Frequency Comb Formation Research Articles

Dynamic gain and frequency comb formation in exceptional-point lasers

Exceptional points (EPs)—singularities in the parameter space of non-Hermitian systems where two nearby eigenmodes coalesce—feature unique properties with applications such as sensitivity enhancement and chiral emission. Existing realizations of EP lasers operate with static populations in the gain medium. By analyzing the full-wave Maxwell–Bloch equations, here we show that in a laser operating sufficiently close to an EP, the nonlinear gain will spontaneously induce a multi-spectral multi-modal instability above a pump threshold, which initiates an oscillating population inversion and generates a frequency comb. The efficiency of comb generation is enhanced by both the spectral degeneracy and the spatial coalescence of modes near an EP. Such an “EP comb” has a widely tunable repetition rate, self-starts without external modulators or a continuous-wave pump, and can be realized with an ultra-compact footprint. We develop an exact solution of the Maxwell–Bloch equations with an oscillating inversion, describing all spatiotemporal properties of the EP comb as a limit cycle. We numerically illustrate this phenomenon in a 5-μm-long gain-loss coupled AlGaAs cavity and adjust the EP comb repetition rate from 20 to 27 GHz. This work provides a rigorous spatiotemporal description of the rich laser behaviors that arise from the interplay between the non-Hermiticity, nonlinearity, and dynamics of a gain medium.

Synthetic reflection self-injection-locked microcombs

Laser-driven microresonators have enabled chip-integrated light sources with unique properties, including the self-organized formation of ultrashort soliton pulses and frequency combs (microcombs). While poised to impact major photonic applications such as spectroscopy, sensing and optical data processing, microcombs still necessitate complex scientific equipment to achieve and maintain suitable single-pulse operation. Here to address this challenge, we demonstrate microresonators with programmable synthetic reflection providing tailored injection feedback to the driving laser. Synthetic reflection achieves independence from random sample scattering properties and, when designed appropriately, enables deterministic access to self-injection-locked microcombs operating exclusively in the single-soliton regime. These results provide a route to easily operable microcombs at scale for portable sensors, autonomous navigation or extreme-bandwidth data processing. The novel concept of synthetic reflection may also be generalized to other integrated photonic systems.

Dispersion engineering in a Brillouin fiber laser cavity for Kerr frequency comb formation

We conduct numerical and experimental investigations on Kerr comb generation in a nonlinear and non-reciprocal fiber cavity by leveraging both stimulated Brillouin backscattering and cascaded four-wave mixing. By engineering the net cavity dispersion to be either normal or anomalous, we enable the formation of diverse patterns and localized structures in the cavity field. The comb’s properties depend crucially on the mismatch between the frequency spacing of the bichromatic pump and the free spectral range of the Brillouin laser cavity in both cases. Particularly, in the anomalous regime, adjusting this parameter yields coherent, stable frequency combs in the modulation instability regime. This allows control and expansion of the spectral bandwidth up to 2 THz in normal dispersion and to 6 THz under anomalous net dispersion. This versatile and easily reconfigurable method holds potential for applications in high-speed communications and microwave synthesis.

Frequency combs in optically injected terahertz ring quantum cascade lasers

Quantum cascade lasers (QCLs) have emerged as promising candidates for generating chip-scale frequency combs in mid-infrared and terahertz wavelengths. In this work, we demonstrate frequency comb formation in ring terahertz QCLs using the injection of light from a distributed feedback (DFB) laser. The DFB design frequency is chosen to match the modes of the ring cavity (near 3.3 THz), and light from the DFB is injected into the ring QCL via a bus waveguide. By controlling the power and frequency of the optical injection, we show that combs can be selectively formed and controlled in the ring cavity. Numerical modeling suggests that this comb is primarily frequency-modulated in character, with the injection serving to trigger comb formation. We also show that the ring can be used as a filter to control the output of the DFB QCL, potentially being of interest in terahertz photonic integrated circuits. Our work demonstrates that waveguide couplers are a compelling approach for injecting and extracting radiation from ring terahertz combs and offer exciting possibilities for the generation of new comb states in terahertz, such as frequency-modulated waves, solitons, and more.

Nonlinear dynamics and Kerr frequency comb formation in lattices of coupled microresonators

Recently, substantial progress has been made in the understanding of microresonators frequency combs based on dissipative Kerr solitons (DKSs). However, most of the studies have focused on the single-resonator level. Coupled resonator systems can open new avenues in dispersion engineering and exhibit unconventional four-wave mixing (FWM) pathways. However, these systems still lack theoretical treatment. Here, starting from general considerations for the N-(spatial) dimensional case, we derive a model for a one-dimensional lattice of microresonators having the form of the two-dimensional Lugiato-Lefever equation (LLE) with a complex dispersion surface. Two fundamentally different dynamical regimes can be identified in this system: elliptic and hyperbolic. Considering both regimes, we investigate Turing patterns, regularized wave collapse, and 2D (i.e., spatio-temporal) DKSs. Extending the system to the Su-Schrieffer-Heeger model, we show that the edge-state dynamics can be approximated by the conventional LLE and demonstrate the edge-bulk interactions initiated by the edge-state DKS.

Efficient computation of coherent multimode instabilities in lasers using a spectral approach

Coherent multimode instabilities are responsible for several phenomena of recent interest in semiconductor lasers, such as the generation of frequency combs and ultrashort pulses. These techonologies have proven disruptive in optical telecommunications and spectroscopy applications. While the standard Maxwell-Bloch equations (MBEs) encompass such complex lasing phenomena, their integration is computationally expensive and offers limited analytical insight. In this paper, we demonstrate an efficient spectral approach to the simulation of multimode instabilities via a quantitative analysis of the instability of single-frequency lasing in ring lasers, referred to as the Lorenz-Haken (LH) instability or the RNGH instability in distinct parameter regimes. Our approach, referred to as CFTD, uses generally non-Hermitian Constant Flux modes to obtain projected Time Domain equations. CFTD provides excellent agreement with finite-difference integration of the MBEs across a wide range of parameters in regimes of non-stationary inversion, including frequency comb formation and spatiotemporal chaos. We also develop a modal linear stability analysis using CFTD to efficiently predict multimode instabilities in lasers. The combination of numerical accuracy, speedup, and semi-analytic insight across a variety of dynamical regimes make the CFTD approach ideal to analyze multimode instabilities in lasers, especially in more complex geometries or coupled laser arrays.

Coupling dynamics of dissipative localized structures: From polarized vector solitons to soliton molecules

Dissipative solitons are well known as representative nonlinear localized wave packets resulting from the composite balance of dispersion, nonlinearity, gain and loss in optical cavities. Since the last three decades, dissipative solitons keep as one of the most active research topics in the framework of nonlinear physics, not only for fundamental researches but also for various industrial applications. From one hand, due to the rich nonlinear dynamics, dissipative solitons have been considered as an ideal testbed to study the pumping-dissipation-bifurcation complexities. On the other hand, the emergences of dissipative solitons are tightly linked with the emission of ultrashort laser pulses, as well as the formation of broadband optical frequency combs. Compared with single-soliton counterpart, the multi-component dissipative solitons have exhibited even more fascinating properties and much wider range of applications, therefore the coupling dynamics of dissipative solitons is the blooming and emergent research area in the last decade. From this point of view, this review article covers the latest developments of compound dissipative solitons, not only in passive Kerr resonators, but also in mode-locked laser cavities. Ranging from polarized vector solitons to soliton molecules, the rising degree of freedom of these multi-component localized structures is boosting the discovery of novel nonlinear dynamics and underpin the various photonic applications in light science.

Low-voltage dielectric elastomer actuators by electro-mechanical resonance syntonization

Generally, a serious practical limitation of dielectric elastomer (DE)-based capacitors is the need for high voltage supply (in the order of 1 kV) to activate them. High voltages require a power level that is currently challenging due to the limit in the operating range of existing function generators. These high voltages are also dangerous for humans, thereby overshadowing many applications of dielectric elastomers. The purpose of this work is to develop a new simple actuation technique to introduce low-voltage driven DE-based capacitors, in which the electrical resonant frequency is syntonized to the mechanical natural frequency by tuning the circuit inductance. This results in extensive voltage amplification across the DE capacitor. In turn, this leads the DE membrane to oscillate with a remarkable large motion using a small voltage which is of one-tenth the magnitude of the input voltage required to drive such systems in the absence of electro-mechanical (EM) resonance syntonization. The efficiency of the proposed approach is demonstrated in the context of nonlinear vibration analysis. The results show that the voltage amplitude across the DE capacitor is amplified substantially while the electrical mode is syntonized with the mechanical one, and as a result, the DE motion’s amplitude is at least two hundred times greater than that of the unmatched system. Furthermore, for unbiased AC voltages with large amplitudes, the electro-mechanical modal interaction causes the system to exhibit the formation of frequency combs in the frequency spectrum of the system’s response. The implementation of this method using a simple electrical circuit just requires adequate matching between the electrical and the mechanical natural frequencies that depends on the inductance value. Our proposal effectively eliminates the need for a high source voltage generator which has been the main limitation in designing DE-based capacitors.

Sensitive dependence of the linewidth enhancement factor on electronic quantum effects in quantum cascade lasers

The linewidth enhancement factor (LEF) describes the coupling between amplitude and phase fluctuations in a semiconductor laser and has recently been shown to be a crucial component for frequency comb formation in addition to linewidth broadening. It necessarily arises from causality, as famously formulated by the Kramers–Kronig relation, in media with nontrivial dependence of the susceptibility on intensity variations. While thermal contributions are typically slow, and thus can often be excluded by suitably designing the dynamics of an experiment, the many quantum contributions are harder to separate. In order to understand and, ultimately, design the LEF to suitable values for frequency comb formation, soliton generation, or narrow laser linewidth, it is, therefore, important to systematically model all these effects. In this comprehensive work, we introduce a general scheme for computing the LEF, which we employ with a nonequilibrium Green's function model. This direct method, based on simulating the system response under varying optical intensity and extracting the dependence of the susceptibility to intensity fluctuations, can include all relevant electronic effects and predicts the LEF of an operating quantum cascade laser to be in the range of 0.1–1, depending on laser bias and frequency. We also confirm that many-body effects, off-resonant transitions, dispersive (Bloch) gain, counter-rotating terms, intensity-dependent transition energy, and precise subband distributions all significantly contribute and are important for accurate simulations of the LEF.

Spin-wave frequency combs

We experimentally demonstrate the generation of spin-wave frequency combs based on the nonlinear interaction of propagating spin waves in a microstructured waveguide. By means of time- and space-resolved Brillouin light scattering spectroscopy, we show that the simultaneous excitation of spin waves with different frequencies leads to a cascade of four-magnon scattering events, which ultimately results in well-defined frequency combs. Their spectral weight can be tuned by the choice of amplitude and frequency of the input signals. Furthermore, we introduce a model for stimulated four-magnon scattering, which describes the formation of spin-wave frequency combs in the frequency and time domain.

A normal form for frequency combs and localized states in Kerr-Gires-Tournois interferometers.

We elucidate the mechanisms that underlay the formation of temporal localized states and frequency combs in vertical external-cavity Kerr-Gires-Tournois interferometers. We reduce our first-principles model based upon delay algebraic equations to a minimal pattern formation scenario. It consists in a real cubic Ginzburg-Landau equation modified by high-order effects such as third-order dispersion and nonlinear drift, which are responsible for generating localized states via the locking of domain walls connecting the high and low intensity levels of the injected micro-cavity. We interpret the effective parameters of the normal form in relation with the configuration of the optical setup. Comparing the two models, we observe an excellent agreement close to the onset of bistability.

Multimode Physics in the Mode Locking of Semiconductor Quantum Dot Lasers

Quantum dot lasers are an attractive option for light sources in silicon photonic integrated circuits. Thanks to the three-dimensional charge carrier confinement in quantum dots, high material gain, low noise and large temperature stability can be achieved. This paper discusses, both theoretically and experimentally, the advantages of silicon-based quantum dot lasers for passive mode-locking applications. Using a frequency domain approach, i.e., with the laser electric field described in terms of a superposition of passive cavity eigenmodes, a precise quantitative description of the conditions for frequency comb and pulse train formation is supported, along with a concise explanation of the progression to mode locking via Adler’s equation. The path to transform-limited performance is discussed and compared to the experimental beat-note spectrum and mode-locked pulse generation. A theory/experiment comparison is also used to extract the experimental group velocity dispersion, which is a key obstacle to transform-limited performance. Finally, the linewidth enhancement contribution to the group velocity dispersion is investigated. For passively mode-locked quantum dot lasers directly grown on silicon, our experimental and theoretical investigations provide a self-consistent accounting of the multimode interactions giving rise to the locking mechanism, gain saturation, mode competition and carrier-induced refractive index.

Silicon integrated terahertz quantum cascade ring laser frequency comb

We demonstrate terahertz quantum cascade lasers realized in “ideal” ring resonators without discontinuities from, e.g., contacting pads. We realize this by mounting rings episide-down on a silicon substrate by a die-bonding technique. This technique allows one to realize ideal conditions for optical confinement as well as heat dissipation and provides the basis for future Si integrated THz devices. The lasers emit light around 3.8 THz and show much reduced threshold current densities. When operated in continuous-wave operation, frequency comb formation with a spectral bandwidth of 70 GHz is observed. Frequency comb operation is indicated by a narrow beat note signal at 8.55 GHz with a signal-to-noise ratio up to 40 dB. The experimentally measured spectral behavior of ring devices is described accurately by the results obtained from numerical simulations based on the Maxwell–Bloch formalism.

Nearly Quantum-Limited Josephson-Junction Frequency-Comb Synthesizer

While coherently-driven Kerr microcavities have rapidly matured as a platform for frequency comb formation, such microresonators generally possess weak Kerr coefficients; consequently, triggering comb generation requires millions of photons to be circulating inside the cavity. This suppresses the role of quantum fluctuations in the comb's dynamics. In this paper, we realize a minimal version of coherently-driven Kerr-mediated microwave frequency combs in the circuit QED architecture, where the quantum vacuum's fluctuations are the primary limitation on comb coherence. We achieve a comb phase coherence of up to 35~$\mu$s, approaching the theoretical device quantum limit of 55~$\mu$s, and vastly longer than the modes' inherent lifetimes of 13~ns. The ability within cQED to engineer stronger nonlinearities than optical microresonators, together with operation at cryogenic temperatures, and excellent agreement of comb dynamics with quantum theory indicates a promising platform for the study of complex dynamics of quantum nonlinear systems

Reversible Self-Replication of Spatiotemporal Kerr Cavity Patterns.

We uncover a novel and robust phenomenon that causes the gradual self-replication of spatiotemporal Kerr cavity patterns in cylindrical microresonators. These patterns are inherently synchronized multifrequency combs. Under proper conditions, the axially localized nature of the patterns leads to a fundamental drift instability that induces transitions among patterns with a different number of rows. Self-replications, thus, result in the stepwise addition or removal of individual combs along the cylinder's axis. Transitions occur in a fully reversible and, consequently, deterministic way. The phenomenon puts forward a novel paradigm for Kerr frequency comb formation and reveals important insights into the physics of multidimensional nonlinear patterns.

Frequency comb generation in a pulse-pumped normal dispersion Kerr mini-resonator.

Kerr microresonators driven in the normal dispersion regime typically require the presence of localized dispersion perturbations, such as those induced by avoided mode crossings, to initiate the formation of optical frequency combs. In this work, we experimentally demonstrate that this requirement can be lifted by driving the resonator with a pulsed pump source. We also show that controlling the desynchronization between the pump repetition rate and the cavity free-spectral range (FSR) provides a simple mechanism to tune the center frequency of the output comb. Using a fiber mini-resonator with a radius of only 6 cm, we experimentally present spectrally flat combs with a bandwidth of 3 THz whose center frequency can be tuned by more than 2 THz. By driving the cavity at harmonics of its 0.54 GHz FSR, we are able to generate combs with line spacings selectable between 0.54 and 10.8 GHz. The ability to tune both the center frequency and frequency spacing of the output comb highlights the flexibility of this platform. Additionally, we demonstrate that under conditions of large pump-cavity desynchronization, the same cavity also supports a new, to the best of our knowledge, form of Raman-assisted anomalous dispersion cavity soliton.

Thermal instabilities, frequency-comb formation, and temporal oscillations in Kerr microresonators

We analyze the consequences of dissipative heating in driven Kerr microresonators theoretically and numerically, using a thermal Lugiato-Lefever model. We show that thermal sensitivity modifies the stability range of continuous wave in a way that blocks direct access to broadband frequency-comb forming waveforms, and we propose a deterministic access path that bypasses the thermal instability barrier. We describe a novel thermal instability that leads to thermooptical oscillations via a Hopf bifurcation.

Optical Frequency Combs in Quadratically Nonlinear Resonators.

Optical frequency combs are one of the most remarkable inventions in recent decades. Originally conceived as the spectral counterpart of the train of short pulses emitted by mode-locked lasers, frequency combs have also been subsequently generated in continuously pumped microresonators, through third-order parametric processes. Quite recently, direct generation of optical frequency combs has been demonstrated in continuous-wave laser-pumped optical resonators with a second-order nonlinear medium inside. Here, we present a concise introduction to such quadratic combs and the physical mechanism that underlies their formation. We mainly review our recent experimental and theoretical work on formation and dynamics of quadratic frequency combs. We experimentally demonstrated comb generation in two configurations: a cavity for second harmonic generation, where combs are generated both around the pump frequency and its second harmonic and a degenerate optical parametric oscillator, where combs are generated around the pump frequency and its subharmonic. The experiments have been supported by a thorough theoretical analysis, aimed at modelling the dynamics of quadratic combs, both in frequency and time domains, providing useful insights into the physics of this new class of optical frequency comb synthesizers. Quadratic combs establish a new class of efficient frequency comb synthesizers, with unique features, which could enable straightforward access to new spectral regions and stimulate novel applications.

Coherent master equation for laser modelocking

Modelocked lasers constitute the fundamental source of optically-coherent ultrashort-pulsed radiation, with huge impact in science and technology. Their modeling largely rests on the master equation (ME) approach introduced in 1975 by Hermann A. Haus. However, that description fails when the medium dynamics is fast and, ultimately, when light-matter quantum coherence is relevant. Here we set a rigorous and general ME framework, the coherent ME (CME), that overcomes both limitations. The CME predicts strong deviations from Haus ME, which we substantiate through an amplitude-modulated semiconductor laser experiment. Accounting for coherent effects, like the Risken-Nummedal-Graham-Haken multimode instability, we envisage the usefulness of the CME for describing self-modelocking and spontaneous frequency comb formation in quantum-cascade and quantum-dot lasers. Furthermore, the CME paves the way for exploiting the rich phenomenology of coherent effects in laser design, which has been hampered so far by the lack of a coherent ME formalism.

Frequency-Modulated Combs Obey a Variational Principle.

Laser dynamics encompasses universal phenomena that can be encountered in many areas of physics, such as bifurcation and chaos, mode competition, resonant nonlinearities, and synchronization-or locking-of oscillators. When a locking process occurs in a multimode laser, an optical frequency comb is produced, which is an optical spectrum consisting of equidistant modes with a fixed phase relationship. Describing the formation of self-starting frequency combs in terms of fundamental laser equations governing the field inside the cavity does not allow one, in general, to grasp how the laser synchronizes its modes. Our finding is that, in a particular class of lasers where the output is frequency modulated with small or negligible intensity modulation, a greatly simplified description of self-locking exists. We show that in quantum cascade lasers-solid-state representatives of these lasers characterized by an ultrashort carrier relaxation time-the frequency comb formation obeys a simple variational principle, which was postulated over 50years ago and relies on the maximization of the laser output power. The conditions for the breakdown of this principle are also experimentally identified, shedding light on the behavior of many different types of lasers, such as dye, diode, and other cascade lasers. This discovery reveals that the formation of frequency-modulated combs is an elegant example of an optimization problem solved by a physical system.