Fundamental Physical Processes Research Articles

Understanding the origins of the heliosphere: integrating observations and measurements from Parker Solar Probe, Solar Orbiter, and other space- and ground-based observatories

Context.The launch of Parker Solar Probe (PSP) in 2018, followed by Solar Orbiter (SO) in February 2020, has opened a new window in the exploration of solar magnetic activity and the origin of the heliosphere. These missions, together with other space observatories dedicated to solar observations, such as the Solar Dynamics Observatory, Hinode, IRIS, STEREO, and SOHO, with complementary in situ observations from WIND and ACE, and ground based multi-wavelength observations including the DKIST observatory that has just seen first light, promise to revolutionize our understanding of the solar atmosphere and of solar activity, from the generation and emergence of the Sun’s magnetic field to the creation of the solar wind and the acceleration of solar energetic particles.Aims.Here we describe the scientific objectives of the PSP and SO missions, and highlight the potential for discovery arising from synergistic observations. Here we put particular emphasis on how the combined remote sensing and in situ observations of SO, that bracket the outer coronal and inner heliospheric observations by PSP, may provide a reconstruction of the solar wind and magnetic field expansion from the Sun out to beyond the orbit of Mercury in the first phases of the mission. In the later, out-of-ecliptic portions of the SO mission, the solar surface magnetic field measurements from SO and the multi-point white-light observations from both PSP and SO will shed light on the dynamic, intermittent solar wind escaping from helmet streamers, pseudo-streamers, and the confined coronal plasma, and on solar energetic particle transport.Methods.Joint measurements during PSP–SO alignments, and magnetic connections along the same flux tube complemented by alignments with Earth, dual PSP–Earth, and SO-Earth, as well as with STEREO-A, SOHO, and BepiColumbo will allow a better understanding of the in situ evolution of solar-wind plasma flows and the full three-dimensional distribution of the solar wind from a purely observational point of view. Spectroscopic observations of the corona, and optical and radio observations, combined with direct in situ observations of the accelerating solar wind will provide a new foundation for understanding the fundamental physical processes leading to the energy transformations from solar photospheric flows and magnetic fields into the hot coronal plasma and magnetic fields and finally into the bulk kinetic energy of the solar wind and solar energetic particles.Results.We discuss the initial PSP observations, which already provide a compelling rationale for new measurement campaigns by SO, along with ground- and space-based assets within the synergistic context described above.

The Relaxation of Reconnected Open Magnetic Field Lines in the Earth’s Magnetosphere

Abstract Magnetic reconnection is a fundamental and important physical process that can release magnetic energy and change magnetic topology. A statistic study of reconnected magnetic field lines has been carried out by Cluster spacecraft 1 during 58 current sheet crossing events. We calculated the values of at different distances from reconnection site to describe the loosing process of magnetic field lines. Our results suggest that current sheets in ion diffusion regions have small values of . As the distance from reconnection site increases, the reconnected magnetic field lines relax, and subsequently have relatively large values of . However, such large values of are found to be closely related to open magnetic field lines that connect the Earth’s magnetosphere and the solar wind.

Noncontact evaluation of full elastic constants of perovskite MAPbBr3 via Photoacoustic eigen-spectrum analysis in one test

Elasticity is one basic property of hybrid organic-inorganic perovskites. It highly relates to many fundamental processes in solid physics. The investigation of elasticity is of interest not only to explore the intrinsic properties of a material, but also to improve their potential application performance. In this study, we predict photoacoustic eigen-spectrum (PAES) of single crystal. Then by solving the inverse problem of the generation of PAES, we propose a noncontact method to determine a complete set of elastic constants of single crystal in one test. Experiments confirm the proposed method accurately determines all elastic constants of MAPbBr3. Since this method is totally noncontact and does not require multiple specimens cutting along different crystal axes, it could be more competent for rare, tiny and brittle specimen, or when the specimen is immersed in turbid or opaque medium. Benefitting from these superiorities, the proposed method might be found prominent values in materials science and applications.

The Beam Plasma Interactions Experiment: An Active Experiment Using Pulsed Electron Beams

The 1970s and 1980s were heydays for using active electron beam experiments to probe some of the fundamental physical processes that occur throughout the heliosphere and in astrophysical contexts. Electron beam experiments were used to study spacecraft charging and spacecraft-plasma coupling; beam-plasma interaction physics; magnetic bounce and drift physics; auroral physics; wave generation; and military applications. While these experiments were enormously successful, they were also limited by the technologies that were available at that time. New advances in space instrumentation, data collection, and accelerator technologies enable a revolutionary new generation of active experiments using electron beams in space. In this paper we discuss such an experiment, the Beam Plasma Interactions Experiment (Beam PIE), a sounding rocket experiment designed to (a) advance HEMT-based RF linear accelerator electron accelerator technology for space applications and (b) study the production of whistler and X-mode waves by modulated electron beams.

Harmonic generation at the nanoscale

Nonlinear photon conversion is a fundamental physical process that lies on the basis of many modern disciplines, from bioimaging and theranostics in nanomedicine to material characterization in materials science and nanotechnology. It also holds great promise in laser physics with applications in information technology for optical signal processing and in the development of novel coherent light sources. The capability to efficiently generate harmonics at the nanoscale will have an enormous impact on all these fields, since it would allow one to realize much more compact devices and to interrogate matter in extremely confined volumes. Here, we present a perspective on the most recent advances in the generation of nonlinear optical processes at the nanoscale and their applications, proposing a palette of future perspectives that range from material characterization and the development of novel compact platforms for efficient photon conversion to bioimaging and sensing.

Advances and Challenges in Observations and Modeling of the Global-Sun Dynamics and Dynamo

AbstractComputational heliophysics has shed light on the fundamental physical processes inside the Sun, such as the differential rotation, meridional circulation, and dynamo-generation of magnetic fields. However, despite the substantial advances, the current results of 3D MHD simulations are still far from reproducing helioseismic inferences and surface observations. The reason is the multi-scale nature of the solar dynamics, covering a vast range of scales, which cannot be solved with the current computational resources. In such a situation, significant progress has been achieved by the mean-field approach, based on the separation of small-scale turbulence and large-scale dynamics. The mean-field simulations can reproduce solar observations, qualitatively and quantitatively, and uncover new phenomena. However, they do not reveal the complex physics of large-scale convection, solar magnetic cycles, and the magnetic self-organization that causes sunspots and solar eruptions. Thus, developing a synergy of these approaches seems to be a necessary but very challenging task.

Microwave gas-discharge device OVOD-1a sanitizing indoor air

A new UV scanning system OVOD-1a for the indoor air environment, based on high-performance microwave gas-discharge lamps developed at GPI RAS, is described. The first experiments demonstrating the air-cleaning capabilities of UV equipment were carried out. It is shown that in laboratory rooms used for the stay of livestock bred in agriculture, the energy cost of almost complete purification of the air environment from viral and fungal components is of the order of 10−2 kW × h/m3. B acter ial sanita tio n o f the laboratory p re mise s o f the research physical Institute is carried out with an energy cost of ≍ 3 10−3 kW×h/m3. The fundamental physical processes underlying microwave UV lamps, which are the main component of the OVOD-1a sanitation system, are discussed.

Assessing the Regulatory Requirements of Lead-Based Perovskite Photovoltaics

Nicole Moody, Samuel Sesena, Dane W. deQuilettes, Benjia Dak Dou, Richard Swartwout, Anna Johnson, Udochukwu Eze, Roberto Brenes, Matthew Johnston, Vladimir Bulovic, and Moungi G. Bawendi are members of Tata-MIT GridEdge Solar, an interdisciplinary research program at the Massachusetts Institute of Technology working toward scalable design and manufacturing of lightweight, flexible solar cells. Joseph T. Buchman and Christy L. Haynes are part of the Center for Sustainable Nanotechnology, a multi-institutional partnership aimed at understanding the fundamental chemical and physical processes that govern the transformations and interactions of nanoparticles in the environment.

Fundamental investigation of photoacoustic signal generation from single aerosol particles at varying relative humidity

Photoacoustic (PA) spectroscopy enjoys widespread applications across atmospheric sciences. However, experimental biases and limitations originating from environmental conditions and particle size distributions are not fully understood. Here, we combine single-particle photoacoustics with modulated Mie scattering to unravel the fundamental physical processes occurring during PA measurements on aerosols. We perform measurements on optically trapped droplets of varying sizes at different relative humidity. Our recently developed technique – photothermal single-particle spectroscopy (PSPS) – enables fundamental investigations of the interplay between the heat flux and mass flux from single aerosol particles. We find that the PA phase is more sensitive to water uptake by aerosol particles than the PA amplitude. We present results from a model of the PA phase, which sheds further light onto the dependence of the PA phase on the mass flux phenomena. The presented work provides fundamental insights into photoacoustic signal generation of aerosol particles.

Unified prediction of reshocked Richtmyer–Meshkov mixing with K-L model

Hydrodynamic instabilities, including Rayleigh–Taylor, Richtmyer–Meshkov (RM), and Kelvin–Helmholtz, induced turbulent mixing broadly occur in both natural phenomena, such as supernova explosions, and high-energy-density applications, such as inertial confinement fusion. Reshocked RM mixing is the most fundamental physical process that is closely related to practical problems, as it involves three classical instabilities. In complex applications, the Reynolds-averaged Navier–Stokes model analysis continues to play a major role. However, there are very few turbulence models that facilitate unified predictions of the outcome of reshocked RM mixing experiments under different physical conditions. Thus, we aim to achieve this objective using the K-L model based on three considerations: deviatoric shear stress is considered when constructing Reynolds stress tensor; the model coefficients used are derived based on a new systematic procedure; the performance of different numerical schemes are studied to ensure high resolution but basically no numerical oscillation. Consequently, a unified prediction is obtained for the first time for a series of reshocked RM mixing experiments under incident shock Mach numbers Ma = 1.2–1.98, Atwood numbers At = ±0.67, and test section lengths 8 cm ≤ δ ≤ 110 cm. The results reveal the feasibility of demonstrating different reshocked RM processes using a single model, without adjusting the model coefficients, which sheds light on the further application of the present model to practical engineering, such as inertial confinement fusion.

Comparison of electron heating and energy loss mechanisms in an RF plasma jet operated in argon and helium

The μ-APPJ is a well-investigated atmospheric pressure RF plasma jet. Up to now, it has mainly been operated using helium as feed gas due to stability restrictions. However, the COST-Jet design including precise electrical probes now offers the stability and reproducibility to create equi-operational plasmas in helium as well as in argon. In this publication, we compare fundamental plasma parameters and physical processes inside the COST reference microplasma jet, a capacitively coupled RF atmospheric pressure plasma jet, under operation in argon and in helium. Differences already observable by the naked eye are reflected in differences in the power-voltage characteristic for both gases. Using an electrical model and a power balance, we calculated the electron density and temperature at 0.6 W to be , 1.2 eV and , 1.7 eV for argon and helium, respectively. In case of helium, a considerable part of the discharge power is dissipated in elastic electron-atom collisions, while for argon most of the input power is used for ionization. Phase-resolved optical emission spectroscopy reveals differently pronounced heating mechanisms. Whereas bulk heating is more prominent in argon compared to helium, the opposite trend is observed for sheath heating. This also explains the different behavior observed in the power-voltage characteristics.

Joining mechanism of bulk metallic glasses in their supercooled liquid region

Abstract Bulk metallic glasses (BMGs) are promising engineering materials due to their high strength, high fracture toughness and excellent corrosion resistance. However, the wide application of BMGs has been limited by the casting sample size. Joining of BMGs in their supercooled liquid region (SCLR) has shown the possibility to get rid of the casting size limitation. In this work, the physical mechanism of joining BMGs in their supercooled liquid region is systematically investigated. Specifically, the effects of joining temperature and time on the joint strength are studied by experiments, and the effects of joint strain and bonding morphologies are simulated by finite element analysis. It is observed that the joint strength is solely determined by the area fraction of the bonded regions, and the bonded regions increase with the joining temperature and joining time but are almost independent of the bonding morphologies. Based on the experiments and simulations, three microscopic processes that are oxide deforming and cracking, pristine BMGs flowing to contact and forming metallic bonds are identified to optimize the joint performance. By correlating the joining conditions with the three responsible microscopic processes, BMGs can be joined with predictable performance. Our work provides the fundamental physical processes for joining of BMGs in their SCLR, which could offer solution to the size limitation in application of BMGs.

How photocorrosion can trick you: a detailed study on low-bandgap Li doped CuO photocathodes for solar hydrogen production.

The efficiency of photoelectrochemical tandem cells is still limited by the availability of stable low band gap electrodes. In this work, we report a photocathode based on lithium doped copper(ii) oxide, a black p-type semiconductor. Density functional theory calculations with a Hubbard U term show that low concentrations of Li (Li0.03Cu0.97O) lead to an upward shift of the valence band maximum that crosses the Fermi level and results in a p-type semiconductor. Therefore, Li doping emerged as a suitable approach to manipulate the electronic structure of copper oxide based photocathodes. As this material class suffers from instability in water under operating conditions, the recorded photocurrents are repeatedly misinterpreted as hydrogen evolution evidence. We investigated the photocorrosion behavior of LixCu1-xO cathodes in detail and give the first mechanistic study of the fundamental physical process. The reduced copper oxide species were localized by electron energy loss spectroscopy mapping. Cu2O grows as distinct crystallites on the surface of LixCu1-xO instead of forming a dense layer. Additionally, there is no obvious Cu2O gradient inside the films, as Cu2O seems to form on all LixCu1-xO nanocrystals exposed to water. The application of a thin Ti0.8Nb0.2Ox coating by atomic layer deposition and the deposition of a platinum co-catalyst increased the stability of LixCu1-xO against decomposition. These devices showed a stable hydrogen evolution for 15 minutes.

A Computational Systems Approach to Rational Design of Nose-to-Brain Delivery of Biopharmaceutics

In this work, a computational systems approach, comprising models at different time and length scales, is developed to elucidate the fundamental chemical, physical, transport, and biological processes in relation to the design of a novel nose-to-brain drug delivery system for the treatment of neurodegenerative diseases. In particular, a kinetic model is established to describe the formation of a hydrogel patch, via the enzymatic cross-linking of tyramine-modified hyaluronic acid, on the olfactory cleft. A fluid transport model is employed to describe the flow of a cross-linkable viscoelastic polymer solution through an applicator in terms of tube and reactive fluid characteristics (e.g., tube geometry, volumetric flow rate, and viscosity). The spreading of the deposited HA droplet on a mucus substrate is modeled via the development of a dynamic droplet deformation model. Subsequently, a dynamic drug release model is formulated to quantify the release rate of an active pharmaceutical ingredient (e.g., long-acting insulin analogues) from a distributed population of drug-loaded polymeric carriers embedded into a hydrogel matrix in terms of molecular and morphological properties of the hydrogel–drug carriers system. Finally, the drug flux from the hydrogel–mucosa interface to the olfactory bulb via the epithelium and lamina propria olfactory sublayers is modeled with a series of dynamic mass transport models. The various mathematical models are integrated together following a multiscale modeling approach to aid the identification of key design system parameters and material properties that can lead to the optimization of the complex drug carriers–hydrogel, droplet deposition, film formation, and drug delivery system to achieve a desired therapeutic effect over a two-week delivery time.

Selective suppression of normal modes in coupled oscillators

In this paper we present experimentally and discuss quantitatively two experiments, in which we show how to suppress in turn selectively one of the two normal modes of a system made of two oscillators (each consisting of a cart and a spring), mutually coupled by an interaction spring. This way, while friction is usually considered an undesirable side effect, the role of dissipation is highlighted. We also discuss, from a didactic perspective, how the experiments presented can be useful to introduce fundamental physical concepts and processes.

Hanbury Brown-Twiss Correlations for a Driven Superatom.

Hanbury Brown-Twiss interference and stimulated emission, two fundamental processes in atomic physics, have been studied in a wide range of applications in science and technology. We study interference effects that occur when a weak probe is sent through a gas of two-level atoms that are prepared in a singly excited collective (Dicke or "superatom") state and for atoms prepared in a factorized state. We measure the time-integrated second-order correlation function g^{(2)} of the output field as a function of the delay τ between the input probe field and radiation emitted by the atoms and find that, for the Dicke state, g^{(2)} is twice as large for τ=0 as it is for γ_{e}τ≫1 (γ_{e} is an excited state decay rate), while for the product state, this ratio is equal to 3/2. The results agree with those of a theoretical model in which any effects related to stimulated emission are totally neglected-the coincidence counts measured in our experiment arise from Hanbury Brown-Twiss interference between the input field and the field radiated by the atoms.

Microwave gasdischarge source of biologically active UV radiation and ozone as efficient means for sanitation of the indoor air

A new system of UV sanitization of the air environment in the premises of OVOD-1a, based on high-efficiency microwave gasdischarge lamps developed in GPI RAS, is described. The first experiments demonstrating the air purification capabilities of UV equipment were carried out. It is shown that in the laboratory premises used for the stay of livestock breeding in agriculture, the energy price of almost complete purification of the air from viral and fungal components is about η ≈ 10−2kW·h/m3. Bacterial sanitation of laboratory space is carried out with an energy cost of η ≈ 3·10−2kW·h/m3. The fundamental physical processes underlying microwave UV lamps, which are the main component of OVOD-1a sanitation system, are discussed.

Self-Arranged Levitating Droplet Clusters: A Reversible Transition from Hexagonal to Chain Structure.

Water microdroplets condense over locally heated water-vapor interfaces and levitate in an ascending vapor-air flow forming self-assembled ordered monolayer clusters. The droplets do not coalesce due to complex aerodynamic interactions between them. The droplet cluster formation is governed by the condensation/evaporation balance and by coupling of heat flux and vapor flow with aerodynamic forces. Here, we report the observations of a reversible structural transition from the ordered hexagonal-structure cluster to the chain-like structure and provide an explanation of its mechanism and conditions under which the transition occurs. The phenomenon provides new insights on the fundamental physical and chemical processes with microdroplets including their role in reaction catalysis in nature and their potential for aerosol and microfluidic applications.

Multiphoton quantum-state engineering using conditional measurements

The quantum theory of electromagnetic radiation predicts characteristic statistical fluctuations for light sources as diverse as sunlight, laser radiation, and molecule fluorescence. Indeed, these underlying statistical fluctuations of light are associated with the fundamental physical processes behind their generation. In this contribution, we experimentally demonstrate that the manipulation of the quantum electromagnetic fluctuations of two-mode squeezed vacuum states leads to a family of quantum-correlated multiphoton states with tunable mean photon numbers and degree of correlation. Our technique relies on the use of conditional measurements to engineer the excitation mode of the field through the simultaneous subtraction of photons from two-mode squeezed vacuum states. The experimental generation of nonclassical multiphoton states by means of photon subtraction unveils novel mechanisms to control fundamental properties of light. As a remarkable example, we demonstrate the engineering of a quantum state of light with up to ten photons, exhibiting nearly Poissonian photon statistics, that constitutes an important step towards the generation of entangled lasers. Our technique enables a robust protocol to prepare quantum states with multiple photons in high-dimensional spaces and, as such, it constitutes a novel platform for exploring quantum phenomena in mesoscopic systems.

Microstructural effects on permeability of Nitrocellulose membranes for biomedical applications

Nitrocellulose membrane (NC), as a paper-like matrix with microscale porous structures, has found widespread applications in biomedical fields due to its excellent biological features and physiochemical properties. In these biomedical applications, diffusion, convection, and binding reaction of biomolecules (e.g., acids and proteins) in NC through wicking flow is the fundamental physical process. However, the optimization of NC based biomedical devices has been limited by the lack of the understanding on the wicking flow behavior of NC membranes from the microstructural point of view. To address this, we experimentally and theoretically investigated the microstructural effects on the wicking flow behaviors (e.g., permeability, effective pore radius) of NC membrane and found that the wicking flow is highly dependent on the pore-morphology characterizing parameters (e.g., porosity and pore size). We further developed a theoretical model yielding a closed-form solution to predict the microstructure-permeability relation, which was validated by our experimental results. Our theoretical model would be a powerful tool for tailoring the wicking flow behavior of NC membranes through controlling the microstructural parameters, and thus for optimizing NC membrane-based biomedical devices from the view point of material design in the future.