Effects of increased pressure on the thermochemistry of turbulent flame-wall interaction (FWI) were investigated within this study. Quantitative, pointwise measurements of three state parameters, i.e., gas-phase temperature, CO2 and CO mole fraction, were performed by means of dual-pump coherent anti-Stokes Raman spectroscopy (CARS) and two-photon laser-induced fluorescence (LIF) of CO. The flame front was simultaneously tracked by planar OH-LIF imaging. The measurements were carried out in a fully premixed methane-air flame in an enclosed side-wall quenching burner test rig under atmospheric and pressurized conditions (3 bar absolute pressure). An evaluation of near wall flame front topologies showed that the interaction of the flame with the wall is predominantly characterized by one single, extended reaction zone, similar to a so-called head-on quenching configuration. The dominance of this quenching scenario occurred most likely due to the confined burner configuration preventing an unhindered expansion of the hot exhaust gases. Thermochemical states were studied using pairwise correlations of temperature, CO2 and CO mole fraction. Regarding the measurements at atmospheric pressure, an overall good agreement with other studies on atmospheric FWI in a similar unconfined burner was observed considering differences concerning the flow field and the burner configuration. For the thermochemistry measurements at elevated pressure, similar trends as for the atmospheric measurements were identified. A comparison of both operating cases suggested that FWI processes were more strongly affected by heat losses at elevated pressure, but differences are moderately pronounced. To the authors’ best knowledge, these experiments are the first attempt to explore the near-wall thermochemistry of FWI processes at elevated pressure using multi-parameter measurements. As the near-wall measurements were further complicated by effects arising with increasing pressure, e.g., intensified beam steering and reduced length scales, implications on the application of the laser diagnostics are reported.
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