Elevated Aerosol Layers Research Articles

Association between sea-land breeze and particulate matter in five coastal urban locations in India

Particulate matter less than 2.5 μm particle diameter (PM2.5) is the most significant environmental issue globally. PM2.5 is an integral component of air quality monitoring and management, human health, weather, climate, and epidemiological research. In this work, we investigate the seasonal variation in PM2.5 mass concentrations and the association between the sea-land breeze system and particulate matter in five coastal urban locations in India (Kolkata, Visakhapatnam, Chennai, Thiruvananthapuram, and Mumbai). The relative occurrence of high PM2.5 mass concentrations was the greatest during the winter season (December through February) while the relative occurrence of low PM2.5 mass concentrations was the greatest during the monsoon season (June through September). Amongst locations, Kolkata experiences the highest PM2.5 loading in winter while Thiruvananthapuram experiences the lowest PM2.5 loading in monsoon. Indo-Gangetic Plain (IGP) outflow onto the Bay of Bengal significantly impacts locations along the eastern coast of India with reduced impact from north (Kolkata) to south (Chennai). The sea-breeze component analysis revealed daily cycles of the sea-land breeze with varying magnitudes of the breeze between the different seasons. Overall, we found a negative association between the sea-land breeze magnitude and PM2.5 mass concentrations, implying that the weakened sea-land breeze may deteriorate air quality in coastal locations due to poor ventilation. The vertical profiles of aerosol extinction showed elevated aerosol layers within 1 km from the surface in almost all locations. The decreasing trend in the land-sea temperature contrast in coastal locations is expected to deteriorate air quality in coastal locations in the warming future. Nevertheless, critical analyses using ground-based remote sensing techniques are required for a better understanding the impact of sea-land breeze dynamics on air quality in coastal locations.

Estimation of Aerosol Layer Height from OLCI Measurements in the O2A-Absorption Band over Oceans

The aerosol layer height (ALH) is an important parameter that characterizes aerosol interaction with the environment. An estimation of the vertical distribution of aerosol is necessary for studies of those interactions, their effect on radiance and for aerosol transport models. ALH can be retrieved from satellite-based radiance measurements within the oxygen absorption band between 760 and 770 nm (O2A band). The oxygen absorption is reduced when light is scattered by an elevated aerosol layer. The Ocean and Land Colour Imager (OLCI) has three bands within the oxygen absorption band. We show a congruent sensitivity study with respect to ALH for dust and smoke cases over oceans. Furthermore, we developed a retrieval of the ALH for those cases and an uncertainty estimation by applying linear uncertainty propagation and a bootstrap method. The sensitivity study and the uncertainty estimation are based on radiative transfer simulations. The impact of ALH, aerosol optical thickness (AOT), the surface roughness (wind speed) and the central wavelength on the top of atmosphere (TOA) radiance is discussed. The OLCI bands are sufficiently sensitive to ALH for cases with AOTs larger than 0.5 under the assumption of a known aerosol type. With an accurate spectral characterization of the OLCI O2A bands better than 0.1 nm, ALH can be retrieved with an uncertainty of a few hundred meters. The retrieval of ALH was applied successfully on an OLCI dust and smoke scene. The found ALH is similar to parallel measurements by the Tropospheric Monitoring Instrument (TROPOMI). OLCI’s high spatial resolution and coverage allow a detailed overview of the vertical aerosol distribution over oceans.

Characteristics of elevated aerosol layer over the Indian east coast, Kattankulathur (12.82oN, 80.04°E): A northeast monsoon region

The elevated aerosol layer (EAL) plays a vital role in weather and climate by modifying the Earth's radiation budget. In the present study, the EAL occurrence and its characteristics in the pre-monsoon season using micropulse lidar (MPL) observations during 2016–2018 and Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) during 2007–2018 over Kattankulathur is being reported. We have collected 147 days (101 cases) of MPL (CALIPSO) observations during clear sky conditions in the pre-monsoon 2016–2018 (2007–2018), out of which EAL is observed for 56 days (61 cases). The EAL width is generally found to be ~2.0 km and occurs between ~1.0 km and 5.0 km. Three different types of EALs are categorized based on their altitudinal occurrence using the zero-crossing method. The EALs with their base at ~1.0–1.5 km, ~1.5–2.0 km, and ~ 2.0–3.0 km are taken as types I, II, and III, which occur for 9, 20, and 27 days, respectively. The EAL significantly modifies the total columnar aerosol optical depth (AOD). It is found that AOD, in total, within ABL and EAL, are ~0.72 (0.61), 0.28 (0.25), and 0.45 (0.36) using MPL (CALIPSO), respectively. The aerosols within ABL contribute ~38 % (41 %) while EAL ~ 62 % (59 %) to the total AOD obtained using MPL (CALIPSO). We observed that the ABL and EAL are characterized by different aerosol subtypes, such as dust marine (31 %) and smoke (~ 27 %) aerosols. Other aerosol subtypes, such as dust and polluted dust, commonly occur within the ABL (54 %) and EAL (52 %).

Multi‐Year CALIPSO Observations of Ubiquitous Elevated Aerosol Layer in the Free Troposphere Over South Asia: Sources and Formation Mechanism

AbstractThe vertical distribution of aerosols in the lower troposphere is critically important for assessing their impact on Earth's radiation budget and modulation of cloud microphysics. This study analyzed cloud‐free aerosol extinction coefficient (βext), aerosol subtypes, and particulate depolarization ratios obtained from CALIOP (Cloud‐Aerosol Lidar with Orthogonal Polarization) over the six regions of India during 2008–2018. We investigated unprecedented climatology of the physical and optical characteristics of elevated aerosol layers (EALs) along with their source and formation mechanism. The key findings include: (a) EALs over the Indian region were persistent between 4 and 6 km during all seasons, (b) geometrical layer thickness of EALs increased up to 36.7% and 25% from the annual mean during summer and fall seasons, respectively, compared to that of spring and winter, (c) dust and polluted dust accounted for up to 50%–80% from near‐surface to 6 km and up to 80%–90% of the EALs between 4 and 6 km, respectively for all the seasons and regions, (d) we anticipated that locally confined recirculation coupled with stratified stable layer capped within turbulent layers could be a possible mechanism of formation of stratified EALs between 4 and 6 km during winter‐spring‐fall, while in summer, vertical transport of pollutants from the PBL to mid‐troposphere due to enhanced deep convection served as a key formation mechanism of the EALs, (e) the second Modern‐Era Retrospective analysis for Research and Applications Global Modeling Initiative model reasonably simulated the shape and vertical gradient of βext with significant differences in magnitude below 4 km; however, it fails to reproduce EALs for all seasons and regions during the study period.

Boundary Layer Height Characteristics in Mexico City from Two Remote Sensing Techniques

The Atmospheric Boundary Layer (ABL) height is a key parameter in air quality research as well as for numerical simulations and forecasts. The identification of thermally stable layers, often with radiosondes, has been a common approach for estimating ABL height, though with limited temporal coverage. Remote sensing techniques offer essentially continuous measurements. Nevertheless, ABL height retrievals from different methods can vary greatly when compared, which is particularly notable for topographically complex terrains, such as that surrounding Mexico City. This study, employing one year of data in Mexico City, reveals that the daytime convective boundary layer height (retrieved from Doppler lidar data) is typically lower than the aerosol layer height (retrieved from ceilometer data). Although both estimated heights evolved diurnally, the more elevated aerosol layer decays more slowly, suggesting that the mechanisms that elevate aerosols are not limited to convective motions. Additionally, both diurnal and seasonal variability are investigated, comparing remotely sensed-retrieved heights with thermally stable layers estimated from radiosonde data. Multiple stable layers often develop, those at higher levels have similar values to the ceilometer-retrieved heights, while stable layers at lower heights are similar to Doppler lidar height retrievals. The present research constitutes the first detailed analysis of ceilometer backscatter and Doppler lidar thresholding methods for estimating ABL height over Mexico City, and our results illustrate the complexity of mixing mechanisms on the ABL in this region of complex orography.

Evaluating convective planetary boundary layer height estimations resolved by both active and passive remote sensing instruments during the CHEESEHEAD19 field campaign

Abstract. During the Chequamegon Heterogeneous Ecosystem Energy-balance Study Enabled by a High-density Extensive Array of Detectors 2019 (CHEESEHEAD19) field campaign, held in the summer of 2019 in northern Wisconsin, USA, active and passive ground-based remote sensing instruments were deployed to understand the response of the planetary boundary layer to heterogeneous land surface forcing. These instruments include radar wind profilers, microwave radiometers, atmospheric emitted radiance interferometers, ceilometers, high spectral resolution lidars, Doppler lidars, and collaborative lower-atmospheric mobile profiling systems that combine several of these instruments. In this study, these ground-based remote sensing instruments are used to estimate the height of the daytime planetary boundary layer, and their performance is compared against independent boundary layer depth estimates obtained from radiosondes launched as part of the field campaign. The impact of clouds (in particular boundary layer clouds) on boundary layer depth estimations is also investigated. We found that while all instruments are overall able to provide reasonable boundary layer depth estimates, each of them shows strengths and weaknesses under certain conditions. For example, radar wind profilers perform well during cloud-free conditions, and microwave radiometers and atmospheric emitted radiance interferometers have a very good agreement during all conditions but are limited by the smoothness of the retrieved thermodynamic profiles. The estimates from ceilometers and high spectral resolution lidars can be hindered by the presence of elevated aerosol layers or clouds, and the multi-instrument retrieval from the collaborative lower atmospheric mobile profiling systems can be constricted to a limited height range in low-aerosol conditions.

Visibility, aerosol optical depth, and low-visibility events in Bangkok during the dry season and associated local weather and synoptic patterns.

Visibility and aerosol optical depth (AOD) characterization, and their relationship with PM10 and local and synoptic meteorology, were studied for January-March in 2014 and 2015 over Bangkok. Visibility degradation intensifies in the dry season as compared to the wet season due to increase in PM10 and unfavorable meteorological conditions. The average visibility is lower in January and February as compared to the other months. Relatively higher AOD in March despite lower PM10 is attributed to the synergetic effect of moderate relative humidity, secondary aerosols, elevated aerosol layer due to summertime convection, and biomass burning. Larger variability in visibility and PM10 in winter months is due to more synoptic weather fluctuations while AOD shows similar variability for all months attributed partly to fires. Higher PM10 and moderate-to-high relative humidity cause lower visibility in the morning while it improves in afternoon as PM10 and relative humidity decrease. AOD is higher in the afternoon as compared to that in the morning and evening as it is less sensitive to diurnal change in aerosols and meteorology at the surface level. Visibility and AOD relationships with PM10 are dependent on relative humidity. Weaker winds lead to lower visibility, higher PM10, and higher AOD irrespective of wind direction. Stronger winds improve visibility and decrease PM10 for all directions while AOD is higher for all directions except eastern and northeastern. The back-trajectory results show that the transport of pollutant and moist air is coupled with the synoptic weather and influence visibility and AOD. Two low-visibility events were investigated. The first event is potentially caused by the combined effect of local emissions and their accumulation due to stagnant weather conditions, secondary aerosols, and forest fires in the nearby regions. The second event can be attributed to the local emission and fires in the nearby area with hygroscopic growth of aerosols due to moist air from the Gulf of Thailand. Based on these findings, some policy implications have also been given.

The vertical aerosol type distribution above Israel – 2 years of lidar observations at the coastal city of Haifa

Abstract. For the first time, vertically resolved long-term lidar measurements of the aerosol distribution were conducted in Haifa, Israel. The measurements were performed by a PollyXT multi–wavelength Raman and polarization lidar. The lidar was measuring continuously over a 2-year period from March 2017 to May 2019. The resulting data set is a series of manually evaluated lidar optical property profiles. To identify the aerosol types in the observed layers, a novel aerosol typing method that was developed at TROPOS is used. This method applies optimal estimation to a combination of lidar-derived intensive aerosol properties to determine the statistically most-likely contribution per aerosol component in terms of relative volume. A case study that shows several elevated aerosol layers illustrates this method and shows, for example, that coarse dust particles are observed up to 5 km height over Israel. From the whole data set, the seasonal distribution of the observed aerosol components over Israel is derived. Throughout all seasons, coarse spherical particles like sea salt and hygroscopically grown continental aerosol were observed. These particles originate from continental Europe and were transported over the Mediterranean Sea. Sea-salt particles were observed frequently due to the coastal site of Haifa. The highest contributions of coarse spherical particles are present in summer, autumn, and winter. During spring, mostly coarse non-spherical particles that are attributed to desert dust were observed. This is consistent with the distinct dust season in spring in Israel. An automated time–height-resolved air mass source attribution method identifies the origin of the dust in the Sahara and the Arabian deserts. Fine-mode spherical particles contribute significantly to the observed aerosol mixture during all seasons. These particles originate mainly from the industrial region at the bay of Haifa.

Assessment of Influence of Urban Aerosol Vertical Profile on Clear-Sky Diffuse Radiance Pattern

Abstract Aerosol particles spread in the atmosphere play an important role in solar light scattering and thus co-determine the sky radiance/luminance pattern as well as diffuse irradiances/illuminances at the ground. The particular influence is given by their optical properties and by their distribution in the atmosphere. The dependence of the aerosol extinction coefficient on altitude is usually described by the exponential law, which results from the averaging of a large number of aerosol realizations. This is also frequently the case of simulating of the solar diffuse radiance/luminance distribution over the sky, when it is based on solving the radiative transfer problem. However, the aerosol vertical profile can sometimes be significantly different from the exponential one. Mainly in the urban environment, the aerosol is often well-mixed within the atmospheric boundary layer, so its volume extinction coefficient is almost constant there. Under specific conditions also the so-called elevated aerosol layer may occur. This work investigates how such different profiles affect the clear sky radiance pattern and consequently also the ground-based horizontal diffuse irradiance. The numerical simulations revealed that the discrepancies are negligible in practice. So, it appears that the aerosol vertical distribution does not play any important role in sky radiance calculations, and the standard exponential law is general enough to cover also various specific aerosol conditions.

Characteristics of Turbulence and Aerosol Optical and Radiative Properties during Haze–Fog Episodes in Shenyang, Northeast China

The characteristics of turbulence in the planetary boundary layer (PBL) and the aerosol optical and radiative properties during haze and haze–fog mixed episodes on 22–27 January 2021, in Shenyang, a provincial city in Northeast China, were analyzed using meteorological and aerosol observations. During the haze episode, the hourly mean PM2.5 concentration reached a maximum of 337 µg m−3 and visibility decreased to 1.6 km. The PM2.5 concentration decreased gradually during the haze–fog mixed episode as a result of the scavenging effects of fog, but visibility mostly remained below 1 km owing to high ambient relative humidity (>90%). During the haze–fog mixed episode, an increasing proportion of PM2.5 led to a higher ratio of the backward to the total scattering coefficient. As fog occurred, downward shortwave radiation arriving at the surface was significantly reduced, and upward longwave radiation increased and almost equaled the downward longwave radiation, which can be used as a good indicator for distinguishing haze and fog. Mechanical turbulence was weak during both episodes, and latent heat flux varied within a wider range during the haze–fog mixed episode. The PBL dynamic structure affected the vertical distribution of aerosols/fog droplets. Aerosol-rich layers appeared at altitudes below 0.5 km and above 0.6 km during the haze episode. The elevated aerosol layer was related to the aerosol transport from upstream polluted areas caused by strong upper-level turbulence, and it began to mix vertically after sunrise because of convective turbulence. Aerosols and fog droplets were mostly trapped in a shallower PBL with a height of 0.2–0.4 km during the haze–fog mixed episode because of weaker turbulence.

Natural processes dominate the pollution levels during COVID-19 lockdown over India

The lockdown measures that were taken to combat the COVID-19 pandemic minimized anthropogenic activities and created natural laboratory conditions for studying air quality. Both observations and WRF-Chem simulations show a 20–50% reduction (compared to pre-lockdown and same period of previous year) in the concentrations of most aerosols and trace gases over Northwest India, the Indo Gangetic Plain (IGP), and the Northeast Indian regions. It is shown that this was mainly due to a 70–80% increase in the height of the boundary layer and the low emissions during lockdown. However, a 60–70% increase in the pollutants levels was observed over Central and South India including the Arabian sea and Bay of Bengal during this period, which is attributed to natural processes. Elevated (dust) aerosol layers are transported from the Middle East and Africa via long-range transport, and a decrease in the wind speed (20–40%) caused these aerosols to stagnate, enhancing the aerosol levels over Central and Southern India. A 40–60% increase in relative humidity further amplified aerosol concentrations. The results of this study suggest that besides emissions, natural processes including background meteorology and dynamics, play a crucial role in the pollution concentrations over the Indian sub-continent.

Vertical distribution characteristics of aerosol particles over the Guanzhong Plain

Haze pollution occurs frequently in Xi'an-centerd Guanzhong Plain (GZP) in winter. In this study, a vehicle-based lidar system was used for monitoring the vertical distribution of aerosol particulates during a typical winter haze episode over GZP. Fixed-point lidar observations were combined with field observations of particle charging in Xi'an city to investigate the distribution of atmospheric particles and the process of formation of particulate pollution. Mobile lidar observations were conducted over three navigation routes in Xi'an and its neighboring cities to investigate the origin and transport of aerosol particles, and meteorological interactions over GZP. The results demonstrated that local emissions were the main cause of near-surface particulate pollution. Fluctuations in humidity promoted particle charging and enhanced particle growth. Polluted dust particles entrained by air mass could be transported from the northwest to high-altitude areas of Xi'an. Mobile lidar observations showed that aerosol particles in the Xi'an-Xianyang area exhibited a clear vertically stratified structure under 1900 m height; there was only one aerosol layer concentrated within 900 m from the ground in Baoji and the near-ground extinction coefficient was relatively high. A larger aerosol optical depth (AOD) was observed in Xi'an-Xianyang than in Baoji, indicating that AOD could be affected by the elevated aerosol layers within the boundary layer. The combined methods of fixed and mobile lidar measurements, and satellite information can be applied in other regions and supply detailed information for air quality models.

Evolution of Aerosols in the Atmospheric Boundary Layer and Elevated Layers during a Severe, Persistent Haze Episode in a Central China Megacity

Aerosol vertical profiling is crucial to understand the formation mechanism and evolution processes of haze, which have not yet been comprehensively clarified. In this study, we investigated a severe, persistent haze event in Wuhan (30.5° N, 114.4° E), China during 5–18 January 2013 by the use of a polarization lidar, a Cimel sun photometer, meteorological datasets, and the hybrid single-particle Lagrangian integrated trajectory (HYSPLIT) model, focusing on the time–height evolution of aerosols in both the atmospheric boundary layer (ABL) and elevated layers. During the haze period, the integrated particle depolarization ratio was 0.05 ± 0.02, and the fine mode fraction reached 0.91 ± 0.03, indicating haze particles were rather spherical and predominately submicron, that is, of anthropogenic nature. Compared with the clear period, columnar aerosol optical depth at 500 nm tripled to 1.32 ± 0.31, and the strongest enhancement in aerosol concentration occurred from near the ground to an altitude of 1.2 km during the haze period. The daytime evolution of aerosol vertical distribution in the ABL exhibited a distinct pattern under haze weather. Abundant particles accumulated below 0.5 km in the morning hours due to stable meteorological conditions, including a strong surface-based inversion (4.4–8.1 °C), late development (from 1000–1100 LT) of the convective boundary layer, and weak wind (<4 m∙s−1) in the lowermost troposphere. In the afternoon, improved ventilation delivered an overall reduction in boundary layer aerosols but was insufficient to eliminate haze. Particularly, the morning residual layer had an optical depth of 0.29–0.56. It influenced air quality indirectly by weakening convective activities in the morning and directly through the fumigation process around noon, suggesting it may be an important element in aerosol–ABL interactions during consecutive days with haze. Our lidar also captured the presence of the elevated aerosol layers (EALs) embodying regional/long-range transport. Most of the EALs were observed to subside to <1.2 km and exacerbate the pollution level. Backward trajectory analysis and lidar data revealed the EALs originated from the transport of anthropogenic pollutants from the Sichuan Basin, China, and of dust from the deserts in the northwest. They were estimated to contribute ~19% of columnar aerosol-loading, pointing to a non-negligible role of transport during the intense pollution episode. The results could benefit the complete understanding of aerosol–ABL interactions under haze weather and air quality forecasting and control in Wuhan.

Processes controlling the vertical aerosol distribution in marine stratocumulus regions – a sensitivity study using the climate model NorESM1-M

Abstract. The vertical distribution of aerosols plays an important role in determining the effective radiative forcing from aerosol–radiation and aerosol–cloud interactions. Here, a number of processes controlling the vertical distribution of aerosol in five subtropical marine stratocumulus regions in the climate model NorESM1-M are investigated, with a focus on the total aerosol extinction. A comparison with satellite lidar data (CALIOP, Cloud–Aerosol Lidar with Orthogonal Polarization) shows that the model underestimates aerosol extinction throughout the troposphere, especially elevated aerosol layers in the two regions where they are seen in observations. It is found that the shape of the vertical aerosol distribution is largely determined by the aerosol emission and removal processes in the model, primarily through the injection height, emitted particle size, and wet scavenging. In addition, the representation of vertical transport related to shallow convection and entrainment is found to be important, whereas alterations in aerosol optical properties and cloud microphysics parameterizations have smaller effects on the vertical aerosol extinction distribution. However, none of the alterations made are sufficient for reproducing the observed vertical distribution of aerosol extinction, neither in magnitude nor in shape. Interpolating the vertical levels of CALIOP to the corresponding model levels leads to better agreement in the boundary layer and highlights the importance of the vertical resolution.

Micro-Pulse Lidar observations of elevated aerosol layers over the Himalayan region

The present study investigates the characteristics of elevated aerosol layer (EAL) using high spatio-temporal Boundary Layer Lidar observations over Manora Peak (29.4° N; 79.2° E; 1958m above mean sea level), Nainital located in the Himalayan region. We have chosen four EAL cases on June 17, 2006 (C1); December 12, 2007 (C2); February 06 (C3) and May 07, 2008 (C4) over the observational site. The occurrence of EAL is generally found at an altitude ~ 2–4 km above ground level over the site. It is found that the westerly/northwesterly winds with magnitudes of about 6–9 ms−1 are conducive for the generation and strengthening of EAL. A 7-days airmass backward trajectory analysis reveals that the lower (higher) altitude source originates from the west coast (northwest) regions. Furthermore, the atmospheric radiative forcing estimated using Santa Barbara DISORT (discrete ordinates radiative transfer) Atmospheric Radiative Transfer (SBDART) model reveals that the atmosphere heats up with 1.35 K day−1 and 1.32 K day−1 due to the presence of EAL on C1 and C4, respectively. Our results confirm that the occurrence of EALs causes atmospheric warming, that can impact on the regional radiation budget over the Himalayan region.

Vertical and spatial distribution of elevated aerosol layers obtained using long-term ground-based and space-borne lidar observations

In this study, long-term ground-based and space-borne lidar measurements are used to understand the vertical (surface to 30 km) and spatial distribution of aerosols. First, the vertical distribution of aerosol extinction (AE) covering from near surface to 30 km is provided by combining Micro Pulse Lidar and Mie lidar observations co-located over a tropical station Gadanki (13.5oN, 79.2oE), India. The presence of two elevated aerosol layers, one between 2 and 5 km (lower troposphere) and the other between 15 and 18 km (Upper Troposphere and Lower Stratosphere (UTLS)), are simultaneously observed during the Indian summer monsoon season. Second, the spatial extent of these elevated aerosol layers obtained using Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) measurements reveals the presence of the lower layer extending from Africa to South Asia during both pre–monsoon and monsoon seasons. However, the UTLS layer is confined from middle-east to the China Sea only during monsoon season, also known as Asian Tropopause Aerosol Layer (ATAL). Third, aerosol sub-types obtained for these elevated aerosol layers using CALIPSO measurements reveals the dominance of polluted dust (44.6%) whereas the occurrence frequency of polluted continental, dust and elevated smoke is ~19.6%, 20.7% and 13.1%, respectively, for the lower layer. However, the frequency of volcanic ash and sulfate aerosols is ~50.3% and 49.7%, respectively, for the UTLS layer. Depolarization ratio (color ratio) values varies between 0.21 and 0.34 (>0.6) in the lower layer while the values >0.15 (<0.6) are present in the UTLS layer during monsoon season revealing the influence of non-spherical and coarse mode particles in the lower layer while spherical and fine mode particles in the UTLS region over the site. This information is very much useful in estimating reliable radiative forcing due to these elevated aerosol layers on the background atmosphere involved in assessing their impact on the regional climate.

A novel lidar gradient cluster analysis method of nocturnal boundary layer detection during air pollution episodes

Abstract. The observation of the nocturnal boundary layer height (NBLH) plays an important role in air pollution and monitoring. Through 39 d of heavy pollution observation experiments in Beijing (China), as well as an exhaustive evaluation of the gradient, wavelet covariance transform, and cubic root gradient methods, a novel algorithm based on the cluster analysis of the gradient method (CA-GM) of lidar signals is developed to capture the multilayer structure and achieve night-time stability. The CA-GM highlights its performance compared with radiosonde data, and the best correlation (0.85), weakest root-mean-square error (203 m), and an improved 25 % correlation coefficient are achieved via the GM. Compared with the 39 d experiments using other algorithms, reasonable parameter selection can help in distinguishing between layers with different properties, such as the cloud layer, elevated aerosol layers, and random noise. Consequently, the CA-GM can automatically address the uncertainty with multiple structures and obtain a stable NBLH with a high temporal resolution, which is expected to contribute to air pollution monitoring and climatology, as well as model verification.

Dust dominates high-altitude snow darkening and melt over high-mountain Asia

Westerly driven, long-range transportation of dust particles in elevated aerosol layers (EALs) is a persistent phenomenon during spring and summer over the Indian subcontinent. During the snow accumulation season, EALs transport substantial amounts of dust to the snow-covered slopes of high-mountain Asia (HMA). Here we use multiple satellite-based estimates to demonstrate a robust physical association between the EALs and dust-induced snow darkening over HMA. Results from a fully coupled atmosphere–chemistry–snow model support these observations, revealing across HMA a signature of increasing dust-induced snow darkening with surface elevation that peaks near 4,500 m. Moreover, the influence of dust on snow darkening is greater than that of black carbon above 4,000 m. Our findings suggest a discernible role of dust in the observed spatial heterogeneity of snowmelt and snowline trends over HMA and highlight an increasing contribution of dust to snowmelt as the snowline rises with warming. Dust deposition in high-mountain Asia lowers snow albedo and hastens melt. Satellite data and models show that dust arrives via transport in elevated aerosol layers and outweighs black carbon impacts at high altitudes, suggesting a growing importance of dust on snowmelt as snowlines rise with warming.

An Investigation of the Elevated Aerosol Layer Using a Polarization Lidar Over a Tropical Rural Site in India

Polarization lidar observations were made to study the transport of an elevated aerosol layer over Gadanki, India (13.45° N, 79.17° E) during the pre-monsoon period of the year 2009. Observations show significant aerosol layering within and above the boundary layer. Coordinated observations with radiosondes were carried out from 2 to 10 April 2009. Temporal and spatial variations of the parameters are studied for the boundary layer (≈ 2.5 km) and up to 5 km. The backscattering coefficient and the depolarization ratio are observed to increase and decrease with an increase in humidity, respectively. Clouds are not formed, indicating less efficiency of the aerosol in acting as condensation nuclei. The transport of the elevated aerosol layer is investigated using a back-trajectory analysis, revealing that the transported layer originating from the central Indian region has a depolarization ratio of at least 0.05. From model analysis and satellite fire-count data, it is inferred that the source of the aerosol layer is wildfire events over the central Indian region. The elevated smoke-aerosol layer (not mixing with the boundary layer) has implications for the altering of the temperature profile of the atmosphere and the suppression of cloud formation.

Enhancement of Atmospheric Stability by Anomalous Elevated Aerosols During Winter in China

AbstractChanges in anthropogenic aerosols with a low level of scientific cognition affect the atmospheric environment and radiative balance of the Earth. We determine anomalous elevated aerosol layers (EALs) and their source and effects on regional atmospheric stability in China by using 2007–2016 data from multiple satellite observations and models. Anomalous EALs occur during winter over Eastern China, and they are mainly distributed above 2 km and can even spread up to 4–5 km despite the disadvantageous atmospheric convection conditions during winter. Anthropogenic pollutants that mainly originate from local‐range transport with enhanced atmospheric updraft play a dominant role (about 60%) in this situation. Furthermore, anomalous EALs result in considerable warming in the upper atmosphere (+0.32 K/day) and cooling on the surface (−0.04 K/day) over Eastern China. They decrease surface incident radiation by an average of 3.4 W/m2. The opposite heating rate change in the upper atmosphere and surface caused by anomalous EALs consequently increases the low atmospheric stability by an average of 0.39 K, and this increment weakens the dissipation of atmospheric dispersion. Related studies have indicated that increased atmospheric stability can severely exacerbate atmospheric pollution near the surface.