Deep underground projects are in a complex in-situ stress environment, and rock burst disasters induced by the hard and brittle failure of the rock mass are prone to occur around the tunnel openings. In this study, we aim to investigate the impacts of geological weak surfaces in rock masses on rockbursts and the spatiotemporal evolution of microcracks during the development of rockbursts. To achieve this objective, two sets of cubic specimens containing a circular through-hole were designed. One set of specimens had prefabricated unfilled cracks around the openings. Subsequently, the rockburst development process within the deep tunnel was replicated by subjecting both groups of specimens to identical gradient loading using a true triaxial test system. During the test, a micro camera was used to record the failure of the borehole wall in real-time, and an acoustic emission monitoring system was utilized to capture the stress waves released during structural damage. Finally, a multi-level synergistic analysis of the rockburst damage mechanism was carried out based on the macro-imaging data and micro-acoustic emission data. The results show that failure in high-stress environments within tunnels mainly includes microcrack initiation, particle ejection, crack propagation, local cracking, slabbing spalling, damage penetration, and rockburst damage. The time–frequency domain information of acoustic emission signals is highly perceptive and representative of the structural damage state of the specimens. The mutation characteristics observed in time-domain parameters, such as acoustic emission amplitude, event rate, ringing, and cumulative energy, correspond to drastic alterations in the internal structure of the rock. The distribution characteristics of frequency-domain parameters, such as acoustic emission peak frequency, dominant frequency energy, and frequency centroid, reflect different crack scales and damage modes. The diffusion of frequency centroid indicates that the damage and failure patterns within the rock are evolving towards a more complex direction. The energy magnitude of acoustic emissions represents the damage intensity during the development of rockburst. The root causes of induced structural-control type rockbursts in deep hard brittle rock masses are the combined effects of localized high-stress concentrations and large-scale discontinuous geological structures, such as natural joints, fissures, and structural planes. The naturally occurring large-scale through-type geological weak surfaces within the rock mass reduce the strength of the surrounding rock, alter the location of stress concentration, and change the initial damage characteristics. Moreover, they promote the evolution of rockbursts, thereby increasing their destructive intensity.