E-skin Devices Research Articles

Micropatterned elastic ionic polyacrylamide hydrogel for low-voltage capacitive and organic thin-film transistor pressure sensors

Electronic skins (E-skins) have attracted great research interest because of their promising applications in stretchable optoelectronics, soft robotics, and personalized healthcare devices. However, it remains a great challenge to fabricate E-skin devices that meet strict practical requirements such as high sensitivity, low-power operation and noise-proof ability. Here, we developed a novel elastic ionic polyacrylamide hydrogel (EIPH) with a high capacitance for the development of low-voltage organic thin-film transistor (OTFT) pressure sensors. The EIPH was prepared by photopolymerization of an acrylamide monomer in an aqueous solution of poly (acrylic acid) and CaCl2 and was then in situ micropatterned on an indium-tin oxide electrode. The fabricated capacitive sensor with 10-µm-wide EIPH micropillar structures achieved a high sensitivity of 2.33 kPa−1 with a capacitance sensitivity of 103.8 nF/kPa. This capacitance sensitivity is more than 100 times higher than that of conventional capacitive pressure sensors due to the formation of an electrical double layer. The micropatterned EIPH was adopted as a dielectric layer in the fabrication of the OTFT-based pressure sensors. Such an EIPH-based OTFT pressure sensor not only greatly enhanced the sensitivity, i.e., 7.7 times higher than its capacitive counterparts, but also largely reduced the operation voltage to 2 V.

Tough and Water-Insensitive Self-Healing Elastomer for Robust Electronic Skin.

An electronic (e-) skin is expected to experience significant wear and tear over time. Therefore, self-healing stretchable materials that are simultaneously soft and with high fracture energy, that is high tolerance of damage or small cracks without propagating, are essential requirements for the realization of robust e-skin. However, previously reported elastomers and especially self-healing polymers are mostly viscoelastic and lack high mechanical toughness. Here, a new class of polymeric material crosslinked through rationally designed multistrength hydrogen bonding interactions is reported. The resultant supramolecular network in polymer film realizes exceptional mechanical properties such as notch-insensitive high stretchability (1200%), high toughness of 12 000 J m-2 , and autonomous self-healing even in artificial sweat. The tough self-healing materials enable the wafer-scale fabrication of robust and stretchable self-healing e-skin devices, which will provide new directions for future soft robotics and skin prosthetics.

A Triple-Mode Flexible E-Skin Sensor Interface for Multi-Purpose Wearable Applications.

This study presents a flexible wireless electronic skin (e-skin) sensor system that includes a multi-functional sensor device, a triple-mode reconfigurable readout integrated circuit (ROIC), and a mobile monitoring interface. The e-skin device’s multi-functionality is achieved by an interlocked micro-dome array structure that uses a polyvinylidene fluoride and reduced graphene oxide (PVDF/RGO) composite material that is inspired by the structure and functions of the human fingertip. For multi-functional implementation, the proposed triple-mode ROIC is reconfigured to support piezoelectric, piezoresistance, and pyroelectric interfaces through single-type e-skin sensor devices. A flexible system prototype was developed and experimentally verified to provide various wireless wearable sensing functions—including pulse wave, voice, chewing/swallowing, breathing, knee movements, and temperature—while their real-time sensed data are displayed on a smartphone.

A Dual-Organic-Transistor-Based Tactile-Perception System with Signal-Processing Functionality.

Organic-device-based tactile-perception systems can open up new opportunities for the next generation of intelligent products. To meet the critical requirements of artificial perception systems, the efficient construction of organic smart elements with integrated sensing and signal processing functionalities is highly desired, but remains a challenge. This study presents a dual-organic-transistor-based tactile-perception element (DOT-TPE) with biomimetic functionality by the construction of organic synaptic transistors with integrated sensing transistors. The unique geometry of the DOT-TPE permits instantaneous sensing of pressure stimuli and synapse-like processing of an electric signal in a single element. More importantly, these organic-transistor-based tactile-perception elements can be built into arrays to serve as bionic tactile-perception systems. The combined biomimetic functionality of tactile-perception systems, together with their promising features of flexibility and large-area fabrication, makes this work represent a step forward toward novel e-skin devices for artificial intelligence.

Fabrication of graphene/free-standing nanofibrillar PEDOT/P(VDF-HFP) hybrid device for wearable and sensitive electronic skin application

In this work, we describe a simple method for the fabrication of a new class of graphene/free-standing nanofibrillar PEDOT/P(VDF-HFP) nanohybrid E-skin device. This E-skin exhibits enhanced contact surface area and piezo-resistivity with an extremely high gauge factor (320) under tensile strain, which combine to yield very high sensitivity to pressure (limit of detection=0.5Pa). Signals from even very weak motion, such as changes in facial expression and the pulse in the wrist, can be detected. Furthermore, this E-skin is sufficiently durable and reproducible. The E-skin device does not exhibit measurable changes in performance or observable signs of physical deterioration, even after over 1000 strain cycles, and is wearable and sufficiently biocompatible to be placed inside clothing or against human skin without causing irritation.

Silk‐Molded Flexible, Ultrasensitive, and Highly Stable Electronic Skin for Monitoring Human Physiological Signals

Flexible and transparent E-skin devices are achieved by combining silk-molded micro-patterned polydimethylsiloxane (PDMS) with single-walled carbon nanotube (SWNT) ultrathin films. The E-skin sensing device demonstrates superior sensitivity, a very low detectable pressure limit, a fast response time, and a high stability for the detection of superslight pressures, which may broaden their potential use as cost-effective wearable electronics for healthcare applications.