Fate Of Sediments Research Articles

Concentrations, potential sources and behavior of organochlorines and phenolic endocrine-disrupting chemicals in surficial sediment of the Shaying River, eastern China

Levels and distributions of organochlorine pesticides (OCPs) and phenolic endocrine-disrupting chemicals (EDCs) in surficial sediments of the Shaying River, the largest tributary of the Huaihe River in eastern China, were investigated to understand their relationship with the hydrodynamics. Concentrations of total hexachlorocyclohexane isomers (ΣHCHs) and dichlorodiphenyltrichloroethanes (ΣDDT) were in the range of 26.7–119 and 9.64–214 ng g−1 with mean values of 104 and 80.7 ng g−1, respectively. Residues of HCHs in sediments can be considered as originating from the application of both technical mixtures and lindane in the past. According to the spatial distribution of (DDD + DDE)/ΣDDT ratios, the influence of recent DDT inputs was dominant upstream, whereas DDD prevailed downstream, due to anaerobic degradation. Concentrations of total phenolic EDCs (ΣEDCs) including nonylphenol (NP), octylphenol (OP) and bisphenol A (BPA) ranged widely from 425 to 3,953 ng g−1 with the highest level occurring in the middle reach. This accumulation could be attributed to the retransfer of surficial sediment from upstream, where the main sources are located. Spatial distribution of contaminants indicated that riverine hydrodynamics can significantly affect their behavior and fate in sediment. This evidence was further verified by multivariate statistical techniques such as Cluster Analysis (CA), Principle Component Analysis (PCA) and Discriminant Analysis (DA). The CA identified three distinct clusters reflecting the large complexity of river system like geography setting, hydrodynamic condition, etc. This finding was also confirmed by the DA. Furthermore, a PCA demonstrated that about 80.8 % of total spatial variance can be explained by the first three factors, which also indicated that contaminant spatial distributions are driven by local inputs, biodegradation and riverine hydrodynamics.

Introduction to the special issue ‘Tracer Applications in Sediment Research’

Introduction to the special issue ‘Tracer Applications in Sediment Research’

Lead Pollution Remanence in an Urban River System: A multi-scale temporal and spatial study

This work aims at studying the fate of sediments contaminated with tetraethyl Pb from leaded gasoline using a two-dimension upscaling approach, from a small urban subcatchment, the Orge River (900 km 2 ) to the whole Seine River basin (64700 km 2 ), in France. In France, the leaded gasoline reduction started in 1986 and leaded gasoline was completely banned after 2000. This work aims at assessing whether the ban of leaded gasoline is related to changes in Pb contamination sources of these river suspended sediment particles (SPM) and bed sediment. Sediment cores and samples collected in the course of previous research projects of the Seine River contamination were used as temporal archives. The study of the isotopic lead ratio showed the fast decrease of the contamination of urban river suspended particulate matter due to the “gasoline” lead source from 2000 to 2011. This source mostly disappeared in the SPM from the Seine River basin that includes urban areas but also agricultural and industrial activities. Nevertheless, it is still present in the small urban catchment of the Orge River. The results on bed sediments showed a different pattern, where the “gasoline” source is still active in densely populated areas, either in the Seine River in the 20 km downstream Paris, or along the Orge River.

Infiltration of Martian outflow channel floodwaters into lowland cavernous systems

The hydrosphere of Mars has remained mostly concealed within the subsurface for the past ∼3.5 Gyr. Localized rupturing of the permafrost‐capped crust led to voluminous groundwater discharges that carved some of the largest known channels in the solar system. However, our knowledge of the nature of the flows and their ultimate fate remains incomplete, partly because diagnostic landforms at outflow channel termini have been largely destroyed or buried. The Hebrus Valles outflow channels were excavated by fluid discharges that emanated from two point sources, and they mostly terminate in systems of fractures and depressions within the northern plains. Our investigation indicates that outflow channel floodwaters were captured and reabsorbed into the subsurface in zones where caverns developed within the northern plains. These findings imply that the study region comprises the only known location in the Martian northern lowlands where the fate of outflow channel discharges can be assessed with confidence. We propose that evacuation of subsurface materials via mud volcanism was an important process in cavern formation. Our conceptual model provides a hypothesis to account for the fate of sediments and fluids from some of the Martian outflow channels. It also reveals a mechanism for lowland cavern formation and upper crustal volatile enrichment after the development of the Martian global cryosphere.

Transport‐limitations on fluvial sediment supply to the sea

The ability to understand and predict the flux and fate of sediment delivered to the sea by rivers remains an outstanding scientific challenge. Approaches to this challenge are necessarily synthetic, spanning wide ranges in spatial and temporal scales. Here a conventional sediment transport theory used by engineers and sedimentologists at reach and channel scales is applied at the basin scale. Specifically, a straightforward expression proposed by Bagnold and modified accordingly predicts the observed importance of combined wetness and steepness of a source basin as a control of sediment supply to the sea. The reasonable, key assumption underlying the application of sediment transport theory in this context is that the river‐mouth sites for which suspended‐sediment loads are reported are alluviated, and thus characterized by transport‐limited flux of sediment. This analysis also indicates the potential significance of additional, as yet poorly documented factors constraining sediment supply to the sea. These factors, some of which appear to covary systematically with climate, include river‐profile concavity, river‐mouth channel width and friction, and the characteristic size of sediment in transport.

Is the von Kármán constant affected by sediment suspension?

Is the von Kármán constant affected by sediment suspension? The presence of suspended sediment in channels and fluvial streams has been known for decades to affect turbulence transfer mechanism in sediment‐laden flows, and, therefore, the transport and fate of sediments that determine the bathymetry of natural water courses. This study explores the density stratification effects on the turbulent velocity profile and its impact on the transport of sediment. There is as yet no consensus in the scientific community on the effect of sediment suspension on the von Kármán parameter,κ. Two different theories based on the empirical log‐wake velocity profile are currently under debate: One supports a universal value ofκ = 0.41 and a strength of the wake, Π, that is affected by suspended sediment. The other suggests that both κ and Π could vary with suspended sediment. These different theories result in a conceptual problem regarding the effect of suspended sediment on κ, which has divided the research area. In this study, a new mixing length theory is proposed to describe theoretically the turbulent velocity profile. The analytical approach provides added insight defining κas a turbulent parameter which varies with the distance to the bed in sediment‐laden flows. The theory is compared with previous experimental data and simulations using ak‐εturbulence closure to the Reynolds averaged Navier Stokes equations model. The mixing length model indicates that the two contradictory theories incorporate the stratified flow effect into a different component of the log‐wake law. The results of this work show that the log‐wake fit with a reducedκ is the physically coherent approximation.

Dynamics of Particle Clouds in Ambient Currents with Application to Open-Water Sediment Disposal

Flow visualization experiments were performed in a glass-walled recirculating flume to observe the fate of sediments released instantaneously in a current. For releases at the surface, criteria were developed to characterize ambient currents as weak, transitional, or strong as a function of particle size. In weak ambient currents, particle clouds were advected downstream with a velocity equal to the ambient current, but otherwise their behavior and structure were similar to those in quiescent conditions. A substantial portion of the mass initially released, up to 30%, was not incorporated into the parent cloud and formed the trailing stem. This percentage was dependent on the initial release variables, with the greatest sensitivity on particle size. The loss of sediment during descent, defined as the fraction of mass missing a designated target with a radius equal to the water depth, was quantified and found to increase sharply with current speed. Laws of geometric, kinematic, and dynamic similitude provide a basis for scaling laboratory results to the real world and formulating guidelines to reduce the losses that could result from open-water sediment disposal. DOI: 10.1061/(ASCE)HY.1943-7900.0000659. © 2013 American Society of Civil Engineers. CE Database subject headings: Sediment; Particles; Thermal factors; Dredging; Currents. Author keywords: Sediment disposal; Particle cloud; Current; Thermal; Dredged material.

(Dis)Connectivity in catchment sediment cascades: a fresh look at the sediment delivery problem

ABSTRACTThe concept of the sediment delivery problem was introduced into the literature in 1983 by Des Walling. This concept describes how only a fraction of sediment eroded within a catchment will reach the basin outlet and be represented as sediment yield, and that sediment storage mechanisms operating within a catchment explain this discrepancy. Since this paper was published, geomorphologists have been examining in great detail the fate of sediment eroded from the landsurface, and the pathways and timeframes of sediment transport and storage in catchments. However, to fully understand the internal dynamics of sediment flux requires a ‘fresh look at the sediment delivery problem’. A framework is required that can incorporate the various processes involved in sediment movement from source areas through a basin to its outlet, and can take account of the spatial distribution of, and timeframes over which, these processes operate.This paper presents a conceptual framework for analysis of catchment (dis)connectivity that incorporates both spatial and temporal variability in the operation of the sediment cascade. This approach examines where blockages occur to disrupt these longitudinal, lateral and vertical linkages in catchments. Depending on the position of blockages (termed buffers, barriers and blankets), and their sediment residence time, various parts of a catchment may be actively contributing sediment to the sediment cascade and be switched on, or inactive and switched off. This paper discusses how such a framework can be used to model response times to disturbance and explain the manifestation of geomorphic change in catchments. The paper then highlights challenges geomorphologists face in applying such a framework to understand the internal dynamics of the catchment sediment cascades, and forecast how environmental change might affect the operation of sediment fluxes into the future. Copyright © 2012 John Wiley & Sons, Ltd.

Coherence of river and ocean conditions along the US West Coast during storms

The majority of water and sediment discharge from the small, mountainous watersheds of the US West Coast occurs during and immediately following winter storms. The physical conditions (waves, currents, and winds) within and acting upon the proximal coastal ocean during these winter storms strongly influence dispersal patterns. We examined this river–ocean temporal coherence for four coastal river–shelf systems of the US West Coast (Umpqua, Eel, Salinas, and Santa Clara) to evaluate whether specific ocean conditions occur during floods that may influence coastal dispersal of sediment. Eleven years of corresponding river discharge, wind, and wave data were obtained for each river–shelf system from USGS and NOAA historical records, and each record was evaluated for seasonal and event-based patterns. Because near-bed shear stresses due to waves influence sediment resuspension and transport, we used spectral wave data to compute and evaluate wave-generated bottom-orbital velocities. The highest values of wave energy and discharge for all four systems were consistently observed between October 15 and March 15, and there were strong latitudinal patterns observed in these data with lower discharge and wave energies in the southernmost systems. During floods we observed patterns of river–ocean coherence that differed from the overall seasonal patterns. For example, downwelling winds generally prevailed during floods in the northern two systems (Umpqua and Eel), whereas winds in the southern systems (Salinas and Santa Clara) were generally downwelling before peak discharge and upwelling after peak discharge. Winds not associated with floods were generally upwelling on all four river–shelf systems. Although there are seasonal variations in river–ocean coherence, waves generally led floods in the three northern systems, while they lagged floods in the Santa Clara. Combined, these observations suggest that there are consistent river–ocean coherence patterns along the US West Coast during winter storms and that these patterns vary substantially with latitude. These results should assist with future evaluations of flood plume formation and sediment fate along this coast.

Modeling reservoir sedimentation associated with an extreme flood and sediment flux in a mountainous granitoid catchment, Japan

Extreme events, such as large storms and floods, have a major effect on the transport of sediment and contaminants and, hence, on water quality. To be realistic, models designed to predict the short-term transport and fate of sediment and contaminants must include large floods and storms, an idea not incorporated into existing models based on uniform sediment flux. Sediment transport in and to river channels in mountainous terrain is strongly influenced by precipitation, particularly when heavy precipitation triggers a surface landslide in the catchment area. This study provides a quantitative measure of such sediment transport. The Yahagi Dam watershed was modeled using a 50-m grid-based digital elevation model (DEM), and flow directions were determined for each of the slopes present. The study objective was to develop a general algorithm for simulating water flow and sediment movement in a dammed mountain basin using water and sediment dynamics modeling. The nonuniform flow model used for stream channels can incorporate energy loss around dam reservoirs, and the resulting algorithm can estimate all phenomena related to sediment movement. The new method was verified by applying it to the Tokai rainfall disaster and the Yahagi Dam basin, Japan. In this basin, the volume of bedload sediment deposited is 993 × 10 3 m 3/y, suspended-load sediment is 669 × 10 3 m 3/y, and wash load sediment is 900 × 10 3 m 3/y, as determined from sediment production in each tributary of the Yahagi River. Most sediment is probably introduced during extreme flood events owing to lithological factors, and thus extreme rain events that now accompany climate change are very important in sediment supply. During extreme flood events, the river's effective tractive force ( τ* e, d90) exceeds the critical tractive force ( τ* c), especially upstream of the Yahagi Dam. Rainfall-related sediment disasters can be accurately predicted using water- and sediment-dynamics models that are founded on realistic geomorphological characteristics and sediment flux of rivers.

Incorporation of Subducted Slab-derived Sediment and Fluid in Arc Magmas: B-Be-10Be- Nd Systematics of the Kurile Convergent Margin, Russia

We present an investigation of B^Be^Be^eNd systematics of the incoming crust and across the wide, active Kurile arc in the NW Pacific ocean basin to address the role of recent sediment incorporation in arc magmas as a function of depth to the Wadati^Benioff zone. The Be flux ratio (8^14%) through the arc constrains the fate of sediments subducted at the trench and requires that a minimum !10 m of the sediment column must reach the depths of magma generation. Enrichments in subducted sediment-derived Be in rear-arc lavas are comparable with those in the volcanic front, despite longer subduction transit times, and require a mechanism for the prolonged release of Be from the subducting slab. Cross-arc Be enrichments, together with drastic reductions in B/Be, imply a protracted stability of their primary mineralogical host in subducted sediment, white mica (phengite).The persistence of phengite constrains slab surface temperatures to be 59508C to 165 km depth and limits the extent of partial melting of the slab to520%. The simplest interpretation of combined incoming sediment and cross-arc B/Be^Be/Be^eNd systematics is that the agent of element transfer changes from aqueous fluid-dominated beneath the volcanic front to melt-like beneath the deeper regions of the arc.

Fate of sediments delivered to the sea by Asian large rivers: Long-distance transport and formation of remote alongshore clinothems

Fate of sediments delivered to the sea by Asian large rivers: Long-distance transport and formation of remote alongshore clinothems

Characterising the origin, nature and fate of sediment exported from catchments perturbed by active tectonics

ABSTRACTChanges to the tectonic boundary conditions governing erosional dynamics in upland catchments have a significant effect on the nature and magnitude of sediment supply to neighbouring basins. While these links have been explored in detail by numerical models of landscape evolution, there has been relatively little work to quantify the timing, characteristics and locus of sediment release from upland catchments in response to changing tectonic boundary conditions that are well‐constrained independently. We address this challenge by quantifying the volume and granulometric characteristics of sediment exported from modern rivers draining across active normal faults in the Central Apennines in Italy. We demonstrate that catchments undergoing a transient response to tectonics are associated with significant volumetric export of material derived primarily from the zone upstream of the fault, producing bi‐modal grain‐size distributions with elevated D84 values within the transient reach. This is in direct contrast to the headwaters, where the fluvial capacity to transport sediment is low and the grain‐size distribution of material in transit is fine and uni‐modal. The grain‐size response is driven by landslides feeding coarse material directly into the channel, and we show the amplitude of the signal is modulated by the degree of tectonic perturbation, once the threshold for bedrock landsliding is exceeded. Additionally, we evaluate the length‐scale over which this transient grain‐size signal propagates downstream into the basin. We show that the coarse‐fraction sediment released is retained in the proximal hanging‐wall if rates of tectonic subsidence are high and if the axial river system is small or far from the fault‐bounded mountain front. Our results therefore provide some of the first quantitative data to evaluate how transient landscape responses affect the locus, magnitude and calibre of sediment supply to basins.

Storm-driven sediment transport in Massachusetts Bay

Massachusetts Bay is a semi-enclosed embayment in the western Gulf of Maine about 50 km wide and 100 km long. Bottom sediment resuspension is controlled predominately by storm-induced surface waves and transport by the tidal- and wind-driven circulation. Because the Bay is open to the northeast, winds from the northeast (‘Northeasters’) generate the largest surface waves and are thus the most effective in resuspending sediments. The three-dimensional oceanographic circulation model Regional Ocean Modeling System (ROMS) is used to explore the resuspension, transport, and deposition of sediment caused by Northeasters. The model transports multiple sediment classes and tracks the evolution of a multilevel sediment bed. The surficial sediment characteristics of the bed are coupled to one of several bottom-boundary layer modules that calculate enhanced bottom roughness due to wave–current interaction. The wave field is calculated from the model Simulating WAves Nearshore (SWAN). Two idealized simulations were carried out to explore the effects of Northeasters on the transport and fate of sediments. In one simulation, an initially spatially uniform bed of mixed sediments exposed to a series of Northeasters evolved to a pattern similar to the existing surficial sediment distribution. A second set of simulations explored sediment-transport pathways caused by storms with winds from the northeast quadrant by simulating release of sediment at selected locations. Storms with winds from the north cause transport southward along the western shore of Massachusetts Bay, while storms with winds from the east and southeast drive northerly nearshore flow. The simulations show that Northeasters can effectively transport sediments from Boston Harbor and the area offshore of the harbor to the southeast into Cape Cod Bay and offshore into Stellwagen Basin. This transport pattern is consistent with Boston Harbor as the source of silver found in the surficial sediments of Cape Cod Bay and Stellwagen Basin.

The source and fate of sediment and mercury in the Tapajós River, Pará, Brazilian Amazon: Ground- and space-based evidence

We present results of mercury (Hg) in surface waters and soils and an analysis of satellite imagery from the Tapajós River basin, Brazilian Amazon, and the Reserva Garimpeira do Tapajós, the legal gold mining district of the basin. Hg bound to suspended sediment was roughly 600 and 200 times the concentration of dissolved Hg per litre of water, in impacted and pristine areas, respectively. Suspended sediments thus represent the major pathway of river-borne Hg. Median concentrations of Hg in suspended load from both impacted and pristine waters were 134 ppb, and 80% of samples were below 300 ppb—in the range of naturally occurring surficial materials in the tropics. Regionally, riverine Hg fluxes were proportional to the concentration of total suspended solids. This shows that the dominant source of Hg is the sediment itself rather than anthropogenic mercury discharge from the small-scale mines. To independently test this conclusion, a mass balance was performed. A conservative calculation of the annual export of mercury (Hg) from the Creporí River (a minimum) was 1.6 tonnes for the year 1998—it could be significantly larger. This amount of Hg is difficult to account for by anthropogenic discharge alone, confirming that enhanced physical erosion caused by sluicing and dredging operations is the dominant source of Hg. We therefore conclude that gold mining operations are primarily responsible for elevated Hg concentrations. The dominant source of contamination is not, however, the loss of Hg in the gold amalgamation process. Rather, the disturbance and mobilization of large quantities of Hg-rich sediment and floodplain soil into the water column during mining operations is the source of contamination. These findings shift the focus of remediation and prevention efforts away from Hg control toward soil and sediment erosion control. The minimization or elimination of Hg losses in the mining process remains important for the health of local peoples and environments, but keeping basin soils and sediments in place would be a much more effective means of minimizing Hg fluxes to the region's rivers. To gain a spatial and historical perspective on the source and extent of emissions, satellite imagery was used. We were able to reconstruct historical mining activity, locate impacted areas, and estimate historical Hg fluxes with the imagery. To do so, the spectral characteristics of satellite images were calibrated to the concentration of suspended sediment in the rivers, which, in turn, is proportional to the Hg concentration. This analysis shows that mining-induced sediment plumes have been a dominant source of sediment to the Tapajós River system for decades. As well, the intensity and location of these emissions has varied through time. For example, sediment discharge from the Creporí River was greater in 1985 than in 1998; and the tributaries on the west bank of the Tapajós were actively being mined in 1985 but had been abandoned in 1998. This type of information should greatly assist in understanding original and ongoing sources of emissions, and in managing prevention and remediation efforts.

Predicting the fate of sediment and pollutants in river floodplains.

Geological processes such as erosion and sedimentation redistribute toxic pollutants introduced to the landscape by mining, agriculture, weapons development, and other human activities. A significant portion of these contaminants is insoluble, adsorbing to soils and sediments after being released. Geologists have long understood that much of this sediment is stored in river floodplains, which are increasingly recognized as important nonpoint sources of pollution in rivers. However, the fate of contaminated sediment has generally been analyzed using hydrodynamic models of in-channel processes, ignoring particle exchange with the floodplain. Here, we present a stochastic theory of sediment redistribution in alluvial valley floors that tracks particle-bound pollutants and explicitly considers sediment storage within floodplains. We use the theory to model the future redistribution and radioactive decay of 137Cs currently stored on sediment in floodplains at the Los Alamos National Laboratory (LANL) in New Mexico. Model results indicate that floodplain storage significantly reduces the rate of sediment delivery from upper Los Alamos Canyon, allowing 50% of the 137Cs currently residing in the valley floor to decay radioactively before leaving LANL. A sensitivity analysis shows that the rate of sediment overturn in the valley (and hence, the total amount of radioactive 137Cs predicted to leave LANL) is significantly controlled by the rate of sediment exchange with the floodplain. Our results emphasize that flood plain sedimentation and erosion processes can strongly influence the redistribution of anthropogenic pollutants in fluvial environments. We introduce a new theoretical framework for examining this interaction, which can provide a scientific basis for decision-making in a wide range of river basin management scenarios.

Aerobic co-metabolism of sulfur, nitrogen and oxygen heterocycles by three marine bacterial consortia.

Bacterial samples were collected from three marine beaches in coastal Newfoundland, Canada, and enriched by growth on 1-methylnaphthalene. The most prominent bacterial cell type for each consortium was isolated in a serial dilutions test, and a substrate utilization profile was obtained for each using the Biolog MicroStation System. Each bacterial community was tested for its ability to co-metabolize sulfur heterocycles (benzothiophene: BT, 3-methylbenzothiophene: 3-MBT, and dibenzothiphene: DBT), a nitrogen heterocycle (carbazole: CARB), and an oxygen heterocycle (dibenzofuran: DBF). Co-metabolism of the starting material was determined using gas chromatography-mass spectroscopy (GC-MS), and formation of products was investigated by GC-MS and Fourier transform infrared (FTIR) spectroscopy. Bacterial growth was monitored turbidimetrically to determine the dry weight (microgram) of cells/ml. The 2-ringed heterocycles were co-metabolized faster and to a greater extent than the 3-ringed compounds. Co-metabolism of BT was not statistically different from that for 3-MBT and, likewise, a comparison of the 3-ringed heterocycles showed no significant differences in degradation rates. Statistical examination showed that no one culture demonstrated a significantly greater ability to co-metabolize the heterocycles studied. This study represents the first comprehensive investigation of the ability of local bacteria to co-metabolize a range of aromatic compounds and provides a preliminary understanding of their fate in sediments should contamination by these compounds occur.

Reconsidering the Physics of the Chesapeake Bay Estuarine Turbidity Maximum

A series of cruises was carried out in the estuarine turbidity maximum (ETM) region of Chesapeake Bay in 1996 to examine physical and biological variability and dynamics. A large flood event in late January shifted the salinity structure of the upper Bay towards that of a salt wedge, but most of the massive sediment load delivered by the Susquehanna River appeared to bypass the ETM zone. In contrast, suspended sediments delivered during a flood event in late October were trapped very efficiently in the ETM. The difference in sediment trapping appeared to be due to increases in particle settling speed from January to October, suggesting that the fate of sediments delivered during large events may depend on the season in which they occur. The ETM roughly tracked the limit of salt (defined as the intersection of the 1 psu isohaline with the bottom) throughout the year, but it was often separated significantly from the limit of salt with the direction of separation unrelated to the phase of the tide. This was due to a lag of ETM sediment resuspension and transport behind rapid meteorologically induced or river flow induced motion of the salt limit. Examination of detailed time series of salt, suspended sediment, and velocity collected near the limit of salt, combined with other indications, led to the conclusion that the convergence of the estuarine circulation at the limit of salt is not the primary mechanism of particle trapping in the Chesapeake Bay ETM. This convergence and its associated salinity structure contribute to strong tidal asymmetries in sediment resuspension and transport that collect and maintain a resuspendable pool of rapidly settling particles near the salt limit. Without tidal resuspension and transport, the ETM would either not exist or be greatly weakened. In spite of this repeated resuspension, sedimentation is the ultimate fate of most terrigenous material delivered to the Chesapeake Bay ETM. Sedimentation rates in the ETM channel are at least an order of magnitude greater than on the adjacent shoals, probably due to focusing mechanisms that are poorly understood.

The role of soil erosion and fluvial processes in the post-fallout redistribution of Chernobyl-derived caesium-137: a case study of the Lapki catchment, Central Russia

The central area of the Russian Plain received substantial amounts Cs-137 fallout as a result of the Chernobyl accident in 1986, with inventories exceeding 40 kBq m −2 in many of the areas close to Chernobyl. Concern over the longer-term fate of this contamination has focused attention on the need to predict the post-fallout redistribution of the radiocaesium and, thus, future changes in the spatial distribution of contamination in the landscape. Since radiocaesium reaching the land surface as fallout is rapidly and strongly adsorbed by soil and sediment particles, any attempt to predict its post-fallout redistribution must focus on erosion and sediment delivery processes and must rely heavily on a knowledge of the geomorphological processes involved. This paper reports a detailed investigation of post-fallout Cs-137 redistribution in the 2.18-km 2 Lapki catchment in the Middle-Russian Upland, which has required consideration of soil erosion processes, sediment delivery pathways, sediment delivery ratios and sediment sinks. The time elapsed since the Chernobyl accident is currently insufficient to result in significant reduction of Cs-137 inventories in eroding areas, but areas of deposition on both the lower slopes and on the balka sides and bottoms are already marked by significant increases in Cs-137 inventories. The results obtained emphasise that any attempt to develop meaningful predictions of the longer-term redistribution of Chernobyl-derived Cs-137 fallout within the Russian Plain must be based on a sound and detailed understanding of the linkage between the slopes and the balka systems and the fate of sediment entering the balka systems.

Modern accumulation rates and a sediment budget for the Eel shelf: a flood-dominated depositional environment

The northern California continental margin is periodically impacted by geologically significant storms, which have a marked influence on terrigenous sediment supply, flood deposition, and long-term accumulation of fine-grained sediment on the Eel shelf. Accumulation of Eel River muds on the adjacent shelf was investigated using 210Pb and 137Cs geochronologies, in order to understand the fate of sediment discharged by the Eel River and to relate patterns of net sediment accumulation (100-yr time scale) to sediment dynamics. 210Pb data demonstrate that modern accumulation of river mud occurs from the 50-m isobath seaward. Across-shelf accumulation rates decrease from maximum mid-shelf values of 0.6–1.7 g cm −2 yr −1 to values of 0.2–0.4 g cm −2 yr −1 at the shelf break, with a spatially weighted mean of 0.5 g cm −2 yr −1 (0.4 cm/yr) for the entire shelf. 210Pb xs sediment-depth profiles from the region of highest accumulation rate are characterized by subsurface intervals of low and uniform activity, which are produced by flood deposition. In some cores, particular 210Pb xs activity intervals may be associated with major Eel River floods of 1955, 1964, and 1974. It is postulated that, because of the coincidence of high-river-flow events and southerly winds during cyclonic winter storms, net northward transport allows for preferential deposition of fine-grained sediment north of the river mouth. Over the past ∼100 years, fluvial sediment input combined with marine dispersal processes have produced a mid-shelf depocenter, evident by both the spatial distribution of 210Pb accumulation rates and by clay-rich flood layers partially preserved in shelf deposits. A fine-grained sediment budget for the dispersal system, based on hydrological data and 210Pb geochronologies, demonstrates that a maximum of ∼20% (3×10 9 kg/yr) of the mean annual supply of fluvial mud (14×10 9 kg/yr) is trapped on the shelf. The results of this study demonstrate that: (1) short-term sedimentation processes associated with floods can influence sediment accumulation on longer time scales; and (2) a major fraction of fine-grained sediment supplied to tectonically active margins by flood-prone mountainous rivers bypasses narrow continental shelves.