Femtosecond Laser Filament Research Articles

Fractional-order hybridly polarized vector beams: generation, focusing, propagation, and spatial self-phase modulation

As a class of integer-order vector beams, hybridly polarized vector beams (HPVBs) are widely used in focus shaping, femtosecond laser filamentation, linear and nonlinear polarization evolution, etc. Recently, fractional-order vector beams have gained widespread interest due to their more control parameters, rich photophysical properties, and novel nonlinear optical phenomena. In this work, we report the experimental generation, focusing and propagation characteristics, and spatial self-phase modulation (SSPM) phenomenon of fractional-order HPVBs. It is shown that during the focusing and propagation processes, the intensity pattern of fractional-order HPVBs develops from a near-Gaussian structure in the incident plane to an asymmetric structure in both the focal field and the far field. Meanwhile, their distributions of state of polarization (SoP) also evolve, although it remains a hybrid polarization distribution overall. When the focused fractional-order HPVBs pass through the nonlinear optical sample, the far-field self-diffraction intensity pattern displays an irregular concentric multi-ring structure with a hybrid polarization distribution. It is found that the nonlinear medium not only modulates the far-field intensity pattern of fractional-order HPVBs but also controls their SoP distribution. This symmetric breaking HPVB has potential application prospects in optical micro-manipulation, light-matter interaction, optical spin-orbit conversion, etc.

Generating nano/microliter droplets with on-demand repetition rates by femtosecond filament-fabricated superhydrophobic bevel needle nozzles

Nano- and micro-droplets provide a platform for microanalysis of a variety of biochemical reactions with less consumption of reagents and large-extent elimination of cross-contamination, but stable generation of such monodisperse droplets with an on-demand size and repetition rate should be first established. Here, we present a simple and robust approach to generate nano/microliter (nL/μL) droplets with predetermined size and repetition rate by using femtosecond laser filament-fabricated stainless bevel needle nozzles (BNNs). We demonstrate that hierarchically heterogeneous micro/nanostructures can be directly formed on both the inner and outer surfaces of BNNs by femtosecond laser filament processing, and that after a heat treatment the fabricated BNNs show an excellent superhydrophobic property with the water contact angle of ∼160° and the rolling-off angle of ∼0.4°. With the superhydrophobic BNNs (19–27 gauge), we produce monodisperse water droplets (2.5 μL–87 nL) with nearly the same sizes as the needle diameters, and dispense them repeatedly with on-demand repetition rates from sub-1 Hz to more than 100 Hz over several orders of the flow rate. The results provide a new way for generating microdroplets on demand for various droplet-based applications.

High efficiency femtosecond laser ablation of alumina ceramics under the filament induced plasma shock wave

Femtosecond laser filament enables energy transfer over long distances, which is of great value for studying long-range ablation. However, the energy coupling of filament with the plasma generated by the ablation process leads to a very complex behavior which limits the ablation efficiency. This study systematically investigated the ablation mechanism of laser-induced filament in alumina ceramic. The plasma shock wave was initially investigated using spectral detection techniques combined with Sedov-Taylor theory. The results indicated that the maximum plasma shock wave reached 30 MPa under the irradiated by a 1 mJ fs laser. The theoretical analysis confirmed the effectiveness of the filament-induced plasma shock wave in enhancing the ablation rate of alumina ceramic. In this context, the experimental studies were conducted with varying filament positions and pulse energies, and the corresponding ablation rates for each parameter were investigated. The filament in the ablation process was found to has a secondary sputtering effect, which is an effective contributor to enhance the ablation rate. The corresponding ablation depth reach to 550 μm while achieving an ablation rate of 3.1 μm3/μJ. Finally, the coupling mechanism between the femtosecond laser filament and the plasma shock wave was systematically revealed. This research will facilitate future laser remote ablation applications with high efficiency.

Pressure scaling of femtosecond laser filamentation in air: Prospects for long-range atmospheric propagation

The principal trend of the last decades is the use of laser systems generating ultrashort (femtosecond) laser pulses of gigawatt and terawatt power in various spheres of human activity, in particular, in atmospheric researches. One of the important challenges within this problem is the use of the unique nonlinear optical phenomena manifesting in the atmosphere as pulse self-focusing, light-induced ionization of the medium, plasma generation and laser filamentation for remote laser diagnostics of the aerosol-gas constituents and efficient delivery of concentrated optical energy over long distances in the atmosphere. This brings to the forefront the problem of increasing the actual length of the nonlinear interaction of an ultrashort laser pulse with medium to kilometer distances whereas real physical length of most existing optical paths is usually limited by several hundred meters. We propose and theoretically substantiate an effective way to solve the problem of long-range atmospheric filamentation by transforming the propagation medium itself using short laboratory traces and optical cuvettes with gases of increased (over-atmospheric) pressure. Following the scaling laws of the optical characteristics of pressurized medium, the coefficients describing the interaction between optical wave and medium increase along with the increase in gas pressure. By the numerical simulations in the framework of the nonlinear Schrodinger equation, we show that this makes it possible to emulate kilometers-long atmospheric traces for laser beams of centimeter diameter and terawatt pulse power on the laboratory scale (tens of meters).

Spatial distribution of self-seeded air lasers induced by the femtosecond laser filament plasma

The femtosecond laser filament-induced air laser plays a significant role for the remote sensing of air pollutants. The spatial distributions of air laser intensity were investigated experimentally in previous studies. However, the mechanism of the air laser propagation properties inside the filament plasma has not been quite clear yet. Moreover, few studies have been dedicated to the reproduction of the air laser profile from nitrogen molecules propagating in the filament plasma based on the numerical simulation method. In this study, the lasing action of the air laser from the transition of the first negative (0,0) band of nitrogen ions at 391 nm was simulated during the femtosecond laser filamentation. The beam profile of the air laser changes from a Gaussian or super-Gaussian shape to an outer ring structure by increasing the filament length or nitrogen ion density, which is in accord with the previous experimental result. A multiple-diffraction effect has been proposed to clarify the mechanism of the outer rings beam pattern formation, which is induced by the dynamical interaction between the lasing effect and diffraction effect of the air laser propagating inside the filament plasma. In addition, the amplified air laser power as a function of both the filament length and nitrogen ion density was investigated. Our study would pave the way to improve the energy conversion efficiency and directivity of remote air lasers, which would be significant for remote sensing applications.

Energy deposition in air by moderately focused femtosecond laser filaments

Energy deposition in air by moderately focused femtosecond laser filaments

A Retrospective Study: Are the Multi-Dips in the THz Spectrum during Laser Filamentation Caused by THz–Plasma Interactions?

During the process of terahertz (THz) wave generation via femtosecond laser filamentation in air, as well as through the mixing of THz waves with externally injected plasma filaments, THz waves engage in interactions with the plasma. A characteristic feature of this interaction is the modulation of the THz radiation spectrum by the plasma, which includes the generation of THz spectral dips. This information is essential for understanding the underlying mechanisms of THz–plasma interactions or for inferring plasma parameters. However, a current debate exists on the number of THz spectral dips observed after the interaction, with different opinions of single versus multiple dips, thus leaving the interaction mechanisms still ambiguous. In this work, we retrospectively analyzed the experimental appearance of multiple dips in the THz spectrum and found that the current observations of such dips are predominantly a result of the water vapor absorption with a low spectral resolution. Additionally, we observed that altering the acquisition width of the temporal THz signal also influenced the dips’ number. Hence, in future research, simultaneous attention should be paid to the following two aspects of THz–plasma interactions: (1) It is necessary to ensure a sufficiently wide time-domain window to accurately represent the spectral dip characteristics. (2) The spectral dips should be carefully distinguished from the water absorption lines before being further studied. On the other hand, for the case of a single dip in the THz spectrum, we also put forward a new viewpoint of the resonance between surface plasmon waves and THz waves, which should also be taken into consideration in future studies.

Specificity of DNA damage formation induced by femtosecond near-infrared laser filamentation in water

We investigated the deoxyribonucleic acid (DNA) damage induced by laser filamentation, which was generated by focusing femtosecond near-infrared Ti:Sapphire laser light in water at several repetition rates ranging from 1000 Hz to 10 Hz. Using plasmid DNA (pUC19), the single-strand break, double-strand break, nucleobase lesions, and the fragmented DNA were analyzed and quantified by agarose gel electrophoresis. Additionally, the H2O2 concentration after irradiation was determined. We observed that (1) the DNA damage per laser shot and (2) the enzyme-sensitive base lesions per total DNA damage decreased as the laser repetition rate increased. Furthermore, (3) extraordinarily short DNA fragments were likely to be produced, compared with those produced using X-rays, and (4) most OH radicals could be eliminated by recombination to generate H2O2, preventing them from damaging the DNA. The Monte-Carlo simulation of the strand break formation implies that the observed dependency of strand break efficiency on the laser repetition rate is mainly due to diffusion of DNA molecules. These findings quantitatively and qualitatively revealed that an intense laser pulse induces a specific DNA damage profile that is not induced by X-rays, a sparsely ionizing radiation source.

Pulse repetition-rate effect on the critical power for self-focusing of femtosecond laser in air

The femtosecond laser filamentation is of significant interest due to its remarkable characteristics, and determining the critical power of self-focusing is essential for the process of filamentation. In this work, the critical power for self-focusing of intense femtosecond laser pulses at different repetition rates is experimentally measured according to the focus-shift method. A bimodal fitting method is proposed to more accurately determine the self-focusing critical power. It is found that the self-focusing critical power decreases as the laser repetition rate increases. A numerical simulation of the filamentation process based on the modified nonlinear Schrödinger equation effectively explains the experimental results obtained. This work provides valuable insights for the generation and application of high repetition rate femtosecond laser filamentation.

Real-Time Demonstration of Multi-Gigabit/s Free- Space Optical Communications Employing Femtosecond Laser Filaments in Complex Environment

Real-Time Demonstration of Multi-Gigabit/s Free- Space Optical Communications Employing Femtosecond Laser Filaments in Complex Environment

Laguerre-Gaussian laser filamentation for the control of electric discharges in air.

We study the use of Laguerre-Gaussian (LG) femtosecond laser filament with multi GW peak power to guide electric sparks in the atmosphere. We demonstrate that an LG beam with a vortex phase or with 6 azimuthal phase steps generates a filamentation regime, where a longer and more uniform energy deposition is produced compared to a normal beam with a flat phase. Such filaments can guide electric discharges over much longer distances. This technique could significantly extend the guiding range of laser filaments for lightning control and other long-range atmospheric experiments involving filamentation.

Temporal variations in NO, N2O, and NO2 generation in filament-induced atmospheric plasmas

Ultra-short pulse lasers generate filaments in air, inducing changes in molecular concentration and the formation of new molecules. However, our understanding of the specific chemical reactions triggered by these filaments remains limited. This study aimed to investigate the NxOy species produced by femtosecond laser filaments in a sealed chamber. We employed mid-infrared laser spectroscopy to analyze the resulting products over the reaction time. The research revealed that filament plasma generates NO, N2O, and NO2. Notably, N2O was detected for the first time in filament plasmas generated in the air. The production of NxOy species depends on the initial pressure and is influenced by factors such as plasma properties and molecular collisions. We measured the equilibrium concentrations of NO, N2O, and NO2 under atmospheric conditions, finding them to be 67, 38, and 518 ppm, respectively. Furthermore, comparative experiments conducted in zero air illustrated significantly higher concentrations of NO and NO2 under identical pressure conditions, indicating a significant negative impact of other air molecules on the generation of these species. These findings provide valuable insight into the understanding of filament-induced atmospheric chemical reactions and the generation of NxOy species.

Impact of gravitational force on high repetition rate filamentation of femtosecond laser pulses in the atmosphere

We study the influence of the gravitational force on the generation of low-density channels of air left in the path of femtosecond laser filaments at high repetition rate. We observe a more important density variation along the filament longitudinal axis in the case of a vertically created filament as compared to a horizontal one. This leads to a more important reduction of the electrical breakdown field using vertical filament. This geometry induced difference is only observed at high repetition rate because it is directly related to the cumulative effect appearing above 100 Hz.

A convenient acoustic measurement of femtosecond filamentation based on a cell phone

The acoustic diagnostic method has been widely used in diagnosing femtosecond filamentation. In this work, acoustic measurements of femtosecond laser filamentation and weakly air-ionized region are conducted using a readily available portable device - a cell phone. The signal is extracted by employing digital signal processing method of Fourier transformation filtering. The results demonstrate that the method can be used for effective measurements even in noisy environments. This greatly enhances the accuracy and portability of the acoustic method, providing a practical approach for improving acoustic diagnostics.

Femtosecond laser one-step direct-writing high quality volume Bragg grating.

Volume Bragg grating is one-step fabricated with femtosecond laser direct-writing technology inside a high nonlinearity chalcogenide glass of As2S3. As the generated femtosecond laser filamentation effect could combined with the cylindrical lens focusing method, a two-dimensional refractive index change interface could spontaneously grow along the incident direction with either the laser pulse energy or number increasing. A number of two-dimensional refractive index change interfaces are periodically arranged to stack into a volume Bragg grating. Through periodically moving the sample stage, a grating of 2 mm × 2 mm × 1.7 mm can be fabricated in 15 minutes. And the maximum diffraction efficiency of grating reached 95.49% under the optimal parameters. This study provides a new processing strategy for femtosecond laser direct-writing volume Bragg grating with high processing efficiency and excellent structural performance.

Stable, intense supercontinuum light generation at 1 kHz by electric field assisted femtosecond laser filamentation in air

Supercontinuum (SC) light source has advanced ultrafast laser spectroscopy in condensed matter science, biology, physics, and chemistry. Compared to the frequently used photonic crystal fibers and bulk materials, femtosecond laser filamentation in gases is damage-immune for supercontinuum generation. A bottleneck problem is the strong jitters from filament induced self-heating at kHz repetition rate level. We demonstrated stable kHz supercontinuum generation directly in air with multiple mJ level pulse energy. This was achieved by applying an external DC electric field to the air plasma filament. Beam pointing jitters of the 1 kHz air filament induced SC light were reduced by more than 2 fold. The stabilized high repetition rate laser filament offers the opportunity for stable intense SC generation and its applications in air.

Rapid diagnosis of femtosecond laser filament by single laser shot-induced acoustic pulses [Invited]

Rapid diagnosis of femtosecond laser filament by single laser shot-induced acoustic pulses [Invited]

Pulse repetition rate effect on the plasma inside femtosecond laser filament in air

Pulse repetition rate effect on the plasma inside femtosecond laser filament in air

Fluorescence and lasing of neutral nitrogen molecules inside femtosecond laser filaments in air: mechanism and applications.

High power femtosecond laser pulses launched in air undergo nonlinear filamentary propagation, featuring a bright and thin plasma channel in air with its length much longer than the Rayleigh length of the laser beam. During this nonlinear propagation process, the laser pulses experience rich and complex spatial and temporal transformations. With its applications ranging from supercontinuum generation, laser pulse compression, remote sensing to triggering of lightning, the underlying physical mechanism of filamentation has been intensively studied. In this review, we will focus on the fluorescence and cavity-free lasing effect of the plasma filaments in air. The different mechanisms underlying the fluorescence of the excited neutral nitrogen molecules will be throughly examined and it is concluded that the electron collision excitation is the dominant channel for the formation of the excited nitrogen molecules. The recently discovered "air lasing" effect, a cavity-free bidirectional lasing emission emitted by the filaments, will be introduced and its main properties will be emphasized. The applications of the fluorescence and lasing effect of the neutral nitrogen molecules will be introduced, with two examples on spectroscopy and detection of electric field. Finally, we discuss the quenching effect of the lasing effect in atmosphere and the mechanisms responsible will be analyzed. An outlook for the achievement of backward lasing in air will be briefly presented.

Gorilla Glass Cutting Using Femtosecond Laser Pulse Filaments

Due to high durability, scratch resistance, and impact resistance, Gorilla glasses are a popular choice for protective screens of smartphones, tablets, and laptops. Precise cutting of Gorilla glasses is very important to maintain the overall aesthetics and user experience, which is very challenging. We demonstrated for the first time the cutting of Gorilla glass by means of femtosecond laser filamentation technique. To achieve laser filamentation, a femtosecond laser beam was focused and irradiated in different depths of the sample Gorilla glasses. The filament length varied with the change in the focus position of the laser beam. The effective numerical aperture of the objective lens rises due to the presence of dielectric material (i.e., the Gorilla glass itself) before the focus position of the femtosecond laser beam inside the glass samples. As a consequence, the focal distance of the incident laser beam was prolonged and focused in a very tiny spot with extremely high energy density. Consequently, filaments (i.e., high aspect ratio micro-voids) were evident inside the Gorilla glass samples. The filament length is controllable by changing the irradiation parameters of the laser beam, including magnification and numerical aperture of the lens, laser energy, and thickness of the Gorilla glass before the target focal point. The filament-engraved Gorilla glass samples go through mechanical cleaving process with 400 MPa pressure on both sides of the laser scanning line for smooth cutting of Gorilla glass. The proposed glass cutting technique show promises for commercial application.