Enhancement Of Light-matter Interaction Research Articles

Electrically Tunable and Robust Bound States in the Continuum Enabled by 2D Transition Metal Dichalcogenide

AbstractHigh quality factor (Q‐factor) resonance can effectively enhance light–matter interactions, but suffers from radiative losses caused by fabrication imperfections and material impurities. Merging bound states in the continuum (BICs) becomes a promising candidate to address this challenge since they generate a large high‐Q region in momentum space against undesired external perturbations. However, it is only achieved by altering the geometric parameters of the structure, which constrains its dynamical tunability once the fabrication is ready, limiting its performance in modulators and photodetectors. Here, a convenient approach is proposed to manipulating the merging BIC by electrically tuning the material properties, aiming at on‐chip photonic devices. The asymmetric merging BIC is achieved and tuned by reducing the in‐plane structural symmetry from to , which enables the inversion of topological charge and reconfigurable polarization distribution in the momentum space. Such tunable merging BIC promises various potential applications including vortex generation, optical communication, and nanolasers.

Enhanced Light–Tellurium Interaction through Evanescent Wave Coupling for High Speed Mid‐Infrared Photodetection

AbstractMid‐infrared (MIR) waveguide‐integrated photodetector is essential for various applications in the fields of sensing and optical communications. However, it is challenging to integrate traditional MIR photoactive materials such as HgCdTe or III−V compounds with complementary metal‐oxide‐semiconductor (CMOS)‐compatible silicon platform due to the lattice mismatch. Tellurium (Te), a novel van der Waals (vdW) material with a narrow bandgap, high carrier mobility, and great air stability, is a promising candidate for high‐performance MIR detection. Here, high‐quality Te nanosheets are synthesized using a hydrothermal method and their carrier dynamics are characterized by transient reflection spectrum. The effect of mobility anisotropy on response speed is investigated intuitively by a free space phototransistor. Combining the strong evanescent wave of a waveguide architecture with the synergy effect between the carrier collection path and the highest mobility crystal orientation in Te, an integrated Te photodetector with enhanced light–matter interaction and reduced carrier transit time is achieved. For the first time, the MIR waveguide‐integrated Te photodetector with a responsivity of 2.3 A W−1 and a bandwidth of 4 GHz at 2015 nm is realized, which is the highest speed MIR photodetector based on narrow bandgap vdW materials to date.

Exciton resonances for atomically-thin optics

Metasurfaces enable flat optical elements by leveraging optical resonances in metallic or dielectric nanoparticles to obtain accurate control over the amplitude and phase of the scattered light. While highly efficient, these resonances are static and difficult to tune actively. Exciton resonances in atomically thin 2D semiconductors provide a novel and uniquely strong resonant light–matter interaction, which presents a new opportunity for optical metasurfaces. Their resonant properties are intrinsic to the band structure of the material, do not rely on nanoscale patterns, and are highly tunable using external stimuli. In this tutorial, we present the role that exciton resonances can play for atomically thin optics. We describe the essentials of metasurface physics and provide background on exciton physics and a comprehensive overview of excitonic materials. Excitons demonstrate to provide new degrees of freedom and enhanced light–matter interactions in hybrid metasurfaces through coupling with metallic and dielectric metasurfaces. Using the high sensitivity of excitons to the medium's electron density, the first demonstrations of electrically tunable nanophotonic devices and atomically thin optical elements are also discussed. The future of excitons in metasurfaces looks promising, while the main challenge lies in large-area growth and precise integration of high-quality materials.

Optical pulling and pushing forces via Bloch surface waves

For flexible tailoring of optical forces, as well as for extraordinary optomechanical effects, additional degrees of freedom should be introduced into a system. Here, we demonstrate that photonic crystals are a versatile platform for optical manipulation due to both Bloch surface waves (BSWs) and the complex character of the reflection coefficient paving a way for controlled optomechanical interactions. We demonstrate enhanced pulling and pushing transversal optical forces acting on a single dipolar bead above a one-dimensional photonic crystal due to directional excitation of BSWs. Our results demonstrate angle- or wavelength-assisted switching between BSW-induced optical pulling and pushing forces. Easy to fabricate for any desired spectral range, photonic crystals are shown to be prospective for precise optical sorting of nanoparticles, which are difficult to sort with conventional optomechanical methods. Our approach opens opportunities for novel, to the best of our knowledge, optical manipulation schemes and platforms, and enhanced light-matter interaction in optical trapping setups.

Moiré-driven electromagnetic responses and magic angles in a sandwiched hyperbolic metasurface

Recent moiré configurations provide a new platform for tunable and sensitive photonic responses, as their enhanced light–matter interactions originate from the relative displacement or rotation angle in a stacking bilayer or multilayer periodic array. However, previous findings are mostly focused on atomically thin condensed matter, with limitations on the fabrication of multilayer structures and the control of rotation angles. Structured microwave moiré configurations are still difficult to realize. Here, we design a novel moiré structure, which presents unprecedented capability in the manipulation of light–matter interactions. Based on the effective medium theory and S -parameter retrieval process, the rotation matrix is introduced into the dispersion relation to analyze the underlying physical mechanism, where the permittivity tensor transforms from a diagonal matrix to a fully populated one, whereas the permeability tensor evolves from a unit matrix to a diagonal one and finally becomes fully filled, so that the electromagnetic responses change drastically as a result of stacking and rotation. Besides, the experiment and simulation results reveal hybridization of eigenmodes, drastic manipulation of surface states, and magic angle properties by controlling the mutual rotation angles between two isolated layers. Here, not only a more precisely controllable bilayer hyperbolic metasurface is introduced to moiré physics, the findings also open up a new avenue to realize flat bands at arbitrary frequencies, which shows great potential in active engineering of surface waves and designing multifunctional plasmonic devices.

Active absorption modulation by employing strong coupling between magnetic plasmons and borophene surface plasmons in the telecommunication band

The tunable and highly confined plasmon in 2D materials paves the way for designing 2D materials capable of manipulating light on a subwavelength scale, making them suitable for the design of optical modulators in ultracompact sizes. Herein, a continuously adjustable modulator in the telecommunication band is theoretically presented by the strong coupling between the magnetic plasmons (MPs) and borophene surface plasmons (BSPs). A remarkable Rabi splitting is observed and the coupling process is theoretically investigated by the model of two coupled oscillators. Results show that the splitting energy is determined by the coupling strength, which can be modulated by adjusting the distance between the borophene monolayer and silver grating. Moreover, by manipulating the electron density of the borophene to drive both two modes coupled or decoupled, the absorption can be continuously adjustable almost from 0 to 1 at 1544 nm, and the maximum modulation depth can be up to 94.8%. This work may provide a method to enhance light–matter interactions by the coupled multi-modes and design borophene-based plasmonic modulator.

Plasmonic Nanoparticles Embedded in Nanomembrane Microcavity for Flexible Optical Tuning

AbstractThe combination of plasmonic nanoparticles and optical microcavities has attracted broad interest for both fundamental and applied studies. However, the conventional scheme of plasmonic nanoparticles being located at microcavity outer surfaces suffers from serious problems such as significant radiative/scattering losses and chemical/mechanical instabilities. Here, silver nanoparticles (NPs) and dispersed ions embedded in nanomembrane‐formed whispering‐gallery‐mode (WGM) microtube cavities are prepared by ion implantations as compact and stable optoplasmonic microcavities. Upon low ion fluence implantation, dispersed silver ions are generated in the tube cavity wall, leading to a redshift of the WGM resonant cavity modes due to the increased refractive index. The silver ions start to aggregate into plasmonic NPs in the cavity wall when increasing implantation ion fluences. The competition and transition between redshift induced by the refractive index increase and blueshift induced by the formation of plasmonic NPs are investigated. Moreover, quality factor enhancement of the WGM modes is observed owing to the improved light confinement caused by the presence of NPs. This work demonstrates a convenient approach for the fabrication of stable optoplasmonic microcavities and fine tuning of resonant modes, indicating wide applications such as wavelength selective tuning and enhanced light–matter interactions.

Strong Coupling of Tamm Plasmons and Fabry-Perot Modes in a One-Dimensional Photonic Crystal Heterostructure

The coupling between multiple modes in subwavelength scale has attracted a lot of attention due to the interesting physics favored by the enhancement of light-matter interaction. In this contribution, we propose a planar hybrid plasmonic-photonic crystal structure, which enables the tunable coupling between Tamm plasmon-polariton and Fabry-Perot cavity modes. Then, a strong coupling can be achieved through evoking the Tamm-mode dependence of the top-layer thickness of the hybrid structure, which is indicated by an anticrossing with a spectrum splitting of 9.298 meV. The effect enables the spatial confinement of polaritons and the formation of hybrid one-dimensional plasmon-polariton modes. In order to account for the splitting of the orthogonally polarized resonances, a detailed investigation on the TE-TM splitting is also performed through the angular-dependence analysis. We note that the value of the TE-TM splitting strongly depends on the thicknesses of dielectric layer and the distance between two distributed Bragg reflector (DBR) stacks. We show that the cavity modes are extremely sensitive to the distance between the DBR stacks and propose using this feature for strain sensing. Thus, our structure may not only offer a platform for study of interesting physics (e.g., spin optronics), but may also provide a route for high-accuracy strain sensors.

Unidirectional bound states in the continuum in Weyl semimetal nanostructures

Recently studied bound states in the continuum (BICs) enable perfect localization of light and enhance light–matter interactions although systems are optically open. They have found applications in numerous areas, including optical nonlinearity, light emitters, and nano-sensors. However, their unidirectional nature in nonreciprocal devices is still elusive because such trapping states are easily destroyed when the symmetry of an optical system is broken. Herein, we propose nonreciprocal and dynamically tunable BICs for unidirectional confinement of light and symmetry-protected BICs at Γ -point by introducing antiparallel magnetism into the optical system. We demonstrate that such BICs can be achieved by using topological magnetic Weyl semimetals near zero-index frequency without any structural asymmetry, and are largely tunable via modifying the Fermi level. Our results reveal a regime of extreme light manipulation and interaction with emerging quantum materials for various practical applications.

Edge states in plasmonic meta-arrays

Abstract Photonic edge states provide a novel platform to control and enhance light–matter interactions. Recently, it becomes increasing popular to generate such localized states using the bulk-edge correspondence of topological photonic crystals. While the topological approach is elegant, the design and fabrication of these complex photonic topological crystals is tedious. Here, we report a simple and effective strategy to construct and steer photonic edge state in a plasmonic meta-array, which just requires a small number of plasmonic nanoparticles to form a simple lattice. To demonstrate the idea, different lattice configurations, including square, triangular, and honeycomb lattices of meta-arrays, are fabricated and measured by using an ultrahigh spatial resolution photoemission electron microscopy. The properties of edge states depend on the geometric details such as the row and column number of the lattice, as well as the gap distance between the particles. Moreover, numerical simulations show that the excited edge states can be used for the generation of the quantum entanglement. This work not only provides a new platform for the study of nanoscale photonic devices, but also open a new way for the fundamental study of nanophotonics based on edge states.

Guided-mode resonance with reduced bandwidth in mid-infrared absorption and thermal emission.

Narrowband resonance plays an important role in many optical applications, especially for the development of wavelength-selective properties and enhanced light-matter interaction. In this paper, we demonstrate metal-insulator-metal (MIM) waveguide gratings, which exhibit guided-mode resonance (GMR) with reduced bandwidth in mid-infrared absorption and thermal emission. Our fabricated MIM waveguide grating consists of a copper substrate, a lossless ZnSe film, and a top gold stripe grating. Our measurements reveal strong GMRs with a bandwidth of 1.29% of the central wavelength in both mid-infrared absorption and thermal emission spectra. By varying structural parameters of the MIM waveguide grating, strong absorptions and thermal emissions of GMRs are observed and tuned within the 3-5 µm wavelength range. These results manifest the great potential of engineering infrared properties by using GMR and could be useful for spectral control in a variety of infrared devices.

Ultra-slow light with high normalized delay–bandwidth product and refractive-index sensing in photonic crystal coupled-cavity waveguide

Ultra-slow light can enhance light–matter interactions and effectively realize all-optical buffering and modulation. In this paper, we present an efficient design for a two-dimensional square-lattice photonic crystal coupled-cavity waveguide, which can realize multi-frequency band slow-light transmission in the near-infrared band (1500–1640 nm).Through adjusting intercavity spacing N and structural parameters of elliptical air holes, high group index ng (202.46) within the bandwidth of 5.04 nm and improved normalized delay–bandwidth​ product of 0.6583 can be obtained at the wavelength of 1550.05 nm. Moreover, the designed devices can effectively function as a slow light sensor with the wavelength sensitivity of 585 nm/RIU. Multiple functions can be achieved synchronously in only one structure, which is essential in complex optical integrated circuits.

Opportunities and Challenges for Alternative Nanoplasmonic Metals: Magnesium and Beyond.

Materials that sustain localized surface plasmon resonances have a broad technology potential as attractive platforms for surface-enhanced spectroscopies, chemical and biological sensing, light-driven catalysis, hyperthermal cancer therapy, waveguides, and so on. Most plasmonic nanoparticles studied to date are composed of either Ag or Au, for which a vast array of synthetic approaches are available, leading to controllable size and shape. However, recently, alternative materials capable of generating plasmonically enhanced light–matter interactions have gained prominence, notably Cu, Al, In, and Mg. In this Perspective, we give an overview of the attributes of plasmonic nanostructures that lead to their potential use and how their performance is dictated by the choice of plasmonic material, emphasizing the similarities and differences between traditional and emerging plasmonic compositions. First, we discuss the materials limitation encapsulated by the dielectric function. Then, we evaluate how size and shape maneuver localized surface plasmon resonance (LSPR) energy and field distribution and address how this impacts applications. Next, biocompatibility, reactivity, and cost, all key differences underlying the potential of non-noble metals, are highlighted. We find that metals beyond Ag and Au are of competitive plasmonic quality. We argue that by thinking outside of the box, i.e., by looking at nonconventional materials such as Mg, one can broaden the frequency range and, more importantly, combine the plasmonic response with other properties essential for the implementation of plasmonic technologies.

Optical Metasurfaces for Energy Conversion.

Nanostructured surfaces with designed optical functionalities, such as metasurfaces, allow efficient harvesting of light at the nanoscale, enhancing light–matter interactions for a wide variety of material combinations. Exploiting light-driven matter excitations in these artificial materials opens up a new dimension in the conversion and management of energy at the nanoscale. In this review, we outline the impact, opportunities, applications, and challenges of optical metasurfaces in converting the energy of incoming photons into frequency-shifted photons, phonons, and energetic charge carriers. A myriad of opportunities await for the utilization of the converted energy. Here we cover the most pertinent aspects from a fundamental nanoscopic viewpoint all the way to applications.

1D quasi-bound states in the continuum with large operation bandwidth in the ω∼k space for nonlinear optical applications

The phenomenon of bound state in the continuum (BIC) with an infinite quality factor and lifetime has emerged in recent years in photonics as a new tool to manipulate light–matter interactions. However, most of the investigated structures only support BIC resonances at very few discrete points in the ω ∼ k space. Even when the BIC is switched to a quasi-BIC (QBIC) resonance through perturbation, its frequency will still be located within a narrow spectral band close to that of the original BIC, restricting their applications in many fields where random or multiple input frequencies beyond the narrow band are required. In this work, we demonstrate that a new set of QBIC resonances can be supported by using a special binary grating consisting of two alternatingly aligned ridge arrays with the same period and zero-approaching ridge width difference on a slab waveguide. These QBIC resonances are distributed continuously over a broad band along a line in the ω ∼ k space and can thus be considered as 1D QBICs. With the Q factors generally affected by the ridge difference, it is now possible to arbitrarily choose any frequencies on the dispersion line to achieve significantly enhanced light–matter interactions, facilitating many applications where multiple input wavelengths are required; e.g., sum or difference frequency generations in nonlinear optics.

Plasmonic Waveguides: Enhancing quantum electrodynamic phenomena at nanoscale

The emerging field of plasmonics can lead to enhanced light matter interactions at extremely nanoscale regions. Plasmonic (metallic) devices promise to efficiently control both classical and quantum properties of light. Plasmonic waveguides are usually used to excite confined electromagnetic modes at the nanoscale that can strongly interact with matter. The analysis of these nanowaveguides exhibits similarities with their low frequency microwave counterparts. In this article, we review ways to study plasmonic nanostructures coupled to quantum optical emitters from a classical electromagnetic perspective. These quantum emitters are mainly used to generate single photon quantum light that can be employed as a quantum bit or qubit in the envisioned quantum information technologies. We demonstrate different ways to enhance a diverse range of quantum electrodynamic phenomena based on plasmonic configurations by using the classical dyadic tensor Green function formalism. More specifically, spontaneous emission and superradiance are analyzed by using the Green function based field quantization. The exciting new field of quantum plasmonics will lead to a plethora of novel optical devices for communications and computing applications operating in the quantum realm, such as efficient single-photon sources, quantum sensors, and compact on-chip nanophotonic circuits.

Terahertz hybrid optical-plasmonic modes: tunable resonant frequency, narrow linewidth, and strong local field enhancement.

Hybrid optical-plasmonic modes have the characteristics of low loss and small mode volume, which will result in the strong localization and enhancement of electromagnetic field. Such advantages of hybrid optical-plasmonic mode are important for the enhancement of light-matter interactions. Here, terahertz (THz) hybrid modes of Fabry-Perot resonances (FPRs) and spoof surface plasmon polaritons (SSPPs) in the modified Otto scheme are investigated both in theoretical and experimental aspects. The device structure is composed of a metal grating silicon waveguide (MGSW) and a metal slit grating (MSG). The two components are vertically stacked with a variable air gap between them. The THz hybrid modes are originated from the far-field coupling of the FPRs and the SSPP supported by the air gap and the MSG, respectively. By changing the thickness of the air gap, the resonant frequency of the FPR-SSPP modes can be tuned in a frequency range of about 0.1 THz. An anti-crossing behavior between two reflection dips corresponding to the guided-mode resonance in the MGSW and the FPR-SSPP mode is observed, which leads to the narrowing of the reflection dips in the anti-crossing region. Numerical simulations show that at the resonant frequencies of FPR-SSPP mode, there is a huge volume-averaged electromagnetic energy enhancement of about 1600 times in the grooves of the MSG, which is around 8.7 times larger than that induced by the SSPP directly launched by free-space electromagnetic field. The hybrid FPR-SSPP modes can be used to construct THz sensors and detectors with high sensitivity.

Nonlinear response of Q-boosting metasurfaces beyond the time-bandwidth limit

Abstract Resonant nanostructures, such as photonic metasurfaces, have created an unprecedented case for enhanced light–matter interactions through local field engineering. However, the presence of resonances fundamentally limits the bandwidth of such interactions. Here, we report on amending the nonlinear optical response of a semiconducting metasurface through Q-boosting, where the Q-factor of a metasurface rapidly increases with time. The coupled-mode theory reveals overcoming the bandwidth limit by coupling a broadband signal to a bandwidth-matched resonance and Q-boosting at a timescale faster than a resonator lifetime. A control–excitation experiment simulation using a tailored Q-boosting silicon-germanium metasurface predicts the third-harmonic enhancement by factors of 8 (peak) and 4.5 (integrated) against the best-case static metasurface. An analysis of free-carrier losses based on experimental data shows robustness to nonradiative losses and offers a viable pathway to increasing the light–matter interactions beyond the bandwidth limit, with implications in nonlinear and quantum optics, sensing, and telecommunication technologies.

Engineering a mechanically stable hybrid photonic crystal cavity coupled to color defects in diamond

Wavelength scale photonic, high-quality factor (Q-factor), cavities are crucial for enhancing light–matter interaction. Such on-chip hybrid devices could potentially provide a route towards scalable quantum technologies with color defects in diamond. A variety of designs for photonic crystal cavities have been proposed; however, the challenging and multi-step fabrication processes required for such designs limit the experimentally observed Q-factors in addition to significant radiation loss. One possible way to minimize the radiation loss in a one-dimensional (1D) photonic crystal cavity is by introducing a so-called Gaussian defect region around the cavity. In this work, we propose a versatile approach to design a Gaussian defect region by changing the lattice parameter in a 1D photonic crystal. Further, to circumvent the problem of creating freestanding cavities for achieving high-Q factor in a 1D photonic crystal cavity, we propose a novel hybrid diamond-titanium dioxide (TiO2) based materials for color defects in diamond, in particular the nitrogen-vacancy (NV−) center. Our proposed mechanically stable and high-Q cavity could be crucial for on-chip integration of different nanophotonic components for chip-scale photonic devices. We show via simulations that Q-factor 105 can be achieved with the device.

Non-Ultrawide Bandgap Semiconductor GaSe Nanobelts for Sensitive Deep Ultraviolet Light Photodetector Application.

In this paper, the authors report the fabrication of a sensitive deep ultraviolet (DUV) photodetector by using an individual GaSe nanobelt with a thickness of 52.1nm, which presents the highest photoresponse at 265nm illumination with a responsivity and photoconductive gain of about 663AW-1 and 3103 at a 3V bias, respectively, comparable to or even better than other reported devices based on conventional wide bandgap semiconductors. According to the simulation, this photoelectric property is associated with the wavelength-dependent absorption coefficient of the GaSe crystal, for which incident light with shorter wavelengths will be absorbed near the surface, while light with longer wavelengths will have a larger penetration depth, leading to a blueshift of the absorption edge with decreasing thickness. Further finite element method (FEM) simulation reveals that the relatively thin GaSe nanobelt exhibits an enhanced transversal standing wave pattern compared to its thicker counterpart at a wavelength of 265nm, leading to an enhanced light-matter interaction and thereby more efficient photocurrent generation. The device can also function as an effective image sensor with acceptable spatial resolution. This work will shed light on the facile fabrication of a high-performance DUV photodetector from non-ultrawide bandgap semiconductors.