Excitation Of Modes Research Articles

Can classical mechanics sense conical intersection?

Conical intersection (CI) leads to fast electronic energy transfer. However, Hamm and Stock [Phys. Rev. Lett. 109, 173201 (2012)] showed the existence of a vibrational CI and its role in vibrational energy relaxation. In this paper, we further investigate the vibrational energy relaxation using an isolated model Hamiltonian system of four vibrational modes with two distinctively different timescales (two fast modes and two slow modes). We show that the excitation of the slow modes plays a crucial role in the energy relaxation mechanism. We also analyze the system from a mixed quantum-classical (surface hopping method) and a completely classical point of view. Notably, surface hopping and even classical simulations also capture fast energy relaxation, which is a signature of CI's existence.

The role of density breaks in driving spiral structure in disc galaxies

ABSTRACT It is well established that stellar discs are destabilized by sharp features in their phase space, driving recurrent spiral modes. We explore the extent to which surface-density breaks in disc galaxies – which represent sharp changes in the gradient of the disc density – drive new spiral modes. We employ linear perturbation theory to investigate how disc breaks alter the eigenmode spectrum of an otherwise pure exponential disc. We find that the presence of a density break gives rise to a set of new, vigorously growing, modes. For a given multiplicity, these edge modes occur in pairs, with closely separated resonances between each pair. The growth rate of edge modes decreases when the break is weakened or moved outward to lower-density regions of the disc. Both down- and up-bending profiles excite edge modes, whose origin can be best understood via the gravitational torques they exert on the underlying disc. When the profile is down-bending (Type II) the faster growing mode is the inner one while in the up-bending (Type III) case the outer mode is faster growing. In both cases, the faster growing mode has a corotation almost coincident with the break. We show that the torques of the edge modes tend to smoothen the break.

A semi-analytical wavelet finite element method for wave propagation in rectangular rods

Prior knowledge of the dispersion curves and mode shapes of guided waves provides valuable information for wave mode selection and excitation in the field of non-destructive evaluation (NDE) and structural health monitoring (SHM). They are typically computed by the matrix methods, the finite element (FE) and semi-analytical finite element (SAFE) methods. However, the former is prone to numerical instability, and the latter two are limited by the refinement level of the FE mesh. In this paper, a semi-analytical wavelet finite element (SAWFE) method is presented to characterize wave propagation in rectangular rods. The piecewise polynomial interpolation functions of the SAFE method are replaced by two-dimensional scaling functions of the B-spline wavelet on the interval (BSWI). To demonstrate the accuracy of the proposed SAWFE technique, the propagation of guided waves in an aluminium plate is studied first. Then, the propagation of guided waves in rectangular rods of arbitrary aspect ratio is investigated. The results of this work clearly show that the SAWFE method presented here has higher accuracy and efficiency than the SAFE method.

Enhanced upconversion luminescence of NaYF4:Er nanocrystals based on the synergy between whispering gallery mode excitation and förster resonant energy transfer

The upconversion luminescence at the visible band was excited by the high power density whispering gallery mode (WGM) on the surface of the microsphere. Under the WGM excitation, Er3+ of NaYF4:Er3+ directly absorbed three photons at 1525 nm, followed by the generation of upconversion luminescence. We used WS2 quantum dots (QDs) as donors and NaYF4:Er3+ upconversion nanoparticles (UCNPs) as acceptors to enhance upconversion luminescence by Förster resonant energy transfer (FRET). The physical mixture composed of monolayer WS2 and NaYF4:Er3+ nanoparticles was coated on SiO2 microsphere by immersion method. Excited by high power density WGM, three photons were absorbed by WS2-QDs based on the quantum size effect to generate excited electrons as donors and UCNPs as acceptors based on FRET, subsequently, the energy of the electrons were transferred to the luminescence center Er3+ to improve the upconversion luminescence efficiency. The mechanism model of upconversion luminescence enhancement based on FRET of WS2–NaYF4:Er3+ was proposed, and the enhancement effect was experimentally studied and demonstrated. To study the distance dependence of energy transfer between QD and UCNP pairs, we covered the surface of the silica microsphere with a controlled concentration of WS2 mixed with NaYF4:Er3+ nano-particles. When the mixed concentration of WS2-QDs was 0.15%, the upconversion luminescence reached the highest efficiency. The results showed that a twofold upconversion luminescence enhancement can be experimentally achieved. The proposed approach for enhancing the upconversion luminescence could benefit the improvement of imaging signal-to-noise ratio (SNR) using UCNPs for fluorescent labels in life sciences.

Manipulating topological charge of nested skyrmion bags by microwave magnetic fields

Nested skyrmion bags, as magnetic solitons with arbitrary integer topological charges (Q), hold potential for applications in data encoding. A crucial issue is the local manipulation of skyrmions within nested skyrmion bags to control the total Q. In this study, we explore different possible ground states and resonant excitation spectra of nested skyrmion bags through micromagnetic simulations. More importantly, we demonstrate that the manipulation of the Q of nested skyrmion bags can be achieved by using microwave magnetic fields, i.e., the inner, middle, and outer skyrmions within the nested skyrmion bags are selectively excited by using the diverse out-of-plane excitation modes. By calculating the energy of skyrmions, we further analyze the relationship between the annihilation of skyrmions at different positions and the out-of-plane microwave magnetic fields. Our findings present a promising approach for manipulating the Q of nested skyrmion bags, potentially advancing their application in storage and logic devices.

A cyan-green-emitting garnet-structured Lu3-xScxAl2-yScyAl3-zSczO12: Ce3+ phosphor ceramics towards high-color-quality laser-driven lighting

For the laser-driven lighting, traditional phosphor ceramics (PCs), such as Y3Al5O12: Ce3+ (YAG: Ce) PC and Lu3Al5O12: Ce3+ (LuAG: Ce) PC, usually show a wide “cyan cavity” due to the ultra-narrow emission bandwidth (∼2 nm) of the blue laser diode (LD). In this regard, the attainable color rendering (Ra) is always <90 even via the combination of “YAG: Ce/LuAG: Ce + CaAlSiN3:Eu2+”. Evidently, the “cyan gap” is the bottleneck issue to attain high-color-quality laser-driven lighting. As such, we develop a novel cyan-green-emitting garnet-structured solid-solution Lu3-xScxAl2-yScyAl3-zSczO12: Ce3+ (abbreviated as LuScAG: Ce) PCs, derived from the LuAG: Ce PC. A comparative study is conducted to unearth its microstructure, luminescence properties and promising availability. It can be found that the LuScAG: Ce PCs shows large full width at half maximum (FWHM) and abundant cyan emission. Upon material optimization, bright cyan-green emission can be generated with internal quantum efficiency (IQE) of 87.4 % and FWHM of 87.17 nm. Remarkably, this new material yields high-power emitting light with luminous flux (LF) of 3230 lm and luminous efficacy (LE) of 89.7 lm/W upon 36.0 W blue LD driven in rotatory excitation mode, which can serve as an efficient laser color converter. As expected, due to the achieved affluent cyan emissive components of developed LuScAG: Ce PCs, the lighting source based on “LuScAG: Ce PC + CASN: Eu phosphor-in-glass film (PiGF)” shows high color quality with Ra of 90.6 and R12 (related with the cyan cavity) of 85.0.

Coverage extended MMF-based indoor OWC using overfilled launch and diversity reception

Speckle patterns generated as coherent optical beams are reflected by scattering elements. Multimode fibers (MMFs) can modify the transverse intensity distribution of speckle patterns with macro perturbations, i.e., pressures, providing a simple and low-cost way to achieve equivalent beam-steering for indoor optical wireless communications (OWCs) with divergent optical beams. However, the received optical power (ROP) variance severely limits the mobility of user terminals. In this paper, the issue is alleviated by using the overfilled launch of MMFs and the diversity gain of multi-receivers. By adjusting the axial spatial coupling distance between the MMF and the single mode fiber (SMF) emitting coherent laser, the number of excited modes of MMF can be significantly increased at 1550 nm with negligible coupling and bending losses. In addition, the signal-to-noise ratio (SNR) enhancement obtained by applying two receivers is theoretically analyzed for the case when either thermal noise or shot noise is dominant. The experimental results demonstrate that the proposed scheme can efficiently compensate for the ROP inhomogeneity, and at the same time it can extend the achievable full steering angle up to 12° at a 1.5-m free-space distance for bit error rate (BER) values of less than 3.8 × 10−3.

Tunable C4-Symmetry-Broken Metasurfaces Based on Phase Transition of Vanadium Dioxide (VO2).

Coupling is a ubiquitous phenomenon observed in various systems, which profoundly alters the original oscillation state of resonant systems and leads to the unique optical properties of metasurfaces. In this study, we introduce a terahertz (THz) tunable coupling metasurface characterized by a four-fold rotation (C4) symmetry-breaking structural array achieved through the incorporation of vanadium dioxide (VO2). This disruption of the C4 symmetry results in dynamically controlled electromagnetic interactions and couplings between excitation modes. The coupling between new resonant modes modifies the peak of electromagnetic-induced transparency (EIT) within the C4 symmetric metasurfaces, simulating the mutual interference process between modes. Additionally, breaking the C4 symmetry enhances the mirror asymmetry, and imparts distinct chiral properties in the far-field during the experimental process. This research demonstrates promising applications in diverse fields, including biological monitoring, light modulation, sensing, and nonlinear enhancement.

The quasi-classical trajectory study of vibrational mode-specific dynamics of the multi-channel reaction OH− + CH3F

The vibrational mode-specific dynamics of the multiple channel reaction, OH− + CH3F, namely the effects of excitations of the CF stretching (v1), CH3 rocking (v3), CH3 umbrella (v4), CH3 deformation (v5), CH symmetric stretching (v7) and CH asymmetric stretching (v8) as well as the OH stretching (vOH) on the reactivity of different product channels, were investigated by running extensive quasi-classical trajectories on a latest accurate full-dimensional potential energy surface. Integral cross sections (ICS), differential cross sections (DCS), product state populations, and product energy distributions for different vibrational excitation modes were calculated and analyzed. The Sudden Vector Projection model is also employed to rationalize these dynamic results.

Excitation of hybrid modes in plasmonic nanoantennas coupled with GeSiSn/Si multiple quantum wells for the photoresponse enhancement in the short-wave infrared range

Hybrid structures represented by a plasmonic nanoantenna array located on the surface of GeSiSn/Si multiple quantum wells (MQWs) grown on a silicon-on-insulator (SOI) substrate by molecular-beam epitaxy were developed for applications in the short-wave infrared range. Using numerical modeling methods, the electromagnetic characteristics of metasurfaces based on aluminum nanoantennas located on the surface of GeSiSn/Si nanoheterostructures were studied. It is shown that the spectral and spatial overlap of localized plasmons in nanoantennas and waveguide modes in the semiconductor film leads to the formation of hybrid modes with a Fano-type resonance profile. The possibility of significant photoluminescence (PL) enhancement of GeSiSn/Si MQWs through the use of hybrid plasmonic structures is demonstrated. The PL enhancement reached to 250 % at the wavelength of 1.9 μm, coinciding with the maximum of the reflectance spectrum for the hybrid structure. Based on the hybrid system, represented by the plasmonic nanoantenna array on the top part of GeSiSn/Si MQWs, p-i-n photodiodes were fabricated. The photocurrent enhancement was approximately 7 times at wavelengths of 1.73 µm and 1.8 µm. The excitation of separately localized plasmons and waveguide modes is demonstrated, and their hybridization is also studied.

Evaluation of array capacitive sensor for local concentration measurement of gas–solid particles flow by coupled fields based on CFD-DEM

An array capacitive sensor adopting two excitation modes is designed for measuring local particle concentration in gas–solid two-phase flow. Considering the difficulty in obtaining instantaneous flow parameters under dynamic experiments, a 3D dynamic simulation model coupling gas–solid two-phase fluid and electrostatic fields is proposed to quantitatively evaluate the sensor performance. In the coupling model, Computational Fluid Dynamics and Discrete Element Method are applied to establish two-phase fluid field for particle micro-distribution. The method of defining particle shape and position is used to set permittivity distribution in electrostatic field for coupling gas–solid fluid field and electrostatic field of array capacitive sensor. Using the method of reconstructed image and data fitting, the performance of two excitation modes are evaluated under a typical dynamic flow with structure of stratified flow. Experimental result validates the simulation conclusions and proves the effectiveness of the coupling simulation model for evaluating capacitive sensors in gas–solid flow systems.

Impact of Hybrid Electromagnetic Surface Modes on the Formation of Low Spatial Frequency LIPSS: A Universal Approach

AbstractIn this article, the impact of the excited electromagnetic surface modes in a comprehensive investigation of the formation of laser‐induced periodic surface structures (LIPSS) is analyzed. It is demonstrated that the electromagnetic origin of low spatial‐frequency LIPSS (LSFL) is the frequency detuning between propagating and localized modes due to their coupling/hybridization. The influence of the pattern profile, inhomogeneity, and material type on the coupling strength, electric‐field spatial distribution, and associated near‐field scattering are highlighted. Exploiting the potential of the approach, evidence of a universal manifestation of LSFLs is provided irrespective of the material and the authors are able to predict and validate the experimentally‐proven lower limit of LSFL periodicity (i.e., λL/2, where λL stands for the laser wavelength). Furthermore, the analysis of the electromagnetic modes predicts that the periodicity of LSFL is practically unaffected by the laser fluence, while a suppression of LSFL at high excitation levels or large number of pulses is also predicted. It is also shown that plasmonic‐active materials are not necessary for LSFL formation perpendicular to polarization. Toward these directions, an important generic metric, namely the resonance quality factor, is additionally inserted. The approach can, thus, serve as a guide for controlling laser‐induced surface topography.

Upconversion dual-photosensitizer-expressing bacteria for near-infrared monochromatically excitable synergistic phototherapy.

Synergistic phototherapy stands for superior treatment prospects than a single phototherapeutic modality. However, the combined photosensitizers often suffer from incompatible excitation mode, limited irradiation penetration depth, and lack of specificity. We describe the development of upconversion dual-photosensitizer-expressing bacteria (UDPB) for near-infrared monochromatically excitable combination phototherapy. UDPB are prepared by integrating genetic engineering and surface modification, in which bacteria are encoded to simultaneously express photothermal melanin and phototoxic KillerRed protein and the surface primary amino groups are derived to free thiols for biorthogonal conjugation of upconversion nanoparticles. UDPB exhibit a near-infrared monochromatic irradiation-mediated dual-activation characteristic as the photothermal conversion of melanin can be initiated directly, while the photodynamic effect of KillerRed can be stimulated indirectly by upconverted visible light emission. UDPB also show living features to colonize hypoxic lesion sites and inhibit pathogens via bacterial community competition. In two murine models of solid tumor and skin wound infection, UDPB separately induce robust antitumor response and a rapid wound healing effect.

Selective excitation of high-order modes in two-dimensional cavity resonator integrated grating filters.

The selective spatial mode excitation of a bi-dimensional grating-coupled micro-cavity called a cavity resonator integrated grating filter (CRIGF) is reported using an incident beam shaped to reproduce the theoretical emission profiles of the device in one and subsequently two dimensions. In both cases, the selective excitation of modes up to order 10 (per direction) is confirmed by responses exhibiting one (respectively two) spectrally narrowband resonance(s) with a good extinction of the other modes, the latter being shown to depend on the parity and order(s) of the involved modes. These results pave the way toward the demonstration of multi-wavelength spatially selective reflectors or fiber-to-waveguide couplers. Also, subject to an appropriate choice of the materials constituting the CRIGF, this work can be extended to obtain mode-selectable laser emission or nonlinear frequency conversion.

Coherent states of the Laguerre-Gauss modes.

Large quantum photonic systems hold promise for surpassing classical computational limits, yet their state preparation remains a challenge. We propose an alternative approach to study multiparticle dynamics by mapping the excitation mode of these systems to physical properties of the Laguerre-Gauss modes. We construct coherent states establishing a direct link between excitation number dynamics and the evolution of the Laguerre-Gauss modes. This highlights the photon transverse spatial degree of freedom as a versatile platform for testing the fundamental aspects of quantum multiparticle systems.

Measurement of the Excitation Spectrum of a Dipolar Gas in the Macrodroplet Regime.

The excitation spectrum of a cigar-shaped strongly dipolar quantum gas at the crossover from a Bose-Einstein condensate to a trapped macrodroplet is predicted to exhibit peculiar features-a strong upward shift of low momentum excitation energies together with a strong multiband response for high momenta. By performing Bragg spectroscopy over a wide range of momenta, we observe both key elements and also confirm the predicted stiffening of excitation modes when approaching the macrodroplet regime. Our measurements are in good agreement with numerical calculations taking into account finite size effects.

P -wave states Tbb− from diquarks

We investigate the P-wave states Tbb− in the isospin singlet and three excited modes [excitation occurring in the diquark [bb]c1s1 (ρ-mode), antidiquark [u¯d¯]c2s2 (r-mode), or between them (λ-mode)] from diquarks in a quark model. We analyze the dynamical behaviors of the diquark [bb]c1s1, antidiquark [u¯d¯]c2s2, and their correlations in the states Tbb− by decomposing the interactions from various sources in the model. The absolute dominant color-spin configuration, more than 99%, in the ρ-mode with 1P11 is [bb]3¯0[u¯d¯]30. Its energy is lower by about 18 MeV than the threshold B¯B¯ so that it can establish a compact bound state. The chromomagnetic and meson-exchange interactions in the antidiquark [u¯d¯]30 are responsible for its binding mechanism. Two other excited modes are higher than their respective threshold. The color configuration 6⊗6¯ need to be handled discreetly in the tetraquark states. Published by the American Physical Society 2024

Non-Abelian chiral soliton lattice in rotating QCD matter: Nambu-Goldstone and excited modes

The ground state of QCD with two flavors at a finite baryon chemical potential under rapid rotation is a chiral soliton lattice (CSL) of the η meson, consisting of a stack of sine-Gordon solitons carrying a baryon number, due to the anomalous coupling of the η meson to the rotation. In a large parameter region, the ground state becomes a non-Abelian CSL, in which due to the neutral pion condensation each η soliton decays into a pair of non-Abelian sine-Gordon solitons carrying S2 moduli originated from Nambu-Goldstone (NG) modes localized around it, corresponding to the spontaneously broken vector symmetry SU(2)V. There, the S2 modes of neighboring solitons are anti-aligned, and these modes should propagate in the transverse direction of the lattice due to the interaction between the S2 modes of neighboring solitons. In this paper, we calculate excitations including gapless NG modes and excited modes around non-Abelian and Abelian (η) CSLs, and find three gapless NG modes with linear dispersion relations (type-A NG modes): two isospinons (S2 modes) and a phonon corresponding to the spontaneously broken vector SU(2)V and translational symmetries around the non-Abelian CSL, respectively, and only a phonon for the Abelian CSL because of the recovering SU(2)V. We also find in the deconfined phase that the dispersion relation of the isospinons becomes of the Dirac type, i.e. linear even at large momentum.

Unravelling the excitation mechanism of very long-period (VLP) tremors in the Gulf of Guinea: evidence for vibrations of thin surface crustal plates

SUMMARY The Gulf of Guinea exhibits a continuous emission of narrow-band and long-period signals (16, 26 and 27 s) on teleseismic records, yet the underlying excitation mechanism remains unclear. This study establishes a connection between these tremors and the vibration of thin, decoupled crustal plates at unexplored volcanoes in the gulf. We first formulate the damped plate oscillation equation, by incorporating the vibration of the thin surface crustal plate and magma flow in the subsurface sill. The findings reveal that a fundamental-mode vibration with a period of several dozen seconds can be induced by a crustal plate that is less than 1.0 km thick but extends over tens of kilometres in both length and width, given a subsurface sill depth exceeding 10.0 cm. The thin plate hypothesis also allows for excitation of a few overtone modes, but such waves in higher frequencies diminish over long distances, leaving only the monotonous fundamental-mode vibration at teleseismic stations. The long duration of Guinea tremors at each recurrence is attributed to the presence of low viscosity basaltic magma, which influences the damping factor. Direct wave loads at the shallow gulf serve as the primary vibration source, accounting for seasonal variations and recurring patterns. Sporadic energy bursts may also occur due to large storms. Radiation patterns of Guinea tremors are linked to the geometric structure of the thin plate. Our theoretical estimates of tremor spectra closely align with observed data, confirming the model’s accuracy in capturing reported Guinea tremor characteristics. This study provides valuable insights into the origins of very long-period tremors at continental volcanoes.

A Small-Signal Stability Analysis Method Based on Minimum Characteristic Locus and Its Application in Controller Parameter Tuning

A small-signal stability analysis method based on minimum characteristic locus (MCL) was recently proposed by the authors. The method is found to be particularly useful in analyzing various oscillation modes in a unified way. The present work continues this line of research. After providing a brief review of the basic principle of MCL method, the paper proceeds to show the mathematical relationship between the stability margin obtained using an MCL method, and that obtained by traditional modal analysis method. Next, a sensitivity analysis procedure is proposed to study quantitatively the effects of control parameters on the stability of the system. Third, the properties of the so-called exciter mode are explained in detail, in particular, explicit formulas of exciter mode frequency and power system stabilizer (PSS) critical gain are derived. Finally, taking PSS4B as an example, a controller parameter tuning method is proposed. The effectiveness and practicability of the proposed method are verified by case studies of Kundur's four-machine-two-area system and China's Yunnan power grid.