Twin-roll casting (TRC) has seen a significant interest in recent years due to its short process, low energy consumption, and low emission. The research included both numerical simulation and experimental validation to examine the flow and temperature field distribution of the TRC process. The “U-shaped” buffer groove is identified as beneficial for maintaining a stable liquid level distribution in the molten pool through comparison with various flow distributor structures. The solidified billet shell dispersion around the casting roller in the molten pool is observed to undergo three distinct stages: stable growth, thickness fluctuation, and rapid growth. The inclusion of two circular side outlets, each with a diameter ranging from 8 to 10 mm, proves advantageous in maintaining a stable distribution of the liquid level within the molten pool. The edge outlet size ranges from 7 to 9 mm, and ensuring a U-shaped buffer groove width/flow distribution of 1.25–1.58 aids in enhancing casting stability.