Ferromagnetic Spin Research Articles

Designing van der Waals layers for ferromagnetic quantum spin Hall phase

Most theoretically predicted and experimentally confirmed quantum spin Hall effects (QSHEs) are limited to zero-moment magnets. In this study, we theoretically anticipate the QSHE in ferromagnets and the quantum anomalous Hall effect (QAHE) in antiferromagnets through van der Waals stacked layers, where the magnetization direction is confined to the in-plane. We introduce a search rule for constructing ferromagnetic (FM) quantum spin Hall insulator (QSHI) and antiferromagnetic (AFM) quantum anomalous Hall insulator (QAHI) and further predict a real material of the LuN2/GaS/LuN2 van der Waals multilayer by first-principles calculations. Our results demonstrate the superposition and elimination of Chern numbers under mirror symmetry and time-reversal symmetry, and they further indicate that FM QSHI and AFM QAHI can be converted through deflection magnetization. These findings broaden the material class for QSHE and QAHE and propose a scheme for constructing FM QSHI and AFM QAHI.

Exotic Kondo effect in two one-dimensional spin-1/2 chains coupled to two localized spin-1/2 magnets

We study an exotic Kondo effect in a system consisting of two one-dimensional XX Heisenberg ferromagnetic spin-1/2 chains (denoted by α=u,d for up and down chains) coupled to a quantum dot consisting of two localized spin-1/2 magnets. Using the Jordan–Wigner transformation on the Heisenberg Hamiltonian of the two chains, this system can be expressed in terms of non-interacting spinless fermionic quasiparticles. As a result, the Hamiltonian of the whole system is expressed as an Anderson model for spin-1/2 fermions interacting with a spin-1/2 impurity. Thus, we study the scattering of fermionic quasiparticles (propagating along spin chains) by a pair of localized magnetic impurities. At low temperature, the localized spin-1/2 magnets are shielded by the chain “spins” via the Kondo effect. We calculate the Kondo temperature TK and derive the temperature dependence of the entropy, the specific heat and the “magnetic susceptibility” of the dot for T≫TK. Our results can be generalized to the case of antiferromagnetic XX chains.

Theoretical studies on a 2D quasi discrete Ferromagnetic spin system with NNN interactions

Theoretical studies on a 2D quasi discrete Ferromagnetic spin system with NNN interactions

Time fractional (2 + 1)-dimensional Heisenberg ferromagnetic spin chain equation: its Lie symmetries, exact solutions and conservation laws

Abstract In this paper, Lie symmetry analysis method is applied to (2+1)-dimensional time-fractional Heisenberg ferromagnetic spin chain equation. We obtain all the Lie symmetries admitted by the governing equation and reduce the corresponding (2+1)-dimensional fractional partial differential equations with Riemann-Liouville fractional derivative to (1+1)-dimensional counterparts with Erd'{e}lyi-Kober fractional derivative. Then we obtain the power series solutions of the reduced equations, prove their convergence and analyze their dynamic behavior graphically. In addition, the conservation laws for all the obtained Lie symmetries are constructed by the new conservation theorem and the generalization of Noether operators.

Double-pole anti-dark solitons for a Lakshmanan-Porsezian-Daniel equation in an optical fiber or a ferromagnetic spin chain

Under investigated in this paper is a Lakshmanan-Porsezian-Daniel equation that describes the nonlinear spin excitations in a (1+1)-dimensional isotropic biquadratic Heisenberg ferromagnetic spin chain with the octupole-dipole interaction or the propagation of the ultrashort pulses in a long-distance and high-speed optical fiber transmission system. Under certain parameter conditions, we simultaneously take the multi-pole phenomena and breather-to-soliton transitions into account, then utilize the second-order generalized Darboux transformation to derive the double-pole anti-dark solitons and graphically illustrate them. Asymptotic analysis is conducted to examine the interaction properties of double-pole anti-dark solitons, including their characteristic lines, amplitudes, phase shifts, slopes and position differences. Unlike the double-pole anti-dark solitons found in the Hirota equation, the ones in this study exhibit a distinct feature: Different soliton components share the same amplitude.

A Spin‐Polarized Electron‐Induced MXene‐KBi0.9Co0.1Fe2O5 Photocatalyst for Enhanced Dye Degradation

In photocatalysts aimed to degrade environmental pollutants, photons are generally used as primary stimuli to generate electron–hole pairs to target the chemical bonds to disintegrate. Recently, electron spin has been reported as an essential degree of freedom to improve the performance of photocatalysts. In this work, spin‐polarized electrons and holes are introduced into a brownmillerite KBi0.9Co0.1Fe2O5 semiconductor and a two‐dimensional (2D) MXene composite system by application of an external magnetic field. The spin polarization properties are monitored by measuring the magnetoresistance effect of the MXene‐KBCFO device, which is related to the carrier transfer efficiency. Remarkably, the photocatalytic performance of MXene‐KBCFO is significantly enhanced by the simultaneous application of an external magnetic field and illumination due to the increased number of spin‐polarized photoexcited carriers caused by the synergy effect of the 2D MXene heterostructure together with the ferromagnetic spin ordering. This results in increased reaction hotspots, effective built‐in electric field, extended carrier lifetime, and reduced charge recombination owing to parallel alignment of electron spin orientation. The results show that the efficiency and stability of photocatalytic dye degradation can be effectively enhanced by manipulating the spin‐polarized electrons in the MXene‐based oxide‐perovskite heterostructure photocatalyst.

Nonequilibrium phase transitions in a 2D ferromagnetic spins with effective interactions

Nonequilibrium phase transitions in a 2D ferromagnetic spins with effective interactions

New method for constructing phase diagrams in 2D centered tetragonal Ising nanoparticles using the cellular automata approach

In this study, both ferromagnetic and antiferromagnetic spin configurations of a 2D-centered tetragonal Ising nanoparticle with two types of exchange interactions (J and Jr) are considered. A newly introduced algorithm using Cellular Automata simulation method, which is relied on counting the states with a magnitude of magnetization per site exceeding a threshold value mt, is used to compute the value of the reduced critical temperature. The sensitivity of the critical temperature value to the lattice size and exchange interactions (The ratio of Jr/J denoted by r parameter) are examined. The results show that the value of the critical temperature increases with increasing lattice size with a decreasing slope. Moreover, the same behavior was observed in ferromagnetic and antiferromagnetic cases.

Microwave‐to‐Optics Conversion Using Magnetostatic Modes and a Tunable Optical Cavity

AbstractQuantum computing, quantum communication, and quantum networks rely on hybrid quantum systems operating in different frequency ranges. For instance, the superconducting qubits work in the gigahertz range, while the optical photons used in communication are in the range of hundreds of terahertz. Due to the large frequency mismatch, achieving the direct coupling and information exchange between different information carriers is generally difficult. Accordingly, a quantum interface is demanded, which serves as a bridge to establish information linkage between different quantum systems operating at distinct frequencies. Recently, the magnon mode in ferromagnetic spin systems has received significant attention. While the inherent weak optomagnonic coupling strength restricts the microwave‐to‐optical photon conversion efficiency using magnons, the versatility of the magnon modes, together with their readily achievable strong coupling with other quantum systems, endow them with many distinct advantages. Here, the magnon‐based microwave‐light interface is realized by adopting an optical cavity with adjustable free spectrum range and different kinds of magnetostatic modes in two microwave cavity configurations. By optimizing the parameters, a conversion efficiency of with bandwidth of 24 MHz is achieved. The impact of various parameters on the microwave‐to‐optics conversion is analyzed. The study provides useful guidance and insights to further enhancing the microwave‐to‐optics conversion efficiency using magnons.

Investigation of thermodynamical stability and generation of large half-metallic gap along with optical properties in N-doped YHfO3 (YHO) (Y = Ca, Sr, and Ba) perovskite materials by first principle calculations

Considerable energy gap (Eg) in insulating channel, high spin-filtering, significant mean free path, and high magnetic transition temperature (TC) escalate half-metallic (HM) ferromagnetic (FM) materials very enticing for spintronic applications. Herein, ab-initio calculations have been executed comprehensively to inquest the structural, thermodynamical, electronic, magnetic, and optical properties of pure as well as nitrogen (N)-doped YHfO3 (YHO) (Y = Ca/Sr/Ba) materials with one N atom added at one of the oxygen (O) site. First, the thermodynamical stability of both bulk and doped YHO systems has been examined by estimating the formation enthalpies (ΔHf) by Convex Hull analysis, which confirms the practical realization of these materials on experimental grounds. Moreover, mechanical stability of these systems is affirmed by estimating the necessary elastic constants and respective parameters. Strikingly, all doped systems possess complete (100%) splitting in spin↑ and spin↓ channels at Fermi level and depict HM FM character with significant Eg of 3.31, 3.49, and 3.24 eV in spin↓ channels for CaHO (CHO), SrHO (SHO), and BaHO (BHO) systems, respectively. It is also found that N 2p orbitals are totally responsible for the emergence of metatallicity and magnetic character in all these doped structures. Moreover, the ground state long range FM stability between two added N atoms in doped systems is affirmed by computing the difference of total energies of FM and anti-ferromagnetic (AFM) spin ordering (ΔE) along with estimated TC at different distances. Lastly, it is found that N-doped systems have a lower optical energy loss than pristine YHO systems in the incident photon energy range of 0-50 eV. Hence, the present study proposes that an unconventional doping approach with intrinsically non-magnetic element in a variety of YHO perovskite systems could be a useful method to alter their various physical properties and forecast their potential applications in the development of novel spintronic and optoelectronic devices.

Correlated normal state fermiology and topological superconductivity in UTe2

UTe2 is a promising candidate for spin-triplet superconductors, in which a paramagnetic normal state becomes superconducting due to spin fluctuations. Here, we theoretically show that electron correlation induces a dramatic change in the normal state fermiology with an emergent correlated Fermi surface (FS) driven by Kondo resonance at low temperatures. This emergent correlated FS can account for various unconventional superconducting properties in a unified way. In particular, the geometry of the correlated FS can naturally host topological superconductivity in the presence of odd-parity pairings, which become the leading instability due to strong ferromagnetic spin fluctuations. Moreover, two pairs of odd-parity channels appear as nearly degenerate solutions which may lead to time-reversal breaking multicomponent superconductivity. The resulting time-reversal-breaking superconducting state is a Weyl superconductor in which Weyl points migrate along the correlated FS as the relative magnitude of nearly degenerate pairing solutions varies.

Pioneering the plethora of soliton for the (3+1)-dimensional fractional heisenberg ferromagnetic spin chain equation

Abstract In this scholarly article, we investigate the complex structured (3+1)-dimensional Fractional Heisenberg Ferromagnetic Spin Chain equation (FHFSCE) with conformable fractional derivatives. We develop a diverse glut of soliton solutions using an improved version of the G ′ G -expansion method, namely the r + G ′ G -expansion method. The constraints for the existence of these solutions are painstakingly explained. Our findings are clearly communicated through a number of 3D and 2D graphical representations displaying periodic, multiple periodic, kink, and shock soliton solutions. These soliton solutions are expressed in several mathematical function forms, such as hyperbolic, trigonometric, and rational functions. Our findings support the suggested method’s efficacy as a powerful symbolic algorithm for discovering innovative soliton solutions within nonlinear evolution systems.

Vanadium embedded in monolayer silicene: Energetics and proximity-induced magnetism

Using the density-functional theory approach, including Hubbard U correction, we investigate the defect structures consisting of vanadium (V) atoms embedded in a monolayer silicene. Specifically, we consider V–V atom pairs in antiferromagnetic (AFM), ferromagnetic (FM), and non-magnetic states, which are embedded in substitutional and interstitial sites. We determine the ground-state structures, formation and binding energies, electronic structures, induced magnetization, as well as the spin-exchange coupling between the V–V pair. For the substitutional vanadium atom pair, the stability of the AFM and FM spin configurations depends on the sublattice sites in which the V atoms are sited. When the V pair is located on a similar sublattice site type, the AFM spin alignment is more energetically favored, whereas when the pair is located in a different sublattice site, the FM interactions are more stable. However, the relative stability of the AFM or FM configurations changes rapidly as the separation between the V pair increases. Regarding the interstitial-hole V–V pair configurations, the most stable structure is when the pair is at the nearest-neighbor hole sites and is in an FM alignment. Also, at larger separations, the AFM or FM hole configurations are approximately degenerate in energy. Furthermore, we elucidate on the Ruderman–Kittel–Kasuya–Yosida, direct-exchange, and the superexchange interaction mechanisms in the vanadium-embedded silicene. In addition, we estimate a Curie temperature (Tc) of up to ∼500 K for a silicene structure containing a V pair in the FM spin alignment. Such a high Tc, in addition to the stability of the material, suggests that vanadium-embedded silicene is a potential candidate material for spintronic device applications.

Dynamical analysis and the soliton solutions of (2+1)-dimensional Heisenberg ferro-magnetic spin chains model with beta fractional derivative

This paper investigates the soliton solutions and dynamical analysis of (2+1)-dimensional Heisenberg ferro-magnetic spin chains model with beta fractional derivative, which is transformed into the ordinary differential equation. By using the second-order complete discriminant system, the soliton solutions are presented. By utilizing the theory of planar dynamical system, the phase portraits of the dynamical system and its disturbance system are drawn. Moreover, three-dimensional, two-dimensional, and contour plots of soliton solutions for (2+1)-dimensional Heisenberg ferro-magnetic spin chains model with beta fractional derivative have also been plotted.

Non-trivial evolution of the Dirac cone in chromium doped Dirac semimetal Cd3As2

The magnetic doping of Dirac semimetals breaks their time-reversal symmetry thus giving rise to anomalous transport phenomena promising for applications. While the Dirac cone (DC) manifestations were observed in the electron transport of (Cd1−xCrx)3As2 alloys up to x = 0.06, their mechanism remains challenging. To address this challenge, we performed DFT calculations of the (Cd0.96Cr0.04)3As2 alloy with the non-magnetic (NM), ferromagnetic (FM), and antiferromagnetic (AFM) spin orders. It was found that the NM state is unstable, while the FM state has the lowest energy. The band structure analysis revealed that Cr 3d states are distributed in energy not uniformly, but with Cr-free windows, in which the Dirac spectrum can survive. The only exception is the Dirac point vicinity, where a narrow gap is formed. Outside the window, the DC band strongly hybridizes with the Cr 3d states and disappears. Near EF, such a Cr-free window with the DC band exists only in the FM↓ state and is absent in the NM, FM↑, and AFM states. The Fermi surface of FM (Cd1−xCrx)3As2 has two parts: the DC↓ sheet with the velocity vF ≈ 1∙106 m/s and several sheets with low vF, originating from Cr 3d↑ states. As an example of transport properties, the dc conductivity of FM (Cd1−xCrx)3As2 was estimated. We found that at T→0 K the DC↓ electrons have a very large transport lifetime and therefore dominate in the conductivity. In this dominance, the role of the Cr-free window is double: it ensures the DC↓ surviving and greatly reduces an admixture of Cr 3d↓ orbitals to DC↓ states, so suppressing the scattering of DC↓ electrons by doped Cr atoms. This mechanism looks rather general and may be applied to the design of magnetic topological alloys.

Magnetic relaxation between ferromagnetic and helix spin configurations in holmium films

Multiple noncollinear spin structures and transitions between them initiated by field and temperature have attracted attention due to the extraordinary coexistence of complicated spin phases in Ho. We explore the magnetic relaxation dynamics within thin films undergoing transitions between ferromagnetic (FM) and helix states. When measuring susceptibility in a relatively high frequency range (∼100–1500 Hz) and magnetic viscosity at lower frequency (∼0.01 Hz), we focus on 400 nm thick Ho film. Notably, sharp variations in the real and imaginary components of magnetic susceptibility are discerned during the FM – Helix transition, occurring at temperatures between 15 and 30 K. Hysteresis effects in the magnetic susceptibility components are identified during cyclic variations in the external field, indicating a relatively rapid process with a timescale of approximately 10 ms accompanying the FM – Helix transition. The slow relaxation process is also found to exhibit sensitivity to this transition. Furthermore, the field dependence of magnetic viscosity displays a marked decline at the FM – Helix transition. The research methodologies proposed for the investigation of relaxation processes in materials with multiphase spin structures are deemed universally applicable and offer insights into transitions between spin states in materials manifesting non collinear spin structures.

Enhanced spin pumping in heterostructures of coupled ferrimagnetic garnets

Spin pumping has significant implications for spintronics, providing a mechanism to manipulate and transport spins for information processing. Understanding and harnessing spin currents through spin pumping is critical for the development of efficient spintronic devices. The use of a magnetic insulator with low damping enhances the signal-to-noise ratio in crucial experiments such as spin-torque ferromagnetic resonance (FMR) and spin pumping. A magnetic insulator coupled with a heavy metal or quantum material offers a more straightforward model system, especially when investigating spin-charge interconversion processes to greater accuracy. This simplicity arises from the absence of unwanted effects caused by conduction electrons unlike in ferromagnetic metals. Here, we investigate the spin pumping in coupled ferrimagnetic (FiM) Y3Fe5O12 (YIG)/Tm3Fe5O12 (TmIG) bilayers combined with heavy-metal (Pt) using the inverse spin Hall effect. It is observed that magnon transmission occurs at both of the FiMs FMR positions. The enhancement of spin pumping voltage (Vsp) in the FiM garnet heterostructures is observed. The plausible reason might be the interfacial exchange coupling between FiMs. The modulation of Vsp is achieved by tuning the bilayer structure. Further, the spin mixing conductance for these coupled systems is found to be ≈1018 m−2. Our findings describe a coupled FiM system for the investigation of magnon coupling providing opportunities for magnonic devices.

Hawking-Page transition on a spin chain

The accessibility of the Hawking-Page transition in AdS5 through a one-dimensional (1D) Heisenberg spin chain is demonstrated. We use the random matrix formulation of the Loschmidt echo for a set of spin chains, and randomize the ferromagnetic spin interaction. It is shown that the thermal Loschmidt echo, when averaged, detects the predicted increase in entropy across the Hawking-Page transition. This suggests that a 1D spin chain exhibits characteristics of black hole physics in 4+1 dimensions. We show that this approach is equally applicable to free fermion systems with a general dispersion relation. Published by the American Physical Society 2024

Analytical solutions and soliton behaviors in the space fractional Heisenberg ferromagnetic spin chain equation

This study investigates soliton solutions to the (2 + 1)-dimensional space fractional Heisenberg ferromagnetic spin chain equation incorporating beta fractional derivatives that explain the nonlinear propagation of spin wave in the ferromagnetic material with magnetic interactions including the both classical and semi-classical frameworks. This model has applications in spintronics, plasma physics, magnet theory, and condensed matter physics. Employing the two-potential extended Kudryashov and (G′/G, 1/G)-expansion methods, we derive some original and generic solutions composed of trigonometric functions, hyperbolic functions, and their rational forms. For particular values of the parameters, these solutions offer V-shaped, bell-shaped, kink, periodic, flat kink, and singular periodic solitons. The physical behavior of these solitons is demonstrated through three-dimensional, contour, and two-dimensional plots. The results are important in the study of phase transitions in ferromagnetic materials, lattice vibrations in condensed matter, and the propagation of shock waves in plasma. This study also demonstrates the potential and reliability of the employed strategies.

Stability aspects of a perturbed 3-dimensional Heisenberg ferromagnetic spin system

Using Glauber’s coherent state approach along with the Dyson–Maleev bosonic representation of spin operators, we examine the nonlinear spin dynamics of a 3-dimensional Heisenberg ferromagnetic spin system with bilinear and anisotropic interactions in the semi-classical limit. By combining the multiple-scale technique with quasi-discreteness approximation, we create a perturbed Cubic Nonlinear Schrödinger equation. We perform a multiple-scale perturbation analysis to see how discreteness affects the soliton excitations. We created the perturbed soliton, and the perturbation analysis demonstrates that the soliton’s amplitude and velocity remain unchanged. Moreover, graphical illustrations and analytical solutions are provided to illustrate the aspects of modulational instability.