Dynamics Of Impurity Research Articles

Markovian to non-Markovian phase transition in the operator dynamics of a mobile impurity

We study a random unitary circuit model of an impurity moving through a chaotic medium. The exchange of information between the medium and impurity is controlled by varying the velocity of the impurity, v_dvd, relative to the speed of information propagation within the medium, v_BvB. Above supersonic velocities, v_d> v_Bvd>vB, information cannot flow back to the impurity after it has moved into the medium, and the resulting dynamics are Markovian. Below supersonic velocities, v_d< v_Bvd<vB, the dynamics of the impurity and medium are non-Markovian, and information is able to flow back onto the impurity. We show the two regimes are separated by a continuous phase transition with exponents directly related to the diffusive spreading of operators in the medium. This is demonstrated by monitoring an out-of-time-order correlator (OTOC) in a scenario where the impurity is substituted at an intermediate time. During the Markovian phase, information from the medium cannot transfer onto the replaced impurity, manifesting in no significant operator development. Conversely, in the non-Markovian phase, we observe that operators acquire support on the newly introduced impurity. We also characterize the dynamics using the coherent information and provide two decoders which can efficiently probe the transition between Markovian and non-Markovian information flow. Our work demonstrates that Markovian and non-Markovian dynamics can be separated by a phase transition, and we propose an efficient protocol for observing this transition.

Lattice dynamics of 119Sn impurity in a bcc-Cr crystal

The chromium crystal doped with119Sn isotope was studied using the nuclear resonance inelastic x-ray scattering and first principles calculations. The Sn partial phonon density of states (PDOS) was obtained for three temperatures that correspond to different magnetic states of Cr. At all temperatures, the energy spectrum consists of a broad band around 18 meV and a narrow peak at 43 meV. The additional peak around 39 meV is observed only in the magnetically ordered phases, indicating the influence of magnetic order in chromium on lattice dynamics. The partial PDOS calculated with the antiferromagnetic order on Cr atoms show a very good agreement with the experimental data. It is revealed that the high-energy peak is lying above the phonon spectra of the pure bcc-Cr crystal. These are the local modes with the increased energies due to a strongly reduced distance between Sn and the nearest-neighbor Cr atoms.

Slow dynamics of a mobile impurity interacting with an Anderson insulator

We investigate dynamics of a single mobile impurity immersed in a bath of Anderson localized particles and focus on the regime of relatively strong disorder and interactions. In that regime, the dynamics of the system is particularly slow, suggesting, at short times, an occurrence of many-body localization. Considering longer time scales, we show that the latter is a transient effect and that, eventually, the impurity spreads sub-diffusively and induces a gradual delocalization of the Anderson insulator. The phenomenology of the system in the considered regime of slow dynamics includes a sub-diffusive growth of mean square displacement of the impurity, power-law decay of density correlation functions of the Anderson insulator and a power-law growth of entanglement entropy in the system. We observe a similar regime of slow dynamics also when the disorder in the system is replaced by a sufficiently strong quasi-periodic potential.

Dynamical formation of two-fold fragmented many-body state induced by an impurity in a double-well

We unravel the correlated quantum quench dynamics of a single impurity immersed in a bosonic environment confined in an one-dimensional double-well potential. A particular emphasis is placed on the structure of the time-evolved many-body (MB) wave function by relying on a Schmidt decomposition whose coefficients directly quantify the number of configurations that are macroscopically populated. For a non-interacting bosonic bath and weak postquench impurity-bath interactions, we observe the dynamical formation of a two-fold fragmented MB state which is related to intra-band excitation processes of the impurity and manifests as a two-body phase separation (clustering) between the two species for repulsive (attractive) interactions. Increasing the postquench impurity-bath coupling strength leads to the destruction of the two-fold fragmentation since the impurity undergoes additional inter-band excitation dynamics. By contrast, a weakly interacting bath suppresses excitations of the bath particles and consequently the system attains a weakly fragmented MB state. Our results explicate the interplay of intra- and inter-band impurity excitations for the dynamical generation of fragmented MB states in multi-well traps and for designing specific entangled impurity states.

A single ion immersed in an ultracold gas: from cold chemistry to impurity physics

A single ion in an ultracold gas is a versatile experimental platform to study interactions between charged and neutral particles in a controllable manner. When the gas density is large enough, a single ion can be viewed as an impurity in a sea of ultracold atoms or molecules. On the other hand, that single ion can also undergo a chemical reaction with atoms or molecules in the gas. This article discusses the dynamics of a charged impurity in an ultracold bath and the interplay between cold chemistry and impurity physics.

Interaction between an Impurity and Nonlinear Excitations in a Polariton Condensate.

Exploring the dynamics of a mobile impurity immersed in field excitations is challenging, as it requires to account for the entanglement between the impurity and the surrounding excitations. To this end, the impurity's effective mass has to be considered as finite, rather than infinite. Here, we theoretically investigate the interaction between a finite-mass impurity and a dissipative soliton representing nonlinear excitations in the polariton Bose-Einstein condensate (BEC). Using the Lagrange variational method and the open-dissipative Gross-Pitaevskii equation, we analytically derive the interaction phase diagram between the impurity and a dissipative bright soliton in the polariton BEC. Depending on the impurity mass, we find the dissipative soliton colliding with the impurity can transmit through, get trapped, or be reflected. This work opens a new perspective in understanding the impurity dynamics when immersed in field excitations, as well as potential applications in information processing with polariton solitons.

Quench dynamics of the Anderson impurity model at finite temperature using matrix product states: entanglement and bath dynamics

We study the dynamics of the quenched Anderson model at finite temperature using matrix product states (MPSs). Exploiting a chain mapping for the electron bath, we investigate the entanglement structure in the MPS for various orderings of the two chains, which emerge from the thermofield transformation employed to deal with nonzero temperature. We show that merging both chains can significantly lower the entanglement at finite temperatures as compared to an intuitive nearest-neighbor implementation of the Hamiltonian. Analyzing the population of the free bath modes—possible when simulating the full dynamics of impurity plus bath—we find clear signatures of the Kondo effect in the quench dynamics.

МОНИТОРИНГ СОДЕРЖАНИЯ СОРТОВОЙ ПРИМЕСИ В ПИТОМНИКАХ ПЕРВИЧНОГО И ЭЛИТНОГО СЕМЕНОВОДСТВА ЛЬНА-ДОЛГУНЦА

The most common reason for varietal impurities of long-stalked type in the crops of fiber flax is non-compliance with the basic requirements of internal control when working with several flax varieties on the farm or when carrying out a variety change. During field testing, the identification of biological impurity of the intermediate type is not completely carried out due to the unevenness of the crops. Due to morphological similarity of fiber flax varieties, it is impossible to determine the percentage of mechanical variety impurities of the long-stalked type. The aim of the research is to study the reproduction dynamics of variety impurity of K-7009 long- stalked form of flax, which has a yellow color of seeds, in the seeds of fiber flax contaminated with it after 6-year sowing. The aim is also to clarify the parameter of variety purity of fiber flax seeds of the following categories: genuine seeds (GS) and elite seeds (ES) in State Standard GOST R 52325-2005. The research was carried out in 2015-2020 in the field conditions of the Experimental field of the Federal State Budgetary Scientific Institution "Federal Scientific Center of Bast Cultures" in Tver region. The objects of the study were plants and seeds of Antey fiber flax variety (control). The usage of variety admixture of the long-stalked flax form with a marker trait made it possible to accurately determine its content in the crop in case of seed multiplication in nurseries of primary seed growing, superelite (GS) and elite (ES). It was found that variety contamination of fiber flax seeds with variety admixture in the amount of 0.2-1.0% did not affect the yield of seeds and straw. As a result of five-year reproduction of seeds in the crops of GS category, an increase in the amount of variety impurity was noted by 0.1-1.3%, in the ES category - by 0.3-2.1% compared to initial contamination. Based on the obtained experimental data, it was recommended to reduce variety purity index for the category of genuine fiber flax seeds in State Standard GOST R 52325-2005 to 99.5%, elite - to 90%.

Transient dynamics of a magnetic impurity coupled to superconducting electrodes: Exact numerics versus perturbation theory

Impurities coupled to superconductors offer a controlled platform to understand the interplay between superconductivity, many-body interactions, and nonequilibrium physics. In the equilibrium situation, local interactions at the impurity induce a transition from the spin-singlet to the spin-doublet ground state, resulting in a supercurrent sign reversal ($0\text{\ensuremath{-}}\ensuremath{\pi}$ transition). In this work, we apply the exact time-dependent density matrix renormalization group method to simulate the transient dynamics of such superconducting systems. We also use a perturbative approximation to analyze their properties at longer times. These two methods agree for a wide range of parameters. In a phase-biased situation, the system gets trapped in a metastable state characterized by a lower supercurrent compared to the equilibrium case. We show that local Coulomb interactions do not provide an effective relaxation mechanism for the initially trapped quasiparticles. In contrast, other relaxation mechanisms, such as coupling to a third normal lead, make the impurity spin relax for parameter values corresponding to the equilibrium 0 phase. For parameters corresponding to the equilibrium $\ensuremath{\pi}$ phase the impurity converges to a spin-polarized stationary state. Similar qualitative behavior is found for a voltage-biased junction, which provides an effective relaxation mechanism for the trapped quasiparticles in the junction.

Dynamical Quantum Cherenkov Transition of Fast Impurities in Quantum Liquids.

The challenge of understanding the dynamics of a mobile impurity in an interacting quantum many-body medium comes from the necessity of including entanglement between the impurity and excited states of the environment in a wide range of energy scales. In this Letter, we investigate the motion of a finite mass impurity injected into a three-dimensional quantum Bose fluid as it starts shedding Bogoliubov excitations. We uncover a transition in the dynamics as the impurity's velocity crosses a critical value that depends on the strength of the interaction between the impurity and bosons as well as the impurity's recoil energy. We find that in injection experiments, the two regimes differ not only in the character of the impurity velocity abatement but also exhibit qualitative differences in the Loschmidt echo, density ripples excited in the Bose-Einstein condensate, and momentum distribution of scattered bosonic particles. The transition is a manifestation of a dynamical quantum Cherenkov effect and should be experimentally observable with ultracold atoms using Ramsey interferometry, rf spectroscopy, absorption imaging, and time-of-flight imaging.

Stochastic-field approach to the quench dynamics of the one-dimensional Bose polaron

We consider the dynamics of a quantum impurity after a sudden interaction quench into a one-dimensional degenerate Bose gas. We use the Keldysh path integral formalism to derive a truncated Wigner like approach that takes the back action of the impurity onto the condensate into account already on the mean-field level and further incorporates thermal and quantum effects up to one-loop accuracy. This framework enables us not only to calculate the real space trajectory of the impurity but also the absorption spectrum. We find that quantum corrections and thermal effects play a crucial role for the impurity momentum at weak to intermediate impurity-bath couplings.Furthermore, we see the broadening of the absorption spectrum with increasing temperature.

Dynamics of spin-polarized impurity in ultracold Fermi gas

We show that the motion of spin-polarized impurity (ferron) in ultracold atomic gas is characterized by a certain critical velocity which can be traced back to the amount of spin imbalance inside the impurity. We have calculated the effective mass of ferron in two dimensions. We show that the effective mass scales with the surface of the ferron. We discuss the impact of these findings; in particular, we demonstrate that ferrons become unstable in the vicinity of a vortex.

Dynamical torque from Shiba states ins-wave superconductors

Magnetic impurities inserted in a $s$-wave superconductor give rise to spin-polarized in-gap states called Shiba states. We study the back-action of these induced states on the dynamics of the classical moments. We show that the Shiba state pertains to both reactive and dissipative torques acting on the precessing classical spin that can be detected through ferromagnetic resonance measurements. Moreover, we highlight the influence of the bulk states as well as the effect of the finite linewidth of the Shiba state on the magnetization dynamics. Finally, we demonstrate that the torques are a direct measure of the even and odd frequency triplet pairings generated by the dynamics of the magnetic impurity. Our approach offers non-invasive alternative to the STM techniques used to probe the Shiba states.

Impurity dephasing in a Bose–Hubbard model

We study the dynamics of a two-level impurity embedded in a two-dimensional Bose–Hubbard (BH) model at zero temperature from an open quantum system perspective. Results for the decoherence across the whole phase diagram are presented, with a focus on the critical region close to the transition between superfluid and Mott insulator. In particular we show how the decoherence and the deviation from a Markovian behaviour are sensitive to whether the transition is crossed at commensurate or incommensurate densities. The role of the spectrum of the BH environment and its non-Gaussian statistics, beyond the standard independent boson model, is highlighted. Our analysis resorts on a recently developed method (2020 Phys. Rev. Res. 2 033276) – closely related to slave boson approaches – that enables us to capture the correlations across the whole phase diagram. This semi-analytical method provides us with a deep insight into the physics of the spin decoherence in the superfluid and Mott phases as well as close to the phase transitions.

Non-equilibrium quantum dynamics and formation of the Bose polaron

Advancing our understanding of non-equilibrium phenomena in quantum many-body systems remains one of the greatest challenges in physics. Here we report on the experimental observation of a paradigmatic many-body problem, namely the non-equilibrium dynamics of a quantum impurity immersed in a bosonic environment1,2. We use an interferometric technique to prepare coherent superposition states of atoms in a Bose–Einstein condensate with a small impurity-state component, and monitor the evolution of such quantum superpositions into polaronic quasiparticles. These results offer a systematic picture of polaron formation3–7 from weak to strong impurity interactions. They reveal three distinct regimes of evolution with dynamical transitions that provide a link between few-body processes and many-body dynamics. Our measurements reveal universal dynamical behaviour in interacting many-body systems and demonstrate new pathways to study non-equilibrium quantum phenomena. Quantum impurities immersed in a bosonic environment can evolve into polaronic quasiparticles, so-called polarons. Interferometric measurement reveals this transition, which involves three different regimes dominated by few-body and many-body dynamics.

System of models for assessment and forecast of heat- and mass-transfer in the system “catchment-watercourse-water body”

Development of a system of models describing the processes of heat and mass transfer in the system “catchment - watercourse – reservoir” enabling the assessment of impact of economic activity and climate change on the state of water bodies. The layout of a water system model using the developed and working models of processes is performed in accordance with the determining factors: the requirements of the task; structural features of the research object; the presence and location of points of the observation network as a source of initial information for modeling. The developed system of models includes six deterministic models and one stochastic one. The deterministic models include the model of water runoff from the catchment ILHM, model of chemicals removal from the catchment ILLM, model of water flow, sediment transport and dissolved impurities in an open channel (1D, 2D, 3D), 1D model of thermal regime and mixing of reservoir FLake, 1D model of dynamics of non-conservative impurity in reservoir FLakeEco, 2D model of currents and sediment transport in shallow reservoir, 3D model of heat and mass transfer in reservoir. The stochastic component of the system is the SWM weather model, which is a stochastic generator of meteorological elements.

Transport of a Single Cold Ion Immersed in a Bose-Einstein Condensate.

We investigate transport dynamics of a single low-energy ionic impurity in a Bose-Einstein condensate. The impurity is implanted into the condensate starting from a single Rydberg excitation, which is ionized by a sequence of fast electric field pulses aiming to minimize the ion's initial kinetic energy. Using a small electric bias field, we study the subsequent collisional dynamics of the impurity subject to an external force. The fast ion-atom collision rate, stemming from the dense degenerate host gas and the large ion-atom scattering cross section, allow us to study a regime of frequent collisions of the impurity within only tens of microseconds. Comparison of our measurements with stochastic trajectory simulations based on sequential Langevin collisions indicate diffusive transport properties of the impurity and allows us to measure its mobility. Our results open a novel path to study dynamics of charged quantum impurities in ultracold matter.

Dynamics of impurity in the environment of Dirac fermions

We study the dynamics of a nonmagnetic impurity interacting with the surface states of a 3D and 2D topological insulator (TI). Employing the linked cluster technique we develop a formalism for obtaining the Green’s function of the mobile impurity interacting with the low-energy Dirac fermions. We show that for the non-recoil case in 2D, the Green’s function in the long-time limit has a power-law decay in time implying the breakdown of the quasiparticle description of the impurity. The spectral function in turn exhibits a weak power-law singularity. In the recoil case, however, the reduced phase-space for scattering processes implies a non-zero quasiparticle weight and the presence of a coherent part in the spectral function. Performing a weak coupling analysis we find that the mobility of the impurity reveals a T−3/2 divergence at low temperatures. In addition, we show that the Green’s function of an impurity interacting with the helical edge modes (surface states of 2D TI) exhibit power-law decay in the long-time limit for both the non-recoil and recoil case (with low impurity momentum), indicating the break down of the quasiparticle picture. However, for impurity with high momentum, the quasiparticle picture is restored. The mobility of the heavy impurity interacting with the helical edge modes exhibits unusual behaviour. It has an exponential divergence at low temperatures which can be tuned to a power-law divergence, T−4, by the application of the magnetic field.

Quantum Rydberg Central Spin Model.

We consider dynamics of a Rydberg impurity in a cloud of ultracold bosonic atoms in which the Rydberg electron undergoes spin-changing collisions with surrounding atoms. This system realizes a new type of quantum impurity problems that compounds essential features of the Kondo model, the Bose polaron, and the central spin model. To capture the interplay of the Rydberg-electron spin dynamics and the orbital motion of atoms, we employ a new variational method that combines an impurity-decoupling transformation with a Gaussian ansatz for the bath particles. We find several unexpected features of this model that are not present in traditional impurity problems, including interaction-induced renormalization of the absorption spectrum that eludes simple explanations from molecular bound states, and long-lasting oscillations of the Rydberg-electron spin. We discuss generalizations of our analysis to other systems in atomic physics and quantum chemistry, where an electron excitation of high orbital quantum number interacts with a spinful quantum bath.

Dynamics of a mobile impurity in a two-leg bosonic ladder

We have analyzed the behavior of a mobile quantum impurity in a bath formed by a two-leg bosonic ladder by a combination of field theory (Tomonaga-Luttinger liquid) and numerical (Density Matrix Renormalization Group) techniques. Computing the Green's function of the impurity as a function of time at different momenta, we find a power law decay at zero momentum, which signals the breakdown of any quasi-particle description of the impurity motion. We compute the exponent both for the limits of weak and strong impurity-bath interactions. At small impurity-bath interaction, we find that the impurity experiences the ladder as a single channel one-dimensional bath, but effective coupling is reduced by a factor of $\sqrt 2$, thus the impurity is less mobile in the ladder compared to a one dimensional bath. We compared the numerical results for the exponent at zero momentum with a semi-analytical expression that was initially established for the chain and find excellent agreement without adjustable parameters. We analyze the dependence of the exponent in the transverse hopping in the bath and find surprisingly an increase of the exponent at variance with the naive extrapolation of the single channel regime. We study the momentum dependence of the impurity Green's function and find that, as for the single chain, two different regime of motion exist, one dominated by infrared metatrophy and a more conventional polaronic behavior. We compute the critical momentum between these two regimes and compare with prediction based on the structure factor of the bath. In the polaronic regime we also compute numerically the lifetime of the polaron. Finally we discuss how our results could be measured in cold atomic experiments.