High-density Beam Research Articles

Analysis and optimization of cesium dynamics for the HUST negative ion source

The high-density beam in the NBI negative ion source relies on surface production on the converter with low work function, which is facilitated by cesium injection. Maintaining the appropriate cesium conditions during the source operation sequence is essential for achieving optimal cesium coverage on the converter. To better understand cesium cycle in the source and to enhance beam production performance during operation sequences, analysis of cesium dynamics and optimization of cesium operation have been carried out. The analysis model is established based on the Monte-Carlo method with cesium sources, cesium transport and surface process during the operation sequence considered. Cesium distribution and converter surface coverage can be obtained from the model using input parameters from the HUST negative ion source. For the operation in the HUST negative ion source, the influence of temperature settings and time sequence is discussed, with suggested parameters for cesium injection proposed to achieve appropriate cesium coverage on converter surface through operation sequences.

Determining the carbon detection limit with magnetic sector dynamic secondary ion mass spectrometry (SIMS)

Dynamic SIMS is often used to evaluate the concentration of impurities in solids because of its high sensitivity, depth profiling capabilities, good depth resolution, and high throughput. Continuous ion beam sputtering with a high-density primary beam provides high sensitivity and reduces the background contribution from residual gases within the analytical chamber. Dynamic SIMS experiments performed with several magnetic sector instruments using various sputtering rate conditions demonstrated a slow decrease of the carbon detection limit with the increase of sputtering rate (SR), when it was varied by changing the sputtering beam density. The dependence data, within the scatter limits, can be fit by a power function of SR with the exponent of about −1/2. The observed detection-limit-dependence curve is common for magnetic sector SIMS instruments, owing to contamination and the design of the analytical chamber. The depth resolution of light-element SIMS analysis (except for oxygen) performed using Cs+ sputtering is limited and cannot be improved by reducing the impact energy of the sputtering beam. A segregation-type depth profile with a long trailing edge was observed in the B, C, and N depth profiles when Cs+ sputtering was employed under ultra-high vacuum conditions. This effect is plausibly associated with preferential sputtering owing to the difference in the surface binding energy, along with the large difference in the mass of the interacting atoms within the collision cascade during sputtering. The depth resolution improved with surface oxidation when Cs + sputtering was combined with backfilling of the analytical chamber using O2. The analytical chamber backfilled with oxygen can be sufficiently replaced with a very low-impact energy-focused oxygen beam, enabling simultaneous oxygen and cesium co-sputtering SIMS analysis. The practical feasibility of using a co-sputtering with focused Cs+ and O2+ sputtering beams to achieve a high depth-resolution for carbon analysis under ultrahigh vacuum conditions was demonstrated.

High-density quasi-monoenergetic proton beam generation from vacuum sandwiched target

An efficient scheme has been proposed for generating a high-density proton beam by enhancing the accelerating field from the interaction of an intense laser with a vacuum sandwiched target. The prime role of the vacuum gap is to reduce the effect of the sudden shock, exerted by the front edge of the intense laser, on the hydrogen layer. It is shown that the accelerated proton beam quality could be significantly enhanced due to the presence of the vacuum gap. We found that the total number of the accelerated protons is about 17.5 (1.7) and the proton beam peak is about 6.5 (3.7) times higher as compared to the single (double) layer target case. The dependence of the proton acceleration on the different layer thickness, density, and laser pulse intensity has also been studied.

The suitability of common reed (Phragmites australis) for load-bearing structural materials

Besides wood, the most widely used natural structural material, dicotyledonous fibre plants such as flax or hemp, and monocotyledonous grasses such as cereal straw or bamboo have been shown to be suitable for application in materials. Common reed is a less well-characterised plant resource in this regard. Therefore, common reed stems were characterised in uniaxial tension in the present study, aiming at acquiring basic information about the mechanical characteristics of this material. Furthermore, laboratory-scale composite beams were manufactured and tested in bending. Compared to wood species with similar density, common reed stem walls showed a comparable average modulus of elasticity of 8 GPa and a very good average tensile strength of 150 MPa. After a mild alkali pre-treatment, reed showed excellent adhesive bonding, enabling the manufacture of high-density composite beams with roughly 130 MPa bending strength and 12–13 GPa modulus of elasticity. Same as untreated common reed stem walls, also reed biocomposite beams compared very favourably with established wood-based materials of similar structure, density, and adhesive content. In summary, it was thus demonstrated that common reed is a highly suitable raw material for bio-based load-bearing structural materials.

Improvement of miniaturized 2.45 GHz ECR plasma flood gun at PKU

In an ion implanter, plasma flood gun (PFG) is used to provide electrons to neutralize the accumulated charge on the wafer surface to avoid breakdown damage. With the development of ion implantation technology, four key requirements have been put forward for PFG. They are simple structure, plasma with high density and low electron temperature, no metal contamination and long life. The existing PFG, such as the filament type PFG, can hardly meet the above requirements at the same time. 2.45 GHz ECR ion source with the advantages of high beam density, high stability, long life time and no filament metal contamination, has shown great potential to work as PFG. Recently, a miniaturized 2.45 GHz permanent magnet electron cyclotron resonance PFG (PMECR-PFG) has been developed at Peking University (PKU). In our previous test, 8.8 mA electron extraction current was obtained with argon gas. In this work, by optimizing the magnetic field configuration to a resonant configuration, the performance of this ECR-PFG was greatly improved. With 100 W microwave power, an 80 mA electron current load was obtained under the extraction voltage of 0.1 kV. To minimize the metal contamination, a three-slit graphite plasma electrode was fabricated and a 50 mA load was generated at only 30 W RF power. During all tests, the gas consumption rate is lower than 0.6 sccm, which is beneficial to maintain the vacuum of implanter beamline.

Determining the oxygen detection limit with magnetic sector dynamic secondary ion mass spectrometry (SIMS)

Dynamic SIMS is often used in evaluating the concentration of impurities in solids because of its high sensitivity and depth profiling capabilities with good depth resolution and high throughput. Continuous ion beam sputtering with a high-density primary beam provides high sensitivity and reduced background contribution from residual gases within the analytical chamber. Numerical simulations along with the data acquired in the real depth profiling experiment show a good agreement of the simple model, assuming that the surface uptake of the oxygen under Cs bombardment depends on the Cs surface retention concentration. In cases where high depth resolution is desired, requiring a low primary ion beam energy, a background subtraction option will help provide better detection limits. It is proposed to perform the background subtraction based on the difference between the continuous and interleaving sputtering modes of dynamic SIMS. The experiments performed on different instruments using different sputtering rate conditions (and different impact energies) show the power function dependence of oxygen detection limit on the reversed sputter rate variation or sputtering beam density. The proposed detection limit dependence curve can be used for analytical specifications benchmarking in most magnetic sector SIMS instruments.

Combined ARFI and Shear Wave Imaging of Prostate Cancer: Optimizing Beam Sequences and Parameter Reconstruction Approaches.

This study demonstrates the implementation of a shear wave reconstruction algorithm that enables concurrent acoustic radiation force impulse (ARFI) imaging and shear wave elasticity imaging (SWEI) of prostate cancer and zonal anatomy. The combined ARFI/SWEI sequence uses closely spaced push beams across the lateral field of view and simultaneously tracks both on-axis (within the region of excitation) and off-axis (laterally offset from the excitation) after each push beam. Using a large number of push beams across the lateral field of view enables the collection of higher signal-to-noise ratio (SNR) shear wave data to reconstruct the SWEI volume than is typically acquired. The shear wave arrival times were determined with cross-correlation of shear wave velocity signals in two dimensions after 3-D directional filtering to remove reflection artifacts. To combine data from serially interrogated lateral push locations, arrival times from different pushes were aligned by estimating the shear wave propagation time between push locations. Shear wave data acquired in an elasticity lesion phantom and reconstructed using this algorithm demonstrate benefits to contrast-to-noise ratio (CNR) with increased push beam density and 3-D directional filtering. Increasing the push beam spacing from 0.3 to 11.6 mm (typical for commercial SWEI systems) resulted in a 53% decrease in CNR. In human in vivo data, this imaging approach enabled high CNR (1.61-1.86) imaging of histologically-confirmed prostate cancer. The in vivo images had improved spatial resolution and CNR and fewer reflection artifacts as a result of the high push beam density, the high shear wave SNR, the use of multidimensional directional filtering, and the combination of shear wave data from different push beams.

Topological structure effects of Laguerre-Gaussian laser on self-collimation acceleration mechanism

Energetic plasma beams can be generated through the interaction between a short-pulse high-intensity laser and solid target. However, obtaining collimated plasma beams with low divergence remains challenging. In this study, we devised a self-collimation scheme driven by a topologically structured Laguerre–Gaussian (LG) laser that irradiates a thin target in three-dimensional particle-in-cell simulations. It was observed that a high-density and narrow plasma beam could be formed by the intrinsic hollow intensity distribution of the LG laser. A magnetic tunnel was generated around the beam and collimated the plasma beam within a radius of hundreds of nanometers. This collimation can be enhanced by increasing the topological charge from l = 1 to l = 3 and then destroyed for a larger l. The collimation method is promising in applications requiring well-collimated energetic plasma beams, such as indirect drive inertial con-finement fusion, laboratory astrophysics, and radiation therapy.

Demonstration of the X-ray imaging capabilities of the newly installed multilayer monochromator at SPring-8 BL20B2

Double multilayer monochromators (DMMs) for 40 keV and 110 keV have been installed at BL20B2 in SPring-8. The DMMs provide X-rays with a few percent bandwidths at those energies. The flux density of the X-rays is more than several hundred times higher than that of monochromatic X-rays with a silicon double crystal monochromator, which enables us to perform high-speed X-ray imaging with a large field of view and high spatial resolution X-ray imaging in those high-energy X-rays. Here characteristics of DMMs and some demonstrations of X-ray imaging using the high flux density beams are shown.

Conceptual Design of a Compact Divertor Heat Load Simulation Device: HIT-PSI

Linear plasma devices have been increasingly applied in investigating plasma–surface interaction (PSI) processes and divertor/scraped-off-layer (D/SOL) physics because of their economy, flexibility, and expandability. However, only a few existing linear plasma devices are able to obtain high heat and particle fluxes. In this work, we report a compact superconducting linear device, with its scientific goals and specific design methods, at Harbin Institute of Technology (HIT), HIT-PSI, capable of implementing an extreme plasma environment with beams of a long discharge pulse, as well as high heat and particle fluxes in the future fusion reactor regime of ITER/CFETR-like parameters. A five-coil integrated superconducting magnet is designed to generate a >2.0 Tesla steady-state magnetic field for confining a long pulse plasma beam with a density of >1020 m−3 produced by a cascaded arc plasma source. With a pump set of 2500 L/s and a water-cooled target system with bias voltage, it is expected to obtain high-density and low-temperature plasma beams with a heat flux of over 10 MW/m2. Subsystems of the platform, including the plasma source, superconducting magnets, vacuum system, and target holder system, are described in detail. In addition, the function and performance of the platform are numerically simulated and represented by SOLPS-ITER code to predict the laboratory simulation results.

An automated liquid jet for fluorescence dosimetry and microsecond radiolytic labeling of proteins

X-ray radiolytic labeling uses broadband X-rays for in situ hydroxyl radical labeling to map protein interactions and conformation. High flux density beams are essential to overcome radical scavengers. However, conventional sample delivery environments, such as capillary flow, limit the use of a fully unattenuated focused broadband beam. An alternative is to use a liquid jet, and we have previously demonstrated that use of this form of sample delivery can increase labeling by tenfold at an unfocused X-ray source. Here we report the first use of a liquid jet for automated inline quantitative fluorescence dosage characterization and sample exposure at a high flux density microfocused synchrotron beamline. Our approach enables exposure times in single-digit microseconds while retaining a high level of side-chain labeling. This development significantly boosts the method’s overall effectiveness and efficiency, generates high-quality data, and opens up the arena for high throughput and ultrafast time-resolved in situ hydroxyl radical labeling.

Characterization of overlapping betatron resonances above the phase advance of 90° per cell

The space-charge-induced resonance band just above the betatron phase advance of 90\ifmmode^\circ\else\textdegree\fi{} per cell is of great practical importance. The instability is closely related to the linear collective mode and can thus give rise to severe emittance growth at high beam density. In a circular machine, this type of second-order resonance occurs not only at half-integer tunes but also near quarter-integer tunes, depending on the lattice superperiodicity. Self-consistent numerical simulations are carried out to elucidate the resonance feature above the 90\ifmmode^\circ\else\textdegree\fi{} cell tune. The present results suggest the existence of three different resonance mechanisms working there; namely, the fourth-order incoherent resonance in the beam tail, the second-order and fourth-order coherent resonances in the beam core. It is reconfirmed that no serious emittance growth occurs even if particles deep inside the core satisfy the incoherent resonance condition. The recently proposed stop-band diagram, free from the concept of incoherent tune spread, appears to be consistent with the numerical observations.

Synergetic combination of photoluminescence spectroscopy with microsecond X-ray footprinting

X-ray Footprinting uses broadband X-rays for in situ hydroxyl radical labeling to map protein interactions and conformation. High flux density beams are essential to overcome radical scavengers and enhance labeling efficiency. However, conventional sample delivery environments, such as capillary-flow, burns and breaks under the high power density of an unattenuated focused X-ray broadband beam. An alternative is to use a liquid jet, and we have previously demonstrated that use of this container-less form of sample delivery can increase labeling by tenfold at an unfocused X-ray source.

Optimizing the geometry of aerodynamic lens injectors for single-particle coherent diffractive imaging of gold nanoparticles.

Single-particle X-ray diffractive imaging (SPI) of small (bio-)nanoparticles (NPs) requires optimized injectors to collect sufficient diffraction patterns to allow for the reconstruction of the NP structure with high resolution. Typically, aerodynamic lens-stack injectors are used for NP injection. However, current injectors were developed for larger NPs (>100 nm), and their ability to generate high-density NP beams suffers with decreasing NP size. Here, an aerodynamic lens-stack injector with variable geometry and a geometry-optimization procedure are presented. The optimization for 50 nm gold-NP (AuNP) injection using a numerical-simulation infrastructure capable of calculating the carrier-gas flow and the particle trajectories through the injector is also introduced. The simulations were experimentally validated using spherical AuNPs and sucrose NPs. In addition, the optimized injector was compared with the standard-installation 'Uppsala injector' for AuNPs. Results for these heavy particles showed a shift in the particle-beam focus position rather than a change in beam size, which results in a lower gas background for the optimized injector. Optimized aerodynamic lens-stack injectors will allow one to increase NP beam density, reduce the gas background, discover the limits of current injectors and contribute to structure determination of small NPs using SPI.

Concept and application of a linearized ring multipass optics configuration.

A multipass optics (MPO) system is used to increase the optical path length in a limited volume. Well-known concepts such as the White-type cell and the Herriott-type cell are used in many applications. The optical path in these cells leaves a large portion of the cell volume unused. In contrast, MPO systems with astigmatic mirrors have significantly more beam passes per volume, but because of their reduced symmetry along the beam axis they are much more sensitive to misalignment. Our goal is to develop MPO systems that have both: the high beam densities of astigmatic MPO systems and the optical robustness of Herriott-type optics. We show that linearized optical ring resonators, which can be constructed by means of simple 2×2 optical ABCD-matrices, lead to suitable solutions. The concept is demonstrated using a MPO system with a base length of 150 mm and a total beam path length of 19.2 m, optimized for laser beams of 10 µm wavelength. The volume of the cell is 295cm3 with a beam density that is four times higher compared to a standard Herriott-type cell.

High density molecular jets of complex neutral organic molecules with Tesla valves.

Supersonic jets of gas-phase atoms and small molecules have enabled a variety of ultrafast and ultracold chemical studies. However, extension to larger, more complex neutral molecules proves challenging for two reasons: (i) Complex molecules, such as cis-stilbene, exist in a liquid or solid phase at room temperature and ambient pressure and (ii) a unidirectional flow of high-density gaseous beams of such molecules to the interaction region is required. No delivery system currently exists that can deliver dense enough molecular jets of neutral complex molecules without ionizing or exciting the target for use in gas-phase structural dynamics studies. Here, we present a novel delivery system utilizing Tesla valves, which generates more than an order-of-magnitude denser gaseous beam of molecules compared to a bubbler without Tesla valves at the interaction region by ensuring a fast unidirectional flow of the gaseous sample. We present combined experimental and flow simulations of the Tesla valve setup. Our results open new possibilities of studying large complex neutral molecules in the gas-phase with low vapor pressures in future ultrafast and ultracold studies.

Velocity-tunable beam of continuously decelerated polar molecules for cold ion-molecule reaction studies.

Producing high densities of molecules is a fundamental challenge for low-temperature, ion-molecule reaction studies. Traveling-wave Stark decelerators promise to deliver high density beams of cold, polar molecules but require non-trivial control of high-voltage potentials. We have overcome this experimental challenge and demonstrate continuous deceleration of ND3 from 385 to 10m/s, while driving the decelerator electrodes with a 10 kV amplitude sinewave. In addition, we test an alternative slowing scheme, which increases the time delay between decelerated packets of ND3 and non-decelerated molecules, allowing for better energy resolution of subsequent reaction studies. We characterize this source of neutral, polar molecules suitable for energy-resolved reaction studies with trapped ions at cold translational temperatures. We also propose a combined apparatus consisting of the traveling-wave decelerator and a linear ion trap with a time-of-flight mass spectrometer and discuss to what extent it may achieve cold, energy-resolved, ion-neutral reactions.

Measurement of propagation of local and minute contractile response in layered myocardium

The in vivo measurement of the contractile response caused by electrical excitation has been studied to detect myocardial ischemia in its early stages. In the present study, we used our previously proposed local velocity estimator to measure the two-dimensional distribution of the strain rate using high-density beam scanning to obtain propagation of the local and minute contractile response in the heart walls of healthy humans. Alternate layers of contraction and relaxation were observed around the time phase representing the onset of the conduction of electrical excitation. The contraction propagated along the direction of the myocardial fiber in the myocardial layer. These results indicated that the electrical excitation conducted in each myocardial layer and the transmural shearing deformation occurred at the boundary between alternate layers of contraction and relaxation. The measurement of the propagation of the local and minute contractile response can reveal the effective contraction with the transmural shearing deformation.

Electrohydrodynamic emitters of ion beams

We discuss physical processes underlying the generation of ion beams with high emission current density in electrohydrodynamic (EHD) emitters based on liquid metals and alloys and with room temperature ionic liquids. We consider EHD effects that influence the emission of ions (ion production mechanisms) and the kinetics of ion interactions in high-density beams. We analyze the factors determining the emission zone size, sustainability of emission at high and low currents, generation of clusters, increase in energy spread, decrease in brightness, and other features of ion beams. We consider the specific design features of EHD emitters and the problems of practically ensuring their stable operation. Discussed in detail are modern application areas for ion sources with EHD emitters, including technological installations for ion beam lithography, micro- and nanopatterning, ion microscopes and tools for local mass spectrometry of secondary ions, and systems to control and neutralize the potential of spacecraft as well as electrostatic rocket engines (microthrusters). We analyze prospects for further development of EHD emitters themselves and instruments based on them.

Электрогидродинамические источники ионных пучков

Physical processes that determine the generation of ion beams with a high emission current density in electrohydrodynamic emitters are considered. Electrohydrodynamic effects, which are manifested in the features of ion emission, and the kinetics of ion interaction in high-density beams are discussed. The factors that determine the size of the emission zone, stability of emission at high and low currents, cluster generation, increase in energy dispersion, and decrease in beam brightness are analyzed. The problems of the practical maintenance of the stable functioning of the EHD emitters are considered. The practical applications of EHD emitters are considered.