Urban green spaces (UGSs) are considered an important natural approach for improving urban climatic conditions, promoting sustainable urban development, and advancing the global “Carbon Peak and Carbon Neutrality” targets. Previous studies have found that different vegetation spatial morphologies significantly impact the capacity to obstruct and absorb CO2, but it is not yet well understood which morphology can retain and absorb more CO2. This study takes Nantong Central Park as an example and conducts a CFD (Computational Fluid Dynamics) carbon flow simulation for CO2 under different vegetation spatial morphologies to identify their CO2 retention and absorption effects. First, the carbon sink benefits of elements such as “vegetation, soil, and wetlands” within the park were calculated, and the elements with the highest carbon sink benefits were identified. Then, the park was divided into carbon welcoming zones, carbon flow zones, and carbon shadow zones for carbon flow simulation with the highest carbon sink benefits. The results show that in the carbon welcome area, the one-block long fan-shaped plant community with a spatial density of 40 m thickness can best meet the requirements of absorption and induction of a small amount of carbon dioxide, with the smallest air vortex and uniform distribution of carbon dioxide in the surrounding area. In the carbon flow area, combined with the visual effect, the planting pattern of 6 m spacing herringbone combined with natural structure was adopted, which has a good carbon dioxide blocking and absorption capacity. In the carbon-shaded area, a herringbone planting pattern with a total width of 40 m and a base angle of 60° was chosen, which had the strongest hindrance and absorption capacity. Urban park environment optimization can use Fluent simulation to analyze the flow of carbon dioxide between different elements affected by wind dynamics at the same time. Based on the results, the form, layout, and spatial distance are adjusted and optimized. This study can better guide the spatial layout of vegetation and contribute to the realization of the goal of “carbon peak and carbon neutrality”.