Floquet States Research Articles

Photon pumping in a weakly-driven quantum cavity–spin system

We investigate the photon pumping effect in a topological model consisting of a periodically driven spin-1/2 coupled to a quantum cavity mode out of the adiabatic limit. In the strong-drive adiabatic limit, a quantized frequency conversion of photons is expected as the temporal analog of the Hall current. We numerically establish a novel photon pumping phenomenon in the experimentally accessible nonadiabatic driving regime for a broad region of the parameter space. The photon frequency conversion efficiency exhibits strong fluctuations and high efficiency that can reach up 80% of the quantized value for commensurate frequency combinations. We link the pumping properties to the delocalization of the corresponding Floquet states which display multifractal behavior as the result of hybridization between localized and delocalized sectors. Finally we demonstrate that the quantum coherence properties of the initial state are preserved during the frequency conversion process in both the strong and ultra-weak-drive limit.

Chaos and subdiffusion in infinite-range coupled quantum kicked rotors

We map the infinite-range coupled quantum kicked rotors over an infinite-range coupled interacting bosonic model. In this way we can apply exact diagonalization up to quite large system sizes and confirm that the system tends to ergodicity in the large-size limit. In the thermodynamic limit the system is described by a set of coupled Gross-Pitaevskij equations equivalent to an effective nonlinear single-rotor Hamiltonian. These equations give rise to a power-law increase in time of the energy with exponent $\gamma\sim 2/3$ in a wide range of parameters. We explain this finding by means of a master-equation approach based on the noisy behaviour of the effective nonlinear single-rotor Hamiltonian and on the Anderson localization of the single-rotor Floquet states. Furthermore, we study chaos by means of the largest Lyapunov exponent and find that it decreases towards zero for portions of the phase space with increasing momentum. Finally, we show that some stroboscopic Floquet integrals of motion of the noninteracting dynamics deviate from their initial values over a time scale related to the interaction strength according to the Nekhoroshev theorem.

Floquet state depletion in ac-driven circuit QED

We perform Floquet spectroscopy in a GaAs double quantum dot system coupled to a high-impedance superconducting resonator. By applying microwave induced consecutive passages under a double resonance condition, we observe novel Landau-Zener-St\"uckelberg-Majorana interference patterns that stem from a cavity-assisted interference pattern modified by the depletion of the ground state. Our experimental results reveal the stationary state behavior of a strongly driven two-level system, and are consistent with the simulations based on our theoretical model. This study provides an excellent platform for investigating the dynamics of Floquet states in the presence of strong driving.

Spin dynamics under the influence of elliptically rotating fields: Extracting the field topology from time-averaged quantities.

Systems that can be effectively described as a localized spin-s particle subject to time-dependent fields have attracted a great deal of interest due to, among other things, their relevance for quantum technologies. Establishing analytical relationships between the topological features of the applied fields and certain time-averaged quantities of the spin can provide important information for the theoretical understanding of these systems. Here, we address this question in the case of a localized spin-s particle subject to a static magnetic field coplanar to a coexisting elliptically rotating magnetic field. The total field periodically traces out an ellipse which encloses the origin of the coordinate system or not, depending on the values taken on by the static and the rotating components. As a result, two regimes with different topological properties characterized by the winding number of the total field emerge: the winding number is 1 if the origin lies inside the ellipse, and 0 if it lies outside. We show that the time average of the energy associated with the rotating component of the magnetic field is always proportional to the time average of the out-of-plane component of the expectation value of the spin. Moreover, the product of the signs of these two time-averaged quantities is uniquely determined by the topology of the total field and, consequently, provides a measurable indicator of this topology. We also propose an implementation of these theoretical results in a trapped-ion quantum system. Remarkably, our findings are valid in the totality of the parameter space and regardless of the initial state of the spin. In particular, when the system is prepared in a Floquet state, we demonstrate that the quasienergies, as a function of the driving amplitude at constant eccentricity, have stationary points at the topological transition boundary. The ability of the topological indicator proposed here to accurately locate the abrupt topological transition can have practical applications for the determination of unknown parameters appearing in the Hamiltonian. In addition, our predictions about the quasienergies can assist in the interpretation of conductance measurements in transport experiments with spin carriers in mesoscopic rings.

Tuning of a bilayer graphene heterostructure by horizontally incident circular polarized light

We theoretically investigated the Floquet states of bilayer graphene heterostructure under the irradiation by horizontally incident circular polarized light. The in-plane and out-of-plane electric field of the light periodically perturbs the intra-layer and inter-layer hopping, respectively. For circular polarized light, the two components of the electric field has $\pi/2$ phase difference, so that the two types of hopping are periodically perturbed with the $\pi/2$ phase difference, which modify the effective inter-layer hopping. We focus on the model of bilayer graphene in the heterostructure of antiferromagnetic van der Walls spin valve. The amplitude of the irradiation can tune the band gap and topological properties of the bulk state. The spin-polarized quantum anomalous Hall phase with Chern number being one is predicted. The incident angle of the irradiation can tune the band gap and dispersion of the edge states in zigzag nanoribbons.

Light-wave control of correlated materials using quantum magnetism during time-periodic modulation of coherent transport

Light–wave quantum electronics utilizes the oscillating carrier wave to control electronic properties with intense laser pulses. Without direct light–spin interactions, however, magnetic properties can only be indirectly affected by the light electric field, mostly at later times. A grand challenge is how to establish a universal principle for quantum control of charge and spin fluctuations, which can allow for faster-than-THz clock rates. Using quantum kinetic equations for the density matrix describing non–equilibrium states of Hubbard quasiparticles, here we show that time–periodic modulation of electronic hopping during few cycles of carrier–wave oscillations can dynamically steer an antiferromagnetic insulating state into a metalic state with transient magnetization. While nonlinearities associated with quasi-stationary Floquet states have been achieved before, magneto–electronics based on quasiparticle acceleration by time–periodic multi–cycle fields and quantum femtosecond/attosecond magnetism via strongly–coupled charge–spin quantum excitations represents an alternative way of controlling magnetic moments in sync with quantum transport.

Photoinduced anomalous Hall effect in two-dimensional transition metal dichalcogenides

A circularly polarized a.c. pump field illuminated near resonance on two-dimensional transition metal dichalcogenides (TMDs) produces an anomalous Hall effect in response to a d.c. bias field. In this work, we develop a theory for this photo-induced anomalous Hall effect in undoped TMDs irradiated by a strong coherent laser field. The strong field renormalizes the equilibrium bands and opens up a dynamical energy gap where single-photon resonance occurs. The resulting photon dressed states, or Floquet states, are treated within the rotating wave approximation. A quantum kinetic equation approach is developed to study the non-equilibrium density matrix and time-averaged transport currents under the simultaneous influence of the strong a.c. pump field and the weak d.c. probe field. Dissipative effects are taken into account in the kinetic equation that captures relaxation and dephasing. The photo-induced longitudinal and Hall conductivities display notable resonant signatures when the pump field frequency reaches the spin-split interband transition energies. Rather than valley polarization, we find that the anomalous Hall current is mainly driven by the intraband response of photon-dressed electron populations near the dynamical gap at both valleys, accompanied by a smaller contribution due to interband coherences. These findings highlight the importance of photon-dressed bands and non-equilibrium distribution functions in achieving a proper understanding of photo-induced anomalous Hall effect in a strong pump field.

Engineering Dynamical Sweet Spots to Protect Qubits from 1/f Noise

Protecting superconducting qubits from low-frequency noise is essential for advancing superconducting quantum computation. Based on the application of a periodic drive field, we develop a protocol for engineering dynamical sweet spots which reduce the susceptibility of a qubit to low-frequency noise. Using the framework of Floquet theory, we prove rigorously that there are manifolds of dynamical sweet spots marked by extrema in the quasi-energy differences of the driven qubit. In particular, for the example of fluxonium biased slightly away from half a flux quantum, we predict an enhancement of pure-dephasing by three orders of magnitude. Employing the Floquet eigenstates as the computational basis, we show that high-fidelity single- and two-qubit gates can be implemented while maintaining dynamical sweet-spot operation. We further confirm that qubit readout can be performed by adiabatically mapping the Floquet states back to the static qubit states, and subsequently applying standard measurement techniques. Our work provides an intuitive tool to encode quantum information in robust, time-dependent states, and may be extended to alternative architectures for quantum information processing.

Dynamical Symmetries and Symmetry-Protected Selection Rules in Periodically Driven Quantum Systems.

In recent experiments, the light-matter interaction has reached the ultrastrong coupling limit, which can give rise to dynamical generalizations of spatial symmetries in periodically driven systems. Here, we present a unified framework of dynamical-symmetry-protected selection rules based on Floquet response theory. Within this framework, we study rotational, parity, particle-hole, chiral, and time-reversal symmetries and the resulting selection rules in spectroscopy, including symmetry-protected dark states (spDS), symmetry-protected dark bands, and symmetry-induced transparency. Specifically, dynamical rotational and parity symmetries establish spDS and symmetry-protected dark band conditions. A particle-hole symmetry introduces spDSs for symmetry-related Floquet states and also a symmetry-induced transparency at quasienergy crossings. Chiral symmetry and time-reversal symmetry alone do not imply spDS conditions but can be combined to define a particle-hole symmetry. These symmetry conditions arise from destructive interference due to the synchronization of symmetric quantum systems with the periodic driving. Our predictions reveal new physical phenomena when a quantum system reaches the strong light-matter coupling regime, which is important for superconducting qubits, atoms and molecules in optical or plasmonic field cavities, and optomechanical systems.

Microwave-driven persistent currents in a nanoscale quantum ring

Time-dependent electron current through a nanoscale phase-coherent quantum ring with leads, coupled to reservoirs biased by a sinusoidal voltage, is studied. We argue that Floquet states in such samples, driven also by external time-periodic magnetic field, can be coherently manipulated. Some examples show that on-demand structures in the frequency domain, tunable by the joint action of the voltage bias and a microwave pumping, can be generated this way.

Floquet spin states in OLEDs

Electron and hole spins in organic light-emitting diodes constitute prototypical two-level systems for the exploration of the ultrastrong-drive regime of light-matter interactions. Floquet solutions to the time-dependent Hamiltonian of pairs of electron and hole spins reveal that, under non-perturbative resonant drive, when spin-Rabi frequencies become comparable to the Larmor frequencies, hybrid light-matter states emerge that enable dipole-forbidden multi-quantum transitions at integer and fractional g-factors. To probe these phenomena experimentally, we develop an electrically detected magnetic-resonance experiment supporting oscillating driving fields comparable in amplitude to the static field defining the Zeeman splitting; and an organic semiconductor characterized by minimal local hyperfine fields allowing the non-perturbative light-matter interactions to be resolved. The experimental confirmation of the predicted Floquet states under strong-drive conditions demonstrates the presence of hybrid light-matter spin excitations at room temperature. These dressed states are insensitive to power broadening, display Bloch-Siegert-like shifts, and are suggestive of long spin coherence times, implying potential applicability for quantum sensing.

Selective high harmonics generated from a carbon nanotube

Selective high-order harmonic radiation can be generated when circularly polarized driving fields interact with single-walled carbon nanotubes. We obtain a gauge-covariant Hamiltonian for electrons confined to a nanotube surface in the presence of a circularly polarized electromagnetic field. Regularized delta-functions are used to approximate the $${\pi }$$ -bonds in the nanotube unit cells, and the electron dynamics, in the presence of the field, is analyzed. The high harmonic radiation occurs for incident field intensities high enough to induce significant nonlinearities and chaos in the electron dynamics. Both (5, 5) and (10, 10) armchair nanotubes are considered and the electron quantum dynamics is modeled using Floquet–Bloch theory. The behavior of the quasienergy spectrum, Floquet states, and the electron current are described for varying intensities of the incident field. We show that, for incident radiation with frequency $${\omega }$$ , the emitted radiation for a (p, p) armchair nanotube will be $$(2p\pm 1){\omega }$$ , $$(4p\pm 1){\omega }$$ , etc.

Rabi oscillations, Floquet states, Fermi's golden rule, and all that: Insights from an exactly solvable two-level model

Rabi oscillations and Floquet states are likely the most familiar concepts associated with a periodically time-varying Hamiltonian. Here, we present an exactly solvable model of a two-level system coupled to both a continuum and a classical field that varies sinusoidally with time, which sheds light on the relationship between the two problems. For a field of the rotating-wave-approximation form, results show that the dynamics of the two-level system can be mapped exactly onto that for a static field, if one shifts the energy separation between the two levels by an amount equal to ℏω, where ω is the frequency of the field and ℏ is Planck's constant. This correspondence allows one to view Rabi oscillations and Floquet states from the simpler perspective of their time-independent-problem equivalents. The comparison between the rigorous results and those from perturbation theory helps clarify some of the difficulties underlying textbook proofs of Fermi's golden rule, and the discussions on quantum decay and linear response theory.

Quantum frequency locking and downconversion in a driven qubit-cavity system

We study a periodically driven qubit coupled to a quantized cavity mode. Despite its apparent simplicity, this system supports a rich variety of exotic phenomena, such as topological frequency conversion as recently discovered in [Martin et al, PRX 7, 041008 (2017)]. Here we report on a qualitatively different phenomenon that occurs in this platform, where the cavity mode's oscillations lock their frequency to a rational fraction $r/q$ of the driving frequency $\Omega$. This phenomenon, which we term quantum frequency locking, is characterized by the emergence of $q$-tuplets of stationary (Floquet) states whose quasienergies are separated by $\Omega/q$, up to exponentially small corrections. The Wigner functions of these states are nearly identical, and exhibit highly-regular and symmetric structure in phase space. Similarly to Floquet time crystals, these states underlie discrete time-translation symmetry breaking in the model. We develop a semiclassical approach for analyzing and predicting quantum frequency locking in the model, and use it to identify the conditions under which it occurs.

Floquet dynamics in light-driven solids

We demonstrate how the properties of light-induced electronic Floquet states in solids impact natural physical observables, such as transport properties, by capturing the environmental influence on the electrons. We include the environment as dissipative processes, such as inter-band decay and dephasing, often ignored in Floquet predictions. These dissipative processes determine the Floquet band occupations of the emergent steady state, by balancing out the optical driving force. In order to benchmark and illustrate our framework for Floquet physics in a realistic solid, we consider the light-induced Hall conductivity in graphene recently reported by J.~W.~McIver, et al., Nature Physics (2020). We show that the Hall conductivity is estimated by the Berry flux of the occupied states of the light-induced Floquet bands, in addition to the kinetic contribution given by the average band velocity. Hence, Floquet theory provides an interpretation of this Hall conductivity as a geometric-dissipative effect. We demonstrate this mechanism within a master equation formalism, and obtain good quantitative agreement with the experimentally measured Hall conductivity, underscoring the validity of this approach which establishes a broadly applicable framework for the understanding of ultrafast non-equilibrium dynamics in solids.

Analytic expressions for the steady-state current with finite extended reservoirs.

Open-system simulations of quantum transport provide a platform for the study of true steady states, Floquet states, and the role of temperature, time dynamics, and fluctuations, among other physical processes. They are rapidly gaining traction, especially techniques that revolve around "extended reservoirs," a collection of a finite number of degrees of freedom with relaxation that maintains a bias or temperature gradient, and have appeared under various guises (e.g., the extended or mesoscopic reservoir, auxiliary master equation, and driven Liouville-von Neumann approaches). Yet, there are still a number of open questions regarding the behavior and convergence of these techniques. Here, we derive general analytical solutions, and associated asymptotic analyses, for the steady-state current driven by finite reservoirs with proportional coupling to the system/junction. In doing so, we present a simplified and unified derivation of the non-interacting and many-body steady-state currents through arbitrary junctions, including outside of proportional coupling. We conjecture that the analytic solution for proportional coupling is the most general of its form for isomodal relaxation (i.e., relaxing proportional coupling will remove the ability to find compact, general analytical expressions for finite reservoirs). These results should be of broad utility in diagnosing the behavior and implementation of extended reservoir and related approaches, including the convergence to the Landauer limit (for non-interacting systems) and the Meir-Wingreen formula (for many-body systems).

Edge localized Schrödinger cat states in finite lattices via periodic driving

Floquet states have been used to describe the impact of periodic driving on lattice systems, either using a tight-binding model, or by using a continuum model where a Kronig-Penney-like description has been used to model spatially periodic systems in one dimension. A number of these studies have focused on finite systems, and results from these studies are distinct from those of infinite lattice systems as a consequence of boundary effects. In the case of a finite system, there remains a discrepancy in the results between tight-binding descriptions and continuous lattice models. Periodic driving by a time-dependent field in tight-binding models results in a collapse of all quasienergies within a band at special driving amplitudes. In the continuum model, on the other hand, a pair of nearly-degenerate edge bands emerge and remain gapped from the bulk bands as the field amplitude increases. We resolve these discrepancies and explain how these edge bands represent Schr\"odinger cat-like states with effective tunneling across the entire lattice. Moreover, we show that these extended cat-like states become perfectly localized at the edge sites when the external driving amplitude induces a collapse of the bulk bands.

Solvable Model of a Generic Driven Mixture of Trapped Bose-Einstein Condensates and Properties of a Many-Boson Floquet State at the Limit of an Infinite Number of Particles.

A solvable model of a periodically driven trapped mixture of Bose–Einstein condensates, consisting of interacting bosons of mass driven by a force of amplitude and interacting bosons of mass driven by a force of amplitude , is presented. The model generalizes the harmonic-interaction model for mixtures to the time-dependent domain. The resulting many-particle ground Floquet wavefunction and quasienergy, as well as the time-dependent densities and reduced density matrices, are prescribed explicitly and analyzed at the many-body and mean-field levels of theory for finite systems and at the limit of an infinite number of particles. We prove that the time-dependent densities per particle are given at the limit of an infinite number of particles by their respective mean-field quantities, and that the time-dependent reduced one-particle and two-particle density matrices per particle of the driven mixture are condensed. Interestingly, the quasienergy per particle does not coincide with the mean-field value at this limit, unless the relative center-of-mass coordinate of the two Bose–Einstein condensates is not activated by the driving forces and . As an application, we investigate the imprinting of angular momentum and its fluctuations when steering a Bose–Einstein condensate by an interacting bosonic impurity and the resulting modes of rotations. Whereas the expectation values per particle of the angular-momentum operator for the many-body and mean-field solutions coincide at the limit of an infinite number of particles, the respective fluctuations can differ substantially. The results are analyzed in terms of the transformation properties of the angular-momentum operator under translations and boosts, and as a function of the interactions between the particles. Implications are briefly discussed.

Floquet Engineering of Two Weakly Coupled Superconducting Flux Qubits

We explore the periodically driven dynamics of two weakly coupled flux qubits and propose a scheme to generate a maximally entangled state based on Floquet engineering. The periodic driving modifies the quasienergy spectrum of the system and induces crossing of quasienergies, and the weak coupling between them lifts the degeneracy of quasienergies. It is found that the phenomena of entanglement resonance of Floquet state appear at certain values of the driving parameters, which could be demonstrated by virtue of the Rabi-frequency spectrum and average concurrence during one driving period. Our scheme relaxes the experimental difficulty in adjusting the static parameters of the system to establish entanglement, and may open interesting perspectives for devising active decoherence-immune quantum-information devices.

Optically induced topological phase transition in two dimensional square lattice antiferromagnet

The two dimensional square lattice antiferromagnet with spin–orbit coupling and nonsymmorphic symmetry is recently found to be topological insulator (TI). We theoretically studied the Floquet states of the antiferromagnetic crystal with optical irradiation, which could be applicable in opto-spintronic. An optical irradiation with circular polarization induces topological phase transition into quantum Anomalous Hall phase with varying Chern number. At the phase boundaries, the Floquet systems could be semimetal with one, two or three band valleys. A linear polarized optical field induces effective antiferromagnetic exchange field, which change the phase regime of the TI. At the intersection of two phase boundaries, the bulk band structure is nearly flat along one of the high symmetry line in the first Brillouin zone, which result in large density of states near to the Fermi energy in bulk and nanoribbons.