Femtosecond Optical Parametric Oscillator Research Articles

Compact low-repetition-rate femtosecond optical parametric oscillators enabled by Herriott cells

We report the design and characterization of a femtosecond optical parametric oscillator containing an intracavity Herriott cell. Pumped by a 49.16-MHz Yb:fiber laser, the signal wavelength could be tuned over 1440-1530 nm, with the Herriott cell containing 81% of the free-space cavity length required for synchronous operation. We also report a 12.29-MHz OPO using a sub-harmonic pumping approach, extending the Herriott cell OPO concept to low-repetition-rate cavities.

Consideration of non-phase-matched nonlinear effects in the design of quasi-phase-matching crystals for optical parametric oscillators.

Femtosecond optical parametric oscillators (OPOs) are widely used in ultrafast nonlinear frequency conversion and quantum information. However, conventional OPOs based on quasi-phase-matching (QPM) crystals have many parasitic non-phase-matched processes which decrease the conversion efficiency. Here, we propose nine-wave coupled equations (NWCEs) to simulate all phase-matched and non-phase-matched interactions in QPM crystals to improve conventional three-wave coupled equations (TWCEs), especially for the situation of high intensity ultrashort pulses and complexly structured crystals. We discuss how to design the poling period of QPM crystal to maximize the conversion efficiency of signal light for a given OPO system. The simulation reveals that the OPO based on chirped periodically poled lithium niobate (CPPLN) with a certain chirp rate has higher signal wave conversion efficiency than that of a PPLN, and demonstrates that NWCEs illustrate more details of the pulse evolution in the OPO cavity. Starting from a CPPLN, an aperiodically poled lithium niobate (APPLN) design is available by modifying the domain lengths of the crystal and optimizing the OPO output power via dynamical optimization algorithm. The results show that by using a properly designed APPLN crystal, a 1600 nm OPO, when pumped by a femtosecond laser with 1030 nm central wavelength, 150 femtosecond pulse duration and 5 GW/cm2 power intensity at the focus, can achieve very efficient output with a signal light conversion efficiency of 50.6%, which is higher than that of PPLN (25.2%) and CPPLN (40.2%). The scheme in this paper will provide a reference for the design of nonlinear QPM crystals of OPOs and will help to understand the complex nonlinear dynamical behavior in OPO cavities.

Spectrally resolved ultrafast transient dynamics of a femtosecond fiber-feedback optical parametric oscillator.

We report on spectrotemporal transient dynamics in a femtosecond fiber-feedback optical parametric oscillator (FFOPO) system. Burst modulation of the pump beam in combination with dispersive Fourier transformation sampling allows to record single-pulse signal spectra at 41 MHz sampling rate. Therefore, each individual pulse of the signal transients can be spectrally resolved. We characterize the signal output behavior for anomalous as well as for normal intra-cavity dispersion. Amongst steady state output we observed period-doubling cycles and other attractors, which occured at higher intra-cavity nonlinearity levels. The experimental findings are supported by numerical simulations, in order to identify the linear and nonlinear effects, which govern the wavelength tuning behavior of this FFOPO system. We find that steady state operation is preferred and that the wavelength tuning stability of the FFOPO dramatically increases when using a normal dispersion feedback fiber.

Two-photon absorption spectrometers for near infrared

We present a Silicon-based Charge-Coupled Device (Si-CCD) sensor applied as a cost-effective spectrometer for femtosecond pulse characterization in the Near Infrared region in two different configurations: two-Fourier and Czerny-Turner setups. To test the spectrometer's performance, a femtosecond Optical Parametric Oscillator with a tuning range between 1100 and 1700nm and a femtosecond Erbium-Doped Fiber Amplifier at 1582nm were employed. The nonlinear spectrometer operation is based on the Two-Photon Absorption effect generated in the Si-CCD sensor. The achieved spectrometer resolution was 0.6 ± 0.1nm with a threshold peak intensity of 2×106Wcm2. An analysis of the nonlinear response as a function of the wavelength, the response saturation, and the criteria to prevent it are also presented.

High–Efficiency, Widely Tunable MgO: PPLN Optical Parametric Oscillator

We report on the investigation of a high–efficiency, widely tunable femtosecond optical parametric oscillator (OPO) based on a multi–period MgO–doped periodically poled lithium niobite (MgO: PPLN) crystal, pumped by an all–solid–state femtosecond mode–locked Yb: KGW laser at 1030 nm providing 100 fs pulses. With 6 W pump power, the OPO generates 2.68 W of signal power at 1540 nm and 1.2 W of idler power at 3110 nm, which corresponds to the total conversion efficiency adding up to 67.4%. To the best of our knowledge, this is the highest conversion efficiency of a femtosecond OPO. Meanwhile, in order to obtain a broad optical spectrum range, both the grating period and working temperature are tuned, resulting in tunable signals of 1.43–1.78 µm and idlers of 2.44–3.68 µm. This source will be used to generate a femtosecond mid–infrared laser of wavelength range 3.7–6.5 µm and tens milliwatts average power through difference frequency generation (DFG).

Tunable femtosecond optical parametric oscillators resonating at 0.65-1.02 µm and 1.07-2.3 µm.

We present a singly resonant femtosecond optical parametric oscillator (OPO) cavity architecture supporting ultra-broadband wavelength tuning and efficient outcoupling of the generated optical pulses. Experimentally, we demonstrate an OPO with its oscillating wavelength tuned over 652-1017 nm and 1075-2289 nm, spanning nearly 1.8 octaves. This is, as far as we know, the widest resonant-wave tuning range obtained from a green-pumped OPO. We show that intracavity dispersion management is crucial for the stationary and single-band operation of such a broadband wavelength tuning system. This architecture is universal, and therefore can be extended to allow the oscillation and ultra-broadband tuning of OPOs at various spectral regions.

Burst-mode femtosecond fiber-feedback optical parametric oscillator

In multiphoton 3D direct laser writing and stimulated Raman scattering applications, rapid and arbitrary pulse modulation with an extremely high contrast ratio would be very beneficial. Here, we demonstrate a femtosecond fiber-feedback optical parametric oscillator (FFOPO) system in combination with pulse picking in the pump beam. This allows tunable signal output at variable burst rates from DC all the way up to 5 MHz. Furthermore, arbitrary pulse sequences can be generated. The rapid signal buildup dynamics provide individual full-power pulses with only two prepulses. This is possible without the requirement for additional injection seeding. Hereby, the intrinsically high intra-cavity losses of the FFOPO system are found to beneficial, as they enable rapid off-switching of the output as signal ring-down is efficiently suppressed. Possible applications are the reduction of the average power while maintaining a high peak power level, as well as tunable arbitrary pulse sequence generation.

Femtosecond OPO pumped by a high power ytterbium rod-type fiber laser mode locked at harmonic repetition rates

We report on an optical parametric oscillator (OPO) pumped by femtosecond pulses delivered by a large-mode-area, ytterbium-doped, rod-type fiber laser. This femtosecond laser that is mode locked at harmonic repetition rates of 108 MHz, 216 MHz, and 324 MHz provides an average output power of more than 4.5 W and tens of nJ per pulse. The repetition rate is changed by adjusting the pulse polarization inside the laser cavity. Remarkably, at all these repetition rates and without any modification to the cavity, the OPO delivers femtosecond signal pulses that are tunable from 1450 nm to 1700 nm, with an average output power higher than 1 W. Increasing the pump power of the rod-type fiber and decreasing the transmission of the OPO output coupler, we were able to run the OPO at 540 MHz.

Widely tunable, high-power, femtosecond noncollinear optical parametric oscillator in the visible spectral range

Ultrafast visible radiation is of great importance for many applications ranging from spectroscopy to metrology. Because some regions in the visible range are not covered by laser gain media, optical parametric oscillators offer an added value. Besides a high-power broadband laser source, the ability to rapidly tune the frequency of pulses with high-power spectral density offers an extra benefit for experiments such as multicolor spectroscopy or imaging. Here, we demonstrate a broadband, high-power, rapidly tunable femtosecond noncollinear optical parametric oscillator with a signal tuning range of 440–720 nm in the visible range. The oscillator is pumped by the third harmonic of an Yb-fiber laser at 345 nm with a repetition rate of 50.2 MHz. Moreover, the signal wavelength is tuned by changing the cavity length only, and output powers up to 452 mW and pulse durations down to 268 fs are achieved. This is, to the best of our knowledge, the first demonstration of a quickly tunable femtosecond optical parametric oscillator that covers nearly the entire visible spectral range with high output power.

Compact, 2.95-GHz repetition-rate femtosecond optical parametric oscillator with tunable pulse repetition frequency

We report a compact femtosecond optical parametric oscillator (OPO) with a tunable repetition rate that is harmonically pumped using a 52.5 MHz Yb-doped fiber laser system. By reducing the OPO cavity length, the repetition rate can be adjusted successively from 1.935 to 2.95 GHz at 52.5 MHz intervals. The multiplication of the repetition rate is achieved by placing a nonlinear crystal in a compact linear cavity, and the minimum cavity length is 47.8 mm. The maximum signal power (205.2 mW) at 2.04 GHz is obtained at an input pump power of 2.35 W and a central wavelength of 1472 nm. The central wavelength of the signal pulses can be tuned from 1383 to 1596 nm. To the best of our knowledge, 2.95 GHz is the highest repetition rate achieved using a femtosecond OPO based on an ultrashort cavity with a length that is N times (N is an integer) shorter than that of the pump cavity.

Orthogonally polarized tunable dual-wavelength femtosecond optical parametric oscillator.

We demonstrate a femtosecond optical parametric oscillator that can generate orthogonally polarized dual-wavelength femtosecond pulses. Two periodically poled lithium niobate (PPLN) crystals with mutually orthogonal crystal axes are pumped by a single femtosecond fiber laser. The central wavelength of the two orthogonally polarized signal pulses can be continuously tuned from 1387 to 1588 nm with a maximum frequency separation of 27 THz. Because of the orthogonal dual-crystal scheme, the system is immune to the coherent coupling effect, thus overcoming the limitation of minimum frequency separation.

Controlled Generation of Wavelength-Tunable Higher Order Poincaré Sphere Beams From a Femtosecond Optical Parametric Oscillator

Although higher order Poincaré (HOP) beams are attractive due to their unique advantages and various efforts have been made for the generation of HOP sphere beams, the current generation technologies suffer from both limited output power and narrow bandwidth, preventing further practical applications. In this paper, we report on a femtosecond optical parametric oscillator (OPO) which can deliver high average power, on-demand arbitrary HOP sphere beams tunable across a wide spectral range in the near-infrared. The desired beam mode can be achieved by manipulating the geometric phase inside the OPO cavity to map the polarization to orbital angular momentum (OAM). Pumped by a Gaussian beam from an Yb-fiber laser, the generalized vector vortex femtosecond signal beams with spectral coverage from 1367 to 1650 nm are obtained. The device can produce over 200 mW structured beam signal power cross the complete tuning range with as much as 377 mW at 1480 nm for 2 W of input pump power. The proposed configuration, which shows superiorities of high average output power, flexible wavelength tunability and complete mode controlling property, may have direct implications in applications such as quantum optics and material processing.

Cascaded nonlinearity induced spatial domain effects in a high power femtosecond optical parametric oscillator.

We have investigated the effect of cascaded optical nonlinearity on the spatial beam properties of a femtosecond optical parametric oscillator (OPO). The OPO was operated with a tunable phase mismatch by varying the angle of the nonlinear crystal. The cascaded nonlinearity induced self-focusing and defocusing changed resonator's stability and impacted mode properties. With tuning of a phase mismatch, the calculated parabolic part of cascaded nonlinearity lens focal length changes from f ∼ 30 mm (D ∼ 33 m-1 at Δθ ∼ -0.5o) to infinity and back to f ∼ -110 mm (D ∼ -9 m-1 at Δθ ∼ 0.9o) in the LBO nonlinear crystal. Such high power nonlinear lenses in a cavity operated near its stability limit promoted the generation of axially asymmetric or pass-to-pass unstable resonator modes. It was shown that phase mismatched optical parametric oscillation changes the physical character of the resonator from linear to ring-like with two nonlinear crystals having two different focusing powers. Calculations showed that the QCN induced spatial nonlinear phase should lead to severe longitudinal chromatic aberrations for broad spectrum pulses. A numerical simulation in XYZ spatial domain and calculations using ABCD matrix approach confirmed the physical mechanisms underlying the experimental results and allowed for the interpretation of the observed effects.

Dual-Wavelength, High-Repetition-Rate, Compact Femtosecond Optical Parametric Oscillator

We demonstrate a dual-wavelength, compact femtosecond optical parametric oscillator (OPO) with high-repetition-rate, which is harmonically pumped by a ~101 MHz Yb-doped fiber laser system. The dual-wavelength output is realized by exploiting the bidirectional off-axis pumping technique, and the multiplication of repetition rate is derived by placing a nonlinear crystal in a miniaturized V-type cavity with only 16.5 cm length. By adjusting the detuning degree of the pump at one end, the maximum dual-wavelength gap is 66 nm from 1497 to 1563 nm. The time interval between the dual wavelengths can be adjusted freely. This is the first report on a dual-wavelength with the high-repetition-rate of GHz-level, femtosecond OPO system.

Controlled soliton formation in a femtosecond optical parametric oscillator with positive group delay dispersion

Soliton formation in a femtosecond optical parametric pumped by the second harmonic of a Yb: KGW solid-state oscillator was investigated. The intracavity group delay dispersion was positive, and the soliton condition was satisfied by introducing negative nonlinearity from cascaded quadratic nonlinearity (CQN). Controllable CQN was induced by an additional second-harmonic-generating nonlinear crystal inside the same resonator. Close to zero-phase mismatch, high CQN allows higher-order soliton formation, which leads to output power increase, self-phase modulation phase-matched dispersive wave formation, pulse splitting under perturbations of higher orders of nonlinear phase, and stable time/spectral domain oscillations with soliton period. Numerical simulations were employed to aid interpretations of the experimental data.

Exploiting optical nonlinearities for group delay dispersion compensation in femtosecond optical parametric oscillators.

A wavelength tunable femtosecond optical parametric oscillator pumped by the second harmonic of a Yb: KGW solid state oscillator was investigated. The intracavity group delay dispersion was positive, and soliton condition was satisfied by introducing negative nonlinearity from cascaded quadratic nonlinearity (CQN). Two different approaches were investigated - CQN induced by the same amplifying nonlinear crystal or CQN induced by an additional second harmonic generating nonlinear crystal inside the same resonator. The second crystal was shown to correct the resonator misalignment induced by the rotation of the amplifying crystal as the wavelength was tuned in the range of 770-970 nm. It simultaneously compensated positive resonator GDD offsets of +/- 1000 fs2 with +/- 5% SHG power losses, simulating a method for compensation of GDD ripples in a broadband mirror.

Cascaded nonlinearities in high-power femtosecond optical parametric oscillator

A femtosecond optical parametric oscillator (OPO) pumped by the second harmonic of a Yb:KGW solid-state oscillator was investigated. A comparison between lithium triborate (LBO) and barium borate (BBO) crystals was carried out, with particular attention to the impact of phase mismatch on pulse characteristics. The phase mismatch induces cascaded nonlinearity, which acts as an effective nonlinear refractive index. Negative group delay dispersion of the resonator and the effective nonlinear refractive index allows soliton-like pulse formation with varying pulse durations and a bandwidth-limited time-bandwidth product. Deviation from the soliton equation was observed when intracavity power was varied. The measured pulse durations were lower than the classical soliton duration, indicating that the pulses were not classical solitons. A Z-scan experiment was used to determine nonlinear refractive indices under conditions identical to those in the oscillator cavity. Unexpectedly, the signs of nonlinear refraction as measured by the Z scan and indirectly observed in the OPO proved to be the opposite. This sign reversal could be interpreted in terms of the competing cascaded nonlinearities corresponding to self-phase modulation and cross-phase modulation between the signal and the pump pulses in the nonlinear OPO crystal.

Dither-free stabilization of a femtosecond doubly resonant OPO using parasitic sum-frequency mixing.

Stable operation of a doubly resonant femtosecond optical parametric oscillator (OPO) requires submicron matching of the OPO and pump laser cavity lengths, which is normally implemented using a dither-locking feedback scheme. Here we show that parasitic sum-frequency mixing between the pump and resonant pulses of a degenerate femtosecond OPO provides an error signal suitable for actuating the cavity length with the precision needed to maintain oscillation on a single fringe and at maximum output power. Unlike commonly used dither-locking approaches, the method introduces no modulation noise and requires no additional optical components, except for one narrowband filter. The scheme is demonstrated on a Ti:sapphire-pumped sub-40-fs PPKTP OPO, from which data are presented showing a tenfold reduction in relative intensity noise compared with dither locking.

Multi-soliton formation in femtosecond degenerate optical parametric oscillators.

Multi-soliton formation is observed theoretically and experimentally in femtosecond degenerate optical parametric oscillators (OPOs). We show that when the pulse energy of the pump source of a femtosecond OPO is increased to a certain level, the existing soliton will move towards the leading edge of pump pulses due to the enhanced nonlinear acceleration, and the undepleted pump energy will support the generation of more solitons. We have successfully observed the generation of double solitons and triple solitons in experimental demonstrations with the measured pulse characteristics agreeing well with the theoretical ones. The generation of multi-soliton sources may stimulate many novel applications, including data storage, telecommunication, and all-optical signal processing.

Theoretical investigation of pulse-to-pulse instabilities in a synchronously pumped femtosecond optical parametric oscillator

A singly resonant synchronously pumped optical parametric oscillator (SPOPO) based on the experimental setup of J. Opt. Soc. Am. B 36, 131 (2019)JOBPDE0740-322410.1364/JOSAB.36.000131 is studied theoretically. Stable, oscillatory, and chaotic operation modes of the SPOPO are investigated. The need of the self- and cross-phase modulation terms in the theoretical model for the explanation of the instabilities is demonstrated. The theoretical values of the wavelengths of the signal spectrum maxima are found. The evidence of chaos by the calculation of the Lyapunov exponent is provided. The possibilities to avoid the instabilities are discussed.