Burnishing is a cold working process that can be used to improve surface finish and surface hardness of workpieces. Conventionally, diamond or hard metal burnishing tools are used. In the present work, a novel burnishing tool was created by depositing amorphous diamond coating (AD) on a stainless steel tip. This tool was used to improve the surface finish and surface hardness of Nitronic-50 HS stainless steel workpieces. Nitronic-50 HS is used in a wide range of applications in industry. The burnishing process was carried out at different burnishing parameters (force, revolution speed, feed and number of tool passes). Burnishing parameters had a significant effect on the finishing process and they had to be optimized to achieve the best results. Remarkable improvements in surface finish (70% decrease in roughness) and hardness (25% increase) could be achieved with this tool and process in the surface finishing of Nitronic-50 stainless steel workpieces. From the tribological point of view, the AD-coated tip performed slightly better than a corresponding tip modified from a commercial polycrystalline diamond tip. AD coating seems to be very suitable for use in mechanical surface finishing tools such as a burnishing tip.