Femtosecond Optical Parametric Amplifier Research Articles

Unlocking superior performance of broadband powerful mid-IR optical parametric amplifiers with a BaGa2GeS6 crystal pumped at 1.24 µm.

We report on the development of a tunable (1.5-6.5 µm) femtosecond optical parametric amplifier (OPA) based on a novel, to the best of our knowledge, BaGa2GeS6 (BGGS) crystal with a Cr:Forsterite pumping laser. Total conversion efficiency as high as 28% is achieved in a robust two-stage setup resulting in the generation of a 340-µJ 1.67-µm signal and 100-µJ 4.65-µm idler pulses. A 5-optical-cycles 94-fs 6-µm idler pulses are demonstrated with a propriate dispersion compensation by Ge and GaAs plates. An experimental estimate is given for the effective nonlinearity of a BGGS material, which for our nonlinear process reaches 19.5 pm/V for Type II phase matching. The crystal is additionally tested as a final amplifier in a high-energy OPA, where total output reaches 1.2 mJ with more than 40% conversion efficiency. The demonstrated high nonlinearity, high damage threshold, and chemical stability of the polished surface make BGGS crystal an ideal candidate for the development of high-energy OPAs with multi-millijoule pumping lasers.

Broadly tunable femtosecond optical parametric amplifiers in the mid-infrared waveband based on cascaded noncollinear-collinear KTiOAsO4 crystals

We demonstrate a widely tunable, ultrafast optical parametric amplifier (OPA) based on cascaded noncollinear-collinear KTiOAsO4 (KTA) crystals seeded by a white light continuum (WLC) source in the mid-infrared waveband. We show that the parametric gain bandwidth of a collinear KTA crystal closely matches that of a noncollinear KTA crystal, thus avoiding the gain-bandwidth-mismatch-induced reduction of the frequency conversion-efficiency. In addition, we demonstrate the direct amplification of the WLC seed at up to 2.8 μm, which indeed offers a new technical route for manipulating the amplification bandwidth of ultrafast OPAs. This is, as far as we know, the first demonstration of direct amplification of the WLC light at this wave region with a 1-μm pump source.

Reducing wavelength jitter in white-light seeded femtosecond optical parametric chirped-pulse amplifiers.

White light generation (WLG) in bulk material can be used as a versatile broadband seed source for optical parametric chirped pulse amplification (OPCPA) stages. In this case, it is beneficial to optimize the performance of the WLG seeder in combination with the subsequent OPCPA stage. Here, we characterize how small variations in the drive pulse energy affect the white light seeder performance, in particular the wavelength stability of the amplified OPCPA spectrum. To isolate the influence of drive pulse energy on the OPCPA central wavelength, we introduce a phase-sensitive amplitude measurement and carefully optimize the drive pulse focus position (at the bulk) to minimize the sensitivity to the jitter of the drive pulse energy. With additional active stabilization of the delay between pump and seed pulses in the OPCPA, we achieve a central wavelength jitter of 2 × 10-4. With this performance, our source is an ideal front-end for applications in laser-plasma acceleration or free-electron laser seeding.

Femtosecond fluorescence conical optical parametric amplification spectroscopy.

Parametric superfluorescence (PSF), which originated from the optical amplification of vacuum quantum noise, is the primary noise source of femtosecond fluorescence non-collinear optical parametric amplification spectroscopy (FNOPAS). It severely affects the detection limit of FNOPAS to collect the femtosecond time-resolved spectra of extremely weak fluorescence. Here, we report the development of femtosecond fluorescence conical optical parametric amplification spectroscopy (FCOPAS), aimed at effectively suppressing the noise fluctuation from the PSF background. In contrast to traditional FNOPAS configurations utilizing lateral fluorescence collection and dot-like parametric amplification, FCOPAS employs an innovative conical fluorescence collection and ring-like amplification setup. This design enables effective cancellation of noise fluctuation across the entire PSF ring, resulting in an approximate order of magnitude reduction in PSF noise compared to prior FNOPAS outcomes. This advancement enables the resolution of transient fluorescence spectra of 4-dicyanomethylene-2-methyl-6-p-dimethylaminostyryl-4H-pyran (DCM) dye molecules in ethanol, even at an optically dilute concentration of 10-6 mol/l, with significantly enhanced signal-to-noise ratios. This improvement will be significant for extremely weak fluorescence detection on the femtosecond time scale.

Laser Output Performance and Temporal Quality Enhancement at the J-KAREN-P Petawatt Laser Facility

We described the output performance and temporal quality enhancement of the J-KAREN-P petawatt laser facility. After wavefront correction using a deformable mirror, focusing with an f/1.3 off-axis parabolic mirror delivered a peak intensity of 1022 W/cm2 at 0.3 PW power levels. Technologies to improve the temporal contrast were investigated and tested. The origins of pre-pulses generated by post-pulses were identified and the elimination of most pre-pulses by removal of the post-pulses with wedged optics was achieved. A cascaded femtosecond optical parametric amplifier based on the utilization of the idler pulse rather than the signal pulse was developed for the complete elimination of the remaining pre-pulses. The orders of magnitude enhancement of the pedestal before the main pulse were obtained by using a higher surface quality of the convex mirror in the Öffner stretcher. A single plasma mirror was installed in the J-KAREN-P laser beam line for further contrast improvement of three orders of magnitude. The above developments indicate, although it has not been directly measured, the contrast can be as high as approximately 1015 up to 40 ps before the main pulse. We also showed an overview of the digital transformation (DX) of the system, enabling remote and automated operation of the J-KAREN-P laser facility.

Effects of chirp of the white-light continuum seed on the pulse characteristics of collinear femtosecond optical parametric amplifiers

The influence of the chirp of the white-light continuum seed on the pulse characteristics of femtosecond optical parametric amplifiers (OPAs) is studied. Here, we focus on collinear OPAs based on type-I phase-matched BBO crystals. By numerical simulations, we investigate the evolution of the pulse-width, spectral bandwidth and time-bandwidth-product (TBP) of the amplified signal pulses with respect to the chirp of the white-light continuum seed pulses. In particular, we show that by manipulating the white-light continuum seed pulses to be highly chirped, nearly transform-limited optical pulses can be directly obtained from OPAs, without requiring dispersion-compensation elements. Our study demonstrates that chirp management offers a concise and effective technical route for obtaining nearly transform-limited, narrowband optical pulses from femtosecond OPAs, which would benefit many applications, including nonlinear imaging and spectroscopy.

Measurement of three-photon excitation cross-sections of fluorescein from 1154 nm to 1500 nm.

Measurements of three-photon action cross-sections for fluorescein (dissolved in water, pH ∼11.5) are presented in the excitation wavelength range from 1154 to 1500 nm in ∼50 nm steps. The excitation source is a femtosecond wavelength tunable non-collinear optical parametric amplifier, which has been spectrally filtered with 50 nm full width at half maximum band pass filters. Cube-law power dependance is confirmed at the measurement wavelengths. The three-photon excitation spectrum is found to differ from both the one- and two-photon excitation spectra. The three-photon action cross-section at 1154 nm is more than an order of magnitude larger than those at 1450 and 1500 nm (approximately three times the wavelength of the one-photon excitation peak), which possibly indicates the presence of resonance enhancement.

Performance improvement of a nonlinear temporal filter by using cascaded femtosecond optical parametric amplification.

In this paper, we report that the conversion efficiency and spectrum of femtosecond optical parametric amplification (fs-OPA) can be significantly enhanced by employing a compact cascaded femtosecond OPA (CF-OPA) scheme with the self-compensation of the temporal walk-off between two nonlinear gain media. Correspondingly, the gain related temporal contrast can also be improved. The feasibility of the CF-OPA method using three cascaded BBO crystals is numerically and experimentally analyzed. Moreover, by replacing the conventional fs-OPA with the CF-OPA and optimizing the design, the performance of a nonlinear temporal filter combining cross-polarized wave generation and fs-OPA is comprehensively improved. The experimental results demonstrate the superiority of the CF-OPA scheme, which can generate high-performance cleaned pulses at 1 kHz repetition rate with energy of 340μJ, energy fluctuation below 0.9% (RMS), spectral width of 97 nm (FWHM), Fourier-transform-limited pulse width of 12 fs and temporal contrast better than 10-12. To the best of our knowledge, this is the first reported temporal walk-off self-compensated quasi-collinear CF-OPA geometry adopting three cascaded BBO crystals, which can be easily generalized to other wavelengths or nonlinear crystals. The above nonlinear temporal filter with a CF-OPA scheme has the rarest comprehensive parameters, which can provide excellent seed pulses for PW and 10 PW class femtosecond laser systems.

Octave-spanning mid-infrared femtosecond OPA in a ZnGeP2 pumped by a 2.4 μm Cr:ZnSe chirped-pulse amplifier.

We report on the highly efficient, octave-spanning mid-infrared (mid-IR) optical parametric amplification (OPA) in a ZnGeP2 (ZGP) crystal, pumped by a 1 kHz, 2.4 μm, 250 fs Cr:ZnSe chirped-pulse amplifier. The full spectral coverage of 3-10 μm with the amplified signal and idler beams is demonstrated. The signal beam in the range of ∼3 - 5 μm is produced by either white light generation (WLG) in YAG or optical parametric generation (OPG) in ZGP using the common 2.4 μm pump laser. We demonstrate the pump to signal and idler combined conversion efficiency of 23% and the pulse energy of up to 130 μJ with ∼2 μJ OPG seeding, while we obtain the efficiency of 10% and the pulse energy of 55 μJ with ∼0.2 μJ WLG seeding. The OPA output energy is limited by the available pump pulse energy (0.55 mJ at ZGP crystal) and therefore further energy scaling is feasible with multi-stage OPA and higher pump pulse energy. The autocorrelation measurements based on random quasi-phase matching show that the signal pulse durations are ∼318 fs and ∼330 fs with WLG and OPG seeding, respectively. In addition, we show the spectrally filtered 30 μJ OPA output at 4.15 μm suitable for seeding a Fe:ZnSe amplifier. Our ultrabroadband femtosecond mid-IR source is attractive for various applications, such as strong-field interactions, dielectric laser electron acceleration, molecular spectroscopy, and medical surgery.

Numerical study on the characteristics of hybrid seeded femtosecond optical parametric amplifier at mid-infrared wavelength

Abstract In the optical parametric amplifier (OPA) process, the phase of the pump is transmitted to the amplified signal due to the spatial walk-off effect and/or a temporal group velocity mismatch (GVM) effect between coherent light waves. As a result, the quality of amplified signal will be reduced by the phase distortion and variation of beam equality of the pump pulse. By using a pair of OPAs, the signal and idler are chosen as seeding lights in the front and back stages, respectively, so that the phase of the amplified signal can be restored, and the influence of phase distortion and beam equality deterioration of pump pulse can be eliminated. The present article also reports other characteristics of this hybrid seeded scheme, including accepted bandwidth, spectral purity, and conversion efficiency.

Three-Dimensional Printing of Nonlinear Optical Lenses.

In the current paper, a series of nonlinear optical (NLO) active devices was prepared by utilizing stereolithographic three-dimensional printing technique. Microcrystalline NLO active component, urea, or potassium dihydrogen phosphate was dispersed in a simple photopolymerizable polyacrylate-based resin and used as the printing material to fabricate highly efficient transparent NLO lenses. The nonlinear activity of the printed lenses was confirmed by second-harmonic generation measurements using a femtosecond laser-pumped optical parametric amplifier operating at a wavelength of 1195 nm. The three-dimensional printing provides a simple method to utilize a range of NLO active compounds without tedious crystal growing and processing steps. Furthermore, introducing NLO additives in the printing material provides an easy and cost-efficient way to manufacture lenses with NLO functionality.

Influence of wave-front curvature on supercontinuum energy during filamentation of femtosecond laser pulses in water

We demonstrate that using spatially divergent incident femtosecond 1240-nm laser pulses in water leads to an efficient supercontinuum generation in filaments. Optimal conditions were found when the focal plane is placed $100--400\phantom{\rule{4pt}{0ex}}\ensuremath{\mu}\mathrm{m}$ before the water surface. Under sufficiently weak focusing conditions [numerical aperture ($\mathrm{NA})l0.2$] and low-energy laser pulses, the supercontinuum energy generated in divergent beams is higher than the supercontinuum energy generated in convergent beams. Analysis by means of the unidirectional pulse propagation equation shows a dramatic difference between filamentation scenarios of divergent and convergent beams, that explains corresponding features of the supercontinuum generation. Under strong focusing conditions ($\mathrm{NA}\ensuremath{\geqslant}0.2$) and high-energy laser pulses, the supercontinuum generation is suppressed for convergent beams in contrast to divergent beams that nevertheless are shown experimentally to allow supercontinuum generation. The presented technique of the supercontinuum generation in divergent beams in water is highly demanded in a development of femtosecond optical parametric amplifiers.

520-µJ mid-infrared femtosecond laser at 2.8 µm by 1-kHz KTA optical parametric amplifier

We report on a 520-µJ, 1-kHz mid-infrared femtosecond optical parametric amplifier system driven by a Ti:sapphire laser system. The seeding signal was generated from white-light continuum in YAG plate and then amplified in four non-collinear amplification stages and the idler was obtained in the last stage with central wavelength at 2.8 µm and bandwidth of 525 nm. To maximize the bandwidth of the idler, a theoretical method was developed to give an optimum non-collinear angle and estimate the conversion efficiency and output spectrum. As an experimental result, laser pulse energy up to 1.8 mJ for signal wave and 520 µJ for idler wave were obtained in the last stage under 10-mJ pump energy, corresponding to a pump-to-idler conversion efficiency of 5.2%, which meets well with the numerical calculation.

High-contrast front end based on cascaded XPWG and femtosecond OPA for 10-PW-level Ti:sapphire laser.

By combining cross-polarized wave generation and femtosecond optical parametric amplification, a high-contrast front end featuring ultrahigh contrast, a broadband spectrum, an excellent beam profile, and good stability is built for a 10-PW-level Ti:sapphire laser in the Shanghai Superintense Ultrafast Laser Facility (SULF-10PW laser). The front end can deliver a cleaned pulse with a 110 μJ energy at 1 kHz, and the bandwidth of the cleaned pulse exceeds 60 nm (FWHM), which can support a 17 fs compressed pulse duration. The measured output energy fluctuation in one hour is <1.8% in rms value. The measurement-limited contrast is 10-10 at 3 ps before the main pulse. Utilizing the high-contrast front end, single-shot contrast at 10-10 level has been demonstrated in the SULF-10PW laser at a 24 fs pulse duration.

Supercontinuum generation and analysis in extruded suspended-core As2S3 chalcogenide fibers

Compared with the traditional fluoride fibers and tellurite fibers that can work in the near-infrared region, suspended-core fibers based on chalcogenide glasses have wider transmitting regions and higher nonlinear coefficients, thus the mid-infrared supercontinuum generations can be achieved easily. Rather than adopting the traditional fabrication technique of hole-drilling and air filling, we adopted a totally novel extrusion technique to fabricate As2S3 suspended-core fibers with four holes, and its mid-infrared supercontinuum generation was investigated systematically by integrating theoretical simulation and empirical results. The generalized nonlinear SchrOdinger equation was used to simulate the supercontinuum generation in the As2S3 suspended-core fibers. The simulated supercontinuum generation in the As2S3 suspended-core fibers with different pump wavelengths (2–5 µm), increasing powers (0.3–4 kW), and various fiber lengths (1–50 cm) was obtained by a simulative software, MATLAB. The experimental results of supercontinuum generation via femtosecond optical parametric amplification (OPA) were recorded by changing fiber lengths (5–25 cm), pump wavelengths (2.9–5 µm), and pump powers (10–200 kW). The simulated consulting spectra are consistent with the experimental results of supercontinuum generation only if the fiber loss is sufficiently low.

The Xingguang-III laser facility: precise synchronization with femtosecond, picosecond and nanosecond beams

We report a high-intensity laser facility named Xingguang-III that generates femtosecond, picosecond, and nanosecond beams with three wavelengths, i.e. 800 nm, 1053 nm, and 527 nm, respectively. To the best of our knowledge, the laser facility is the first one which produces three beams with different pulse widths and wavelengths. An optical synchronization technique, combining super continuum generation and femtosecond optical parametric amplification, was developed to ensure three beams are from the same source to achieve precise synchronization. The femtosecond beam is a double chirped-pulse-amplification Ti:sapphire laser which applies cross-polarized wave generation to improve the temporal contrast. The picosecond/nanosecond beams utilize the optical parametric amplification + Nd:glass mixed amplification scheme. The output energy and pulse width of the three beams are 20.1 J/26.8 fs, 370.2 J/0.48 ps (shortest), and 575.4 J/1.0 ns, respectively. The smallest synchronization time (peak-to-valley) and the shot-to-shot timing jitter (peak-to-peak) of less than 1.32 ps have been achieved for the femtosecond and picosecond beams.

Astigmatism transfer phenomena in the optical parametric amplification process

We numerically and experimentally investigate the astigmatism transfer phenomena in femtosecond optical parametric amplification (OPA). We model the OPA process based on the coupled second-order three-wave nonlinear propagation equations. The numerical and experimental results support that the input pump pulse astigmatism can be transferred into the idler pulse but not the signal pulse, and the idler pulse astigmatism originating from spatial walk-off is less than the idler pulse astigmatism received from the pump. Thus, we can provide a clear understanding of astigmatism transfer mechanisms in the OPA process, and make better use of broadband tunable OPA sources.

High power multi-color OPCPA source with simultaneous femtosecond deep-UV to mid-IR outputs.

Many experimental investigations demand synchronized pulses at various wavelengths, ideally with very short pulse duration and high repetition rate. Here we describe a femtosecond multi-color optical parametric chirped pulse amplifier (OPCPA) with simultaneous outputs from the deep-UV to the mid-IR with optical synchronization. The high repetition rate of 160 kHz is well suited to compensate for low interaction probability or low cross section in strong-field interactions. Our source features high peak powers in the tens to hundreds of MW regime with pulse durations below 110 fs, which is ideal for pump-probe experiments of nonlinear and strong-field physics. We demonstrate its utility by strong-field ionization experiments of xenon in the near- to mid-IR.

Femtosecond wavelength-tunable OPCPA system based on picosecond fiber laser seed and picosecond DPSS laser pump.

We present a compact and stable femtosecond wavelength-tunable optical parametric chirped pulse amplification (OPCPA) system. A novel OPCPA front-end was constructed using a multi-channel picosecond all-in-fiber source for seeding DPSS pump laser and white light supercontinuum generation. Broadband chirped pulses were parametrically amplified up to 1 mJ energy and compressed to less than 40 fs duration. Pulse wavelength tunability in the range from 680 nm to 930 nm was experimentally demonstrated.

Water-window soft x-ray high-harmonic generation up to the nitrogen K-edge driven by a kHz, 2.1 μm OPCPA source

We report the generation of coherent water-window soft x-ray harmonics in a neon-filled semi-infinite gas cell driven by a femtosecond multi-mJ mid-infrared optical parametric chirped-pulse amplification (OPCPA) system at a 1 kHz repetition rate. The cutoff energy was extended to ∼450 eV with a 2.1 μm driver wavelength and a photon flux of photons/s/1% bandwidth was obtained at 350 eV. A comparable photon flux of photons/s/1% bandwidth was observed at the nitrogen K-edge of 410 eV. This is the first demonstration of water-window harmonic generation up to the nitrogen K-edge from a kHz OPCPA system. Finally, this system is suitable for time-resolved soft x-ray near-edge absorption spectroscopy. Further scaling of the driving pulse's energy and repetition rate is feasible due to the availability of high-power picosecond Yb-doped pump laser technologies, thereby enabling ultrafast, tabletop water-window x-ray imaging.