Laser Frequency Research Articles

Radiation reaction kinetics and collective QED signatures

Observing collective effects originating from the interplay between quantum electrodynamics and plasma physics might be achieved in upcoming experiments. In particular, the generation of electron–positron pairs and the observation of their collective dynamics could be simultaneously achieved in a collision between an intense laser and a highly relativistic electron beam through a laser frequency shift driven by an increase in the plasma density increase. In this collision, the radiation of high-energy photons will serve a dual purpose: first, in seeding the cascade of pair generation; and, second, in decelerating the created pairs for detection. The deceleration results in a detectable shift in the plasma frequency. This deceleration was previously studied considering only a small sample of individual pair particles. However, the highly stochastic nature of the quantum radiation reaction in the strong-field regime limits the descriptive power of the average behavior to the dynamics of pair particles. Here, we examine the full kinetic evolution of generated pairs in order to more accurately model the relativistically adjusted plasma density. As we show, the most effective pair energy for creating observable signatures occurs at a local minimum, obtained at finite laser field strength due to the trade-off between pair deceleration and the relativistic particle oscillation at increasing laser intensity. For a small number of laser cycles, the quantum radiation reaction may re-arrange the generated pairs into anisotropic distributions in momentum space, although, in the one-dimensional simulations considered here, this anisotropy quickly decreases.

Magnetostriction measurements at milli-kelvin temperatures using a Fabry-Pérot interferometer.

This paper demonstrates an optical technique to measure magnetostrictive strain in a cryogenic environment using a Fabry-Pérot resonator spaced by crystal samples. Optical measurement techniques are calibration-free and highly sensitive. This technique was used to measure the magnetostrictive strain of neodymium gallate at a temperature of 49 mK to be λ = 1.3 × 10-5 at 3T, with a sensitivity of 3.0 × 10-8. We highlight the interesting properties of the crystal's magnetic ordering. The sensitivity of this technique was limited by the wavemeter used to measure the laser frequency, and significant improvements in the sensitivity should be possible.

A new method for instrumental profile reconstruction of high-resolution spectrographs

Context. Knowledge of the spectrograph’s instrumental profile (IP) provides important information needed for wavelength calibration and for the use in scientific analyses. Aims. This work develops new methods for IP reconstruction in high-resolution spectrographs equipped with astronomical laser frequency comb (astrocomb) calibration systems and assesses the impact that assumptions on the IP shape have on achieving accurate spectroscopic measurements. Methods. Astrocombs produce ≈ 10 000 bright, unresolved emission lines with known wavelengths, making them excellent probes of the IP. New methods based on Gaussian process regression were developed to extract detailed information on the IP shape from these data. Applying them to HARPS, an extremely stable spectrograph installed on the ESO 3.6m telescope, we reconstructed its IP at 512 locations of the detector, covering 60% of the total detector area. Results. We found that the HARPS IP is asymmetric and that it varies smoothly across the detector. Empirical IP models provide a wavelength accuracy better than 10m s−1 (5m s−1) with a 92% (64%) probability. In comparison, reaching the same accuracy has a probability of only 29% (8%) when a Gaussian IP shape is assumed. Furthermore, the Gaussian assumption is associated with intra-order and inter-order distortions in the HARPS wavelength scale as large as 60 m s−1. The spatial distribution of these distortions suggests they may be related to spectrograph optics and therefore may generally appear in cross-dispersed echelle spectrographs when Gaussian IPs are used. Empirical IP models are provided as supplementary material in machine readable format. We also provide a method to correct the distortions in astrocomb calibrations made under the Gaussian IP assumption. Conclusions. Methods presented here can be applied to other instruments equipped with astrocombs, such as ESPRESSO, but also ANDES and G-CLEF in the future. The empirical IPs are crucial for obtaining objective and unbiased measurements of fundamental constants from high-resolution spectra, as well as measurements of the redshift drift, isotopic abundances, and other science cases.

Optical second harmonic generation in anisotropic multilayers with complete multireflection of linear and nonlinear waves using ♯SHAARP.ml package

Optical second harmonic generation (SHG) is a nonlinear optical effect widely used for nonlinear optical microscopy and laser frequency conversion. Closed-form analytical solution of the nonlinear optical responses is essential for evaluating materials whose optical properties are unknown a priori. A recent open-source code, ♯SHAARP.si, can provide such closed form solutions for crystals with arbitrary symmetries, orientations, and anisotropic properties at a single interface. However, optical components are often in the form of slabs, thin films on substrates, and multilayer heterostructures with multiple reflections of both the fundamental and up to ten different SHG waves at each interface, adding significant complexity. Many approximations have therefore been employed in the existing analytical approaches, such as slowly varying approximation, weak reflection of the nonlinear polarization, transparent medium, high crystallographic symmetry, Kleinman symmetry, easy crystal orientation along a high-symmetry direction, phase matching conditions and negligible interference among nonlinear waves, which may lead to large errors in the reported material properties. To avoid these approximations, we have developed an open-source package named Second Harmonic Analysis of Anisotropic Rotational Polarimetry in Multilayers (♯SHAARP.ml). The reliability and accuracy are established by experimentally benchmarking with both the SHG polarimetry and Maker fringes using standard and commonly used nonlinear optical materials as well as twisted 2-dimensional heterostructures.

Characterization of the ESPRESSO line-spread function and improvement of the wavelength calibration accuracy

ABSTRACT Achieving a truly accurate wavelength calibration of high-dispersion echelle spectrographs is a challenging task but crucially needed for certain science cases, e.g. to test for a possible variation of the fine-structure constant in quasar spectra. One of the spectrographs best suited for this mission is Very Large Telescope/Echelle SPectrograph for Rocky Exoplanets and Stable Spectroscopic Observation (ESPRESSO). Nevertheless, previous studies have identified significant discrepancies between the classical wavelength solutions and the one derived independently from the laser frequency comb. The dominant parts of these systematics were intra-order distortions, most-likely related to a deviation of the instrumental line-spread function from the assumed Gaussian shape. Here, we therefore present a study focused on a detailed modelling of the ESPRESSO instrumental line-spread function. We demonstrate that it is strongly asymmetric, non-Gaussian, different for the two slices and fibres, and varies significantly along the spectral orders. Incorporating the determined non-parametric model in the wavelength calibration process drastically improves the wavelength calibration accuracy, reducing the discrepancies between the two independent wavelength solutions from $50\,\rm{m\,s^{-1}}$ to about $10\, \rm{m\,s^{-1}}$. The most striking success is, however, that the different fibres and slices now provide fully consistent measurements with a scatter of just a couple m s−1. This demonstrates that the instrument-related systematics can be nearly eliminated over most of the spectral range by properly taking into account the complex shape of the instrumental line-spread function and paves the way for further optimizations of the wavelength calibration process.

Growth, optical and thermal properties of YbxHo1-xCa4O(BO3)3 crystals

YbxHo1-xCa4O(BO3)3 (Yb:HoCOB, x = 0, 0.1, 0.2, 0.3) crystals were grown by the Bridgman method for the first time. The crystal structure, rocking curve, transmission spectra, absorption spectra, band structure and thermal properties of Yb:HoCOB were characterized in detail. The maximum half peak width (FMHW) of Yb0.1Ho0.9COB and Yb0.2Ho0.8COB is 26.7″ and 23.8″, respectively, and the effective segregation coefficient is greater than 0.9. In addition, the transmittance of Yb:HoCOB is 88 %. New absorption peaks are introduced by doping Yb3+ at 850–1000 nm. The UV absorption cut-off edge of Yb:HoCOB is red-shifted with increasing Yb3+ doping. The thermal diffusivity and thermal conductivity of Yb:HoCOB decrease with increasing temperature. The specific heat increases with the increasing temperature and finally approaches a constant value. The specific heat of Yb:HoCOB crystal are above 0.670 J/gK at room temperature. Yb:HoCOB with good crystallization quality, high transmittance and high specific heat has the application potential in laser frequency and QPCPA. This work provides a useful exploration for the study of nonlinear optical materials in solid state lasers.

Laser and radio frequency technologists in the treatment of degenerative polysegmental pathologies of the spine in elderly people

The article discusses outcomes after treating 88 elderly patients with degenerative pathologies of the spine, 42 of whom had previous decompression- stabilizing surgical interventions. Clinical manifestations of the disease were characterized by prolonged pain syndrome, lumboishialgia caused by degenerative-dystrophic changes in the arch-process joints and progressive degeneration of the intervertebral discs. Surgical intervention in 65 patients included puncture laser ablation of the medial branch of the spinal nerve in the facet joint. In 23 patients, ablation of the medial branch of the spinal nerve was performed at two (n = 8) and three (n = 15) levels using four-channel radio frequency generator COSMAN G4.Excellent and good results after surgery were found in 58 (65.9%) patients. The researchers assessed intermediate results within 3 years in 55 patients, and 37 (42.01%) of them had a stable positive state. Minimally invasive laser and radiofrequency technologies in the treatment of degenerative polysegmental pathologies of the spine in elderly and old people is justifi ed, and it is an important component of their rehabilitation

Simultaneous effect of medicinal plants as natural photosensitizers and low-level laser on photodynamic inactivation.

Photodynamic inactivation (PDI) technology is a promising alternative to antibiotics. This technology is defined as the inhibition of bacterial growth with photosensitizers while irradiated with low-level laser light in the wavelength of 532 ± 2.08nm. A challenging area in this field is selecting photosensitizers with antibacterial potential. In this paper, to enhance the antibacterial efficiency, the photosensitizers (the selected plant extracts) with a high absorption peak at the selected laser frequency, 532nm, were prepared. Low-concentration ethanolic plant extracts of Hibiscus sabdariffa and Opuntia ficus-indica were found to exhibit significant antibacterial activity against, Acinetobacter baumannii ATCC 19606 and, Staphylococcus aureus ATCC 33591 as two important human pathogenic bacteria. The effectiveness of these natural photosensitizers was measured by determining their Minimum Inhibitory Concentration (MIC) and Minimum Bactericidal Concentration (MBC) values and by performing a time-killing assay in the absence and the presence of laser irradiation. Our results showed that the combination of low-level laser irradiation and the selected photosensitizers had excellent potential for treating in vitro bacterial infections. Therefore, PDI technology has great potential as a viable alternative to traditional antibiotics for combating bacterial infections. This study presents a promising avenue for further exploration of PDI and the use of laser technology in medical science.

Fabrication of Al/Au hybrid SERS substrate using laser engraving for rapid detection of melamine and its analogues by hand-held Raman spectrometer

Surface-enhanced Raman spectroscopy (SERS), combined with a handheld Raman spectrometer, was utilized for the rapid and highly sensitive detection of melamine and its analogues. The investigation focused on the hybrid micro-nano structures of SERS-active substrates, fabricated by laser engraving aluminum (Al) sheets and depositing gold (Au) nanoparticles using magnetron sputtering. The laser engraving frequency was varied to get optimum SERS substrate. The fabricated SERS substrates were tested with rhodamine 6G (R6G) to optimize the Raman signal and subsequently detect melamine and its analogues viz., cyanuric acid, ammeline, ammelide in milk samples. The results demonstrated that a laser frequency of 20 kHz was the optimal condition for fabricating a micro-nano Al template with a depth of 61.21 μm, providing the highest Raman signal for R6G. The limit of detection (LOD) for melamine in mild acid solution and milk samples were determined to be 1x10-5 M and 1x10-4 M, respectively. The laser-engraved Al sheet technique offers a cost-effective approach for SERS substrate fabrication. The integration of the Al/Au hybrid SERS substrate with a hand-held Raman spectrometer demonstrates significant potential for detecting melamine and its analogues in realistic environments.

Optimization and GRA prediction of Al–Cu pulsed laser welding process based on RSM

In this paper, the process parameters of pulsed laser welding of Al–Cu are studied using response surface methodology (RSM) and grey relation analysis (GRA) to propose optimal directions for lap-shear strength of the joints. A single-factor experiment was conducted to find the suitable process parameter windows. The RSM models were established and analyzed with laser power, welding speed, pulse width, and frequency as inputs and joint lap shear, interfacial weld width, and weld-penetration-depth as outputs. With the use of GRA of interfacial weld width and weld penetration depth with the lap-shear force of joints, the improved direction for the lap-shear force of joints can be proposed.

Absolute Ranging with Time Delay Interferometry for Space-Borne Gravitational Wave Detection.

In future space-borne gravitational wave (GW) detectors, time delay interferometry (TDI) will be utilized to reduce the overwhelming noise, including the laser frequency noise and the clock noise etc., by time shifting and recombining the data streams in post-processing. The successful operation of TDI relies on absolute inter-satellite ranging with meter-level precision. In this work, we numerically and experimentally demonstrate a strategy for inter-satellite distance measurement. The distances can be coarsely determined using the technique of arm-locking ranging with a large non-ambiguity range, and subsequently TDI can be used for precise distance measurement (TDI ranging) by finding the minimum value of the power of the residual noises. The measurement principle is introduced. We carry out the numerical simulations, and the results show millimeter-level precision. Further, we perform the experimental verifications based on the fiber link, and the distances can be measured with better than 0.05 m uncertainty, which can well satisfy the requirement of time delay interferometry.

Modulation transfer spectroscopy of the D1 transition of potassium: theory and experiment

We report on a study of modulation transfer spectroscopy of the 4S1/2→4P1/2 (D1) transition of naturally abundant potassium in a room-temperature vapour cell. This transition is critical for laser cooling and optical pumping of potassium and our study is therefore motivated by the need for robust laser frequency stabilisation. Despite the absence of a closed transition, the small ground-state hyperfine splitting in potassium results in strong crossover features in the D1 modulation transfer spectrum. To emphasise this we compare the D1 and D2 spectra of potassium with those of rubidium. Further, we compare our experimental results with a detailed theoretical simulation, examining different pump–probe polarisation configurations to identify the optimal signals for laser frequency stabilisation. We find good agreement between the experiment and the theory, especially for the lin∥lin polarisation configuration.

1/f Noise Mitigation in an Opto-Mechanical Sensor with a Fabry-Pérot Interferometer.

Low-frequency and 1/f noise are common measurement limitations that arise in a variety of physical processes. Mitigation methods for these noises are dependent on their source. Here, we present a method for removing 1/f noise of optical origin using a micro-cavity Fabry-Pérot (FP) interferometer. A mechanical modulation of the FP cavity length was applied to a previously studied opto-mechanical sensor. It effectively mimics an up-conversion of the laser frequency, shifting signals to a region where lower white-noise sources dominate and 1/f noise is not present. Demodulation of this signal shifts the results back to the desired frequency range of observation with the reduced noise floor of the higher frequencies. This method was found to improve sensitivities by nearly two orders of magnitude at 1 Hz and eliminated 1/f noise in the range from 1 Hz to 4 kHz. A mathematical model for low-finesse FP cavities is presented to support these results. This study suggests a relatively simple and efficient method for 1/f noise suppression and improving the device sensitivity of systems with an FP interferometer readout.

Enhancing frequency stability and mode control in a Brillouin random fiber laser with a strongly scattering disordered grating

Random fiber lasers (RFLs) with disordered scattering feedback media provide a range of functionalities and properties. The primary drawback with weak Rayleigh scattering (RS)-based RFLs is their large frequency drift and mode hopping, which are caused by the random walk of photons at different round trips. Here, we present a technique to control the mode propagation of RFLs by using a narrow gain bandwidth from stimulated Brillouin scattering and photon localization from a strongly scattering disordered grating. Multiple scattering of light within the disordered grating leads to photon localization and narrow reflection peaks, which suppresses frequency drift and reduces the number of modes. The compact Brillouin random fiber laser (BRFL) with a 200 m strongly scattering disordered grating enables single-mode lasing with an ultra-narrow linewidth of ∼650 Hz. The results of the real-time spectral evolution obtained by the heterodyne method demonstrate long-term stability of the lasing frequency, confirming the capability of the strongly scattering disordered grating to control mode propagation of the BRFL. The BRFL exhibits an ultra-high frequency stability of 0.48 MHz and mode-hop-free operation up to 120 s. This work provides a perspective on the development of RFLs with high coherence and stability.

Frequency-comb-linearized, widely tunable lasers for coherent ranging

Tunable lasers, with the ability to continuously vary their emission wavelengths, have found widespread applications across various fields such as biomedical imaging, coherent ranging, optical communications, and spectroscopy. In these applications, a wide chirp range is advantageous for large spectral coverage and high frequency resolution. Besides, the frequency accuracy and precision also depend critically on the chirp linearity of the laser. While extensive efforts have been made on the development of many kinds of frequency-agile, widely tunable, narrow-linewidth lasers, wideband yet precise methods to characterize and linearize laser chirp dynamics are also demanded. Here we present an approach to characterize laser chirp dynamics using an optical frequency comb. The instantaneous laser frequency is tracked over terahertz bandwidth at 1 MHz intervals. Using this approach we calibrate the chirp performance of 12 tunable lasers from Toptica, Santec, New Focus, EXFO, and NKT that are commonly used in fiber optics and integrated photonics. In addition, with acquired knowledge of laser chirp dynamics, we demonstrate a simple frequency-linearization scheme that enables coherent ranging without any optical or electronic linearization unit. Our approach not only presents novel wideband, high-resolution laser spectroscopy, but is also critical for sensing applications with ever-increasing requirements on performance.

Ytterbium femtosecond fiber laser ablation synthesis of silicon nanocrystals in water: Laser frequency and pulse energy dependence

The utilization of femtosecond laser pulses in synthesizing spherical silicon nanocrystals (SiNCs) poses great potential in producing stable nanostructures with chemically pure surfaces and easy-to-manipulate optical properties. In this work, we present an approach that enhances the production and optical quality of surfactant-free spherical SiNCs synthesized in water by ablating silicon wafers with ytterbium fiber femtosecond laser operating at different pulse energies and repetition rates. By further post-synthesis laser treatment of SiNCs suspensions, fragmentation of larger aggregates is observed leading to absorption broadening and absorption-band blueshift. Furthermore, the increase in the repetition rate, from 1 to 500 kHz, of laser pulses having energies of 20 and 240 μJ leads to a decrease in the Si wafer ablation efficiency from 35 to 1.15 pg/pulse; and from 440 to 5.2 pg/pulse, respectively. Using laser pulses with energy of 240 μJ and a repetition rate of 50 kHz results in maximum SiNCs productivity of 33 mg/h. The dependence of the nanostructures's size and ablation efficiency on the pulse energy and repetition rate is attributed to thermal effects on the Si/water interface and within the water layer illuminated by the strong laser radiation.

Use Of Laser Phototherapy In The Treatment Of Trigeminal Neuralgia

Responsible for the sensory stimuli of the viscerocranium, the 5th pair of cranial nerves, called the trigeminal nerve due to its 3 branches, is a mixed-function nerve. The diagnosis of Trigeminal Neuralgia is directly related to the symptoms reported by the patient during the anamnesis. The right treatment depends on the correct diagnosis. The exact etiology of TN is still unknown. It affects around 4 to 13 individuals per 100,000 and although it seems to be a neuropathy with a low incidence, it is the most common among facial pain syndromes. A retrospective cross-sectional observational study was carried out. We used data on laser therapy treatment for Trigeminal Neuralgia, received and treated at the Laser Clinic of the Faculty of Dentistry of the Federal University of Bahia, from 2003 to 2022. A total of 119 patients with a diagnosis of Trigeminal Neuralgia were treated, most of them with unilateral pain (89%). After diagnosis, the initial irradiation protocol was determined individually. The laser frequency applied was 808 nm (infrared) due to its greater ability to penetrate and activate chromophores in nerve and bone structures. The amount of energy applied varies from case to case, usually starting with 2 or 3 J per point, which is indicated for cases of regeneration and analgesia. The final status of the treatment is based on the patient’s score according to the visual analog scale, where 10 is the highest pain threshold and 0 is no pain. 65% of the patients related no pain or ate at least under 3 grades before the first degree Laser phototherapy is an effective means of recovery, reducing pain symptoms and improving the quality of life of patients with Trigeminal Neuralgia, and the infrared wave spectrum is the most suitable for this treatment.

Research on Fiber-Optic Optical Coherence Ranging System Based on Laser Frequency Scanning Interferometry.

In this paper, a system for absolute distance measurement is proposed based on laser frequency scanning interferometry (FSI). The system utilizes a digitally tunable laser as the light source and employs synchronized pulses to drive an analog-to-digital converter (ADC) for interference signal acquisition. The frequency domain demodulation for absolute distance measurement is achieved through a three-spectrum line interpolation method based on the Hanning window. The system takes advantage of the spatial filtering characteristics of a single-mode optical fiber and the diffuse reflection properties of light to achieve a high integration of the prism system that forms the interference optical path. The resulting integrated fiber-optic probe is capable of measuring the distance to a non-cooperative target even when oriented at a certain angle with the target. We designed and fabricated a portable prototype. Experimental validation demonstrated that the maximum measurement distance of the system is 73.51 mm with a standard deviation of less than 0.19 μm for optimal measurement results. Even when there is an offset angle, the system maintains good measurement repeatability.

Optical cavity spectroscopy using heterodyne detection with optical feedback laser frequency locking.

We demonstrate an accurate high sensitivity method for cavity spectroscopy. We measure the frequency intervals of transverse electromagnetic modes relative to a fundamental mode in a high finesse optical resonator, and attribute their mode numbers unambiguously. A laser is frequency locked to a fundamental T E M 00 cavity mode by optical feedback, and phase modulation is used to obtain frequency side bands, which may come to resonance with other transverse cavity modes as the radio-frequency of the modulation is tuned. At these resonances, transmission of the side bands is sensitively detected by heterodyning with the carrier. We also analyze the transverse spatial profile of the heterodyne signal for identification of mode numbers. The adjustment of the Gaussian cavity model to the measured frequency intervals yields values of cavity length, mirror radius of curvature, and mirror ellipticity, with high precision to the ppm level.

Lidar Observations of the Fe Layer in the Mesopause and Lower Thermosphere over Beijing (40.5° N, 116.0° E) and Mohe (53.5° N, 122.4° E)

Lidar observations of metal layers play a significant role in research on the chemistry and dynamics of the mesosphere and lower thermosphere. This work reports on Fe lidar observations conducted in Beijing and Mohe. Utilizing the same laser emission system, a 1064 nm seed laser was injected into an Nd: YAG laser to generate a single longitudinal-mode pulse 532 nm laser, which pumped a dye laser to produce a 572 nm laser. The 572 nm laser and the remaining 1064 nm fundamental frequency laser passed through a sum–frequency module to generate a 372 nm laser to detect the Fe layer. According to a total of 52.6 h of observations for 10 nights in Beijing, the Fe layer has an average column density of 1.24 × 1010 cm−2, an RMS width of 4.4 km and a centroid altitude of 89.4 km. In Mohe, observed for 16 nights and a total of 91.5 h, the Fe layer has an average column density of 1.08 × 1010 cm−2, an RMS width of 4.6 km and a centroid altitude of 89.5 km. The probability of the occurrence of sporadic Fe layers was 42.4% in Beijing and 29.4% in Mohe. Compared to simultaneously observed Na layers, the occurrence probabilities of sporadic Fe layers were higher than those of sporadic Na layers in both stations. Based on the two cases observed in Beijing, it is conjectured that the formation mechanism of sporadic metal layers above approximately 100 km has a more significant influence on sporadic Fe layers than on sporadic Na layers. The lower thermospheric Fe layers with densities significantly larger than those of the main layer were observed during two nights in Mohe. This work contributes to the refinement of the global distribution of Fe layers and provides abundant observational data for the modeling and study of the metal layers.