Abstract Background The rapid expansion of modern smart applications, demanding faster data transfer and extensive bandwidth, has prompted the development of new-generation networks like 5G and 6G. These networks encompass additional frequency bands such as sub-6 GHz, millimeter waves, and terahertz bands to meet the growing bandwidth requirements. However, despite the substantial bandwidth available in these bands, several challenges must be addressed to overcome unfavorable propagation characteristics. Moreover, numerous applications necessitate wireless devices with antennas that exhibit high flexibility and exceptional radiation responses, particularly when subjected to bending effects. This requirement highlights the importance of polymers-based antennas that can adapt to changing conditions while maintaining optimal performance. The present comprehensive study delves into the performance evaluation of rectangular and circular microstrip antennas utilizing PMMA (polymethyl methacrylate) polymer substrate with varying thicknesses. Results Notably, CNTs (Carbon Nanotubes) are employed as an alternative to traditional copper for the conductive part and ground plane. Both PMMA-based antennas, integrated with CNTs, exhibit a compact footprint of 27.8 × 47.8 × 1.5 mm3 for the circular antenna and 22.8 × 39.5 × 1.5 mm3 for the rectangular antenna. Impressively, the realized gain of both antennas surpasses 5 dBi, demonstrating robust performance in both flat and bending scenarios across different substrate thicknesses. Conclusions The rectangular antenna achieves a bandwidth of approximately 200 MHz, while the circular microstrip antenna showcase annotable bandwidth of 500 MHz. These exceptional outcomes position the two microstrip antennas as highly suitable for a diverse range of emerging applications within the sub-6 GHz band (the frequency range below 6 GHz in the radio spectrum). Thus, the combination of PMMA substrate, CNTs and the compact form factor of the antennas presents a compelling solution for meeting the demands of modern applications requiring efficient wireless communication with enhanced performance and bandwidth.