CO2 sequestration in geological formations is an efficient step towards mitigating climate change by reducing global warming. The CO2 emitted from natural sources and anthropogenic activities is injected into geological formations. The flow and transport of CO2 during sequestration operations require in-depth knowledge of the effects of the type of geological formation. The present work analyses the CO2 migration and storage in a heterogeneous deep saline aquifer with variable porosity and evolving permeability under non-isothermal flow conditions while upscaling the capillary pressure using the Leverett J-function. The developed numerical model is history-matched with CO2 gas saturation profiles reported using analytical and numerical approaches. The novelty of the present work lies in its ability to capture fine-scale heterogeneities in the aquifer, which is modelled through variation in the porosity (ϕ) distribution and the permeability (k). The thermal-hydraulic numerical analysis projected a pronounced effect of the degree of heterogeneity arising from the variation in porosity and permeability on pressure buildup along the top of the formation decreasing from a maximum of about 6.41 MPa at the injection well to about 0.933 MPa at 1200 m and affecting gas characteristics and transmission. The thermal front could only propagate to a maximum extent of about 142 m from the injection well in aquifers, while gas plume lengths migrated to a maximum plume length of about 1010 m. The permeability and porosity of the aquifer are critically observed to vary during the sequestration by a ratio (k/k0) of about 1.07 to 1.01 and a percentage of about 0.791 % – 3.136 % in the low permeable conditions. Maximum effective storage of CO2 by a factor of 0.95 observed in low-permeable heterogeneous aquifers with normally distributed porosity affirms maintenance of optimum gas injection rates below the fracture gradient in these formations to sequester the CO2 economically.
Read full abstract