Faraday Rotation Research Articles

Orbital magnetism through inverse Faraday effect in metal clusters

Abstract In view of the recent increased interest in light-induced manipulation of magnetism in nanometric length scales this work presents metal clusters as promising elementary units for generating all-optical ultrafast magnetization. We perform a theoretical study of the opto-magnetic properties of metal clusters through ab-initio real-time (RT) simulations in real-space using time-dependent density functional theory (TDDFT). Through ab-initio calculations of plasmon excitation with circularly polarized laser pulse in atomically precise clusters of simple and noble metals, we discuss the generation of orbital magnetic moments due to the transfer of angular momentum from light field through optical absorption at resonance energies. Notably, in the near-field analysis we observe self-sustained circular motion of the induced electron density corroborating the presence of nanometric current loops which give rise to orbital magnetic moments due to the inverse Faraday effect (IFE) in the clusters. The results provide valuable insights into the quantum many-body effects that influence the IFE-mediated light-induced orbital magnetism in metal clusters depending on its geometry and chemical composition. At the same time, they explicitly demonstrate the possibility for harnessing magnetization in metal clusters, offering potential applications in the field of all-optical manipulation of magnetism.

Enhanced Faraday rotation via Kerr nonlinearity in graphene metasurface

Enhanced Faraday rotation via Kerr nonlinearity in graphene metasurface

Enhancing chiral molecule detection: A weak measurement approach utilizing two-dimensional information

This study addresses the critical need for high purity chiral molecules in biological systems by overcoming the challenges associated with the quantitative detection of chiral molecules and their enantiomeric mixtures. We developed an innovative detection approach that leverages the two-dimensional information gleaned from natural optical rotation (NOR) and Faraday optical rotation (FOR) under magnetic fields in chiral molecules, combined with an ultrahigh-resolution weak measurement sensor. This novel weak measurement system achieves unparalleled accuracy in detecting spin angles, with a precision of 1.86 × 10−5°. Notably, our method introduces no chemical reactions or interference with the substances under test. It offers enhanced discrimination capabilities through the dual-dimensional analysis of both natural and Faraday optical rotation, alongside a simple and compact sensor design. Conclusively, our study introduces a novel, high-precision, and multi-dimensional optical detection paradigm for chiral molecules. By incorporating Faraday rotation in the presence of a magnetic field, we expand the informational dimensionality accessible to the original weak measurement sensor, facilitating the quantitative analysis of chiral molecules and their enantiomers. This breakthrough not only furnishes a novel instrument for the exploration and development of chiral pharmaceuticals but also propels the advancement of weak measurement sensing technology forward.

Light-induced orbital magnetism in metals via inverse Faraday effect

We present a microscopic calculation of the inverse Faraday effect in metals. We derive a static local magnetic moment induced on the application of high-frequency light, using the Eilenberger formulation of quasiclassical theory. We include the effect of disorder and formulate a theory applicable across the entire temperature range, in the absence of external applied fields. For light-induced electric fields of amplitude ∼100kV/cm, the induced fields are large ∼0.1T for metallic Nb. The predictions of our theory agree with recent experimental and theoretical results [O. H.-C. Cheng , and J. Hurst , ]. An extension of this approach to superconductors would open a new route of inducing orbital magnetic field and potentially vortices in superconductors. Published by the American Physical Society 2024

Effect of gamma-radiation on the transmission and return losses of FC/APC connectors

The Fibre Optics Current Sensor (FOCS) installed at ITER will use optical fibres to perform plasma current measurements based on the Faraday effect. A connection between the sensing fibre placed on the Vacuum Vessel and the fibre guiding the signal to the data-acquisition hardware will be required. Because of practical reasons, this link contains FC/APC connectors, which guarantee the low return loss required for normal operation of the FOCS. The connectors will be located in the port cell area and will be subject to high levels of nuclear radiation. Radiation may influence both transmission and return losses of the FC/APC connectors and, as a result, degrade the FOCS performance. To address the problem, several FC/APC connectors were exposed to Co60 gamma radiation up to a 550 kGy dose. Transmission through the connectors was monitored during irradiation. The return loss of mated FC/APC connectors was measured before and after irradiation. It was found that radiation-induced changes of both transmission and reflection parameters are acceptable for the FOCS at ITER.

Magnon Supercurrent and the Phase Slippage in an Yttrium Iron Garnet Film

Exactly forty years ago, the spin superfluidity and Bose–Einstein condensation of magnons in superfluid antiferromagnetic 3He-B were discovered. In this work, the existence of spin superfluidity and phase slippage in an yttrium iron garnet film at room temperature is demonstrated using the optical Faraday effect. The s-patial distribution of the phase and amplitude of the spin precession under the conditions of magnon Bose‒Einstein condensation are studied by varying the pump phase difference between two strip lines exciting magnons.

Probing the magnetized gas distribution in galaxy groups and the cosmic web with POSSUM Faraday rotation measures

ABSTRACT We present initial results from the Polarization Sky Survey of the Universe’s Magnetism (POSSUM), analysing 22 817 Faraday rotation measures (RMs) with median uncertainties of 1.2 rad m$^{-2}$ across 1520 deg2 to study magnetized gas associated with 55 nearby galaxy groups ($z\lesssim 0.025$) with halo masses between $10^{12.5}$ and $10^{14.0}$ M$_\odot$. We identify two distinct gas phases: the intragroup medium (IGrM) within 0–2 splashback radii and the warm-hot intergalactic medium (WHIM) extending from 2 to 7 splashback radii. These phases enhance the standard deviation of residual (i.e. Galactic foreground RM-subtracted) RMs by $6.9\pm 1.8$ rad m$^{-2}$ and $4.2 \pm 1.2$ rad m$^{-2}$, respectively. Estimated magnetic field strengths are several μG within the IGrM and 0.1–1 μG in the WHIM. We estimate the plasma $\beta$ in both phases, and show that magnetic pressure might be more dynamically important than in the ICM of more massive clusters or sparse cosmic web filaments. Our findings indicate that ‘missing baryons’ in the WHIM likely extend beyond the gravitational radii of group-mass haloes to Mpc scales, consistent with large-scale, outflow-driven ‘magnetized bubbles’ seen in cosmological simulations. We demonstrate that RM grids are an effective method for detecting magnetized thermal gas at galaxy group interfaces and within the cosmic web. This approach complements X-ray and Sunyaev-Zel’dovich effect methods, and when combined with fast radio burst dispersion measures, data from the full POSSUM survey – comprising approximately a million RMs – will allow direct magnetic field measurements to further our understanding of baryon circulation in these environments and the magnetized universe.

Magnetometry for the Muon g-2 Experiment

The Muon g-2 Experiment at Fermilab aims to measure the muon anomalous magnetic moment with a precision of 140 parts per billion (ppb). The collaboration has published the latest measurement based on the first three Runs (collected from 2018 to 2020) in August 2023 with a precision of 200 ppb. The experiment accumulated three more years of data, from 2020 to 2023, which are currently being analyzed. This additional statistic is sufficient to achieve and possibly exceed the goal of 100 ppb of final statistical uncertainty. As the statistical error reduces, increasing attention is dedicated to studying systematic uncertainties. Among them, one source is a magnetic transient generated by the fast kickers. To center the muon orbit into its final position in the storage ring, three kickers emit a 120 ns magnetic pulse of ∼240 G, right after injection. This, however, induces eddy currents in the kicker aluminum structure that last for several microseconds. To measure the 10 mG magnetic perturbations generated by the eddy currents, the INFN team developed a laser magnetometer based on the Faraday effect. This article describes the technical principles, operations, and data analysis of this very sensitive device.

Photoinduced currents and inverse Faraday effect in graphene quantum dots

Photoinduced currents and inverse Faraday effect in graphene quantum dots

Optical Readout of Single-Molecule Magnets Magnetic Memories with Unpolarized Light.

Magnetic materials are widely used for many technologies in energy, health, transportation, computation, and data storage. For the latter, the readout of the magnetic state of a medium is crucial. Optical readout based on the magneto-optical Faraday effect was commercialized but soon abandoned because of the need for a complex circular polarization-sensitive readout. Combining chirality with magnetism can remove this obstacle, as chiral magnetic materials exhibit magneto-chiral dichroism, a differential absorption of unpolarized light dependent on their magnetic state. Molecular chemistry allows the rational introduction of chirality into single-molecule magnets (SMMs), ultimate nanoobjects capable of retaining magnetization. Here, we report the first experimental demonstration of optical detection of the magnetic state of an SMM using unpolarized light on a novel air-stable Dy-based chiral SMM featuring a strong single-ion magnetic anisotropy. These findings might represent a paradigm shift in the field of optical data readout technologies.

Global preventive feedback of powerful radio jets on galaxy formation

Firmly anchored on observational data, giant radio lobes from massive galaxies hosting supermassive black holes can exert a major negative feedback effect, by endowing the intergalactic gas with significant magnetic pressure hence retarding or preventing gas accretion onto less massive halos in the vicinity. Since massive galaxies that are largely responsible for producing the giant radio lobes, this effect is expected to be stronger in more overdense large-scale environments, such as protoclusters, than in underdense regions, such as voids. We show that by redshift [Formula: see text] halos with masses up to [Formula: see text] are significantly hindered from accreting gas due to this effect for radio bubble volume filling fraction of [Formula: see text], respectively. Since the vast majority of the stars in the universe at [Formula: see text][Formula: see text] 2 to 3 form precisely in those halos, this negative feedback process is likely one major culprit for causing the global downturn in star formation in the universe. It also provides a natural explanation for the rather sudden flattening of the slope of the galaxy rest-frame UV luminosity function around [Formula: see text]. A cross-correlation between protoclusters and Faraday rotation measures may test the predicted magnetic field. Inclusion of this external feedback process in the next generation of cosmological simulations may be imperative.

WITHDRAWN: Perfect asymmetric transmission for linear polarization in background reflection-free bilayer dielectric metasurfaces

In spite of the importance of asymmetric transmission (AT) with near-unity value and significantly high contrast of transmission, such a perfect AT has not yet been realized in reciprocal systems. For single resonance, it is already known that the upper limit of AT is identical to the background amplitude reflection coefficient. Nevertheless, if multiple resonances simultaneously contribute to AT, their coherent coupling enables us to obtain perfect AT, even when background reflection completely vanishes. Taking bilayer dielectric metasurfaces composed of orthogonal silicon nanorods embedded in silica glass as examples, here we show that perfect AT can be realized for linear polarization with characteristics comparable with bulky optical isolators based on Faraday effect: AT of 0.9994 with dramatically high contrast 35.1dB at telecom wavelength, the spectral position of which is tunable by properly changing the structural parameters. The analytical model based on the quasinormal-mode expansion well agrees with numerical results, revealing the concurrent contributions of multiple resonances. The presented perfect AT has the advantages of excellent performances of AT and compact structures without bulky devices for field bias or temporal modulations, enabling practical applications for optical computing, high-contrast polarization multiplexing and conversion.

Magneto‐optical effect of rare‐earth‐rich borate glasses prepared using a levitation technique

AbstractThe magneto‐optical properties of rare‐earth‐rich borate glasses prepared using a levitation technique were thoroughly investigated. Among the series of rare‐earth borate glasses, Tb2O3–B2O3 and Dy2O3–B2O3 glasses displayed remarkably large Faraday effects in the visible region. The Verdet constant of 58Tb2O3–42B2O3 reached −229 rad/T·m at 633 nm, surpassing the value of commercially available single‐crystalline Tb3Ga5O12. Compositions with a higher rare‐earth oxide content (60 mol%) than that of binary glasses facilitated the successful synthesis of Tb2O3–Dy2O3–B2O3 ternary glasses. The Verdet constant linearly increased with increasing Tb2O3 content for the glasses with 40 mol% B2O3. Results indicate that rare‐earth‐rich borate glasses are promising candidates for magneto‐optical applications in the visible region, and that the types and amounts of rare‐earth ion mainly affect these properties.

Magnetooptical Faraday and Kerr effects in nanosized BiYIG/GGG structures

AnnotationMagnetooptical Faraday and Kerr effects are studied in the nanosized BiY2Fe5O12 films within the spectral region of 1.3 eV<E<4.5 eV and magnetic fields of up to 10 kOe. It is shown that the thin-films BiY2Fe5O12 with the thicknesses ranging from 5 to 51 nm obtained by magnetron sputtering on the single-crystalline Gd3Ga5O12 substrates have high magneto-optical quality. The specific Faraday rotation for the nanosized Bi0.5Y1.5Fe5O12-δ films reaches about 140000 deg/cm close to that for bulk BiY2Fe5O12. Meanwhile, the polar Kerr effect reaches about 30 min within the range of 1.6 eV–4.1 eV at the magnetic fields above 2 kOe.It is shown that the strong paramagnetic contribution of Gd3Ga5O12 substrates significantly affects the Faraday and Kerr effect for the films. The defining of magnetooptical parameters and Verdet constant for the Gd3Ga5O12 substrate permitted to separate the substrate contribution and reveal peculiarities of spectral dependences of both Faraday and Kerr effects for magnetic films of various thicknesses. The estimated critical thickness of the film-substrate interface region is as large as 35 lattice constants of BiY2Fe5O12. It is shown that the magnetooptical effects for the thin films with the thickness above the critical one correspond to those for bulk BiY2Fe5O12. For samples with the smallest thicknesses of the film (5 nm) the contributions from magnetically dead and magnetically passive layers lead to a drastic reduction in the observable Faraday and Kerr effects with a dominating contribution from the substrate. The high density of displacement dislocations at the film-substrate interface leads to the decrease the magnetooptical quality of the nanosized films.

Magneto‐Optical Bi‐Substituted Yttrium and Terbium Iron Garnets for On‐Chip Crystallization via Microheaters

AbstractFerrimagnetic iron garnets enable magnetic and magneto‐optical functionality in silicon photonics and electronics. However, garnets require high‐temperature processing for crystallization which can degrade other devices on the wafer. Here bismuth‐substituted yttrium and terbium iron garnet (Bi‐YIG and Bi‐TbIG) films are demonstrated with good magneto‐optical performance and perpendicular magnetic anisotropy (PMA) crystallized by a microheater built on a Si chip or by rapid thermal annealing. The Bi‐TbIG film crystallizes on Si at 873 K without a seed layer and exhibits good magneto‐optical properties with Faraday rotation (FR) of −1700 deg cm−1. The Bi‐YIG film also crystallizes on Si and fused SiO2 at 873 K without a seed layer. Rapidly cooled films exhibit PMA due to the tensile stress caused by the thermal expansion mismatch with the substrates, increasing the magnetoelastic anisotropy by 4 kJ m−3 versus slow‐cooled films. Annealing in the air for 15 s using the microheater yields fully crystallized Bi‐TbIG on the Si chip.

A nebular origin for the persistent radio emission of fast radio bursts.

Fast radio bursts (FRBs) are millisecond-duration, bright (approximately Jy) extragalactic bursts, whose production mechanism is still unclear1. Recently, two repeating FRBs were found to have a physically associated persistent radio source of non-thermal origin2,3. These two FRBs have unusually large Faraday rotation measure values2,3, probably tracing a dense magneto-ionic medium, consistent with synchrotron radiation originating from a nebula surrounding the FRB source4-8. Recent theoretical arguments predict that, if the observed Faraday rotation measure mostly arises from the persistent radio source region, there should be a simple relation between the persistent radio source luminosity and the rotation measureitself7,9. Here we report the detection of a third, less luminous persistent radio source associated with the repeating FRB source FRB 20201124A at a distance of 413 Mpc, substantially expanding the predicted relation into the low luminosity-low Faraday rotation measure regime (<1,000 rad m-2). At lower values of the Faraday rotation measure, the expected radio luminosity falls below the limit-of-detection threshold for present-day radio telescopes. These findings support the idea that the persistent radio sources observed so far are generated by a nebula in the FRB environment and that FRBs with low Faraday rotation measure may not show a persistent radio source because of a weaker magneto-ionic medium. This is generally consistent with models invoking a young magnetar as the central engine of the FRB, in which the surrounding ionized nebula-or the interacting shock in a binary system-powers the persistent radio source.

Low Gilbert damping in Bi/In-doped YIG thin films with giant Faraday effect

Abstract Magnetic films with low Gilbert damping are crucial for magnonic devices, which provide a promising platform for realizing ultralow-energy devices. In this study, low Gilbert damping and coercive field were observed in Bi/In-doped yttrium iron garnet (BiIn:YIG) thin films. The BiIn:YIG (444) films were deposited onto different substrates using pulsed laser deposition. Low coercivity (&lt;1 Oe) with saturation magnetization of 125.09 emu/cc was achieved along the in-plane direction of BiIn:YIG film. The values of Gilbert damping and inhomogeneous broadening of ferromagnetic resonance in BiIn:YIG films were obtained to be as low as 4.05 × 10−4 and 5.62 Oe, respectively. In addition to low damping, the giant Faraday rotation angles (up to 2.9 × 104 deg/cm) were also observed in the BiIn:YIG film. By modifying the magnetic structure and coupling effect between Bi3+ and Fe3+ of Bi:YIG, doped In3+ plays a key role on variation of the magnetic properties. The low damping and giant Faraday effect made the BiIn:YIG film an appealing candidate for magnonic and magneto-optical devices.

Inverse Faraday effect in superconductors with potential impurities

Inverse Faraday effect in superconductors with potential impurities

Large Mid‐Infrared Magneto‐Optic Response from Doped Cadmium Oxide at Its Epsilon‐Near‐Zero Frequency

AbstractThe epsilon‐near‐zero (ENZ) frequency regime of transparent conducting oxide materials is known to yield large enhancements in their optical nonlinearity and electro‐optic response. Here, Faraday rotation is investigated in Gd and In‐doped CdO films and it is found that the Verdet constant peaks at values &gt;3 105 deg T−1 m−1 near the ENZ frequency, which is tunable in the wavelength range 2 &lt; λ&lt; 10 µm by varying the doping concentration. These results are among the highest reported to date in the mid‐infrared spectral range and are in good agreement with the Drude model, which confirms that the magneto‐optic response of doped CdO derives from its free carriers. The combination of a tunable Verdet constant, low optical loss compared to other plasmonic materials, and the ability to deposit CdO on Si with no loss in performance make this material a promising platform for integrated magneto‐optic and magnetoplasmonic devices that operate across the mid‐infrared.

Faraday effect of light caused by plane gravitational wave

A gravitational field can cause a rotation of the polarisation vector of light. This phenomenon is known as the gravitational Faraday effect. We study the gravitational Faraday effect of linearly polarised light propagating in the gravitational field of a weak plane gravitational wave (GW) with “+\\documentclass[12pt]{minimal} \\usepackage{amsmath} \\usepackage{wasysym} \\usepackage{amsfonts} \\usepackage{amssymb} \\usepackage{amsbsy} \\usepackage{mathrsfs} \\usepackage{upgreek} \\setlength{\\oddsidemargin}{-69pt} \\begin{document}$$+$$\\end{document}", “×\\documentclass[12pt]{minimal} \\usepackage{amsmath} \\usepackage{wasysym} \\usepackage{amsfonts} \\usepackage{amssymb} \\usepackage{amsbsy} \\usepackage{mathrsfs} \\usepackage{upgreek} \\setlength{\\oddsidemargin}{-69pt} \\begin{document}$$\ imes $$\\end{document}", and elliptical polarisation modes. The corresponding gravitational Faraday rotation angle is proportional to the GW amplitude and to the squared distance traveled by the light and inversely proportional to the GW squared wavelength. The Faraday rotation is maximal if the light propagates along directions perpendicular to the GW propagation and tilted by π/4\\documentclass[12pt]{minimal} \\usepackage{amsmath} \\usepackage{wasysym} \\usepackage{amsfonts} \\usepackage{amssymb} \\usepackage{amsbsy} \\usepackage{mathrsfs} \\usepackage{upgreek} \\setlength{\\oddsidemargin}{-69pt} \\begin{document}$$\\pi /4$$\\end{document} to the directions of its polarisation. There is no a gravitational Faraday rotation when light and a GW propagate along the same directions, or when light propagates along directions of a GW polarisation. Helicity of an elliptically polarised GW gives cubic order contribution to the Faraday rotation.