yr−1. The highest dust fluxes in the Baie bog were recorded from 1750–1000 cal. BP to 600–100 cal. BP and occur at the same time as periods of high variability in the macrofossil record (i.e. successive layers dominated by Sphagnum or Ericaceae). The timing of these events in the dust and macrofossil records also corresponds to documented cold periods. These two periods have been identified as episodes of climatic instability, which could have been caused by changes in the wind regime.

Extreme eolian delivery of reactive iron to late Paleozoic icehouse seas

The biogeochemical impacts of iron-rich dust to the oceans are known for Earth’s recent record but unexplored for deep time, despite recognition of large ancient dust fluxes, particularly during the late Paleozoic. We report a unique Fe relationship for Upper Pennsylvanian mudrock of eolian origin that records lowstand (glacial) conditions within a carbonate buildup of western equatorial Pangaea (western United States) well removed from other detrital inputs. Here, reactive Fe unambiguously linked to dust is enriched without a corresponding increase in total Fe. More broadly, data from thick coeval loess deposits of western equatorial Pangaea show the same marked enrichment in reactive Fe. This enrichment—atypical compared to modern marine, fluvial, glacial, loess, and soil sediments—suggests an enhancement of the reactivity of the internal Fe pool that increased the bioavailability of the Fe for marine primary production. Regardless of the mechanism behind this enhancement, our data in combination with other evidence for high dust fluxes imply delivery of extraordinarily large amounts of biogeochemically reactive Fe to glacial-stage late Paleozoic seas, and modeling of this indicates major impacts on carbon cycling and attendant climatic feedbacks.

Centennial-scale variability of the Southern Hemisphere westerly wind belt in the eastern Pacific over the past two millennia

Abstract. We present the first high-resolution (sub-annual) dust particle data set from West Antarctica, developed from the West Antarctic Ice Sheet (WAIS) Divide deep ice core (79.468° S, 112.086° W), and use it to reconstruct changes in atmospheric circulation over the past 2400 years. We find a background dust flux of ~4 mg m−2 year−1 and a mode particle size of 5–8 μm diameter. Through comparing the WAIS Divide record with other Antarctic ice core particle records, we observe that coastal and lower-elevation sites have higher dust fluxes and coarser particle size distributions (PSDs) than sites on the East Antarctic plateau, suggesting input from local dust sources at these lower-elevation sites. In order to explore the use of the WAIS Divide dust PSD as a proxy for past atmospheric circulation, we make quantitative comparisons between both mid-latitude zonal wind speed and West Antarctic meridional wind speed and the dust size record, finding significant positive interannual relationships. We find that the dust PSD is related to mid-latitude zonal wind speed via cyclonic activity in the Amundsen Sea region. Using our PSD record, and through comparison with spatially distributed climate reconstructions from the Southern Hemisphere (SH) middle and high latitudes, we infer that the SH westerlies occupied a more southerly position from circa 1050 to 1400 CE (Common Era), coinciding with the Medieval Climate Anomaly (MCA). Subsequently, at ca. 1430 CE, the wind belt shifted equatorward, where it remained until the mid-to-late twentieth century. We find covariability between reconstructions of El Niño–Southern Oscillation (ENSO) and the mid-latitude westerly winds in the eastern Pacific, suggesting that centennial-scale circulation changes in this region are strongly influenced by the tropical Pacific. Further, we observe increased coarse particle deposition over the past 50 years, consistent with observations that the SH westerlies have been shifting southward and intensifying in recent decades.

Mid- and late Holocene dust deposition in western Europe: the Misten peat bog (Hautes Fagnes – Belgium)

Abstract. Dust deposition in southern Belgium is estimated from the geochemical signature of an ombrotrophic peatland. The rare earth elements (REE) and lithogenic elements concentrations, as well as Nd isotopes, were determined by HR-ICP-MS and MC-ICP-MS, respectively, along an ~6 m peat section covering 5300 yr, from 2000 to 7300 cal BP, dated by the 14C method. Changes in REE concentration in the peat correlate with those of Ti, Al, Sc and Zr that are lithogenic conservative elements, suggesting that REE are immobile in the studied peat bogs and can be used as tracers of dust deposition. Peat humification and testate amoebae were used to evaluate hydroclimatic conditions. The range of dust deposition varied from 0.03 to 4.0 g m−2 yr−1. The highest dust fluxes were observed from 2750 to 2550 cal BP and from 5150 to 4750 cal BP, and correspond to cold periods. The &amp;amp;varepsilon;Nd values show a large variability from −13 to −5, identifying three major sources of dusts: local soils, distal volcanic and desert particles.