Hydrogen Gas Target Research Articles

Elastic scattering cross sections and transport of tin ions in extreme ultraviolet lithography sources

Energetic tin ions are created by laser produced plasmas in extreme-ultraviolet lithography sources where hydrogen must be used as a buffer gas to protect critical optical components. In this study, the quantum chemistry code NWChem is used to calculate the interatomic potential between singly ionized tin and molecular hydrogen. The interatomic potential was fit by an inverse-power potential, a modified universal ZBL potential, and a two-piece-Lennard-Jones potential which were in turn used to calculate the classical distance of closest approach, scattering angle, total elastic scattering cross sections. Furthermore, the universal Ziegler-Biersack-Littmark (ZBL) potential was used in the open-source binary collision approximation codes RustBCA as well as Stopping Range in Matter and Transport of Ion in Matter (SRIM/TRIM) to calculate ion ranges, straggling, and stopping cross sections in a hydrogen gas target.

Analytical solution versus the Monte Carlo simulation for studying the H+ beam neutralization in H2 gas target neutralizer

A comparative Study on the conversion of an energetic H+ beam inside a cell neutralizer filled with hydrogen gas target is conducted by two different methods to determine the maximum beam neutralization efficiency and corresponding optimal gas thickness in terms of beam energy, ranging from 1 keV to 10 MeV. One method analytically solves the equations of particle flux with a deterministic response. The other uses the random collisional probability based on the Monte Carlo simulation with non-deterministic response, which is implemented by COMSOL software. Effective reactions of charge exchange and reionization are commonly considered in both methods with the energy-depended collisional cross section. The results obtained from the two methods are compared, demonstrating good fitness with a mean difference of ±1.5 %. This acceptive difference arises often due to statistical errors that occur in the Monte Carlo calculations. Additionally, a close agreement is found between calculated and measured efficiencies.

Production of 99Mo in inverse kinematics heavy ion reactions

Following the successful production of the radioimmunotheranostic nuclide 67Cu through the reaction of a 70Zn beam on a hydrogen gas target, our interest turned to the 99Mo/99mTc generator system. We produced 99Mo in inverse kinematics, with a100Mo beam at 12.0 MeV/nucleon impinging on a 4He gas target. The gas target was kept at liquid nitrogen temperature and pressures of 0.134(3), 0.280(6) and 1.33(3) atm. The produced isotopes and the beam were collected on a thick Al catcher foil. The 99Mo radioisotope can be produced in a one nucleon transfer occurring in peripheral reactions. Two competing factors determine the yield in such reactions, one is the cross-section which favors high mass targets, the other is the effective range which favors low-mass targets. Thus, at low 4He densities, higher beam energy at the exit of the gas target, most of the 99Mo production is generated in the Al foil, while at higher densities, most is generated in the gas target. The activity obtained at the end of the bombardment (given in Becquerel per particle nano-Amps per hour of irradiation), including the 4He gas and Al catcher contribution, were determined as 4.8(14), 2.5(7) and 3.8(11) kBq/(pnAh) for ρgas = 0.83, 0.18 and 0.09 mg/cm3, respectively. These results are competitive to other accelerator production methods; however, the method reported has the additional advantages of needing significantly less amount of expensive enriched isotope and offers an easier and cleaner collection/separation method.

On Producing Long-Lived Spin Polarized Metastable Atoms—Feasibility of Storing Electric Energy

We describe a method of producing long-lived multiply excited spin polarized atoms or ions, the decay of which is strongly delayed or even blocked by intra-ionic magnetic stabilization. Special configurations with huge internal magnetic fields capture only spin polarized electrons in collisions with spin aligned atomic hydrogen gas targets. It is expected that the spin aligned configuration yields an extremely high internal magnetic field which will effectively block spin flip transitions. By this the lifetime of inner shell vacancies is expected to strongly increase.

Constraining the astrophysical p process: Cross section measurement of the Kr84(p,γ)Rb85 reaction in inverse kinematics

One of the biggest questions in nuclear astrophysics is understanding where the elements come from and how they are made. This work focuses on the p process, a nucleosynthesis process that consists of a series of photodisintegration reactions responsible for producing stable isotopes on the proton-rich side of stability. These nuclei, known as the p nuclei, cannot be made through the well-known neutron-capture processes. Currently p-process models rely heavily on theory to provide the relevant reaction rates to predict the final p-nuclei abundances and more experimental data is needed. The present work reports on an experiment performed with the SuN detector at the National Superconducting Cyclotron Laboratory, NSCL, at Michigan State University using the ReA facility to measure the $^{84}$Kr(p,$\gamma$)$^{85}$Rb reaction cross section in inverse kinematics. The reverse $^{85}$Rb($\gamma$,p)$^{84}$Kr reaction is a branching point in the p-process reaction network that was highlighted as an important reaction in sensitivity studies in the production of the $^{78}$Kr p nucleus. A new hydrogen gas target was designed and fabricated and a new analysis technique for background subtraction and efficiency calculations of the detector were developed. The experimental cross section is compared to standard statistical model calculations using the NON-SMOKER and TALYS codes.

Determination of the [formula omitted] cross section at astrophysical energies using a radioactive 7Be ion beam

The reaction Be(p7,γ)8B plays an important role in the Sun, where it determines the high energy component of the solar neutrino spectrum. The importance of this reaction triggered several experiments over the last decades. A combined analysis of their results produces an overall consistent picture for the energy dependence of the cross section, while an inflation of the quoted uncertainties is needed to accommodate the observed discrepancy in the absolute scale of the different data sets. The origin of this discrepancy needs to be understood for a reliable estimate of the astrophysical rate of Be(p7,γ)8B and its uncertainty. In addition, there is a question about possible common systematic effects, considering that all measurements performed so far share the same experimental approach, i.e. an intense proton beam impinging on a Be7 radioactive target. A direct measurement using a radioactive Be7 ion beam on a pure hydrogen gas target has been since long envisioned as a way to improve the situation. First attempts showed the feasibility of an experiment based on the use of a recoil mass separator to collect reaction products with high efficiency, but failed to reach a useful statistical significance because of the low beam intensity. Here we present the results obtained using the intense Be7 beam available at the Tandem Accelerator Laboratory at CIRCE, University of Campania, Italy coupled to the recoil mass separator ERNA in the energy range Ecm=367 to 812 keV. Our results are compatible only with a part of previous measurements, in particular those indicating a low value of the astrophysical S-factor at zero energy S17, thus exacerbating the discrepancy between existing measurements. The analysis of our data together with the results of previous data provides an estimate S17(0)=20.0±0.8 eV⋅b, where systematic uncertainties are inflated to obtain a statistically compatible data set.

Measurement of the Charge-Averaged Elastic Lepton-Proton Scattering Cross Section by the OLYMPUS Experiment.

We report the first measurement of the average of the electron-proton and positron-proton elastic scattering cross sections. This lepton charge-averaged cross section is insensitive to the leading effects of hard two-photon exchange, giving more robust access to the proton's electromagnetic form factors. The cross section was extracted from data taken by the OLYMPUS experiment at DESY, in which alternating stored electron and positron beams were scattered from a windowless gaseous hydrogen target. Elastic scattering events were identified from the coincident detection of the scattered lepton and recoil proton in a large-acceptance toroidal spectrometer. The luminosity was determined from the rates of Møller, Bhabha, and elastic scattering in forward electromagnetic calorimeters. The data provide some selectivity between existing form factor global fits and will provide valuable constraints to future fits.

A novel approach to medical radioisotope production using inverse kinematics

The inverse kinematics methodology using a gas target has been applied to produce medically important radionuclides at the Cyclotron Institute at Texas A&M University. The production of the theranostic radionuclide67Cu (T1/2 = 62 h) through the reaction of a70Zn beam at 15 MeV/nucleon with a hydrogen gas target was performed. The activities at end of irradiation and the thick target yield were obtained for67Cu. A test using the forward-focused neutrons from the primary reaction to irradiatenatZn to produce67Cu is also presented.

New approach to search for parity-even and parity-odd time-reversal violation beyond the Standard Model in a storage ring

Time-reversal breaking and parity-conserving millistrong interactions, suggested in 1965, still remain a viable mechanism of CP-violation beyond the Standard Model. One of its possible manifestations is the T-odd asymmetry in the transmission of tensor-polarized deuterons through a vector-polarized hydrogen gas target. Upon the rotation of the deuteron polarization from the vertical direction into the ring plane, the T-odd asymmetries, odd against the reversal of the proton polarization in the target, will continuously oscillate with first or second harmonics of the spin precession frequency. The Fourier analysis of the oscillating T-odd asymmetries allows for an easy separation from background persistent in conventional experiments employing static vector and tensor polarizations.

Employing [formula omitted] elastic scattering for determination of K-shell ionization cross section of 58Ni19+ in collisions with hydrogen gas target at 95 MeV/u

We present a new experimental method for measuring inner-shell ionization cross sections of low-charged ions colliding with hydrogen gas target in a storage ring. The method is based on a calibration by the well-known differential cross sections of proton elastic scattering on nuclei. K-shell ionization cross section of 1047(100) barn for the 95 MeV/u 58Ni19+ ions colliding with hydrogen atoms was obtained in this work. Compared to the measured ionization cross section, a good agreement is achieved with the prediction by the Relativistic Ionization CODE Modified program (RICODE-M).

Measurement of Ni58(p,p)Ni58 elastic scattering at low momentum transfer by using the HIRFL-CSR heavy-ion storage ring

The very first in-ring reaction experiment at the Cooler Storage Ring at the Heavy Ion Research Facility in Lanzhou (HIRFL-CSR), namely proton elastic scattering on stable $^{58}\mathrm{Ni}$ nuclei, is presented. The circulating $^{58}\mathrm{Ni}^{19+}$ ions with an energy of 95 MeV/u were interacting repeatedly with an internal hydrogen gas target in the experimental storage ring (CSRe). Low-energy proton recoils from the elastic collisions were measured with an ultra-high vacuum compatible silicon-strip detector. Deduced differential cross sections were normalized by measuring $k$-shell x rays from $^{58}\mathrm{Ni}^{19+}$ projectiles due to the $^{58}\mathrm{Ni}^{19+}\text{\ensuremath{-}}{\mathrm{H}}_{2}$ ionization collisions. Compared to the experimental cross sections, a good agreement has been achieved with the theoretical predictions in the measured region, which were obtained by using the global phenomenological optical model potentials. Our results enable new research opportunities for optical model potential studies on exotic nuclides by using the in-ring reaction setup at the HIRFL-CSR facility.

A small proton charge radius from anelectron-proton scattering experiment.

Elastic electron-proton scattering (e-p) and the spectroscopy of hydrogen atoms are the two methods traditionally used to determine the proton charge radius, rp. In 2010, a new method using muonic hydrogen atoms1 found a substantial discrepancy compared with previous results2, which became known as the 'proton radius puzzle'. Despite experimental and theoretical efforts, the puzzle remains unresolved. In fact, there is a discrepancy between the two most recent spectroscopic measurements conducted on ordinary hydrogen3,4. Here we report on the proton charge radius experiment at Jefferson Laboratory (PRad), a high-precision e-p experiment that was established after the discrepancy was identified. We used a magnetic-spectrometer-free method along with a windowless hydrogen gas target, which overcame several limitations of previous e-p experiments and enabled measurements at very small forward-scattering angles. Our result, rp=0.831±0.007stat± 0.012systfemtometres, is smaller than the most recent high-precision e-p measurement5 and 2.7 standard deviations smaller than the average of all e-p experimental results6. The smaller rp we have now measured supports the value found by two previous muonic hydrogen experiments1,7. In addition, our finding agrees with the revised value (announced in 2019) for the Rydberg constant8-one of the most accurately evaluated fundamental constants in physics.

Beam-helicity asymmetries for single-hadron production in semi-inclusive deep-inelastic scattering from unpolarized hydrogen and deuterium targets

A measurement of beam-helicity asymmetries for single-hadron production in deep-inelastic scattering is presented. Data from the scattering of 27.6 GeV electrons and positrons off gaseous hydrogen and deuterium targets were collected by the HERMES experiment. The asymmetries are presented separately as a function of the Bjorken scaling variable, the hadron transverse momentum, and the fractional energy for charged pions and kaons as well as for protons and anti-protons. These asymmetries are also presented as a function of the three aforementioned kinematic variables simultaneously.

Design and operation of a windowless gas target internal to a solenoidal magnet for use with a megawatt electron beam

A windowless hydrogen gas target of nominal thickness $10^{19}$ cm$^{-2}$ is an essential component of the DarkLight experiment, which is designed to utilize the megawatt electron beam at an Energy Recovery Linac (ERL). The design of such a target is challenging because the pressure drops by many orders of magnitude between the central, high-density section of the target and the surrounding beamline, resulting in laminar, transitional, and finally molecular flow regimes. The target system was assembled and operated at Jefferson Lab's Low Energy Recirculator Facility (LERF) in 2016, and subsequently underwent several revisions and calibration tests at MIT Bates in 2017. The system at dynamic equilibrium was simulated in COMSOL to provide a better understanding of its optimal operation at other working points. We have determined that a windowless gas target with sufficiently high density for DarkLight's experimental needs is feasible in an ERL environment.

Radiative electron capture as a tunable source of highly linearly polarized x rays

The radiative electron capture (REC) into the K shell of bare Xe ions colliding with a hydrogen gas target has been investigated. In this study, the degree of linear polarization of the K-REC radiation was measured and compared with rigorous relativistic calculations as well as with the previous results recorded for U92+. Owing to the improved detector technology, a significant gain in precision of the present polarization measurement is achieved compared to the previously published results. The obtained data confirms that for medium-Z ions such as Xe, the REC process is a source of highly polarized x rays which can easily be tuned with respect to the degree of linear polarization and the photon energy. We argue, in particular, that for relatively low energies the photons emitted under large angles are almost fully linear polarized.Received 22 February 2019DOI:https://doi.org/10.1103/PhysRevA.99.052702Published by the American Physical Society under the terms of the Creative Commons Attribution 4.0 International license. Further distribution of this work must maintain attribution to the author(s) and the published article's title, journal citation, and DOI.Published by the American Physical SocietyPhysics Subject Headings (PhySH)PropertiesPolarizationTechniquesCompton scatteringRadiation detectorsAccelerators & BeamsAtomic, Molecular & Optical

A novel approach to medical radioisotope production using inverse kinematics: A successful production test of the theranostic radionuclide 67Cu

A novel method for the production of important medical radioisotopes has been developed. The approach is based on performing the nuclear reaction in inverse kinematics, namely sending a heavy-ion beam of appropriate energy on a light target (e.g. H, d, He) and collecting the isotope of interest. In this work, as a proof-of-concept, we studied the production of the theranostic radionuclide 67Cu (T1/2 = 62 h) via the reaction of a 70Zn beam at 15 MeV/nucleon with a hydrogen gas target. The 67Cu radionuclide alongside other coproduced isotopes, was collected after the gas target on an aluminum catcher foil and their radioactivity was measured by off-line γ-ray analysis. After 36 h post irradiation, apart from the product of interest 67Cu, the main radioimpurity coming from the 70Zn + p reaction was 69mZn (T1/2 = 13.8 h), which can be reduced by further radio-cooling. Moreover, along with the radionuclide of interest produced in inverse kinematics, the production of additional radioisotopes is possible by making use of the forward-focused neutrons from the reaction and allowing them to interact with a secondary target. A preliminary successful test of this concept was realized in the present study. The main requirement to obtain activities appropriate for preclinical studies is the development of high-intensity heavy-ion primary beams.

Test measurement of 7Be(p, $\gamma$ γ )8B with the recoil mass separator ERNA

7Be(p, $\gamma$ )8B has an important role in nuclear astrophysics, having a direct impact on both the high energy component of solar neutrinos and the 7Li abundance after the Big Bang Nucleosynthesis. All direct measurements providing useful information on this reaction so far used the same approach, i.e. a proton beam on a radioactive 7Be target. The overall precision and accuracy of the estimate of the astrophysical rate of this reaction are limited by the discrepancy between the results of existing measurements, possibly due to the complicated stoichiometry and beam induced deterioration of the radioactive targets. The ERNA (European Recoil separator for Nuclear Astrophysics) collaboration planned a new experiment in inverse kinematics exploiting the intense 7Be beam available at CIRCE (Center for Isotopic Research on Cultural and Environmental heritage), Caserta, Italy. The 8B recoils are produced in a windowless hydrogen gas target and detected after the efficient mass separation provided by ERNA. Here we present the commissioning of the experimental setup and a first cross section measurement at $E_{\mathrm{cm}}\approx 812$ keV.

High Energy electron and proton acceleration by circularly polarized laser pulse from near critical density hydrogen gas target

Relativistic electron rings hold the possibility of very high accelerating rates, and hopefully a relatively cheap and compact accelerator/collimator for ultrahigh energy proton source. In this work, we investigate the generation of helical shaped quasi-monoenergetic relativistic electron beam and high-energy proton beam from near critical density plasmas driven by petawatt-circularly polarized-short laser pulses. We numerically observe the efficient proton acceleration from magnetic vortex acceleration mechanism by using the three dimensional particle-in-cell simulations; proton beam with peak energy 350 MeV, charge ~10nC and conversion efficiency more than 6% (which implies 2.4 J proton beam out of the 40 J incident laser energy) is reported. We detailed the microphysics involved in the ion acceleration mechanism, which requires investigating the role of self-generated plasma electric and magnetic fields. The concept of efficient generation of quasi-monoenergetic electron and proton beam from near critical density gas targets may be verified experimentally at advanced high power – high repetition rate laser facilities e.g. ELI-ALPS. Such study should be an important step towards the development of high quality electron and proton beam.

A novel technique for determining luminosity in electron-scattering/positron-scattering experiments from multi-interaction events

The OLYMPUS experiment measured the cross-section ratio of positron–proton elastic scattering relative to electron–proton elastic scattering to look for evidence of hard two-photon exchange. To make this measurement, the experiment alternated between electron beam and positron beam running modes, with the relative integrated luminosities of the two running modes providing the crucial normalization. For this reason, OLYMPUS had several redundant luminosity monitoring systems, including a pair of electromagnetic calorimeters positioned downstream from the target to detect symmetric Møller and Bhabha scattering from atomic electrons in the hydrogen gas target. Though this system was designed to monitor the rate of events with single Møller/Bhabha interactions, we found that a more accurate determination of relative luminosity could be made by additionally considering the rate of events with both a Møller/Bhabha interaction and a concurrent elastic ep interaction. This method was improved by small corrections for the variance of the current within bunches in the storage ring and for the probability of three interactions occurring within a bunch. After accounting for systematic effects, we estimate that the method is accurate in determining the relative luminosity to within 0.36%. This precise technique can be employed in future electron–proton and positron–proton scattering experiments to monitor relative luminosity between different running modes.

Design of SECAR a recoil mass separator for astrophysical capture reactions with radioactive beams

A recoil mass separator SECAR has been designed for the purpose of studying low-energy (p,γ) and (α,γ) reactions in inverse kinematics with radioactive beams for masses up to about A = 65. Their reaction rates are of importance for our understanding of the energy production and nucleosynthesis during explosive hydrogen and helium burning. The radiative capture reactions take place in a windowless hydrogen or He gas target at the entrance of the separator, which consists of four Sections. The first Section selects the charge state of the recoils. The second and third Sections contain Wien Filters providing high mass resolving power to separate efficiently the intense beam from the few reaction products. In the following fourth Section, the reaction products are guided into a detector system capable of position, angle and time-of-flight measurements. In order to accept the complete kinematic cone of recoil particles including multiple scattering in the target in the center of mass energy range of 0.2 MeV to 3.0 MeV, the system must have a large polar angle acceptance of ± 25 mrad. This requires a careful minimization of higher order aberrations. The present system will be installed at the NSCL ReA3 accelerator and will be used with the much higher beam intensities of the FRIB facility when it becomes available.