Light Propagation Effects Research Articles

Large nonlinear optical magnetoelectric response in a noncentrosymmetric magnetic Weyl semimetal

Weyl semimetals resulting from either inversion (P) or time-reversal (T) symmetry breaking have been revealed to show the record-breaking large optical response due to intense Berry curvature of Weyl-node pairs. Different classes of Weyl semimetals with both P and T symmetry breaking potentially exhibit optical magnetoelectric (ME) responses, which are essentially distinct from the previously observed optical responses in conventional Weyl semimetals, leading to the versatile functions such as directional dependence for light propagation and gyrotropic effects. However, such optical ME phenomena of (semi)metallic systems have remained elusive so far. Here, we show the large nonlinear optical ME response in noncentrosymmetric magnetic Weyl semimetal PrAlGe, in which the polar structural asymmetry and ferromagnetic ordering break P and T symmetry. We observe the giant second harmonic generation (SHG) arising from the P symmetry breaking in the paramagnetic phase, being comparable to the largest SHG response reported in Weyl semimetal TaAs. In the ferromagnetically ordered phase, it is found that interference between this nonmagnetic SHG and the magnetically induced SHG emerging due to both P and T symmetry breaking results in the magnetic field switching of SHG intensity. Furthermore, such an interference effect critically depends on the light-propagating direction. The corresponding magnetically induced nonlinear susceptibility is significantly larger than the prototypical ME material, manifesting the existence of the strong nonlinear dynamical ME coupling. The present findings establish the unique optical functionality of P- and T-symmetry broken ME topological semimetals.

In situ estimation of ice crystal properties at the South Pole using LED calibration data from the IceCube Neutrino Observatory

Abstract. The IceCube Neutrino Observatory instruments about 1 km3 of deep, glacial ice at the geographic South Pole. It uses 5160 photomultipliers to detect Cherenkov light emitted by charged relativistic particles. An unexpected light propagation effect observed by the experiment is an anisotropic attenuation, which is aligned with the local flow direction of the ice. We examine birefringent light propagation through the polycrystalline ice microstructure as a possible explanation for this effect. The predictions of a first-principles model developed for this purpose, in particular curved light trajectories resulting from asymmetric diffusion, provide a qualitatively good match to the main features of the data. This in turn allows us to deduce ice crystal properties. Since the wavelength of the detected light is short compared to the crystal size, these crystal properties include not only the crystal orientation fabric, but also the average crystal size and shape, as a function of depth. By adding small empirical corrections to this first-principles model, a quantitatively accurate description of the optical properties of the IceCube glacial ice is obtained. In this paper, we present the experimental signature of ice optical anisotropy observed in IceCube light-emitting diode (LED) calibration data, the theory and parameterization of the birefringence effect, the fitting procedures of these parameterizations to experimental data, and the inferred crystal properties.

Development of NIR-II small animal living fluorescence imaging system

Fluorescence imaging technology can dynamically monitor gene and cell changing in live animals in real-time, with advantages such as high sensitivity, high resolution, and non-invasion. In recent years, it has been widely used in tumor research, gene expression research, drug development research, etc. The imaging wavelength of traditional fluorescence imaging technology falls in the visible and near-infrared-I region. Due to the absorption and scattering effects of light propagation in biological tissues, and the inherent fluorescence of biological tissues, traditional fluorescence imaging techniques still have significant limitations in penetration depth and image signal-to-noise ratio. In this work, a highly integrated near-infrared-II (NIR-II, 900—1880 nm) small animal living fluorescence imaging system is developed by taking the advantages of NIR-II fluorescence imaging technology, such as low absorption, low scattering, and deep penetration depth in biological tissues. And a method of enhancing and correcting fluorescence image is proposed to optimize fluorescence images. In this work, the biological tissue simulation experiments and live animal experiments are conducted to test the performance and imaging effect of the system. The experimental results show that the system has the advantages of deep penetration depth, high signal-to-noise ratio, and high sensitivity. Combined with commercial indocyanine green reagents and aggregation-induced emission dyes, this system can monitor the distribution of blood vessels in real time and continuously monitor deep tissues and organs in mice, and conduct the dynamically monitoring research in living mice in a conscious state. This helps to promote tumor research and drug development research in the field of biomedical imaging to enter a new stage.

Superradiant Detection of Microscopic Optical Dipolar Interactions.

The interaction between light and cold atoms is a complex phenomenon potentially featuring many-body resonant dipole interactions. A major obstacle toward exploring these quantum resources of the system is macroscopic light propagation effects, which not only limit the available time for the microscopic correlations to locally build up, but also create a directional, superradiant emission background whose variations can overwhelm the microscopic effects. In this Letter, we demonstrate a method to perform "background-free" detection of the microscopic optical dynamics in a laser-cooled atomic ensemble. This is made possible by transiently suppressing the macroscopic optical propagation over a substantial time, before a recall of superradiance that imprints the effect of the accumulated microscopic dynamics onto an efficiently detectable outgoing field. We apply this technique to unveil and precisely characterize a density-dependent, microscopic dipolar dephasing effect that generally limits the lifetime of optical spin-wave order in ensemble-based atom-light interfaces.

Propagation effects in high-harmonic generation from dielectric thin films

A theoretical investigation is conducted of high-order harmonic generation (HHG) in silicon thin films to elucidate the effect of light propagation in reflected and transmitted waves. The first-principles simulations are performed of the process in which an intense pulsed light irradiates silicon thin films up to $3\phantom{\rule{0.28em}{0ex}}\ensuremath{\mu}\mathrm{m}$ thickness. Our simulations are carried within the time-dependent density functional theory (TDDFT) with the account of coupled dynamics of the electromagnetic fields and the electronic motion. It was found that the intensity of transmission HHG gradually decreases with the thickness, while the reflection HHG becomes constant from a certain thickness. Detailed analyses show that transmission HHG has two origins: the HHG generated near the front edge and propagates to the back surface and the HHG generated near the back edge and emitted directly. The dominating mechanism of the transmission HHG is found to depend on the thickness of the thin film and the frequency of the HHG. At the film thickness of $1\phantom{\rule{0.28em}{0ex}}\ensuremath{\mu}\mathrm{m}$, the transmission HHG with the frequency below 20 eV is generated near the back edge, while that with the frequency above 20 eV is generated near the front edge and propagates from there to the back surface.

Securing Data in Multimode Fibers by Exploiting Mode-Dependent Light Propagation Effects.

Multimode fibers hold great promise to advance data rates in optical communications but come with the challenge to compensate for modal crosstalk and mode-dependent losses, resulting in strong distortions. The holographic measurement of the transmission matrix enables not only correcting distortions but also harnessing these effects for creating a confidential data connection between legitimate communication parties, Alice and Bob. The feasibility of this physical-layer-security-based approach is demonstrated experimentally for the first time on a multimode fiber link to which the eavesdropper Eve is physically coupled. Once the proper structured light field is launched at Alice's side, the message can be delivered to Bob, and, simultaneously, the decipherment for an illegitimate wiretapper Eve is destroyed. Within a real communication scenario, we implement wiretap codes and demonstrate confidentiality by quantifying the level of secrecy. Compared to an uncoded data transmission, the amount of securely exchanged data is enhanced by a factor of 538. The complex light transportation phenomena that have long been considered limiting and have restricted the widespread use of multimode fiber are exploited for opening new perspectives on information security in spatial multiplexing communication systems.

Temperature-adaptive hydrogel optical waveguide with soft tissue-affinity for thermal regulated interventional photomedicine

Photomedicine has gained great attention due to its nontoxicity, good selectivity and small trauma. However, owing to the limited penetration of light and difficult monitoring of the photo-media therapies, it is challenging to apply photomedical treatment in deep tissue as they may damage normal tissues. Herein, a thermal regulated interventional photomedicine based on a temperature-adaptive hydrogel fiber-based optical waveguide (THFOW) is proposed, capable of eliminating deeply seated tumor cells while lowering risks of overtemperature (causes the death of healthy cells around the tumor). The THFOW is fabricated by an integrated homogeneous-dynamic-crosslinking-spinning method, and shows a remarkable soft tissue-affinity (low cytotoxicity, swelling stability, and soft tissue-like Young’s modulus). Moreover, the THFOW shows an excellent light propagation property with different wavenumbers (especially −0.32 dB cm−1 with 915 nm laser light), and temperature-gated light propagation effect. The THFOW and relevant therapeutic strategy offer a promising application for intelligent photomedicine in deep issue.

Fast light propagating waveguide composed of heterogeneous metamaterials

A symmetrical three-layer fast light waveguide based on photonic crystal heterostructure is proposed in this article. Two types of photonic crystal where their effective optical parameters such as permittivity and permeability are variable from negative to positive at vicinity of the “Dirac-like” point frequency, are designed. Then the symmetrical three-layer light waveguide composed of these two different photonic crystals (heterogeneous structure at the junction between the cladding and the core) are constructed. By analyzing the anomalous dispersion mode of this waveguide, numerically calculated the group velocity to be negative. The light propagation effect of the waveguide is simulated, and it shows that the waveguide can confine light to the core layer well. In addition, observing the backward moving behavior of the wave packet by incident modulated gaussian pulses envelope, further verifying the generation of fast light. These numerical simulation results agree well the analytical analysis. The proposed waveguide structures in this article may improve the sensitivity of optical instruments and offer potential applications in the fields of integrated photonic circuits, on-chip optical interconnect, and fast optical communication and transmission.

A reaction–diffusion model for grayscale digital light processing 3D printing

Digital light processing (DLP) 3D printing is an additive manufacturing process that utilizes light patterns to photopolymerize a liquid resin into a solid. Due to the accuracy of modern digital micromirror devices (DMD) and recent advances in resin chemistry, it is now possible to create functionally graded structures using different light intensity values, also known as grayscale DLP (g-DLP). Different intensities of light lead to differences in the polymer crosslinking density after curing, which ultimately produces a part with gradients of material properties. However, g-DLP is a complicated process. First, the DLP printing is a highly coupled chemical and physical process that involves light propagation, chemical reactions, species diffusion, heat transfer, volume shrinkage, and changes in mechanical behaviors of the curing resin. Second, in g-DLP, light gradients create strong in plane gradients of chemical species concentrations in the curing liquid resin due to the strong dependence of light intensity on the rate of monomer crosslinking. Furthermore, light gradients through the depth create concentration gradients due to the degree of cure dependent light absorption and the use of photoabsorbers. These complex physical features of the printing process must be understood in order to properly control printing parameters such as light exposure time, printing speed, and grayscale variations to achieve accurate mechanical properties. In this paper, a photopolymerization reaction–diffusion model is developed and used in conjunction with experiments to investigate the coupled effects of light propagation, chemical reaction rates, and species diffusion during g-DLP 3D printing. The model is implemented numerically utilizing the finite difference method and simulation results are compared to experimental findings of simple printed structures. The agreement between experimental and model predictions of simple quantities of interest, such as geometric feature sizes, shows that the model can capture the overcure due to free-radical and other species diffusion during printing when grayscale patterns are employed. This model lays the groundwork for future extensions that can incorporate more complex coupled physics such as heat transfer, volume shrinkage, and material property evolution, which are critically important in utilizing g-DLP 3D printing for the fabrication of high-performance parts which excellent geometric and material property tolerances.

Strong-Field Gravity Tests with the Double Pulsar

Continued observations of the Double Pulsar, PSR J0737-3039A/B, consisting of two radio pulsars (A and B) that orbit each other with a period of 2.45hr in a mildly eccentric (e=0.088) binary system, have led to large improvements in the measurement of relativistic effects in this system. With a 16-yr data span, the results enable precision tests of theories of gravity for strongly self-gravitating bodies and also reveal new relativistic effects that have been expected but are now observed for the first time. These include effects of light propagation in strong gravitational fields which are currently not testable by any other method. We observe retardation and aberrational light-bending that allow determination of the pulsar's spin direction. In total, we have detected seven post-Keplerian (PK) parameters, more than for any other binary pulsar. For some of these effects, the measurement precision is so high that for the first time we have to take higher-order contributions into account. These include contributions of A's effective mass loss (due to spin-down) to the observed orbital period decay, a relativistic deformation of the orbit, and effects of the equation of state of super-dense matter on the observed PK parameters via relativistic spin-orbit coupling. We discuss the implications of our findings, including those for the moment of inertia of neutron stars. We present the currently most precise test of general relativity's (GR's) quadrupolar description of gravitational waves, validating GR's prediction at a level of $1.3 \times 10^{-4}$ (95% conf.). We demonstrate the utility of the Double Pulsar for tests of alternative theories by focusing on two specific examples and discuss some implications for studies of the interstellar medium and models for the formation of the Double Pulsar. Finally, we provide context to other types of related experiments and prospects for the future.

Theory of light propagation in arbitrary two-dimensional curved space

As an analog model of general relativity, optics on some two-dimensional (2D) curved surfaces has received increasing attention in the past decade. Here, in light of the Huygens–Fresnel principle, we propose a theoretical frame to study light propagation along arbitrary geodesics on any 2D curved surfaces. This theory not only enables us to solve the enigma of “infinite intensity” that existed previously at artificial singularities on surfaces of revolution but also makes it possible to study light propagation on arbitrary 2D curved surfaces. Based on this theory, we investigate the effects of light propagation on a typical surface of revolution, Flamm’s paraboloid, as an example, from which one can understand the behavior of light in the curved geometry of Schwarzschild black holes. Our theory provides a convenient and powerful tool for investigations of radiation in curved space.

Effect of the finite speed of light in ionization of extended molecular systems

We study propagation effects due to the finite speed of light in ionization of extended molecular systems. We present a general quantitative theory of these effects and show under which conditions such effects should appear. The finite speed of light propagation effects are encoded in the non-dipole terms of the time-dependent Shrödinger equation and display themselves in the photoelectron momentum distribution projected on the molecular axis. Our numerical modeling for the hbox {H}_{2}^{+} molecular ion and the hbox {Ne}_2 dimer shows that the finite light propagation time from one atomic center to another can be accurately determined in a table top laser experiment which is much more readily accessible than the ground breaking synchrotron measurement by Grundmann et al. (Science 370:339, 2020).

On the minimum thickness of doped electron/hole transport layers in organic semiconductor devices

Doped hole (respectively electron) transport layers [HTLs (respectively ETLs)] are commonly used in evaporated organic devices to achieve high work function hole contact (respectively low work function electron contact) in organic LEDs to inject large current, in solar cells to increase the open circuit voltage, and in photodetectors to minimize the dark current. However, optimization of the HTL thickness results from a delicate trade-off. Indeed, on the one hand, to minimize the impact of HTLs on light propagation and series resistance effects, it is commonly admitted that HTLs must be kept as thin as possible. In this work, a model, validated by drift and diffusion simulations, has shown that, depending of the doping level, a minimum thickness between 10 and 20 nm was needed to prevent the transport layer work function from degradation due to field effects. Experiments have been performed on template p-only devices featuring a single HTL of various thicknesses and doping, confirming the validity of the model. Finally, simulations have been performed on a p-i-n device featuring both HTL and ETL. These results constitute precious indications for the design of efficient evaporated organic LEDs, solar cells, or photodetectors.

Advances in IceCube ice modelling & what to expect from the Upgrade

The IceCube Neutrino Observatory instruments about 1 km3 of deep, glacial ice at the geographic South Pole using 5160 photomultipliers to detect Cherenkov light from relativistic, charged particles. Most IceCube science goals rely on precise understanding and modelling of the optical properties of the instrumented ice. A peculiar light propagation effect observed by IceCube is an anisotropic attenuation, which is aligned with the local flow of the ice. Recent efforts have shown this effect is most likely due to curved photon trajectories resulting from the asymmetric light diffusion in the birefringent polycrystalline microstructure of the ice. This new model can be optimized by adjusting the average orientation, size and shape of the ice crystals. We present the parametrization of the birefringence effect in our photon propagation simulation, the fitting procedures and results. The anticipated potential of calibration instrumentation in the upcoming IceCube Upgrade to improve on known shortcomings of the current ice modelling is also discussed.

Atomic Clocks in Space: A Search for Rubidium and Cesium Masers in M- and L-dwarfs

Abstract I searched for the ground state 6.8 and 9.2 GHz hyperfine transitions of rubidium and cesium toward M- and L-dwarfs that show Rb and Cs optical resonance lines. The optical lines can pump the hyperfine transitions, potentially forming masers. These spin-flip transitions of Rb and Cs are the principal transitions used in atomic clocks (the 133Cs hyperfine transition defines the second). If they are detected in stellar atmospheres, these transitions would provide exceptionally precise clocks that can be used as accelerometers, as exoplanet detectors, as probes of the predictions of general relativity, as probes of light propagation effects, and as a means to do fundamental physics with telescopes. Observations of 21 M- and L-dwarfs, however, show no evidence for Rb or Cs maser action, and a previous survey of giant stars made no Rb maser detections.

Kilonova Emission from Black Hole–Neutron Star Mergers. I. Viewing-angle-dependent Lightcurves

Abstract In this paper, we explore the viewing angle effect on black hole–neutron star (BH–NS) merger kilonova lightcurves. We extrapolate the fitting formulae for the mass and velocity of dynamical ejecta across a wide mass ratio range validated with 66 simulations and use them in kilonova lightcurve calculations. The calculated peak luminosity of a BH–NS merger kilonova is typically about a few times 1041 erg s−1, which is always ≲4.5 × 1041 erg s−1. This corresponds to AB absolute magnitudes fainter than ∼−15 mag in the optical and ∼−16 mag in the infrared. The dynamical ejecta usually contribute to the majority of the kilonova emission, as its projected photosphere area is much larger than that of the disk wind outflows. The fitted blackbody temperature and the observed multiband lightcurve shape are insensitive to the line of sight. The peak time of the observed multiband lightcurves, affected by the light-propagation effect, is related to the relative motion direction between the dynamical ejecta and the observer. The predicted peak luminosity, which changes with the projected photosphere area, only varies by a factor of ∼(2–3) (or by ∼1 mag) for different viewing angles. When taking the short-duration gamma-ray burst afterglow into account, for an on-axis geometry, the kilonova emission is usually outshone by the afterglow emission and can only be observed in the redder bands, especially in the K band at late times. Compared with GW 170817/AT 2017gfo, BH–NS merger kilonovae are optically dim but possibly infrared bright, and have lower fitting temperature at the same epoch after the merger.

Optical Phase Transition in Semiconductor Quantum Metamaterials.

Unexpected light propagation effects, such as negative refraction, have been reported in artificial media. Leveraging on the intersubband resonances in heterostructured semiconductors, we show that all possible optical regimes, ranging from classical dieletric and metal to hyperbolic metamaterial types 1 and 2, can be achieved. As a demonstration, we prove that the negative refraction effect can occur at a designed frequency by controlling the electronic quantum confinement.

All-optical spatio-temporal control of electron emission from SiO2 nanospheres with femtosecond two-color laser fields

Field localization by nanostructures illuminated with laser pulses of well-defined waveform enables spatio-temporal tailoring of the near-fields for sub-cycle control of electron dynamics at the nanoscale. Here, we apply intense linearly-polarized two-color laser pulses for all-optical control of the highest energy electron emission from SiO2 nanoparticles. For the size regime where light propagation effects become important, we demonstrate the possibility to control the preferential emission angle of a considerable fraction of the fastest electrons by varying the relative phase of the two-color field. Trajectory based semi-classical simulations show that for the investigated nanoparticle size range the directional steering can be attributed to the two-color effect on the electron trajectories, while the accompanied modification of the spatial distribution of the ionization rate on the nanoparticle surface has only a minor effect.

Moiré tomography for the diagnoses of flow fields with consideration of ray propagation

Abstract Moire tomography has been considered as powerful diagnostic tool to flow fields with advantages of noncontact, compact optical structure, strong anti-vibration capability and large dynamic range. However, the refractive index reconstructions in the existing moire tomography are based on the straight ray assumption, by which the light propagation effects caused by the inhomogeneities of flow fields are not taken into account. In this paper, a spatial-domain filtered back-propagation (FBPP) algorithm for moire tomography is studied from the wave equation in inhomogeneous media. Three advancements can be achieved by the algorithm: (1) the weak scattering effect caused by the inhomogeneities of flow field is considered; (2) the first-order derivative of the projected phase measured by moire deflectometry can be directly employed to quantitatively reconstruct the refractive index; (3) the reconstruction is calculated in pure spatial domain, which can reduce the errors resulted by the conversions in frequency domain in the conventional FBPP algorithm. The feasibility and accuracy of the algorithm is checked by numerical simulations. Finally, the refractive index of an axisymmetric propane-air premixed flame is measured by moire tomography with the proposed reconstruction algorithm and the temperature distribution is deduced.

PT-symmetric system based optical modulator

This paper introduces a novel approach based on linear parity-time (PT) symmetry for realization of an optical modulator. The suggested optical modulator is attained by embedding PT-symmetric couplers within the arms of a Mach–Zehnder interferometer configuration. The asymmetric evolution behavior of light propagation and interference effect play the key role in the proposed PT-symmetric based modulator. The extinction ratio of the proposed modulator is as high as 56.97 dB. Moreover, it is shown that the normalized light intensity of the modulator output exponentially varies by increasing the gain/loss coefficients. Finally, it is demonstrated that just by an active arm (the gain waveguide) of the PT-symmetric coupler, a similar evolution of the light propagation can be achieved along the modulator structure.