Terahertz Pulse Energy Research Articles

Terahertz-driven acceleration of subrelativistic electron beams using tapered rectangular dielectric-lined waveguides

We investigate the use of tapered rectangular dielectric-lined waveguides (DLWs) for the acceleration of low-energy, subrelativistic, electron bunches by the interaction with multicycle narrowband terahertz (THz) pulses. A key challenge exists in this subrelativistic regime; the electron velocity changes significantly as energy is gained. To keep electrons in the accelerating phase, the phase velocity must also be increased to match. We present simulations which demonstrate that the dielectric thickness can be kept constant and the width of the dielectric lining can be tapered along the direction of travel to vary the phase velocity, an approach only possible by the use of a rectangular waveguide geometry. The properties of tapered DLWs are discussed and following this, a design process is presented to demonstrate that the way this tapering can be optimized for different pulse and beam parameters. The minimum accelerating gradient for electron bunch capture is derived and compared to simulations. As examples of this design process, designs are considered based on considerations of the THz source, incoming electron beam, and manufacturing tolerances. A maximum THz pulse energy of 22.5 μJ in the DLW was considered, which represents what is readily achievable using mJ-level regenerative amplifier laser systems together with optical-to-terahertz conversion in lithium niobate crystals. This will be more than double the energy of a 100 keV electron beam, increasing it to 205 keV. We describe the optimization process and present a detailed exploration of the beam dynamics, discussing how the performance will further improve with compressed bunches. Published by the American Physical Society 2024

Zeptojoule detection of terahertz pulses by parametric frequency upconversion.

We combine parametric frequency upconversion with the single-photon counting technology to achieve terahertz (THz) detection sensitivity down to the zeptojoule (zJ) pulse energy level. Our detection scheme employs a near-infrared ultrafast source, a GaP nonlinear crystal, optical filters, and a single-photon avalanche diode. This configuration is able to resolve 1.4 zJ (1.4 × 10-21 J) THz pulse energy, corresponding to 1.5 photons per pulse, when the signal is averaged within only 1 s (or 50,000 pulses). A single THz pulse can also be detected when its energy is above 1185 zJ. These numbers correspond to the noise-equivalent power and THz-to-NIR photon detection efficiency of 1.3 × 10-16 W/Hz1/2 and 5.8 × 10-2%, respectively. To test our scheme, we perform spectroscopy of the water vapor between 1 and 3.7 THz and obtain results that are in agreement with those acquired with a standard electro-optic sampling (EOS) method. Our technique provides a 0.2 THz spectral resolution offering a fast alternative to EOS THz detection for monitoring specific spectral components in spectroscopy, imaging, and communication applications.

Controlling the time shape of terahertz pulses from two-color plasma by combining wavelength dispersion and laser chirp

Using a two-color plasma in air or gas allows for the generation of ultra-broadband and highly intense terahertz (THz) pulses. Precisely controlling the shape of THz pulses, particularly the carrier envelope phase, is crucial for a wide range of technological and scientific applications. Recent research has revealed that the phase difference between the fundamental laser wave and its second harmonic influences the shape of the emitted THz pulse. However, the combined impact of laser chirp and the air-dispersion-induced phase difference between the two colors has not been explored in detail. This study aims to fill this gap. The results show that both of these factors have a significant impact on the THz waveform and emitted pulse energy. Positive and negative chirps lead to distinct effects on the pulse shape. A positively chirped pump laser produces a THz waveform with a negative monopolar shape, while a negatively chirped pump laser results in a positive THz pulse shape. Additionally, our findings indicate that the relationship between THz pulse energy and chirp changes with variations in the specific phase difference between the first and second harmonics. These results underscore the importance of carefully tuning both parameters to achieve maximum generation efficiency for a given waveform.

Recent progress of THz source at the SXFEL

Coherent, wide-tunable frequency and high intensity terahertz (THz) source is under preparation at the Shanghai Soft X-ray free-electron laser facility (SXFEL). The electron bunches modulated by frequency beating light can generate coherent, wide-tunable, high intensity THz radiation from 0.1 to 30 THz through wigglers. The electromagnetic wiggler with peak magnetic field up to 1.75 T is adopted and the parameters of the wiggler are optimized to ensure the generation of strong field THz radiation. Due to the limitation of layout space of the SXFEL, the length of wiggler is limited within 5 meters. By properly increasing the charge of the electron beam, the THz pulse energy can be kept at sub mJ level under the proposed different parameters of the wiggler. In this article, we will present the possible layout of THz source on the SXFEL and the S2E simulation of THz radiation of sub mJ magnitude within the 5-meter wiggler.

High-repetition-rate strong-field terahertz source by optical rectification in DSTMS crystals

Abstract We present the generation of high-repetition-rate strong-field terahertz (THz) pulses from a thin 4-N,N-dimethylamino-4’-N’-methyl-stilbazolium 2,4,6-trimethylbenzenesulfonate (DSTMS) organic crystal pumped by an ytterbium-doped yttrium aluminum garnet laser. The generated THz pulse energy reaches 932.8 nJ at 1 kHz repetition rate, with a conversion efficiency of 0.19% and a peak electric field of 819 kV/cm. At a repetition rate of 10 kHz, it is able to maintain a peak electric field of 236 kV/cm and an average THz power of 0.77 mW. The high-repetition-rate, strong-field THz source provides a convenient tool for the study of THz matter manipulation and THz spectroscopy.

Highly sensitive frequency upconversion detection from 1 to 3 THz with OH1 crystal.

The wide applications of terahertz (THz) wave technology in the ∼1-3 THz range has resulted in a surge in the demand for the performance improvement of THz wave detection technique. In this study, a frequency tunable, highly sensitive frequency upconversion detection based on a 2-(3-(4-hydroxystyryl)-5,5-dime-thylcyclohex-2-enylidene) malononitrile (OH1) crystal at room temperature is demonstrated. Moreover, to effectively increase the signal-to-noise ratio in the low frequency range, a beam isolation enhancer is proposed and its effect is verified. The minimum detectable THz pulse energy reaches about 100 aJ at 1.9 THz. The frequency tuning ranging from 1 to 3 THz. Sensitivity comparison with a 4-dimethylamino-N-methyl-4-stilbazolium tosylate (DAST) crystal system shows that OH1 is a more suitable nonlinear crystal in the 1-2.4 THz range.

Perspectives on ultraintense laser-driven terahertz radiation from plasmas

High-power terahertz (THz) radiation is fundamental to numerous applications in many fields. Ultraintense laser-produced plasmas have attracted ever-increasing interest as a damage-free medium for generating high-peak-power THz pulses. This article gives the authors' perspectives on how the field of ultraintense laser-driven THz radiation from plasmas developed and where the field is headed. In particular, recent advances and some new ideas are outlined in terms of THz genesis, metrology, and applications. In addition to pushing the limits of achievable THz pulse energies and peak powers, much attention will be paid on the tunability of THz properties. Single-shot THz metrology will develop toward multi-dimensional resolution. The resulting extreme THz radiation offers immense opportunities in the THz control over matter and THz-driven strong-field physics. A selection of illustrative application cases in the field of materials, chemistry, and biology are briefly discussed. In the authors' opinion, the concerted advances in these aspects will propel this field into the bright future.

Efficient Co/Pt THz spintronic emitter with tunable polarization

We report on the design of a spintronic emitter based on the Pt(3 nm)/Co(3 nm) structure, which enables the control over terahertz radiation polarization. Utilizing the field-induced magnetization rotation that takes place at low magnetic fields of up to 250 Oe at room temperature, we have achieved the full range of terahertz polarization rotation from 0° to 360°. This rotation became possible due to the uniaxial magnetic anisotropy induced in the plane of the cobalt film during its fabrication. We evaluated the efficiency of the Co/Pt structure in generating terahertz radiation and found that the terahertz pulse energy flux reaches ∼160 nJ/cm2 at an excitation flux of 4 mJ/cm2.

Temporal behavior of the high-power pulsed gas terahertz laser pumped by a fundamental mode TEA CO2 laser.

Optically pumped gas molecular terahertz (THz) lasers are promising for generating high-power and high-beam-quality coherent THz radiation. However, for pulsed gas THz lasers, the temporal behavior of the output THz pulse has rarely been investigated. In this study, the temporal behavior of a pulsed gas THz pumped by a fundamental-mode TEA CO2 laser has been presented for the first time both in simulation and experiment. A modified laser kinetics model based on the density matrix rate equation was used to simulate the temporal behavior and output pulse energy of a pulsed gas THz laser at different gas pressures. The results clearly show that the working gas pressure and pump pulse energy have critical influences on the output THz pulse shape. Three typical pulse shapes were obtained, and the THz pulse splitting caused by gain switching was quantitatively simulated and explained based on the laser dynamic process. Besides, with an incident pump pulse energy of 342 mJ, the maximum output THz pulse energy of 2.31 mJ was obtained at 385 µm, which corresponds to a photon conversion efficiency of approximately 56.1%, and to our knowledge, this is the highest efficiency for D2O gas THz laser. The experimental results agreed well with those of the numerical simulation for the entire working gas pressure range, indicating that our model is a powerful tool and paves the way for designing and optimizing high-power pulsed gas lasers.

Terahertz parametric oscillator with a rhombic ring-cavity

Terahertz parametric oscillator (TPO) with a rhombic ring-cavity is demonstrated. The oscillating cavity is composed of three mirrors and the terahertz emitting-surface. Terahertz frequency can be tuned from 0.9 THz to 2.9 THz just by shifting the position of a cavity mirror. Under a certain round-trip optical length of the Stokes beam, the pump beam size can be larger in the rhombic ring-cavity TPO than that in the conventional resonant-cavity TPO. The maximum terahertz pulse energy in the rhombic ring-cavity TPO is 3.21 μJ, which is about 3 times higher than that in the conventional resonant-cavity TPO.

0.35% THz pulse conversion efficiency achieved by Ti:sapphire femtosecond laser filamentation in argon at 1 kHz repetition rate

In this study, an optical setup for generating terahertz (THz) pulses through a two-color femtosecond laser filament was carefully designed to achieve a precise overlap of two-color laser pulses in space and time. β-barium borate (BBO), α-BBO, and a dual-wavelength plate were used to compensate the phase delay of the two-color lasers. Tilting of α-BBO could further realize the precise spatial overlap of the two beams by counteracting the walk-off effect. The maximum output THz pulse energy reached 21 μJ in argon gas when using a commercial Ti:sapphire laser with a pulse energy of 6 mJ at a 1 kHz repetition rate. The corresponding conversion efficiency exceeded 0.35%.

Active stabilization of terahertz waveforms radiated from a two-color air plasma

Intense laser fields focused into ambient air can be used to generate high-bandwidth current densities in the form of plasma channels and filaments. Excitation with bichromatic fields enables us to adjust the amplitude and sign of these currents using the relative phase between the two light pulses. Two-color filamentation in gas targets provides a route to scaling the energy of terahertz pulses to microjoule levels by driving the plasma channel with a high-energy laser source. However, the structure of plasma channels is highly susceptible to drifts in both the relative phase and other laser parameters, making control over the waveform of the radiated terahertz fields delicate. We establish a clear link between the phase dependence of plasma currents and terahertz radiation by comparing in situ detection of current densities and far-field detection of terahertz electric fields. We show that the current measurement can be used as a feedback parameter for stabilizing the terahertz waveform. This approach provides a route to energetic terahertz pulses with exceptional waveform stability.

Forward terahertz wave generation from liquid gallium in the non-relativistic regime

We characterize a terahertz (THz) source based on plasma in liquid gallium. The dependence of the emitted THz pulse energy on second-order phase, pump pulse energy, and polarization of the short laser pulse is demonstrated. Our study suggests that the THz emission mechanism is due to the ponderomotive force and is aided by a direct-field driven term. The proposed source and accompanying generation mechanism are studied under a non-relativistic regime ( 1 0 15 < I < 1 0 18 W / c m 2 ) for forward directed THz under a single pump excitation scheme.

Effects of high intensity non-ionizing terahertz radiation on human skin fibroblasts.

For the first time, the data have been obtained on the effects of high-intensity terahertz (THz) radiation (with the intensity of 30 GW/cm2, electric field strength of 3.5 MV/cm) on human skin fibroblasts. A quantitative estimation of the number of histone Н2АХ foci of phosphorylation was performed. The number of foci per cell was studied depending on the irradiation time, as well as on the THz pulse energy. The performed studies have shown that the appearance of the foci is not related to either the oxidative stress (the cells preserve their morphology, cytoskeleton structure, and the reactive oxygen species content does not exceed the control values), or the thermal effect of THz radiation. The prolonged irradiation of fibroblasts also did not result in a decrease of their proliferative index.

Development of a 1 TW/35 fs Ti:sapphire Laser Amplifier and Generation of Intense THz Waves Using Two-Color Laser Filamentation

We developed a compact Ti:sapphire laser amplifier system in our laboratory, generating intense laser pulses with a peak power of >1 TW (terawatt), a pulse duration of 34 fs (femtosecond), a central wavelength of 800 nm, and a repetition rate of 10 Hz. The laser amplifier system consists of a mode-locked Ti:sapphire oscillator, a regenerative amplifier, and a single-side-pumped 4-pass amplifier. The chirped-pulse amplification (CPA)-based laser amplifier was found to provide an energy of 49.6 mJ after compression by gratings in air, where the pumping fluence of 1.88 J/cm2 was used. The amplified spontaneous emission (ASE) level was measured to be lower than 10−7, and ps-prepulses were in 10−4 or lower level. The developed laser amplifier system was used for the generation of intense THz (terahertz) waves by focusing the original (800 nm) and second harmonic (400 nm) laser pulses in air. The THz pulse energy was shown to be saturated in the high laser energy regime, and this phenomenon was confirmed by fully electromagnetic, relativistic, and self-consistent particle-in-cell (PIC) simulations.

Enhancing terahertz radiation from femtosecond laser filaments using local gas density modulation

We present a method to enhance the terahertz (THz) wave radiation from a femtosecond laser-induced plasma filament by controlling the local gas density within the filament. We develop a theoretical model for THz generation from a laser-induced air plasma filament and the subsequent propagation process, to account for a varying local gas density. By adjusting the local gas density along the filament, the transient current distribution along the filament and the resulting coherent superposition of terahertz waves can be controlled. The location of the gas jet nozzle and the relative phase between multicolor light fields both affect the transient current distribution and thus the strength of the generated THz field. Compared with the conventional terahertz generation by a two-color filament in a homogeneous gas, a three-color filament can realize an increase by 6.12 times in the generated THz pulse energy, with optimized local gas density modulation. Our results suggest that the THz amplification via local gas density modulation can be further improved with well-designed multicolor pulses.

Terahertz generation by means of ZnGeP2 large aperture photoconductive antenna

The generation of terahertz (THz) radiation using a ZnGeP2 (ZGP) large-aperture photoconductive antenna (PCA) was demonstrated. The semiconductors were excited above and below the bandgap (400 and 800 nm) by a femtosecond Ti:sapphire laser. The THz pulse waveform generated by the ZGP antenna was measured using a time-domain spectroscopy technique. The antenna’s THz pulse energy dependence on the optical pump energy was measured, and saturation fluence and carrier mobility were estimated. The ZGP and a chemical vapor deposited ZnSe-based PCA were compared.

Experimental study of terahertz radiation driven by femtosecond ultraintense laser

Powerful terahertz (THz) radiation sources are crucial to the development of THz science. High-energy strong-field THz pulses have many significant applications such as in the ultrafast control of matter and the THz-driven electron acceleration. In recent years, ultraintense laser-plasma interactions have been proposed as a novel approach to strong-field THz generation. In this paper, the experimental results are presented about the generation of THz radiation from a solid foil irradiated by a 10-TW femtosecond laser pulse. The THz energy as a function of laser energy and defocusing amount is studied. It is found that both the THz energy and the laser-to-THz conversion efficiency increase nonlinearly with the laser energy increasing. At maximum laser energy ~270 mJ, the measured THz pulse energy is 458 μJ, corresponding to a laser-to-THz energy conversion efficiency of 0.17%. No indication of saturation is observed in the experiment, implying that a stronger THz radiation could be achieved with higher laser energy. By simultaneously monitoring the backward scattered laser light spectrum, it is qualitatively understood that the observed THz radiation as a function of laser energy and laser defocusing distance is closely related to the electron heating mechanisms at different laser intensities. The THz spectrum and polarization are characterized by using different band-pass filers and a wire-grid polarizer, respectively. The THz radiation covers an ultrabroad band ranging from 0.2 THz to 30 THz, and shows a radially polarized distribution. By fitting the measured THz spectrum with the theory of coherent transition radiation, the THz pulse duration is inferred to be about 30 fs. At the THz focal spot of ~1 mm in size, the THz field strength is evaluated to be 3.68 GV/m. Such a strong-field THz source will enable the study of extreme THz-matter interactions.

Mechanism study of terahertz radiation regulation in a multi-color laser field

By establishing a theoretical model for terahertz (THz) generation from a laser-induced air plasma filament and the subsequent propagation process, we study the physical mechanisms of THz wave radiation regulation in the multi-color femtosecond laser field. It is proved that the total THz radiation in the far field is affected by three factors: the ionized electron density, transient current distribution along the laser filament, and coherent superposition between THz waves generated by each point along the filament. The results show that the wavelength, relative phase, energy ratio, pulse width, laser frequency ratio, and frequency combination of the multi-color laser are all correlated to their radiated THz energy with different changing laws. The proper regulation of a three-color filament can realize a 4 orders of magnitude increase in the generated THz pulse energy as compared with the conventional THz generation by a two-color filament. These results provide the theoretical basis for the enhancement of THz radiation energy, and they are of great significance for clarifying the physical process of laser filament.

Acceleration of relativistic beams using laser-generated terahertz pulses

Particle accelerators driven by laser-generated terahertz (THz) pulses promise unprecedented control over the energy–time phase space of particle bunches compared with conventional radiofrequency technology. Here we demonstrate acceleration of a relativistic electron beam in a THz-driven linear accelerator. Narrowband THz pulses were tuned to the phase-velocity-matched operating frequency of a rectangular dielectric-lined waveguide for extended collinear interaction with 35 MeV, 60 pC electron bunches, imparting multicycle energy modulation to chirped (6 ps) bunches and injection phase-dependent energy gain (up to 10 keV) to subcycle (2 ps) bunches. These proof-of-principle results establish a route to whole-bunch linear acceleration of subpicosecond particle beams, directly applicable to scaled-up and multistaged concepts capable of preserving beam quality, thus marking a key milestone for future THz-driven acceleration of relativistic beams. Relativistic 35 MeV electron bunches with charges of 60 pC are accelerated in a terahertz-wave-driven dielectric waveguide. When the terahertz pulse energy is 0.8 μJ, an accelerating gradient of 2 MeV m−1 and energy gain of 10 keV are achieved.