Helical Dirac Fermions Research Articles

Magnetic skyrmion crystal at a topological insulator surface

We consider a magnetic skyrmion crystal formed at the surface of a topological insulator. Incorporating the exchange interaction between the helical Dirac surface states and the periodic N\'eel or Bloch skyrmion texture, we obtain the resulting electronic band structure and discuss the constraints that symmetries impose on the energies and Berry curvature. We find substantive qualitative differences between the N\'eel and Bloch cases, with the latter generically permitting a multiband low energy tight-binding representation whose parameters are tightly constrained by symmetries. We explicitly compute the associated Wannier orbitals, which resemble the ringlike chiral bound states of helical Dirac fermions coupled to a single skyrmion in a ferromagnetic background. We construct a two-band tight-binding model with real nearest-neighbor hoppings which captures the salient topological features of the low-energy bands. Our results are relevant to magnetic topological insulators (TIs), as well as to TI-magnetic thin film heterostructures, in which skyrmion crystals may be stabilized.

Phase diagram and phonon-induced backscattering in topological insulator nanowires

We present an effective low-energy theory of electron-phonon coupling effects for clean cylindrical topological insulator nanowires. Acoustic phonons are modelled by isotropic elastic continuum theory with stress-free boundary conditions. We take into account the deformation potential coupling between phonons and helical surface Dirac fermions, and also include electron-electron interactions within the bosonization approach. For half-integer values of the magnetic flux $\Phi_B$ along the wire, the low-energy theory admits an exact solution since a topological protection mechanism then rules out phonon-induced $2k_F$-backscattering processes. We determine the zero-temperature phase diagram and identify a regime dominated by superconducting pairing of surface states. As example, we consider the phase diagram of HgTe nanowires. We also determine the phonon-induced electrical resistivity, where we find a quadratic dependence on the flux deviation $\delta\Phi_B$ from the nearest half-integer value.

Topological Surface Dirac Fermion in BiTeCl-Based Heterostructures

Inversion asymmetric topological insulator promises great potential to realize many intriguing phenomena such as intrinsic topological [Formula: see text]–[Formula: see text] junctions, pyroelectricity and novel topological magneto-electric effects that require inversion asymmetry. Recently, gapless helical surface Dirac fermions were observed in inversion-asymmetric BiTeCl crystal. However, heavy debate about whether BiTeCl is a topological insulator and controversial experimental results of the electronic structure of BiTeCl exist. In this work, through ab-initio calculations, we discovered that a BiTeCl-dominant BiTeCl/Bi2Te3 heterostructure can give rise to the observed band structures with a single surface Dirac fermion. Interestingly, we further suggest that such a BiTeCl/Bi2Te3 heterostructure could be naturally formed by annealing pure BiTeCl single crystals. Our results not only resolve the discrepancy between the previous experiments on heat treated samples and theoretical investigations, but also point out a pathway to design novel materials with sophisticated properties.

Intermediate stages of surface state formation and collapse of topological protection to transport in Bi2Se3

Surface states consisting of helical Dirac fermions have been extensively studied in three-dimensional topological insulators. Yet, experiments to date have only investigated fully formed topological surface states (TSS) and it is not known whether preformed or partially formed surface states can exist or what properties they could potentially host. Here, by decorating thin films of Bi2Se3 with nanosized islands of the same material, we show for the first time that not only can surface states exist in various intermediate stages of formation but they exhibit unique properties not accessible in fully formed TSS. These include tunability of the Dirac cone mass, vertical migration of the surface state wave-function and the appearance of mid-gap Rashba-like states as exemplified by our theoretical model for decorated TIs. Our experiments show that an interplay of Rashba and Dirac fermions on the surface leads to an intriguing multi-channel weak anti-localization effect concomitant with an unprecedented tuning of the topological protection to transport. Our work offers a new route to engineer topological surface states involving Dirac–Rashba coupling by nano-scale decoration of TI thin films, at the same time shedding light on the real-space mechanism of surface state formation in general.

Electrical manipulation of dynamic magnetic impurity and spin texture of helical Dirac fermions

We have theoretically investigated the spin inelastic scattering of helical electrons off a high-spin nanomagnet absorbed on a topological surface. The nanomagnet is treated as a dynamic quantum spin and driven by the spin transfer torque effect. We proposed a mechanism to electrically manipulate the spin texture of helical Dirac fermions rather than by an external magnetic field. By tuning the bias voltage and the direction of impurity magnetization, we present rich patterns of spin texture, from which important fingerprints exclusively associated with the spin helical feature are obtained. Furthermore, it is found that the nonmagnetic potential can create the resonance state in the spin density with different physics as the previously reported resonance of charge density.

Cyclotron resonance in topological insulators: non-relativistic effects

The low-energy Hamiltonian used to describe the dynamics of the helical Dirac fermions on the surface of a topological insulator contains a subdominant non-relativistic (Schrödinger) contribution. This term can have an important effect on some properties while having no effect on others. The Hall plateaus retain the same relativistic quantization as the pure Dirac case. The height of the universal interband background conductivity is unaltered, but its onset is changed. However, the non-relativistic term leads directly to particle–hole asymmetry. It also splits the interband magneto-optical lines into doublets. Here, we find that, while the shape of the semiclassical cyclotron resonance line is unaltered, the cyclotron frequency and its optical spectral weight are changed. There are significant differences in both of these quantities for a fixed value of chemical potential or fixed doping away from charge neutrality depending on whether the Fermi energy lies in the valence or conduction band.

Particle-hole asymmetry in gapped topological insulator surface states

We consider the combined effect of a gap and the Zeeman interaction on the helical Dirac fermions that exist on the surface of a topological insulator. Magneto-optical properties, the magnetization, Hall effect, and the density of states are considered with emphasis on the particle-hole asymmetry, which arises when a subdominant Schr\"odinger piece is included along with the dominant Dirac part of the Hamiltonian. When appropriate, we compare our results with those of a single-valley gapped graphene system for which Zeeman splitting behaves differently. We provide a derivation of the phase offset in the magnetic oscillations brought about by the combined effect of the gap and Schr\"odinger term without requiring the semiclassical Onsager quantization condition. Our results agree with previous discussions based on semiclassical arguments.

Electron-phonon correlations on spin texture of gapped helical Dirac fermions

The metallic surface states of a topological insulator support helical Dirac fermions protected by topology with their spin locked perpendicular to their momentum. They can acquire mass through magnetic doping or through hybridization of states on opposite faces of a thin sample. In this case there can be a component of electron spin oriented perpendicular to the surface plane. The electron-phonon interaction renormalizes the dynamics of the charge carriers through their spectral density. It also modifies the gap channel and a second spectral function enters which, not only determines the out of plane spin component, but also comes into in-plane properties. While the out of plane spin component is decreased below the Fermi momentum ($k_F$), the in plane component increases. There are also correlation tails extending well beyond $k_F$. The angular resolved photo-emission line shapes aquire Holstein side bands. The effective gap in the density of states is reduced and the optical conductivity aquires distinct measurable phonon structure even for modest value of the electron-phonon coupling.

Dielectric screening of surface states in a topological insulator

Hexagonal warping provides an anisotropy to the dispersion curves of the helical Dirac fermions that exist at the surface of a topological insulator. A subdominant quadratic in the momentum term leads to an asymmetry between conduction and valence band. A gap can also be opened through magnetic doping. We show how these various modifications to the Dirac spectrum change the polarization function of the surface states and employ our results to discuss their effect on the plasmons. In the long wavelength limit, the plasmon dispersion retains its square-root dependence on its momentum, $\mathbf{q}$, but its slope is modified and it can acquire a weak dependence on the direction of $\mathbf{q}$. Further, we find the existence of several plasmon branches, one of which is damped for all values of $\mathbf{q}$, and extract the plasmon scattering rate for a representative case.

Photon energy dependence of circular dichroism in angle-resolved photoemission spectroscopy of Bi2Se3Dirac states

Circular dichroism in angle-resolved photoemission spectroscopy (CD-ARPES) has been recently proposed as a sensitive probe of either the spin texture or the orbital momentum texture of helical Dirac fermions at the surface of three-dimensional topological insulators. Recent results obtained on Bi${}_{2}$Te${}_{3}$ point rather towards a final state effect. In this Rapid Communication, we study the prototypical topological insulator Bi${}_{2}$Se${}_{3}$ by CD-ARPES as a function of the photon energy and as a function of thickness. Analysis of the photon energy dependence of CD-ARPES, as well as the existence of a large dichroic signal from massive Dirac fermion states in ulthathin films, confirm that the dichroism is predominantly a final state effect.

Interaction effects on almost flat surface bands in topological insulators

We consider ferromagnetic instabilities of two-dimensional helical Dirac fermions hosted on the surface of three-dimensional topological insulators. We investigate ways to increase the role of interactions by means of modifying the bulk properties which in turn changes both the surface Dirac theory and the screening of interactions. We discuss both the long-ranged part of the Coulomb interactions controlled by the dimensionless coupling constant $\alpha = e^{2}/(\hbar \epsilon v_{F}^{\mathrm{surf}})$ as well as the effects of local interactions parametrized by the ratio $U_{\mathrm{surf}}/D_{\mathrm{surf}}$ of a local interaction on the surface, $U_{\mathrm{surf}}$, and the surface bandwidth, $D_{\mathrm{surf}}$. If large compared to 1, both mechanisms can induce spontaneously surface ferromagnetism, thereby gapping the surface Dirac metal and inducing an anomalous quantum Hall effect. We investigate two mechanisms which can naturally lead to small Fermi velocities $v_{F}^{\mathrm{surf}}$ and a corresponding small bandwidth $D_{\mathrm{surf}}$ at the surface when the bulk band gap is reduced. The same mechanisms can, however, also lead to an enhanced screening of surface interactions. While in all considered cases the long-ranged part of the Coulomb interaction is screened efficiently, $\alpha \lesssim 1$, we discuss situations, where $U_{\mathrm{surf}}/D_{\mathrm{surf}}$ becomes \emph{parametrically}\ large compared to 1, thus inducing surface magnetism.

Reversal of the Circular Dichroism in Angle-Resolved Photoemission fromBi2Te3

The helical Dirac fermions at the surface of topological insulators show a strong circular dichroism which has been explained as being due to either the initial-state spin angular momentum, the initial-state orbital angular momentum, or the handedness of the experimental setup. All of these interpretations conflict with our data from Bi(2)Te(3) which depend on the photon energy and show several sign changes. Our one-step photoemission calculations coupled to ab initio theory confirm the sign change and assign the dichroism to a final-state effect. Instead, the spin polarization of the photoelectrons excited with linearly polarized light remains a reliable probe for the spin in the initial state.

Thermal coherence properties of topological insulator slabs in time-reversal symmetry breaking fields

We first develop a general Green's-function method for the slab geometry, which can handle quite complex conversions between the different polarized radiation modes. Then by using the method, we study the near field thermal coherence properties of a slab of ${Z}_{2}$ topological insulator (TI) with a finite thickness. Under a strong enough external magnetic field, the gapless helical Dirac fermions on the TI surfaces can acquire an energy gap larger than the photon energy of the radiation field at the Dirac point. This gapped surface states can couple strongly with the waveguide modes in the bulk of the TI slab, which thus induces an electromagnetic resonance. Exactly due to the resonance, the coherence properties of the thermal radiation field can be modified dramatically. For ${Z}_{2}$ topological insulators, the parameter regime with the surface Hall conductivity half integer quantized is unique. We demonstrated that within the parameter regime, for a TI slab of a proper thickness, the thermal radiation energy density can be enhanced very much, and the coherence length of the thermal radiation field can be as long as twice that of SiC.

Photoelectron spin-flipping and texture manipulation in a topological insulator

Recently discovered materials called three-dimensional topological insulators constitute examples of symmetry protected topological states in the absence of applied magnetic fields and cryogenic temperatures. A hallmark characteristic of these non-magnetic bulk insulators is the protected metallic electronic states confined to the material's surfaces. Electrons in these surface states are spin polarized with their spins governed by their direction of travel (linear momentum), resulting in a helical spin texture in momentum space. Spin- and angle-resolved photoemission spectroscopy (spin-ARPES) has been the only tool capable of directly observing this central feature with simultaneous energy, momentum, and spin sensitivity. By using an innovative photoelectron spectrometer with a high-flux laser-based light source, we discovered another surprising property of these surface electrons which behave like Dirac fermions. We found that the spin polarization of the resulting photoelectrons can be fully manipulated in all three dimensions through selection of the light polarization. These surprising effects are due to the spin-dependent interaction of the helical Dirac fermions with light, which originates from the strong spin-orbit coupling in the material. Our results illustrate unusual scenarios in which the spin polarization of photoelectrons is completely different from the spin state of electrons in the originating initial states. The results also provide the basis for a novel source of highly spin-polarized electrons with tunable polarization in three dimensions.

Creation of helical Dirac fermions by interfacing two gapped systems of ordinary fermions

Topological insulators are a unique class of materials characterized by a Dirac cone state of helical Dirac fermions in the middle of a bulk gap. When the thickness of a three-dimensional topological insulator is reduced, however, the interaction between opposing surface states opens a gap that removes the helical Dirac cone, converting the material back to a normal system of ordinary fermions. Here we demonstrate, using density function theory calculations and experiments, that it is possible to create helical Dirac fermion state by interfacing two gapped films-a single bilayer Bi grown on a single quintuple layer Bi(2)Se(3) or Bi(2)Te(3). These extrinsic helical Dirac fermions emerge in predominantly Bi bilayer states, which are created by a giant Rashba effect with a coupling constant of ~4 eV·Å due to interfacial charge transfer. Our results suggest that this approach is a promising means to engineer topological insulator states on non-metallic surfaces.

PbTe/PbSnTe heterostructures as analogs of topological insulators

We investigate theoretically the PbTe/PbSnTe heterostructure grown in [111] direction, specifically a quantum wall (potential step of width d) of PbTe embedded in Pb_{1-x}Sn_{x}Te. For x large enough to lead to band inversion, and for large d, there are well-known gapless interface states associated with four L valleys. We show that for d \approx\ 10 nm the three pairs of states from oblique valleys strongly couple, and become gapped with a gap ~10 meV. On the other hand, the interface states from the [111] valley are essentially uncoupled, and they retain their helical character, remaining analogous to states at surfaces of thin layers of three-dimensional topological insulators. This opens up a possibility of studying the physics of two-dimensional helical Dirac fermions in heterostuctures of already widely studied IV-VI semicondcutors.

Electron-phonon scattering in topological insulator thin films

We present a theoretical study of electron-phonon scattering effects in thin films made of a strong topological insulator. The phonons are modeled by isotropic elastic continuum theory with stress-free boundary conditions, and the interaction with the helical surface Dirac fermions is mediated by the deformation potential. We determine the temperature-dependent electrical resistivity $\ensuremath{\rho}(T)$ and the quasiparticle decay rate $\ensuremath{\Gamma}(T)$ observable in photoemission. The low- and high-temperature power laws for both quantities are obtained analytically. Detailed estimates covering the full temperature range are provided for Bi${}_{2}$Se${}_{3}$.

Control over topological insulator photocurrents with light polarization

Three-dimensional topological insulators represent a new quantum phase of matter with spin-polarized surface states that are protected from backscattering. The static electronic properties of these surface states have been comprehensively imaged by both photoemission and tunnelling spectroscopies. Theorists have proposed that topological surface states can also exhibit novel electronic responses to light, such as topological quantum phase transitions and spin-polarized electrical currents. However, the effects of optically driving a topological insulator out of equilibrium have remained largely unexplored experimentally, and no photocurrents have been measured. Here, we show that illuminating the topological insulator Bi(2)Se(3) with circularly polarized light generates a photocurrent that originates from topological helical Dirac fermions, and that reversing the helicity of the light reverses the direction of the photocurrent. We also observe a photocurrent that is controlled by the linear polarization of light and argue that it may also have a topological surface state origin. This approach may allow the probing of dynamic properties of topological insulators and lead to novel opto-spintronic devices.

Spatial fluctuations of helical Dirac fermions on the surface of topological insulators

Surfaces of topological insulators host a new class of states with Dirac dispersion and helical spin texture. Potential quantum computing and spintronic applications using these states require manipulation of their electronic properties at the Dirac energy of their band structure by inducing magnetism or superconductivity through doping and proximity effect. Yet, the response of these states near the Dirac energy in their band structure to various perturbations has remained unexplored. Here we use spectroscopic mapping with the scanning tunneling microscope to study their response to magnetic and non-magnetic bulk dopants in Bi2Te3 and Bi2Se3. Far from the Dirac energy helicity provides remarkable resilience to backscattering even in the presence of ferromagnetism. However, approaching the Dirac point, where the surface states' wavelength diverges bulk doping results in pronounced nanoscale spatial fluctuations of energy, momentum, and helicity. Our results and their connection with similar studies of Dirac electrons in graphene demonstrate that while backscattering and localization are absent for Dirac topological surface states, reducing charge defects is required for both tuning the chemical potential to Dirac energy and achieving high electrical mobility for these novel states.

Topological defects and gapless modes in insulators and superconductors

We develop a unified framework to classify topological defects in insulators and superconductors described by spatially modulated Bloch and Bogoliubov de Gennes Hamiltonians. We consider Hamiltonians $\mathcal{H}(\mathbf{k},\mathbf{r})$ that vary slowly with adiabatic parameters $\mathbf{r}$ surrounding the defect and belong to any of the ten symmetry classes defined by time-reversal symmetry and particle-hole symmetry. The topological classes for such defects are identified and explicit formulas for the topological invariants are presented. We introduce a generalization of the bulk-boundary correspondence that relates the topological classes to defect Hamiltonians to the presence of protected gapless modes at the defect. Many examples of line and point defects in three-dimensional systems will be discussed. These can host one dimensional chiral Dirac fermions, helical Dirac fermions, chiral Majorana fermions, and helical Majorana fermions, as well as zero-dimensional chiral and Majorana zero modes. This approach can also be used to classify temporal pumping cycles, such as the Thouless charge pump, as well as a fermion parity pump, which is related to the Ising non-Abelian statistics of defects that support Majorana zero modes.