Foil Targets Research Articles

Integrated double-plasma-mirror targets for contrast enhancement in laser ion acceleration

We introduce a target concept for laser-driven ion acceleration with ultrashort, highly intense laser pulses that includes an integrated double plasma mirror for contrast enhancement. It comprises three nanometer thin plastic foils, embedded in a small metal structure, which ensures precise mounting. The geometry allows to apply a double plasma mirror directly in front of a target foil within the converging beam, enabling moderate-energy (∼1 J) laser systems to reach the required fluence of several hundred J/cm2 on the plasma mirrors. During an experimental campaign, performed at the Laboratory for Extreme Photonics in Munich, we observed proton energies increased by a factor of three using this new target, which is attributed to an enhanced laser contrast after the integrated double plasma mirrors.

Tandem column isolation of zirconium-89 from cyclotron bombarded yttrium targets using an automated fluidic platform: Anion exchange to hydroxamate resin columns

The development of a tandem column purification method for the preparation of high-purity 89Zr(IV) oxalate is presented. The primary column was a macroporous strongly basic anion exchange resin on styrene divinylbenzene co-polymer. The secondary column, with an internal volume of 33 μL, was packed with hydroxamate resin. A condition of inverted selectivity was developed, whereby the 89Zr eluent solution for the primary column is equivalent to the 89Zr load solution for the secondary column. The ability to transfer 89Zr from one column to the next allows two sequential column clean-up methods to be performed prior to the final elution of the 89Zr(IV) oxalate. This approach assures delivery of high purity 89Zr product and assures a 89Zr product that is eluted in a substantially smaller volume than is possible when using the traditionally-employed single hydroxamate resin column method. The tandem column purification process has been implemented into a prototype automated fluidic system. The system is configured with on-line gamma detection so column effluents can be monitored in near-real time. The automated method was tested using seven cyclotron bombarded Y foil targets. It was found that 95.1 ± 1.3% of the 89Zr present in the foils was recovered in the secondary column elution fraction. Furthermore, elution peak analysis of several 89Zr elution profile radiochromatograms made possible the determination of 89Zr recovery as a function of volume; a 89Zr product volume that contains 90% of the mean secondary column elution peak can be obtained in 0.29 ± 0.06 mL (representing 86 ± 5% of the 89Zr activity in the target). This product volume represents a significant improvement in radionuclide product concentration over the predominant method used in the field. In addition to the reduced 89Zr product elution volume, titrations of the 89Zr product with deferoxamine mesylate salt across two preparatory methods resulted in mean effective specific activity (ESA) values of 279 and 340 T Bq·mmole−1 and mean bindable metals concentrations ([MB]) of 13.5 and 16.7 nmole·g−1. These ESA and [MB] values infer that the 89Zr(IV) oxalate product resulting from this tandem column isolation method has the highest purity reported to date.

Numerical studies on pair production in ultra-intense laser interaction with a thin solid-foil

A theoretical and numerical model of photon and electron–positron pair production in strong-field quantum electrodynamics (QED) is described. Two processes are contained in our QED theoretical model, one is photon emission in the interaction of ultra-intense laser with relativistic electron (or positron), and the other is pair production by a gamma-ray photon interacting with the laser field. This model has been included in a PIC/MCC simulation code named BUMBLEBEE 1D, which is used to simulate the laser plasma interaction. Using this code, the evolutions of electron–positron pair and gamma-ray photon production in ultra-intense laser interaction with aluminum foil target are simulated and analyzed. The simulation results revealed that more positrons are moved in the opposite direction to the incident direction of the laser under the charge separation field.

Enhanced laser proton acceleration by target ablation on a femtosecond laser system

Proton acceleration during the interaction of an ultraintense (6 × 1019 W/cm2) femtosecond (fs) laser pulse with a thin (2.5 μm) foil target pre-ablated by a picosecond (ps) pulse is experimentally and numerically investigated. Enhancements in both proton cut-off energy and charge are observed with the target ablation due to a large number of energetic electrons generated from the preformed preplasma in front of the target. The enhanced proton beams are successfully collected at 4–9 MeV with ±4% energy spread and then transported to the irradiating platform. The results show that for the interaction between fs laser pulse and μm-thickness target, proton energy and charge can be enhanced by target ablation using a ps laser pulse, which is valuable for application like cancer radiotherapy.

Charge-Transfer Processes in Warm Dense Matter: Selective Spectral Filtering for Laser-Accelerated Ion Beams.

We investigate, both experimentally and theoretically, how the spectral distribution of laser accelerated carbon ions can be filtered by charge exchange processes in a double foil target setup. Carbon ions at multiple charge states with an initially wide kinetic energy spectrum, from 0.1 to 18MeV, were detected with a remarkably narrow spectral bandwidth after they had passed through an ultrathin and partially ionized foil. With our theoretical calculations, we demonstrate that this process is a consequence of the evolution of the carbon ion charge states in the second foil. We calculated the resulting spectral distribution separately for each ion species by solving the rate equations for electron loss and capture processes within a collisional radiative model. We determine how the efficiency of charge transfer processes can be manipulated by controlling the ionization degree of the transfer matter.

Multi-keV X-ray area source intensity at SGII laser facility

Experiments for investigating the feasibility of multi-keV backlighters for several different metallic foil targets were performed at the Shenguang II (SGII) laser facility in China. Emission spectra in the energy range of 1.65–7.0 keV were measured with an elliptically bent crystal spectrometer, and the X-ray source size was measured with a pinhole camera. The X-ray intensity near 4.75 keV and the X-ray source size for titanium targets at different laser intensity irradiances were studied. By adjusting the total laser energy at a fixed focal spot size, laser intensity in the range of 1.5–5.0 × 1015 W/cm2, was achieved. The results show that the line emission intensity near 4.75 keV and the X-ray source size are dependent on the laser intensity and increase as the laser intensity increases. However, an observed “peak” in the X-ray intensity near 4.75 keV occurs at an irradiance of 4.0 × 1015 W/cm2. For the employed experimental conditions, it was confirmed that the laser intensity could play a significant role in the development of an efficient multi-keV X-ray source. The experimental results for titanium indicate that the production of a large (∼350 μm in diameter) intense backlighter source of multi-keV X-rays is feasible at the SGII facility.

Highly intensified emission of laser-accelerated electrons from a foil target through an additional rear laser plasma

Highly intensified emission of laser-accelerated electrons from a foil target through an additional rear laser plasma

Ring-like spatial distribution of laser accelerated protons in the ultra-high-contrast TNSA-regime

The spatial distribution of protons accelerated from submicron-thick plastic foil targets using multi-terawatt, frequency-doubled laser pulses with ultra-high temporal contrast has been investigated experimentally. A very stable, ring-like beam profile of the accelerated protons, oriented around the target’s normal direction has been observed. The ring’s opening angle has been found to decrease with increasing foil thicknesses. Two-dimensional particle-in-cell simulations reproduce our results indicating that the ring is formed during the expansion of the proton density distribution into the vacuum as described by the mechanism of target-normal sheath acceleration. Here—in addition to the longitudinal electric fields responsible for the forward acceleration of the protons—a lateral charge separation leads to transverse field components accelerating the protons in the lateral direction.

Simulations of bremsstrahlung emission in ultra-intense laser interactions with foil targets

Bremsstrahlung emission from interactions of short ultra-intense laser pulses with solid foils is studied using particle-in-cell (PIC) simulations. A module for simulating bremsstrahlung has been implemented in the PIC loop to self-consistently account for the dynamics of the laser–plasma interaction, plasma expansion, and the emission of gamma ray photons. This module made it possible to study emission from thin targets, where refluxing of hot electrons plays an important role. It is shown that the angular distribution of the emitted photons exhibits a four-directional structure with the angle of emission decreasing with the increase of the width of the target. Additionally, a collimated forward flash consisting of high energy photons has been identified in thin targets. The conversion efficiency of the energy of the laser pulse to the energy of the gamma rays rises with both the driving pulse intensity, and the thickness of the target. The amount of gamma rays also increases with the atomic number of the target material, despite a lower absorption of the driving laser pulse. The angular spectrum of the emitted gamma rays is directly related to the increase of hot electron divergence during their refluxing and its measurement can be used in experiments to study this process.

Au197(n,2n) reaction cross section in the 15–21 MeV energy range

The cross section of the $^{197}\mathrm{Au}(n,2n)^{196}\mathrm{Au}$ reaction has been determined at six energies ranging from 15.3--20.9 MeV by means of the activation technique, relative to the $^{27}\mathrm{Al}(n,\ensuremath{\alpha})^{24}\mathrm{Na}$ reaction. Quasimonoenergetic neutron beams were produced via the $^{3}\mathrm{H}(d,n)^{4}\mathrm{He}$ reaction at the 5.5 MV Tandem T11/25 accelerator laboratory of NCSR ``Demokritos''. After the irradiations, the induced $\ensuremath{\gamma}$-ray activity of the target and reference foils was measured with high-resolution HPGe detectors. The cross section for the high spin isomeric state (${12}^{\ensuremath{-}}$) was determined along with the sum of the ground (${2}^{\ensuremath{-}}$), the first (${5}^{+}$), and second (${12}^{\ensuremath{-}}$) isomeric states. Theoretical calculations were carried out with the codes empire 3.2.2 and talys 1.8. Optimum input parameters were chosen in such a way as to simultaneously reproduce several experimental reaction channel cross sections in a satisfactory way, namely the ($n,\mathrm{elastic}$), ($n,2n$), ($n,3n$), ($n,p$), ($n,\ensuremath{\alpha}$), and ($n$,total) ones.

Direct measurements of the lifetime of medium-heavy hypernuclei

The lifetime of a Λ particle embedded in a nucleus (hypernucleus) decreases from that of free Λ decay mainly due to the opening of the ΛN→NN weak decay channel. However, it is generally believed that the lifetime of a hypernucleus attains a constant value (saturation) for medium to heavy hypernuclear masses, yet this hypothesis has been difficult to verify. This paper presents a direct measurement of the lifetime of medium-heavy hypernuclei that were hyper-fragments produced by fission or break-up from heavy hypernuclei initially produced with a 2.34 GeV photon-beam incident on thin Fe, Cu, Ag, and Bi target foils. For each event, fragments were detected in coincident pairs by a low-pressure multi-wire proportional chamber system. The lifetime was extracted from decay time spectrum formed by the difference of the time zeros between the pairs. The measured lifetime from each target is actually a statistical average over a range of mass with mean about 1/2 of the target mass and appears to be a constant of about 200 ps. Although this result cannot exclude unexpected shorter or longer lifetimes for some specific hypernuclei or hypernuclear states, it shows that a systematic decrease in lifetime as hypernuclear mass increases is not a general feature for hypernuclei with mean mass up to A≈130. On the other hand, the success of this experiment and its technique shows that the time delayed fissions observed and used by all the lifetime measurements done so far on heavy hypernuclei could likely have originated from hyper-fragments lighter than the assumed masses.

X-ray absorption spectroscopy study of energy transport in foil targets heated by petawatt laser pulses

X-ray absorption spectroscopy is proposed as a method for studying the heating of solid-density matter excited by secondary X-ray radiation from a relativistic laser-produced plasma. The method was developed and applied to experiments involving thin silicon foils irradiated by 0.5–1.5 ps duration ultrahigh contrast laser pulses at intensities between 0.5×1020 and 2.5×1020 W/cm2. The electron temperature of the material at the rear side of the target is estimated to be in the range of 140–300 eV. The diagnostic approach enables the study of warm dense matter states with low self-emissivity.

Diagnosis of warm dense conditions in foil targets heated by intense femtosecond laser pulses using Kα imaging spectroscopy.

Warm dense conditions in titanium foils irradiated with intense femtosecond laser pulses are diagnosed using an x-ray imaging spectroscopy technique. The line shapes of radially resolved titanium Kα spectra are measured with a toroidally bent GaAs crystal and an x-ray charge-coupled device. Measured spectra are compared with the K-shell emissions modeled using an atomic kinetics - spectroscopy simulation code. Kα line shapes are strongly affected by warm (5-40 eV) bulk electron temperatures and imply multiple temperature distributions in the targets. The spatial distribution of temperature is dependent on the target thickness, and a thin target shows an advantage to generate uniform warm dense conditions in a large area.

QED effects induced harmonics generation in extreme intense laser foil interaction

A new mechanism of harmonics generation (HG) induced by quantum electrodynamics (QED) effects in extreme intense laser foil interaction is found and investigated by particle-in-cell (PIC) simulations. When two laser pulses with identical intensities of are counter-incident on a thin foil target, harmonics emission is observed in their reflected electromagnetic waves. Such harmonics radiation is excited due to transversely oscillating electric currents coming from the vibration of QED effect generated pairs. The effects of laser intensity and polarization were studied. By distinguishing the cascade depth of generated photons and pairs, the influence of QED cascades on HG was analyzed. Although the current HG is not an efficient way for radiation source applications, it may provide a unique way to detect the QED processes in the near future ultra-relativistic laser solid interactions.

Radiation Pressure-Driven Plasma Surface Dynamics in Ultra-Intense Laser Pulse Interactions with Ultra-Thin Foils

The dynamics of the plasma critical density surface in an ultra-thin foil target irradiated by an ultra-intense (∼6 × 10 20 Wcm − 2 ) laser pulse is investigated experimentally and via 2D particle-in-cell simulations. Changes to the surface motion are diagnosed as a function of foil thickness. The experimental and numerical results are compared with hole-boring and light-sail models of radiation pressure acceleration, to identify the foil thickness range for which each model accounts for the measured surface motion. Both the experimental and numerical results show that the onset of relativistic self-induced transparency, in the thinnest targets investigated, limits the velocity of the critical surface, and thus the effectiveness of radiation pressure acceleration.

Optimized anion exchange column isolation of zirconium-89 (89Zr) from yttrium cyclotron target: Method development and implementation on an automated fluidic platform

Zirconium-89 (89Zr), produced by the (p, n) reaction from naturally monoisotopic yttrium (natY), is a promising positron emitting isotope for immunoPET imaging. Its long half-life of 78.4 h is sufficient for evaluating slow physiological processes. A prototype automated fluidic system, coupled to on-line and in-line detectors, has been constructed to facilitate development of new 89Zr purification methodologies. The highly reproducible reagent delivery platform and near-real time monitoring of column effluents allows for efficient method optimization. The separation of Zr from dissolved Y metal targets was evaluated using several anion exchange resins. Each resin was evaluated against its ability to quantitatively capture Zr from a load solution high in dissolved Y. The most appropriate anion exchange resin for this application was identified, and the separation method was optimized. The method is capable of a high Y decontamination factor (>105) and has been shown to remove Fe, an abundant contaminant in Y foils, from the 89Zr elution fraction. Finally, the method was evaluated using cyclotron bombarded Y foil targets; the method was shown to achieve >95% recovery of the 89Zr present in the foils. The anion exchange column method described here is intended to be the first 89Zr isolation stage in a dual-column purification process.

Performance of different theories for the angular distribution of bremsstrahlung produced by keV electrons incident upon a target

Different theories of the intrinsic bremsstrahlung angular distribution (i.e., the shape function) have been evaluated using Monte Carlo calculations for various target materials and incident electron energies between 20 keV and 300 keV. The shape functions considered were the plane-wave first Born approximation cross sections (i) 2BS [high-energy result, screened nucleus], (ii) 2BN [general result, bare nucleus], (iii) KM [2BS modified to emulate 2BN], and (iv) SIM [leading term of 2BN]; (v) expression based on partial-waves expansion, KQP; and (vi) a uniform spherical distribution, UNI [a common approximation in certain analytical models]. The shape function was found to have an important impact on the bremsstrahlung emerging from thin foil targets in which the incident electrons undergo few elastic scatterings before exiting the target material. For thick transmission and reflection targets the type of shape function had less importance, as the intrinsic bremsstrahlung angular distribution was masked by the diffuse directional distribution of multiple scattered electrons. Predictions made using the 2BN and KQP theories were generally in good agreement, suggesting that the effect of screening and the constraints of the Born approximation on the intrinsic angular distribution may be acceptable. The KM and SIM shape functions deviated notably from KQP for low electron energies (< 50 keV), while 2BS and UNI performed poorly over most of the energy range considered; the 2BS shape function was found to be too forward-focused in emission, while UNI was not forward-focused enough. The results obtained emphasize the importance of the intrinsic bremsstrahlung angular distribution for theoretical predictions of x-ray emission, which is relevant in various applied disciplines, including x-ray crystallography, electron-probe microanalysis, security and industrial inspection, medical imaging, as well as low- and medium (orthovoltage) energy radiotherapy.

Coherent synchrotron emission in transmission with double foil target

Generation of intense single attosecond pulses from coherent synchrotron emission (CSE), in the transmitted direction of the laser-irradiated double foil targets, has been investigated theoretically and numerically. Unlike conventional CSE in the single foil target case, here the dense electron nanobunch is formed in the vacuum gap between two foils, which is composed of the electrons blown out from the first ultrathin foil. Owing to the existence of the vacuum gap, the electron nanobunch can be accelerated to more energy. In addition, more laser energy can penetrate through the nanobunch and get reflected from the second foil. These reflected lasers and electron nanobunches interact with each other and results in enhanced CSE and consequently, the generation of intense attosecond pulses. Particle-in-cell simulations show that a single attosecond pulse with duration of 18 , photon energy and peak intensity of can be obtained from the double-foil targets irradiated by a laser at intensity of .

High quality ion acceleration through the interaction of two matched counterpropagating transversely polarized Gaussian lasers with a flat foil target

In order to generate high quality ion beams through a relatively uniform radiation pressure acceleration (RPA) of a common flat foil, a new scheme is proposed to overcome the curve of the target while being radiated by a single transversely Gaussian laser. In this scheme, two matched counterpropagating transversely Gaussian laser pulses, a main pulse and an auxiliary pulse, impinge on the foil target at the meantime. It is found that in the two-dimensional (2D) particle-in-cell (PIC) simulation, by the restraint of the auxiliary laser, the curve of the foil can be effectively suppressed. As a result, a high quality monoenergetic ion beam is generated through an efficient RPA of the foil target. For example, two counterpropagating transversely circularly polarized Gaussian lasers with normalized amplitudes ${a}_{1}=120$ and ${a}_{2}=30$, respectively, impinge on the foil target at the meantime, a 1.3 GeV monoenergetic proton beam with high collimation is obtained finally. Furthermore, the effects on the ions acceleration with different parameters of the auxiliary laser are also investigated.

Improved yield and control of spectra from high-intensity laser-generated neutron beams

AbstractKinetic modeling of laser-ion beam generation from the “break-out afterburner” (BOA) has been modeled for several deuteron-rich solid-density target foils. Modeling the transport of these beams in a beryllium converter shows as much as a fourfold increase in neutron yield over the present state of the art through the use of alternative target materials. Additionally, species-separation dynamics during the BOA can be exploited to control the hardness of the neutron spectra, of interest for, for example, enhancing penetrability in shielded material in active neutron interrogation settings.