Electron Scattering Research Articles

Absence of Additional Stretching-Induced Electron Scattering in Highly Conductive Cross-linked Nanocomposites with Negligible Tunneling Barrier Height and Width.

The intrinsic resistance of stretchable materials is dependent on strain, following Ohm's law. Here the invariable resistance of highly conductive cross-linked nanocomposites over 53% strain is reported, where additional electron scattering is absent with stretching. The in situ generated uniformly dispersed small silver nanosatellite particles (diameter=3.6nm) realize a short tunneling barrier width of 4.1nm in cross-linked silicone rubber matrix. Furthermore, the barrier height can be precisely controlled by the gap state energy level modulation in silicone rubber using cross-linkers. The negligible barrier height (0.01eV) and short barrier width, achieved by the silver nanosatellite particles in cross-linked silicone rubber, dramatically increase the electrical conductivity (51710Scm-1) by more than 4 orders of magnitude. The high conductance is also maintained over 53% strain. The quantum tunneling behavior is observed when the barrier height is increased, following the Simmons approximation theory. The transport becomes diffusive, following Ohm's law, when the barrier width is increased beyond 10.3nm. This study provides a novel strain-invariant resistance mechanism in highly conductive cross-linked nanocomposites.

Structural Study of Aqueous Electrolyte Solution by MeV Liquid Electron Scattering.

The impact of ions on water has long been a subject of great interest, as it is closely tied to the hydration structure, dynamics, and properties of electrolyte solutions. Over centuries of investigation, the influence of ions on water's structure remains highly debated. Prevailing techniques, such as neutron and X-ray scattering, primarily focus on the microscopic structure of salt solutions at very high concentrations, mostly above 1 mol/L. In this study, we measured the structure of aqueous potassium iodide (KI) and potassium chloride (KCl) solutions using MeV liquid electron scattering (MeV-LES) across a concentration range of 0.10 to 0.75 mol/L. The obtained results provide detailed insights into the variations in ion-oxygen and oxygen-oxygen correlations as a function of concentration. The observed structural differences between KI and KCl solutions are in line with the structure maker/breaker theory, which suggests that iodide ions exert a more pronounced effect than chloride ions on disrupting the water shell. This work demonstrates the potency of MeV-LES for investigating the atomic structure in liquids, augmenting the modern analytical toolbox.

The Neutron Skin-Thickness of 208Pb Determined by Electron and Proton Scattering

Abstract Electron as well as proton elastic scattering is not able to determine the point proton and point neutron densities, $\rho _\tau (r), (\tau =p,n)$, separately. If both scatterings are analyzed consistently, those densities would be determined uniquely, since the two densities are observed by different combinations from each other. Previous experiments have not provided $\rho _\tau (r)$ uniquely, but the values of the mean square radii of $\rho _p(r)$, $\langle \, r^2\, \rangle _p$, and of $\rho _n(r)$, $\langle \, r^2\, \rangle _n$, are shown to be determined consistently through the fourth moment of the observed charge density, $\langle \, r^4\, \rangle _c$, in 208Pb. The previous analyses of $(\gamma , \pi ^0)$ and $\bar{p}$-nucleus obtained a similar value of $\langle \, r^2\, \rangle _n$, but they do not yield the experimental value of $\langle \, r^4\, \rangle _c$ observed in electron scattering.

Low-Energy Electron Scattering from Ethyl Amine and Propyl Amine: A Comparative Study.

In this study, we investigate the low-energy electron (<20 eV) scattering cross sections for the linear ethyl amine and propyl amine using the R-matrix approach. A theoretical study is conducted, covering various cross sections such as elastic, symmetry-wise elastic, differential, momentum transfer, and electronic excitation. We obtained the ionization cross section using the CSP-ic and BEB methodologies. We unveil the intricate electron-amine interactions within these molecular systems. Additionally, our work extends to a comparative analysis among ethyl amine, propyl amine, and previously studied methyl amine systems. By comparing the obtained results, we discern subtle differences and similarities in the electron scattering behaviors across these structurally related amines. The findings presented herein shed light on fundamental electron-amine interactions, offering valuable insights for diverse fields ranging from chemical kinetics to astrophysics.

Moments of the Charge Distribution Observed through Electron Scattering in 3H and 3He

Abstract The moments of the charge distributions obtained by the sum-of-Gaussians (SOG) analysis of electron-scattering data are examined in $^3$H and $^3$He, together with those obtained by the Fourier–Bessel (FB) analysis. The SOG and FB methods reproduce well the experimental form factors available at present, but provide different charge distributions from each other. As a result, they do not yield the same values of the moments of the charge distribution, although their analyses are called “model-independent.” The moments are sensitive to the tail of the charge distribution. The present experimental data are not enough for SOG and FB analyses to determine with reasonable accuracy the shape of the tails, in a quantum mechanical point of view. New, accurate experimental data at small momentum transfer squared less than 0.1 fm$^{-2}$ are desired.

Elastic Electron Scattering from Be, Mg, and Ca

We present a comprehensive set of theoretical results for differential, integrated, and momentum transfer cross sections for the elastic scattering of electrons by beryllium, magnesium, and calcium at energies below 1 keV. In addition, we provide Sherman function values for elastic electron scattering from calcium in the same energy range. This study extends the application of our method of calculations, already employed for barium and strontium, to all stable alkaline-earth-metal atoms. Our semi-empirical approach to treating target polarization has produced in our earlier work a satisfactory agreement with experimental values and precise theoretical results such as convergent close-coupling calculations for barium. The present data are expected to be of similar high accuracy, based on our previous success in similar calculations for barium and all inert gases.

Elastic and Electronically Inelastic Cross Sections for the Scattering of Electrons by Pyrrole.

Integral and differential cross sections for elastic and electronically inelastic electron scattering from the pyrrole molecule are reported. The cross section calculations employed the Schwinger multichannel method with norm-conserving pseudopotentials. The collision dynamics was described according to a model in which up to 209 energetically accessible channels were treated as open. In the elastic channel, calculations carried out in the interval of energies from 0 to 50 eV revealed the presence of four resonances with peaks located at 2.56 eV (π1*), 3.82 eV (π2*), 4.70 eV (σNH*), and between 8.30 and 9.50 eV (σ*) positions which are in good agreement with previous assignments. Moreover, the role of the multichannel coupling effects in obtaining accurate cross sections was evaluated by comparing the present results with theoretical results recently reported in the literature and early measurements performed for elastic electron collisions with furan. Electronic excitation cross sections involving the transitions from ground state to the 13B2, 13A1, 11A2, and 11A1 excited states of pyrrole driven by electron impact are presented for energies from thresholds up to 50 eV and, whenever possible, critically compared with the data available in the literature.

Improving electrical transport properties of LaxCa0.89-xSr0.11MnO3 films via optimized La content

Optimized LaxCa0.89-xSr0.11MnO3 (x = 0.65, 0.68, 0.71 and 0.74) films were fabricated using spin-coating method. According to double exchange (DE) mechanism and Jahn-Teller effect, the enhancement of peak temperature coefficient of resistivity (TCR) was attributed to low residual resistivity and weak various electron scatterings, including electron–electron, electron–phonon and electron-magnon. Also, peak TCR temperature is not only influenced mainly by the DE mechanism, but also by the Mott transition. Moreover, optimized sintering improved film crystallinity, increasing peak TCR value. The resulting La0.71Ca0.18Sr0.11MnO3 film displayed a peak TCR of 10.74 %/K at 294.11 K. Appropriate chemical composition and sintering promoted the enhancement of electrical transport properties.

Tunable Non-Fermi Liquid Phase from Coupling to Two-Level Systems.

We study a controlled large-N theory of electrons coupled to dynamical two-level systems (TLSs) via spatially random interactions. Such a physical situation arises when electrons scatter off low-energy excitations in a metallic glass, such as a charge or stripe glass. Our theory is governed by a non-Gaussian saddle point, which maps to the celebrated spin-boson model. By tuning the coupling strength we find that the model crosses over from a Fermi liquid at weak coupling to an extended region of non-Fermi liquid behavior at strong coupling, and realizes a marginal Fermi liquid at the crossover. Our results are valid for generic space dimensions d>1.

Electron Scattering from Pyrimidine up to 5 keV

Electron Scattering from Pyrimidine up to 5 keV

Real-time observation of two distinctive non-thermalized hot electron dynamics at MXene/molecule interfaces

The photoinduced non-thermalized hot electrons at an interface play a pivotal role in determining plasmonic driven chemical events. However, understanding non-thermalized electron dynamics, which precedes electron thermalization (~125 fs), remains a grand challenge. Herein, we simultaneously captured the dynamics of both molecules and non-thermalized electrons in the MXene/molecule complexes by femtosecond time-resolved spectroscopy. The real-time observation allows for distinguishing non-thermalized and thermalized electron responses. Differing from the thermalized electron/heat transfer, our results reveal two non-thermalized electron dynamical pathways: (i) the non-thermalized electrons directly transfer to attached molecules at an interface within 50 fs; (ii) the non-thermalized electrons scatter at the interface within 125 fs, inducing adsorbed molecules heating. These two distinctive pathways are dependent on the irradiating wavelength and the energy difference between MXene and adsorbed molecules. This research sheds light on the fundamental mechanism and opens opportunities in photocatalysis and interfacial heat transfer theory.

Ultrafast Electron-Electron Scattering in Metallic Phase of 2H-NbSe_{2} Probed by High Harmonic Generation.

Electron-electron scattering on the order of a few to tens of femtoseconds plays a crucial role in the ultrafast electron dynamics of conventional metals. When mid-infrared light is used for driving and the period of light field is comparable to the scattering time in metals, unique light-driven states and nonlinear optical responses associated with the scattering process are expected to occur. Here, we use high-harmonics spectroscopy to investigate the effect of electron-electron scattering on the electron dynamics in thin film 2H-NbSe_{2} driven by a mid-infrared field. We observed odd-order high harmonics up to 9th order as well as a broadband emission from hot electrons in the energy range from 1.5 to 4.0eV. The electron-electron scattering time in 2H-NbSe_{2} was estimated from the broadband emission to be almost the same as the period of the mid-infrared light field. A comparison between experimental results and a numerical calculation reveals that competition and cooperation between the driving and scattering enhances the nonperturbative behavior of high harmonics in metals, causing a highly nonequilibrium electronic state corresponding to several thousand Kelvin.

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We present a coupled-cluster calculation for the electron-4\\documentclass[12pt]{minimal} \\usepackage{amsmath} \\usepackage{wasysym} \\usepackage{amsfonts} \\usepackage{amssymb} \\usepackage{amsbsy} \\usepackage{mathrsfs} \\usepackage{upgreek} \\setlength{\\oddsidemargin}{-69pt} \\begin{document}$$^4$$\\end{document}He scattering in the region of the quasi-elastic peak. We show the longitudinal and transverse responses separately, and discuss results within two distinct theoretical methods: the Lorentz integral transform and spectral functions. The comparison between them allows to investigate the role of final state interactions, two-body currents and relativistic effects.

Real-Time Ab Initio Investigation on Hot Electron Relaxation Dynamics in Silicon.

The relaxation of hot electrons in semiconductors is pivotal for both energy harvesting processes and optoelectronics. Utilizing a self-developed non-adiabatic molecular dynamics simulation approach in the momentum space (NAMD_k), we have examined the dynamics of hot electrons in silicon. Whether excited from the Γ or L point, the relaxation dynamics exhibit two distinct stages. Initially, within 100 fs, electrons scatter with phonons throughout the Brillouin zone. Subsequently, over a few picoseconds, they further relax toward the conduction band minimum as a whole. This picture of hot electron relaxation is highly consistent with the quasi-equilibrium hot electron ensemble (HEE) concept. Throughout the hot electron relaxation process, energy transfer to phonons is efficient, leading to time-dependent phonon excitation, which is thoroughly analyzed. This investigation provides a novel perspective on hot electron relaxation in silicon, which holds substantive implications for the realm of photovoltaic and optoelectronic device applications.

Compton Scattering of Electrons in the Intergalactic Medium

This paper investigates the distribution and implications of cosmic-ray electrons within the intergalactic medium (IGM). Utilizing a synthesis model of the extragalactic background, we evolve the spectrum of Compton-included cosmic rays. The energy density distribution of cosmic-ray electrons peaks at redshift z ≈ 2, and peaks in the ∼MeV range. The fractional contribution of cosmic-ray pressure to the general IGM pressure progressively increases toward lower redshift. At mean density, the ratio of cosmic-ray electron to thermal pressure in the IGM PCRe/Pth is 0.3% at z = 2, rising to 1.0% at z = 1, and 1.8% at z = 0.1 (considering only the cosmic rays produced locally by Compton scattering). We compute the linear Landau damping rate of plasma oscillations in the IGM caused by the ∼MeV cosmic-ray electrons, and find it to be of order ∼10−6 s−1 for wavenumbers 1.2 ≲ ck/ω p ≲ 5 at z = 2 and mean density (where ω p is the plasma frequency). This strongly affects the fate of TeV e + e − pair beams produced by blazars, which are potentially unstable to oblique instabilities involving plasma oscillations with wavenumber ck/ωp≈secθ (θ being the angle between the beam and wavevector). Linear Landau damping is at least thousands of times faster than either pair beam instability growth or collisional effects; it thus turns off the pair beam instability except for modes with very small θ (ck/ω p → 1, where linear Landau damping is kinematically suppressed). This leaves open the question of whether the pair beam instability is turned off entirely, or can still proceed via the small-θ modes.

Electron Scattering from Stable and Exotic Li Isotopes

The nuclear shell model was used to investigate the bulk properties of lithium isotopes (6,7,8,9,11Li), i.e., the ground state density distributions and C0 and C2 components of charge form factors. The theoretical treatment was based on supposing that the Harmonic-oscillator (HO) potential governs the core nucleons while the valence nucleon(s) move through Hulthen potential. Such assumptions were applied for both stable and exotic lithium isotopes. The HO size parameters ( and ), the core radii ( ) and the attenuation parameters ( and ) were fixed to recreate the available empirical size radii for lithium isotopes under study.

Nonlinear electron scattering by electrostatic waves in collisionless shocks

We present a theoretical analysis of electron pitch-angle scattering by ion-acoustic electrostatic fluctuations present in the Earth's bow shock and, presumably, collisionless shocks in general. We numerically simulate electron interaction with a single wave packet to demonstrate the scattering through phase bunching and phase trapping and quantify electron pitch-angle scattering in dependence on the wave amplitude and wave normal angle to the local magnetic field. The iterative mapping technique is used to model pitch-angle scattering of electrons by a large number of wave packets, which have been reported in the Earth's bow shock. Assuming that successive electron scatterings are not correlated, we revealed that the long-term dynamics of electrons is diffusive. The diffusion coefficient depends on the ratio $\varPhi _0/W$ between the wave packet amplitude and electron energy, $D\propto (\varPhi _0/W)^{\nu }$ . A quasi-linear scaling ( $\nu \approx 2$ ) is observed for sufficiently small wave amplitudes, $\varPhi _0\lesssim 10^{-3}W$ , while the diffusion is nonlinear ( $1&lt;\nu &lt;2$ ) above this threshold. We show that pitch-angle diffusion of ${\lesssim }1$ keV electrons in the Earth's bow shock can be nonlinear. The corresponding diffusion coefficient scales with the intensity $E_{w}^{2}$ of the electrostatic fluctuations in a nonlinear fashion, $D\propto E_{w}^{\nu }$ with $\nu &lt;2$ , while its expected values in the Earth's bow shock are $D\sim 0.1\unicode{x2013}100$ $(T_{e}/W)^{\nu -1/2}\,{\rm rad}^{2}\,{\rm s}^{-1}$ . We speculate that in the Earth's quasi-perpendicular bow shock the stochastic shock drift acceleration mechanism with pitch-angle scattering provided by the electrostatic fluctuations can contribute to the acceleration of thermal electrons up to approximately 1 keV. The potential effects of a finite perpendicular coherence scale of the wave packets on the efficiency of electron scattering are discussed.

Nonresonant Scattering of Energetic Electrons by Electromagnetic Ion Cyclotron Waves: Spacecraft Observations and Theoretical Framework

AbstractElectromagnetic ion cyclotron (EMIC) waves lead to rapid scattering of relativistic electrons in Earth's radiation belts, due to their large amplitudes relative to other waves that interact with electrons of this energy range. A central feature of electron precipitation driven by EMIC waves is deeply elusive. That is, moderate precipitating fluxes at energies below the minimum resonance energy of EMIC waves occur concurrently with strong precipitating fluxes at resonance energies in low‐altitude spacecraft observations. This paper expands on a previously reported solution to this problem: nonresonant scattering due to wave packets. The quasi‐linear diffusion model is generalized to incorporate nonresonant scattering by a generic wave shape. The diffusion rate decays exponentially away from the resonance, where shorter packets lower decay rates and thus widen the energy range of significant scattering. Using realistic EMIC wave packets from δf particle‐in‐cell simulations, test particle simulations are performed to demonstrate that intense, short packets extend the energy of significant scattering well below the minimum resonance energy, consistent with our theoretical prediction. Finally, the calculated precipitating‐to‐trapped flux ratio of relativistic electrons is compared to ELFIN observations, and the wave power spectra is inferred based on the measured flux ratio. We demonstrate that even with a narrow wave spectrum, short EMIC wave packets can provide moderately intense precipitating fluxes well below the minimum resonance energy.

Study of Nuclear Structure and Elastic Electron Scattering Form Factors for Neutron Halo Nuclei (22N ,23O and 24F) Using Full Correlation Functions with Two Size Parameters

The study of neutron-rich nuclei's form factors, root-mean-square radius (rms), and nuclear density distributions is the focus of this work for the nuclei (22N,23 O and 24F). With the use of a strong short-range effect and a strong tensor force, the nucleons distribution function of the two oscillating harmonic particles in a two-frequency shell model operates with two different parameters: the first (bcore), for the inner (core) orbits, and the second (bvalence) for the outer (halo) orbits. This work demonstrated the existence of neutron halo nuclei for the nuclei (22N, 23O and 24F) in the (2s1/2) shell. The computed density distribution of neutron, proton and matter for these nuclei displayed the long tail performance. Using the Borne approximation of the plane wave, the elastic form factor of the electron scattering from the alien nucleus was calculated, this form factor is independent of the neutrons that make up the halo, but rather it results from a difference in the proton density distribution of the last proton in the nuclei. Fortran 95 power station program was used to the neutron, proton and matter density, elastic electron scattering form factor, and rms radii. The calculated outcomes for these exotic nuclei were in good agreement with the experimental data.

Out of field scatter from electron applicator in modern linear accelerators.

Electron out-of-field scatter is generally not given importance mainly in electron fields. However, this is important when applicator down and boost treatments are given usually at an angle from the central axis. The electron scatter dose is found to be far away from the central axis which could be easily ignored. This study aims to investigate the out-of-field radiation doses from electron applicators and their effects on clinical treatment. By identifying the parameters that contribute to out-of-field doses and to explore potential strategies for reducing these doses in order to improve patient outcomes from modern machines. Measurements were performed in water phantom using electron diode for modern Elekta and Varian machines. Dose profiles were acquired at surface and dmax with 0° and 90° collimation angle. Various gantry angles were also studied for some data with IC Profiler. The profiles were normalized with respect to the central axis dose. The scatter dose peaks were found at a distance between 11 and 28cm from the central axis on all machines. However, the peak shifts to 15cm at 90° collimator when beam is tilted. The position and intensity of the dose varies with depth, collimator, and gantry angles for both Elekta and Varian machines. Due to clearance issues more gantry angles were studied for Elekta applicator compared to Varian. In general, Varian TrueBeam has a lower scatter that Elekta Infinity. The 90° collimator angle has a higher scatter compared to zero degree for both machines. There are clinically significant peripheral doses around 3% of the central axis dose from the electron applicator. Elekta has a slightly higher scatter (3%) than Varian (2%) that peaks at 25cm which is clinically important but often overlooked.