A fast and accurate radiative transfer model is the prerequisite in the field of atmospheric remote sensing for limb atmospheric inversion to tackle the drawback of slow calculation speed of traditional atmospheric radiative transfer models. This paper established a fast computing model (ANN-HASFCM) for high-spectral-resolution absorption spectra by using artificial neural networks and PCA (principal component analysis) spectral reconstruction technology. This paper chose the line-by-line radiative transfer model (LBLRTM) as the comparative model and simulated training spectral data in the oxygen A-band (12,900–13,200 cm−1). Subsequently, ANN-HASFCM was applied to the retrieval of the atmospheric density profile with the data of the Global Ozone Monitoring by an Occultation of Stars (GOMOS) instrument. The results show that the relative error between the optical depth spectra calculated by LBLRTM and ANN-HASFCM is within 0.03–0.65%. In the process of using the global-fitting algorithm to invert GOMOS-measured atmospheric samples, the inversion results using Fast-LBLRTM and ANN-HASFCM as forward models are consistent, and the retrieval speed of ANN-HASFCM is more than 200 times faster than that of Fast-LBLRTM (reduced from 226.7 s to 0.834 s). The analysis shows the brilliant application prospects of ANN-HASFCM in limb remote sensing.
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