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Published in last 50 years
It has been found that there is a strong dependence of the rate of benzil hydrogenation on the structure and basicity of maines. This observation is interpreted in terms of heterolytic activation of hydrogen by cobaloxime.
The dehydrochlorination of dihydridochlorocarbonylbis(triphenylphosphine)iridium(III) by organic and inorganic bases is described. The manner in which this reaction provides a formal link between the homolytic activation of hydrogen at a single metal center and the heterolytic activation of hydrogen is discussed.