Experimental Knob Research Articles

Double loop dc-SQUID as a tunable Josephson diode

The development of superconducting electronics requires careful characterization of the components that makeup electronic circuits. Superconducting weak links are the building blocks of most superconducting electronic components and are characterized by highly nonlinear current-to-phase relations (CPRs), which are often not perfectly known. Recent research has found that the Josephson diode effect (JDE) can be related to the high harmonic content of the current-to-phase relation of the weak links embedded in superconducting interferometers. This makes the JDE a natural tool for exploring the harmonic content of weak links beyond single-harmonic CPR. In this study, we present the theoretical model and experimental characterization of a double-loop superconducting quantum interference device (DL-SQUID) that embeds all-metallic superconductor-normal metal-superconductor junctions. The proposed device exhibits the JDE due to the interference of the supercurrents of three weak links in parallel, and this feature can be adjusted through two magnetic fluxes, which act as experimental knobs. We carry out a theoretical study of the device in terms of the relative weight of the interferometer arms and the experimental characterization concerning flux tunability and temperature.

The quest for harnessing nuclear effects in graphene-based devices

The recent successes of superconducting qubits and the demonstration of quantum supremacy over classical bits herald a new era for information processing. Yet, the field is still in its infancy and there exist viable alternative candidates that can also store quantum information. In this review, we will highlight ideas, attempts, and the experimental progress to address nuclear spins in graphene, a readily available Dirac semimetal that consists of a single layer of carbon atoms. Carbon isotopes with a nuclear spin are rare in natural graphene. However, it is possible to enrich the spin-bearing 13C isotopes to produce large-scale graphene sheets, which constitute the testbed to store, transport, and retrieve spin information, or to engineer nanostructures. Here, the hyperfine interaction between the electron spins and the nuclear spins serves as an experimental control knob and mediator to address nuclear polarization and nuclear spin coherence times through electrical measurements. The exploitation of nuclear spins in graphene is thus an alluring perspective. We will discuss methods to synthesize 13C graphene and show experimental approaches and challenges to exploit the relatively weak hyperfine interaction in two-dimensional 13C graphene devices. The ultimate purpose, i.e., the exploitation of nuclear spins in graphene for information processing, is not within reach, but its potential for future applications merits a revisit of the current state-of-the-art.

Local dynamic responses of magnetic reconnection to three-dimensional perturbations in a laboratory plasma

The dynamic responses of magnetic reconnection to localized three-dimensional (3D) magnetic field perturbations imposed by a pair of figure-8-shaped coils are investigated in the Magnetic Reconnection Experiment (MRX) device. Both the magnetic field geometry and current sheet profiles are altered by external perturbations. For the case when the inductive electric field associated with these perturbations aligns with the preexisting reconnection electric field, O-type magnetic structures appear within an elongated current sheet. When these magnetic structures are ejected downstream at the speed close to the ion outflow velocity, the inductive electric field is enhanced considerably. Despite that the imposed perturbation amplitude is larger than 30% of the original reconnecting magnetic field, the overall reconnection process remains robust without current sheet disruptions. This technique to form O-type magnetic structures can serve as an additional experimental knob for future systematic laboratory investigations of 3D magnetic reconnection and related instabilities without disrupting two-dimensional current sheet.

Angle-resolved photoemission spectroscopy with an in situ tunable magnetic field.

Angle-resolved photoemission spectroscopy (ARPES) is a powerful tool for probing the momentum-resolved single-particle spectral function of materials. Historically, in situ magnetic fields have been carefully avoided as they are detrimental to the control of photoelectron trajectory during the photoelectron detection process. However, magnetic field is an important experimental knob for both probing and tuning symmetry-breaking phases and electronic topology in quantum materials. In this paper, we introduce an easily implementable method for realizing an in situ tunable magnetic field at the sample position in an ARPES experiment and analyze magnetic-field-induced artifacts in the ARPES data. Specifically, we identified and quantified three distinct extrinsic effects of a magnetic field: constant energy contour rotation, emission angle contraction, and momentum broadening. We examined these effects in three prototypical quantum materials, i.e., a topological insulator (Bi2Se3), an iron-based superconductor (LiFeAs), and a cuprate superconductor (Pb-Bi2Sr2CuO6+x), and demonstrate the feasibility of ARPES measurements in the presence of a controllable magnetic field. Our studies lay the foundation for the future development of the technique and interpretation of ARPES measurements of field-tunable quantum phases.

Zero-frequency supercurrent susceptibility signatures of trivial and topological zero-energy states in nanowire junctions

We propose a method to distinguish between trivial and topological, Majorana, zero-energy states (ZESs) in both short and long superconductor-normal-superconductor junctions based on Rashba nanowires using phase-biased equilibrium transport measurements. In particular, we show how the sawtooth profile of the supercurrent, due to the Majorana oscillation suppression in the topological phase for sufficiently long superconductor regions, leads to a strong signal in its zero-frequency susceptibility for a phase difference of . This signal is notably insensitive to the chemical potential in the normal region, while trivial ZESs only causes signals in the susceptibility that is highly varying with the chemical potential, thus turning gating of the normal region into a simple experimental control knob. Furthermore, we obtain that, by tuning the junction transparency, critical currents in both short and long junctions undergo a reduction in the number of oscillations as a function of magnetic field only in the topological phase, an effect that find to be intimately linked to Majorana non-locality. Finally, we show that our results also hold at finite temperatures, thus highlighting their potential measurability under realistic experimental conditions.

Thickness-dependent excitonic properties of WSe2/FePS3 van der Waals heterostructures.

van der Waals heterostructures (vdWHs), with their flexible combination of various two-dimensional (2D) materials, are continuously revealing new physics and functionalities. 2D magnetic materials have recently become a focus due to their fascinating electronic and spintronic properties. However, there has rarely been any investigation of the optical properties of 2D magnetic materials-based heterostructures. Herein, we construct a new WSe2/FePS3 heterostructure, in which WSe2 works as a "sensor" to visualize the thickness-dependent properties of FePS3. As characterized by photoluminescence (PL) spectra, whether under or on top of the FePS3, the PL intensity of the monolayer WSe2 is strongly quenched. The quenching effect becomes more obvious as the FePS3 thickness increases. This is because of the efficient charge transfer process occurring at the WSe2/FePS3 interface with type II band alignment, which is faster for thicker FePS3, as is evident from transient absorption measurements. The thickness-dependent charge transfer process and corresponding excitonic properties are further revealed in low-temperature photoluminescence spectra of WSe2/FePS3 heterostructures. Our results show that the thickness of 2D magnetic materials can work as an experimental tuning knob to manipulate the optical performance of conventional 2D semiconductors, endowing van der Waals heterostructures with more unexpected properties and functionalities.

Dissipative discrete time crystals in a pump-modulated Kerr microcavity

Time crystals represent temporal analogues of the spatial self-ordering exhibited by atomic or molecular building blocks of solid-state crystals. The pursuit of discrete time crystals (DTCs) in periodically forced Floquet closed systems has revealed how they can evade thermalization and loss of temporal order. Recently, it has been shown that even with coupling to the ambient and its concomitant noise, some states maintain their time crystalline order, forming dissipative DTCs. Here, we introduce a scheme for the realization and state control of dissipative DTCs hinging on pumping a Kerr optical resonator with a phase-modulated continuous-wave laser. We show the possible symmetry breaking states possess temporal long-range order and analyze the phase noise of the accompanying signature radio frequency (RF) subharmonic. Besides offering a technique for generating high-spectral-purity RF signals, this versatile platform empowers controlled switching between various DTC states through accessible experimental knobs, hence facilitating the future study of DTC phase transitions.

Higher Chern number states in curved periodic nanowires

The coupling between the spin and momentum degrees of freedom due to spin–orbit interactions (SOI) suggests that the strength of the latter can be modified by controlling the motion of the charge carriers. In this paper, we investigate how the effective SOI can be modulated by constraining the motion of charge carriers to curved waveguides thereby introducing real-space geometric curvature in their motion. The change in the SOI can in turn induce topological phase transitions in the system. Specifically, we study how the introduction of periodic sinusoidal curvature in nanowires with intrinsic SOC can induce the onset of mid-gap topologically protected edge states, which can be characterized by a topological invariant or Chern number. The Chern number corresponds to the number of discrete charges that would be pumped across the length of the nanowire when the phase of a sliding gate potential relative to that of the sinusoidal curvature is varied adiabatically over a complete period. In addition, coupling to an external magnetization can be utilized as an experimental knob to modify the Chern number by displacing the energies of the curvature-induced bands relative to one another. The magnetization can be tuned to achieve large discrete jumps in the number of pump charges per phase period.

Quantum non-Hermitian topological sensors

We investigate in the framework of quantum noise theory how the striking boundary sensitivity recently discovered in the context of non-Hermitian (NH) topological phases may be harnessed to devise novel quantum sensors. Specifically, we study a quantum-optical setting of coupled modes arranged in an array with broken ring geometry that would realize a NH topological phase in the classical limit. Using methods from quantum-information theory of Gaussian states, we show that a small coupling induced between the ends of the broken ring may be detected with a precision that increases exponentially in the number of coupled modes, e.g., by heterodyne detection of two output modes. While this robust effect only relies on reaching a NH topological regime, we identify a resonance phenomenon without direct classical counterpart that provides an experimental knob for drastically enhancing the aforementioned exponential growth. Our findings pave the way towards designing quantum NH topological sensors that may observe with high precision any physical observable that couples to the boundary conditions of the device.

Majorana braiding racetracks from charge Chern insulator–superconductor hybrids

Recent experiments have provided evidence for chiral charge order in Kagome superconductors (SCs). This intriguing possibility motivates us to unveil the first pathway to engineer topological superconductivity by harnessing the interplay of charge Chern insulators (CIs) and conventional SCs. We here identify under which conditions a pyramidal SC/CI/SC heterostructure induces an effective 1D spinless p-wave SC that allows pinning Majorana zero modes (MZMs) at termination edges and domain walls. As we reveal, such a MZM track is controlled by the phase difference of the two SCs involved and additional magnetic fields which are required for generating Rashba-like spin-orbit coupling. Further, we show that a SC/CI/SC/CI/SC double-pyramidal hybrid defines a double MZM track, in which braiding occurs by varying the two superconducting phase differences in space and adiabatically in time. Given the geometry of the MZM racetrack, we propose to employ the time-averaged quadrupolar differential conductance to confirm the here-termed MZM track exchange process which is pivotal for braiding. In addition, we identify experimental knobs which enable the fusion of MZM pairs, and the detection of the underlying non-Abelian topological order and twofold many-body ground state degeneracy by encoding it in a topological invariant.

Spin-orbit-driven ferromagnetism at half moiré filling in magic-angle twisted bilayer graphene.

Strong electron correlation and spin-orbit coupling (SOC) can have a profound influence on the electronic properties of materials. We examine their combined influence on a 2-dimensional electronic system at the atomic interface between magic-angle twisted bilayer graphene and a tungsten diselenide crystal. Strong electron correlation within the moiré flatband stabilizes correlated insulating states at both quarter and half filling, and SOC transforms these Mott-like insulators into ferromagnets, evidenced by robust anomalous Hall effect with hysteretic switching behavior. The coupling between spin and valley degrees of freedom is demonstrated through the control of the magnetic order with an in-plane magnetic field, or a perpendicular electric field. Our findings establish an experimental knob to engineer topological properties of moiré bands in twisted bilayer graphene and related systems.

Non-Hermitian higher-order Weyl semimetals

We study non-Hermitian higher-order Weyl semimetals (NHHOWSMs) possessing real spectra and having inversion $\mathcal{I}$ ($\mathcal{I}$-NHHOWSM) or time-reversal symmetry $\mathcal{T}$ ($\mathcal{T}$-NHHOWSM). When the reality of bulk spectra is lost, the NHHOWSMs exhibit various configurations of surface Fermi Arcs (FAs) and Exceptional Fermi Rings (EFRs), providing a setup to investigate them on an equal footing. The EFRs only appear in the region between 2nd-order WNs. We also discover Weyl nodes originating from non-Hermicity, called non-Hermitian Weyl nodes (NHWNs). Remarkably, we find T-NHHOWSMs which host only 2nd-order NHWNs, having both surface and hinge FAs protected by the quantized biorthogonal Chern number and quadrupole moment, respectively. We call this intrinsically non-Hermitian phase exceptional HOWSM. In contrast to ordinary WNs, the NHWNs can instantly deform to line nodes, forming a monopole comet. The NHWNs also show exceptional tilt-rigidity, which is a strong resistance towards titling due to attachment to exceptional structures. This phenomenon can be a promising experimental knob. Finally, we reveal the exceptional stability of FAs called exceptional helicity. Surface FAs having opposite chirality can live on the same surface without gapping out each other due to the complex nature of the spectrum. Our work motivates an immediate experimental realization of NHHOWSMs.

Facile Synthesis of Palladium-Based Nanocrystals with Different Crystal Phases and a Comparison of Their Catalytic Properties.

A relatively unexplored aspect of noble-metal nanomaterials is polymorphism, or their ability to crystallize in different crystal phases. Here, a method is reported for the facile synthesis of Ru@Pd core-shell nanocrystals featuring polymorphism, with the core made of hexagonally close-packed (hcp)-Ru while the Pd shell takes either an hcp or face-centered cubic (fcc) phase. The polymorphism shows a dependence on the shell thickness, with shells thinner than ≈1.4nm taking the hcp phase whereas the thicker ones revert to fcc. The injection rate provides an experimental knob for controlling the phase, with one-shot and drop-wise injection of the Pd precursor corresponding to fcc-Pd and hcp-Pd shells, respectively. When these nanocrystals are tested as catalysts toward formic acid oxidation, the Ru@Pdhcp nanocrystals outperform Ru@Pdfcc in terms of both specific activity and peak potential. Density functional theory calculations are also performed to elucidate the origin of this performance enhancement.

Atom-surface physics: A review

An atom in front of a surface is one of the simplest and fundamental problem in physics. Yet, it allows testing quantum electrodynamics, while providing potential platforms and interfaces for quantum technologies. Despite its simplicity, combined with strong scientific and technological interests, atom-surface physics, at its fundamental level, remains largely unexplored mainly because of challenges associated with precise control of the atom-surface distance. Nevertheless, substantial breakthroughs have been made over the last two decades. With the development of cold and quantum atomic gases, one has gained further control on atom-surface position, naturally leading to improved precision in the Casimir–Polder interaction measurement. Advances have also been reported in finding experimental knobs to tune and even reverse the Casimir–Polder interaction strength. So far, this has only been achieved for atoms in short-lived excited states, however, the rapid progresses in material sciences, e.g., metamaterials and topological materials has inspired new ideas for controlling the atom-surface interaction in long-lived states. In addition, combining nano-photonic and atom-surface physics is now envisioned for applications in quantum information processing. The first purpose of this Review is to give a general overview on the latest experimental developments in atom-surface physics. The second main objective is to sketch a vision of the future of the field, mainly inspired by the abundant theoretical works and proposals available now in the literature.

Planar graphene- NbSe2 Josephson junctions in a parallel magnetic field

Thin transition metal dichalcogenides sustain superconductivity at large in-plane magnetic fields due to Ising spin-orbit protection, which locks their spins in an out-of-plane orientation. Here we use thin NbSe$_2$ as superconducting electrodes laterally coupled to graphene, making a planar, all van der Waals two-dimensional Josephson junction (2DJJ). We map out the behavior of these novel devices with respect to temperature, gate voltage, and both out-of-plane and in-plane magnetic fields. Notably, the 2DJJs sustain supercurrent up to $H_\parallel$ as high as 8.5 T, where the Zeeman energy $E_Z$ rivals the Thouless energy $E_{Th}$, a regime hitherto inaccessible in graphene. As the parallel magnetic field $H_\parallel$ increases, the 2DJJ's critical current is suppressed and in a few cases undergoes suppression and recovery. We explore the behavior in $H_\parallel$ by considering theoretically two effects: a 0-$\pi$ transition induced by tuning of the Zeeman energy and the unique effect of ripples in an atomically thin layer which create a small spatially varying perpendicular component of the field. The 2DJJs have potential utility as flexible probes for two-dimensional superconductivity in a variety of materials and introduce high $H_\parallel$ as a newly accessible experimental knob.

Formation of transient high-β plasmas in a magnetized, weakly collisional regime

We present experimental data providing evidence for the formation of transient ( ${\sim }20\ \mathrm {\mu }\textrm {s}$ ) plasmas that are simultaneously weakly magnetized (i.e. Hall magnetization parameter $\omega \tau > 1$ ) and dominated by thermal pressure (i.e. ratio of thermal-to-magnetic pressure $\beta > 1$ ). Particle collisional mean free paths are an appreciable fraction of the overall system size. These plasmas are formed via the head-on merging of two plasmas launched by magnetized coaxial guns. The ratio $\lambda _{\textrm {gun}}=\mu _0 I_{\textrm {gun}}/\psi _{\textrm {gun}}$ of gun current $I_{\textrm {gun}}$ to applied magnetic flux $\psi _{\textrm {gun}}$ is an experimental knob for exploring the parameter space of $\beta$ and $\omega \tau$ . These experiments were conducted on the Big Red Ball at the Wisconsin Plasma Physics Laboratory. The transient formation of such plasmas can potentially open up new regimes for the laboratory study of weakly collisional, magnetized, high- $\beta$ plasma physics; processes relevant to astrophysical objects and phenomena; and novel magnetized plasma targets for magneto-inertial fusion.

Upping the pressure in bilayer graphene

Superconductivity The discovery of superconductivity and exotic insulating phases in twisted bilayer graphene has established this material as a model system of strongly correlated electrons. To achieve superconductivity, the two layers of graphene need to be at a very precise angle with respect to each other. Yankowitz et al. now show that another experimental knob, hydrostatic pressure, can be used to tune the phase diagram of twisted bilayer graphene (see the Perspective by Feldman). Applying pressure increased the coupling between the layers, which shifted the superconducting transition to higher angles and somewhat higher temperatures. Science , this issue p. [1059][1]; see also p. [1035][2] [1]: /lookup/doi/10.1126/science.aav1910 [2]: /lookup/doi/10.1126/science.aaw4642

Tuning superconductivity in twisted bilayer graphene.

Materials with flat electronic bands often exhibit exotic quantum phenomena owing to strong correlations. An isolated low-energy flat band can be induced in bilayer graphene by simply rotating the layers by 1.1°, resulting in the appearance of gate-tunable superconducting and correlated insulating phases. In this study, we demonstrate that in addition to the twist angle, the interlayer coupling can be varied to precisely tune these phases. We induce superconductivity at a twist angle larger than 1.1°-in which correlated phases are otherwise absent-by varying the interlayer spacing with hydrostatic pressure. Our low-disorder devices reveal details about the superconducting phase diagram and its relationship to the nearby insulator. Our results demonstrate twisted bilayer graphene to be a distinctively tunable platform for exploring correlated states.

Observation of entanglement sudden death and rebirth by controlling a solid-state spin bath

Quantum entanglement, the essential resource for quantum information processing, has rich dynamics under different environments. Probing different entanglement dynamics typically requires exquisite control of complicated system-environment coupling in real experimental systems. Here, by a simple control of the effective solid-state spin bath in a diamond sample, we observe rich entanglement dynamics, including the conventional asymptotic decay as well as the entanglement sudden death, a term coined for the phenomenon of complete disappearance of entanglement after a short finite time interval. Furthermore, we observe counter-intuitive entanglement rebirth after its sudden death in the same diamond sample by tuning an experimental parameter, demonstrating that we can conveniently control the non-Markovianity of the system-environment coupling through a natural experimental knob. Further tuning of this experimental knob can make the entanglement dynamics completely coherent under the same environmental coupling. Probing of entanglement dynamics, apart from its fundamental interest, may find applications in quantum information processing through control of the environmental coupling.

Tuning diamagnetism with current

Solid-State Physics Properties of materials can be tuned by various means, such as chemical doping, magnetic field, or pressure. Sow et al. used electrical currents of modest density to turn the Mott insulator Ca2RuO4 into a semimetal. Concurrently, its diamagnetic response—the ability to counter an externally applied magnetic field—rose to levels higher than in any other nonsuperconducting material. The use of electrical current as a powerful experimental knob may be applicable to other similar materials. Science , this issue p. [1084][1] [1]: /lookup/doi/10.1126/science.aah4297