Femtosecond Extreme Ultraviolet Pulses Research Articles

Explosion of Xenon Clusters Driven by Intense Femtosecond Pulses of Extreme Ultraviolet Light

The explosions of large xenon clusters irradiated by intense, femtosecond extreme ultraviolet pulses at a wavelength of 38 nm have been studied. Using high harmonic generation from a 35 fs laser, clusters have been irradiated by extreme ultraviolet pulses at intensity approaching 10;{11} W/cm;{2}. Charge states up to Xe8+ are observed, states well above those produced by single atom illumination, indicating that plasma continuum lowering is important. Furthermore, the kinetic energy distribution of the exploding ions is consistent with a quasineutral hydrodynamic expansion, rather than a Coulomb explosion.

Two-color photoionization in xuv free-electron and visible laser fields

Two-photon ionization of atomic helium has been measured by combining femtosecond extreme-ultraviolet pulses from the free-electron laser in Hamburg (FLASH at DESY) with intense light pulses from a synchronized neodymium-doped yttrium lithium fluoride laser. Sidebands appear in the photoelectron spectra when the two laser pulses overlap in both space and time. Their intensity exhibits a characteristic dependence on the relative time delay between the ionizing and the dressing pulses and provides an inherent time marker for time-resolved pump-probe experiments. The measurements of the sidebands are in good agreement with theoretical predictions and allow for a direct analysis of two-photon ionization, free from processes related to interference between multiple quantum paths.

Time-frequency characterization of femtosecond extreme ultraviolet pulses.

We present energy-resolved cross-correlation measurements of an extreme ultraviolet (XUV) pulse, generated as the fifth harmonic (15.5 eV) of an intense 80 fs laser pulse centered at 400 nm. Spectrally resolving the cross-correlation signal allows us to characterize the time-dependent frequency of the XUV pulse. We find that the fifth harmonic has a small negative chirp in excess of that predicted by perturbation theory. In addition, by manipulating the chirp of the driving laser we can induce and measure a positive or a negative chirp on the XUV pulse.