Bentonite has been considered as a candidate buffer material for the disposal of high-level radioactive waste (HLW) because of its low permeability, high sorption capacity, self-sealing characteristics and durability in a natural environment. Bentonite erosion caused by groundwater flow may take place at the interface of the compacted bentonite and fractured granite. Surface erosion of bentonite flocs is represented typically as an erosion threshold. Predicting the erosion threshold of bentonite flocs requires taking into account cohesion, which results from interactions between clay particles. Beyond the usual dependence on grain size, a significant correlation between erosion threshold and porosity measurements is confirmed for bentonite flocs. A fractal model for erosion threshold of bentonite flocs is proposed. Cohesion forces, the long-range van der Waals interaction between two clay particles are taken as the resource of the erosion threshold. The model verification is conducted by the comparison with experiments published in the literature. The results show that the proposed model for erosion threshold is in good agreement with the experimental data.