To investigate the relationship between moisture content in cohesive soils during spontaneous liquefaction and their corresponding critical slope failure angles. This study modified the liquid limit test apparatus originally developed by A. Atterberg in 1911, adapting it into a liquid-flow limit test apparatus. On-site soils from three actual cases of slope failures in Xiaolin Village, Jiasian District, Kaohsiung City, as well as soils from slope failures along the banks of Meilong River and Zengwun River were used for experiments involving different soil moisture content and slope failure angles. Based on the experimental findings, the moisture content which cohesive soils undergo spontaneous liquefaction was designated as the Flow Limit (FL), corresponding to the downslope angle at which circular failure occurs. This value represents the critical sliding angle at which spontaneous liquefaction occurs as a results of soil saturation. It also represents the maximum slope angle for exposed mudrock or clay slopes, and establishes the critical slope angle for vegetated slopes. Beyond this critical FL angle, all vegetation is susceptible to loss due to soil liquefaction. Furthermore, this study conducted FL tests on soils from thirteen tree holes in Kaohsiung City, two mountain slopes in Fengshan District, and the silty clay responsible for property damage and injuries during a landslide in Yanchao District on September 29, 2016, as a means of validation. The consistent test results observed reaffirm that different soils exhibit similar spontaneous liquefaction angles and flow limit behavior. These FL test results demonstrate a consistent pattern, reinforcing the notion of distinct curve characteristics that can be replicated across diverse soil compositions.