Restoring vegetation is an effective way to control regional erosion as well as reduce soil erodibility. However, it is not clear how the vegetation restoration duration affects soil erodibility and how it further influences soil erosion processes. Therefore, the soil physicochemical properties and comprehensive soil erodibility index (CSEI) at five sampling sites with 3, 20, 55, 80 and 100 years of vegetation restoration were investigated in this study. A simulated rainfall with intensities of 60, 90, and 120 mm h−1 was conducted on three slopes with gradients of 10°, 20°, and 30° by using rare earth element oxides (Ho2O3 and Sm2O3) as tracers to quantify interrill and rill erosion. The results revealed a decreasing trend in both the CSEI and sediment concentration with increasing vegetation restoration duration. Compared to that at the site with 3 years of vegetation restoration, the CSEI at the sites with 20, 55, 80, and 100 years of restoration was reduced by 35.2 %, 39.7 %, 92.8 %, and 67.1 %, respectively. Interrill erosion dominated the hillslope erosion processes and contributed more than 76.9 % to the total erosion amount. By comparing the measured and estimated erosion rates using the equations provided by the Water Erosion Prediction Project (WEPP), significant prediction errors were found. Therefore, relationships among the CSEI, slope gradient and rainfall intensity were established for interrill and rill erosion rate estimation in vegetation restoration areas. This study provides a theoretical basis for evaluating the soil and water conservation benefits of vegetation restoration and for improving soil erosion prediction models within the context of vegetation restoration.