Solid Lubricant Research Articles

Design, optimization, and verification of self‐lubricating ceramic tool microstructure by MC method

AbstractThe computer‐aided analysis of microstructure evolution during the sintering process of self‐lubricating ceramic tools can unveil the underlying sintering mechanism and optimize experimental parameters. In this study, a novel self‐lubricating ceramic tool material, Al2O3/SiC/h‐BN@Al2O3, was fabricated with Al2O3 as the matrix, SiC as the reinforcement phase, and h‐BN@Al2O3 as the solid lubricant. The Monte Carlo (MC) method was employed to construct a model of self‐lubricating ceramic tool material, consisting of Al2O3/SiC/h‐BN@Al2O3. Subsequently, the sintering process was analyzed to investigate the influence of particle size and content of reinforced SiC, as well as the content of coated solid lubricant h‐BN@Al2O3, sintering pressure, and temperature on the microstructure of the tool. Optimal composition and sintering parameters were determined: 3 vol% for SiC additive amount with a particle size of 0.05 μm; 5 vol% for h‐BN@Al2O3 additive amount; and an optimal sintering temperature at 1650°C. The development of self‐lubricating ceramic tool materials, Al2O3/SiC/h‐BN@Al2O3, was realized through the employment of the aforementioned parameters. Their mechanical properties and microstructure were comprehensively characterized. The bending strength, fracture toughness, and Vickers hardness of the experimentally‐prepared Al2O3/3 vol%SiC/5 vol%h‐BN@Al2O3 self‐lubricating ceramic tool material were determined to be 722.42 MPa, 6.5 MPa·m1/2, and 20.65 GPa, respectively.

Modeling and Optimization of Turning Hastelloy C-276 under Sustainable Machining Environments

Due to their numerous applications in the aerospace, chemical, and nuclear power industries, environmentally responsible superalloy machining is a major problem in the current production environment. Additionally, Ni-based superalloys are regarded as difficult to manufacture because of their great strength under hot and chemically reactive settings. Therefore, it is necessary to machine these materials using adequate cooling and lubricating solutions. Current study has been based on the optimisation and modelling of turning Hastelloy C-276 under dry, flood, and least lubrication system. A Taguchi L-9 arrangement was used as plan of experiment and modeling was enabled through ANOVA, regression analysis and Taguchi optimization. The results depicted optimal parameters for surface roughness and temperature at v2-f1-d1-CE3 and v1-f2-d1-CE3. Likewise, for CRC and shear angle the best combination was observed at v3-f3-d2-CE2. From ANOVA analysis, the benefaction of C.E, depth of cut and feed rate on S.R been listed as 46.70%, 40.44% and 10.66%. Likewise, for temperature cutting speed has benefaction of (53.09%), cooling environment (23.94%), depth of cut (6.10%) and feed rate 5.49% . In similar fashion, CRC and Shear angle were influenced by feed rate and cutting speed having contribution of 62.89% and 5.15% respectively. Furthermore, minimum standard error between the fitted and observed values for S.R., temperature, CRC, and shear angle were calculated as 0.0149, 7.66, 0.267, and 1.80 units. Finally, the marginal reduction of cutting temperature and surface roughness through utilization of MQL implies the sustainable machining conditions.

Stiffening of double-shelled fullerene molecules under uniaxial strains

Onion-like fullerenes (OLFs) have spherical and tunable shell structures that make them perfect solid lubricants, but their molecular mechanical properties are largely unknown as they are extremely difficult to measure. In this computational study, double-shelled OLFs C60@C180, C80@C180, C60@C240 and C80@C240 are subject to uniaxial elastic strains to obtain their mechanical response. Compressive and tensile elastic moduli are calculated using density functional theory with van der Waals correction. We found that the tensile elastic moduli of the single- and double-shelled fullerenes are always larger than the compressive ones by about 50% to 100%. Inserting C80 into C180 causes an increase in compressive elastic modulus from 96.8 GPa to 178.6 GPa, while inserting C60 into C240 cause much smaller increases. The key factor that determines the stiffening effects is the relative sizes of the inner and outer shells.

Tribological behavior and mechanism of Mo2Ti2C3/polyimide composite films under dry friction condition

AbstractPolyimide (PI) has good mechanical properties and thermal stability, while high coefficient (COF) and wear rate limit its wide application. In order to endow PI with better friction and wear resistance, Mo2Ti2C3 MXene was used as solid lubricant to prepare Mo2Ti2C3/PI nanocomposites with different content of Mo2Ti2C3. The effect of the amount of Mo2Ti2C3 on the tribological behavior of PI was explored and the tribological mechanism was also analyzed Tribological tests showed that at 1.2 wt% of Mo2Ti2C3 addition, the composite material demonstrated superior friction and wear resistance, exhibiting a 19.9% decrease in the COF and a 79.7% decrease in the wear rate compared to single PI due to the good self‐lubricating properties of Mo2Ti2C3 MXene. Moreover, Mo2Ti2C3 can also effectively assist PI to form sleek transfer films without interruption or gaps on the steel balls, resulting in a reduced friction COF and wear rate of the material. This work demonstrates that Mo2Ti2C3 MXene is an aussichtsreich additive for polymers to improve the tribological properties and broadens the applications of Mo2Ti2C3/PI composites in friction material area.Highlights Mo2Ti2C3 significantly improves the tribological performance of polyimide. The thermal properties of Mo2Ti2C3/polyimide are enhanced by the introduction of Mo2Ti2C3. The minimum coefficient of Mo2Ti2C3/PI composites was only 0.246 at the 1.2 wt% content of Mo2Ti2C3. The wear rate of Mo2Ti2C3/PI composites was decreased by 79.7% at the 1.2 wt% addition of Mo2Ti2C3. Mo2Ti2C3 promotes the establishment of tribo‐film to protect the Mo2Ti2C3/PI composites from friction.

Combining Carbon Nanoparticle Coatings and Laser Surface Texturing for Enhanced Lubricity Under High Loads

Developing new lubrication concepts greatly contributes to improving the energy efficiency of mechanical systems. Nanoparticles such as those based on carbon allotropes or 2D materials have received widespread attention due to their outstanding mechanical and tribological performance. However, these systems are limited by a short wear life. Combining nanoparticle coatings with laser surface texturing has been demonstrated to substantially improve their durability due to the reservoir effect which prevents immediate particle removal from the contact. In this study, we investigate the high-load (20 N) tribological performance of AISI 304 austenitic stainless-steel substrates, which are line-patterned by laser interference patterning and subsequently coated with different carbon nanoparticle coatings (carbon nanotubes, carbon onions, carbon nanohorns) against alumina and 100Cr6 counter bodies. In addition to that, benchmark testing is performed with conventional solid lubricant coatings (graphite, MoS2, WS2). Electrophoretic deposition is used as the main coating technique along with air spraying (for WS2). All coatings substantially improve friction compared to the purely laser-patterned reference. Among all coating materials, carbon nanotubes demonstrate superior lubricity and the longest wear life against 100Cr6 and alumina counter bodies. Detailed characterization of the resulting wear tracks by energy-dispersive X-ray spectroscopy, scanning electron microscopy, and confocal laser scanning microscopy provides insights into the friction mechanisms of the various solid lubricant particles. Further, material transfer is identified as an important aspect for effective and long-lasting lubrication.

Solid lubrication performance of Ti2CTx coatings with reduced friction and extended durability

MXene research in tribology has predominantly focused on Ti3C2Tx, overlooking the untapped potential of other promising MXenes with equally intriguing properties. Thus, to enhance tribological reliability in industrial applications, Ti2CTx coatings were applied to 316 stainless steel as a solid lubricant. Using a linear ball-on-disk tribometer under 460 MPa pressure, we found that Ti2CTx coatings reduced friction by 82% and wear rate by 70% compared to uncoated steel. Advanced characterizations showed that this improved tribology is linked to nanostructured carbon-rich protective tribofilms resulting from the contact pressure-induced graphitization of Ti2CTx MXenes sheets. Our research comprehensively elucidates the tribological effectiveness of multi-layer Ti2CTx, which is pivotal to design advanced lubricants for contemporary mechanical applications.

Synergistic lubrication effects of Sn–Ag–Cu and MXene–Ti3C2 to improve tribological properties of M50 bearing steel with microporous channels

Purpose This paper aims to study the synergistic lubrication effects of Sn–Ag–Cu and MXene–Ti3C2 to improve the tribological properties of M50 bearing steel with microporous channels. Design/methodology/approach M50 matrix self-lubricating composites (MMSC) were designed and prepared by filling Sn–Ag–Cu and MXene–Ti3C2 in the microporous channels of M50 bearing steel. The tribology performance testing of as-prepared samples was executed with a multifunction tribometer. The optimum hole size and lubricant content, as well as self-lubricating mechanism of MMSC, were studied. Findings The tribological properties of MMSC are strongly dependent on the synergistic lubrication effect of MXene–Ti3C2 and Sn–Ag–Cu. When the hole size of microchannel is 1 mm and the content of MXene–Ti3C2 in mixed lubricant is 4 wt.%, MMSC shows the lowest friction coefficient and wear rate. The Sn–Ag–Cu and MXene–Ti3C2 are extruded from the microporous channels and spread to the friction interface, and a relatively complete lubricating film is formed at the friction interface. Meanwhile, the synergistic lubrication of Sn–Ag–Cu and MXene–Ti3C2 can improve the stability of the lubricating film, thus the excellent tribological property of MMSC is obtained. Originality/value The results help in deep understanding of the synergistic lubrication effects of Sn–Ag–Cu and MXene–Ti3C2 on the tribological properties of M50 bearing steel. This work also provides a useful reference for the tribological design of mechanical components by combining surface texture with solid lubrication. Peer review The peer review history for this article is available at: https://publons.com/publon/10.1108/ILT-12-2023-0381/

Carbon nanotubes used to enhance the wear properties of AlSi10Mg/CNTs nanocomposites prepared through additive manufacturing

In this work, varying weight percentages of carbon nanotubes (CNTs) were reinforced in the AlSi10Mg alloy, and prepared nanocomposites through additive manufacturing. The distribution of CNTs in the metal matrix were achieved through functionalization and ball milling. The dispersion of CNTs were investigated through FESEM, TEM, and Raman spectroscopy. To study the wear properties, the prepared samples underwent wear tests at various loads and speeds. The wear properties, worn surfaces, and microhardness were thoroughly investigated. The results unveiled that the incorporation of CNTs led to a decrease in the wear rate and a reduction in the coefficient of friction. It was observed that CNTs functioned as a solid lubricant, resulting in a significant reduction in both the coefficient of friction and wear rate. The microstructures of the worn surfaces and wear channels became smaller and smoother after the addition of CNTs, and smaller-sized debris was produced.

Electrodeposited MoxSyOz/Ni Tribological Coatings.

Deposition of molybdenum disulfide (MoS2) coatings using physical vapor deposition (PVD) and mechanical burnishing has been widely assessed for solid lubricants in space applications but still suffers from line-of-sight constraints on complex geometries. Here, we highlight one of the first demonstrations of electrodeposited MoxSyOz and MoxSyOz/Ni thin-film coatings from aqueous solutions of ammonium tetrathiomolybdate for solid lubricant applications and their remarkable ability to provide low coefficients of friction and high wear resistance. Characterization of the coating morphology shows amorphous microstructures with a high oxygen content and cracking upon drying. Even so, electrodeposited MoxSyOz can achieve low steady-state coefficients of friction (μ ∼ 0.05-0.06) and wear rates (2.6 × 10-7 mm3/(N m)) approaching those of physical vapor deposited coatings (2.3 × 10-7 mm3/(N m)). Additionally, we show that adding dopants such as nickel increased the wear rate (7.5 × 10-7 mm3/(N m)) and initial coefficient of friction (μi = 0.23) due to compositional modifications such as dramatic sub-stoichiometry (S/Mo ∼ 1) and expression of a NiOx surface layer, although doping did reduce the degree of cracking upon drying.

Tribological performance and composition optimization of semi-metallic friction materials applied for carbon ceramic brake disc

The tribological performance of C/C–SiC paired semi-metallic brake pads suitable for automobiles was investigated in this study. Factors on tribological properties of semi-metallic brake pads such as the contents of phenolic resin, copper fibers, steel fibers and MoS2 were tested by the orthogonal experimental. According to the SAE-J2522 test procedure, an optimized compositional formulation was derived based on the brake test results combined with fuzzy comprehensive evaluation. The wear mechanism of brake pairs was discussed, and the compositional formulation of the brake pad was further optimized after the analysis of the friction surface morphology before and after braking. The results showed that copper fibers had the greatest effect on the friction performance of brake pads. Copper fibers contributed to stabilization of the coefficient of friction (COF) and effectively improved the wear resistance. However, at higher braking speeds (≥120 km/h), the copper fibers were converted from fibrous to flaky and softened, acting as a solid lubricant on the friction surface, resulting in a low COF of brake pads. The tribological performance of brake pads could be improved by reducing the content of copper fiber and increasing the content of hard particles.

Influence of GNPs solid lubricant on the fabrication of Cu/SS304L composite micro channels

The different solution-processed concentrations of graphene solid lubricant (0 – 30 mg/mL) were applied on the surface of copper/stainless steel 304 L composite foils. A variable trend of rolling force occurs, with a first falling and then rising trend and the lowest rolling force was obtained at 25 mg/mL for 3.82 kN. Besides, the height of ridges and aspect ratio were improved with an increased solution-processed concentration. On the valley surfaces, the GNPs filled up the cracks, flattened the grooves and eliminated the micro scratches. This indicates the self-repairing and self-polishing mechanisms of GNPs in the micro rolling process. The sliding and exfoliation of GNPs also contributed to the reduced roughness and improved quality of the sample surfaces.

Highly Interfacial Active Gemini Surfactants as Simple and Versatile Emulsifiers for Stabilizing, Lubricating and Structuring Liquids

AbstractTo date, locking the shape of liquids into non‐equilibrium states usually relies on jamming nanoparticle surfactants at an oil/water interface. Here we show that a synthetic water‐soluble zwitterionic Gemini surfactant can serve as an alternative to nanoparticle surfactants for stabilizing, structuring and additionally lubricating liquids. By having a high binding energy comparable to amphiphilic nanoparticles at the paraffin oil/water interface, the surfactant can attain near‐zero interfacial tensions and ultrahigh surface coverages after spontaneous adsorption. Owing to the strong association between neighboring surfactant molecules, closely packed monolayers with high mechanical elasticity can be generated at the oil/water interface, thus allowing the surfactant to produce not only ultra‐stable emulsions but also structured liquids with various geometries by using extrusion printing and 3D printing techniques. By undergoing tribochemical reactions at its sulfonic terminus, the surfactant can endow the resultant emulsions with favorable lubricity even under high load‐bearing conditions. Our study may provide new insights into creating complex liquid devices and new‐generation lubricants capable of combining the characteristics of both liquid and solid lubricants.

Highly Interfacial Active Gemini Surfactants as Simple and Versatile Emulsifiers for Stabilizing, Lubricating and Structuring Liquids.

To date, locking the shape of liquids into non-equilibrium states usually relies on jamming nanoparticle surfactants at an oil/water interface. Here we show that a synthetic water-soluble zwitterionic Gemini surfactant can serve as an alternative to nanoparticle surfactants for stabilizing, structuring and additionally lubricating liquids. By having a high binding energy comparable to amphiphilic nanoparticles at the paraffin oil/water interface, the surfactant can attain near-zero interfacial tensions and ultrahigh surface coverages after spontaneous adsorption. Owing to the strong association between neighboring surfactant molecules, closely packed monolayers with high mechanical elasticity can be generated at the oil/water interface, thus allowing the surfactant to produce not only ultra-stable emulsions but also structured liquids with various geometries by using extrusion printing and 3D printing techniques. By undergoing tribochemical reactions at its sulfonic terminus, the surfactant can endow the resultant emulsions with favorable lubricity even under high load-bearing conditions. Our study may provide new insights into creating complex liquid devices and new-generation lubricants capable of combining the characteristics of both liquid and solid lubricants.

Design of ternary solid lubricants SiO2/Ti3C2/PTFE for wear-resistant, self-lubricating polyimide composites

BackgroundPolyimide is widely used in aerospace, electronics and electrical appliances, automotive, chemical and other fields due to its high temperature stability, excellent mechanical properties. However, polymer materials are often subjected to severe wear and tear under complex operating conditions due to their poor lubrication performance. Therefore, the improvement of lubrication performance is a key strategy to extend the service life of polyimide. MethodsHerein, a ternary solid lubricant SiO2/Ti3C2/PTFE (STP) is innovatively prepared by solution dispersion for reducing the friction of polyimide to increase the lubricity. Specifically, SiO2 and PTFE are intercalated accordion-like Ti3C2 nanosheets, thereby causing the nanosheets to slide relative to each other under external frictional stress. Then, STP was introduced into polyimide to prepare the ultra-wear-resistant and self-lubricating composites by blending. Significant findingsThe results of the study showed that the STP significantly enhanced the lubrication properties of the composites, the lowest coefficient of friction (0.29) of the composites is 22.81 % lower than that of the polyimide. In addition, the inclusion of hybrids helps to form a transfer film, which effectively improves the abrasion performance of polyimide, and the lowest wear rate (0.18 × 10−5 mm3/(N·m)) was 93.35 % lower than that of polyimide.

Recycling Automotive Plastic Waste: Residual Polyvinyl Butyral (rPVB) as Solid Lubricant in Polyoxymethylene (POM) Blends

Polyoxymethylene (POM) is an engineering thermoplastic commonly used in tribological applications due to its low friction and auto-lubrication properties. To improve its performance further and broaden its applications to higher sliding speeds and loads, it is commonly reinforced with different particles, fibers, or solid lubricants. In this study, the effect of adding residual polyvinyl butyral (rPVB) from automotive windshields production lines on the tribological performance of POM during pin-on-disk wear tests at different loads (12, 15, and 18 N) and sliding speeds (0.25, 0.50, and 0.75 m/s) is investigated. It was found that rPVB acts as a solid lubricant, reducing the coefficient of friction (CoF) up to 50%. It is suggested that the formation of a protective layer of adhered material on the wear track is the mechanism behind CoF reduction. Melt flow index, Shore D hardness and elastic properties decrease linearly with rPVB content. However, the reduction in tensile strength, and thus shear strength of the blends, seems to be more significant on their CoF behavior than the reduction in hardness. No trend was found for wear resistance. Under certain sliding conditions rPVB decreased volume loss, but in other cases it increased it. It is suggested that, for the conditions analyzed in this study, adding 10 wt% of rPVB to a POM matrix results in the best balance of tribological performance, with an overall CoF reduction of 36%, and an average volume loss increase of only 1%.

Large‐Scale Numerical Simulation of the Solid Lubricant Behavior in the Leg Joints of Insects

AbstractSemi‐solid lubricant in the leg joints of insects is represented by tiny cylindrical fragments. The dynamics of lubricant behavior between contact surfaces at the joint scale are investigated using numerical simulation. Results of modeling show that lubricant fragments tend to stick together and form clots of varying shapes and sizes under the influence of shear motion. Formation of such clots, accompanied by constant loss and reproduction of the lubricant, allows maintaining of fluctuating clearance between contact surfaces and helps to reduce friction. Foreign contaminant particles penetrating an open insect joint are removed by the lubricant, to which they stick, reducing abrasive wear.

Understanding the effect of solid lubricants on scratch behavior in epoxy resins: An experimental and statistical approach

AbstractEpoxy resins inherently have low resistance to scratching. To increase the scratch resistance of epoxy resins, reinforcing solid lubricants into the resin is an option. For this purpose, in this study, polytetrafluoroethylene (PTFE) and graphite were reinforced in two different epoxy resins (rigid and toughened) at different reinforcement ratios (5, 10, and 15 wt%). The effects of solid lubricant reinforcement on the scratch behavior of rigid and toughened epoxy resins were examined both experimentally and statistically. Scratch tests were performed throughout a distance of 10 mm using a test apparatus under a load of 15 N and a scratch speed of 30 mm/min. Following the scratch tests, the COF (Coefficient of Friction) values, scratch hardness, scratch width, and depth of all samples were determined and compared to neat epoxy for each resin. In general, it has been determined that solid lubricant reinforcement at higher reinforcement ratios has a positive effect on the COF value (15 wt%). In the case of 15 wt% graphite reinforced rigid and toughened epoxy, a decrease of 15.90% and 17.77%, respectively, was obtained in the COF value compared to the neat epoxy. After the scratch tests, statistical analysis was performed according to RSM to support the experimental results, and ANOVA tables were obtained.Highlights Epoxy adhesives exhibit low scratch resistance. Examining the impact of PTFE and graphite reinforcement on scratch behavior. Two types of epoxy and varied reinforcement ratios (5, 10, and 15 wt%) were studied. Solid lubricant reinforcement to epoxy positively affected scratch behavior.

STUDY ON MECHANICAL PROPERTIES OF DEVELOPED ECO-FRIENDLY BRAKE PADS USING GRAY RELATIONAL ANALYSIS IN BOX BEHNKEN DESIGN OF EXPERIMENT

Over the years, asbestos has been a leading material for developing automobile brake pads. However, due to its hazardous nature to human health, many researchers have found that organic materials possess the potential for replacement. The organic materials used in this research were the hybrid of coconut fruit fibre CFF and oyster sea shell OSS. These materials were gathered from the river bank, dried, crushed, washed, ground, sieved, and moulded with different additives: CuO (abrasive), graphite (friction modifier or solid Lubricant), epoxy resin (binder), hardener (catalyst) by Box Behnken design BBD of L27 experiment. Therefore, an experimental test on mechanical properties was performed to check the developed brake pad's characterization. Then, grey relational analysis was used to analyze grey relational grade GRG to convert a multiple response process optimization problem into a single response optimization using maximization of maximum GRG. The optimum parameter values producing the highest value of grey relational grade were chosen as rank one, pertained to the factors setup for experiment number S3232 having moulding pressure of 11.25MPa, moulding temperature of 180oC, and heat treatment time of 180min. The optimized response values obtained from the experiment sample S3232 give the highest values on all the responses, i.e., density of 3.483g/cm3, hardness of 52.91BHN, compressive strength of 2.78MPa, ultimate tensile strength of 3.92MPa, impact energy of 17.87N, cold water absorption of 0.2863%, hot water absorption of 0.4785%, and oil absorption of 0.4402%. After that, the optimized brake pad sample (S3232) was applied to the automobile and was suitable for braking owing to its high mechanical properties.

Enhancing oil pressure dynamics in a high-performance racing engine with innovative lubrication system tuning

This work focuses on fine-tuning the oil pressure dynamics of a single-seater formula car, a participant in international engineering competition organized by the Society of Automotive Engineers (SAE). Adhering to competition guidelines, the Honda CBR600RR 05-06® motorcycle engine, renowned for its 600 c.c. displacement and exceptional power-to-weight ratio, emerges as a popular choice. However, as this engine is originally equipped with a wet sump lubrication system (featuring deep wet sumps to prevent oil starvation during turns), this presents challenges when adapted to Formula Society of Automotive Engineers (FSAE) cars. Cornering leads to significant pressure drops, as sloshing exposes the pickup port, causing consequential engine issues. To tackle sloshing-related challenges and pressure loss during lateral and longitudinal g-forces, a dry sump lubrication system was introduced in the Formula car. The dry sump system also lowers the engine’s center of gravity, by reducing sump height. However, transitioning to the dry sump system and integrating it with the existing engine demanded extensive design modifications to various components, including the oil reservoir, lubrication lines, scavenging pump, and oil ports. These adjustments were essential to achieve the targeted elevation in oil pressures at higher engine RPMs. A relationship between the engine oil pressure and the engine RPM was developed as part of the study.

Comparison of conventional hydrothermal and microwave‐assisted synthesized g‐C3N4/MoS2 nanocomposite coated steel substrate by tribological measurement

AbstractMolybdenum disulfide is an effective solid lubricant, but it suffers from oxidation and moisture absorption issues, resulting in insufficient wear resistance and a shortened lifespan. This study introduces an innovative approach, integrating graphitic carbon nitride with molybdenum disulfide via advanced microwave‐assisted synthesis, offering precise control over synthesis parameters. The research assesses the tribological performance, comparing it with conventional hydrothermal synthesis. The study extensively investigates the morphology, microstructure, and tribology of a g‐C3N4/MoS2 nanocomposite created through novel microwave (g‐C3N4/MoS2‐MW) and hydrothermal techniques (g‐C3N4/MoS2‐HT). MoS2 exhibits a flower‐like structure, while graphitic carbon nitride has a layered structure, as confirmed by elemental analysis via energy‐dispersive X‐ray spectroscopy. X‐ray diffraction identifies g‐C3N4 peaks at 13.0° (100) and 27.5° (002) and hexagonal MoS2 peaks at 14° (002), 32.7° (100), 35.8° (102), and 58.3° (110). The Fourier‐transform infrared spectrum reveals peaks at 1237.4 and 808 cm−1 (aromatic and triazine ring breathing modes in g‐C3N4), 1407.1 and 1638.9 cm−1 (C=N and C−C heterocyclic structures), and 3432 cm−1 (vibrations due to −NH and −OH). The coefficients of friction for microwave‐assisted and traditional hydrothermal synthesized nanocomposites are 0.22 and 0.34, respectively. The wear depths are 98 microns and 141 microns, with a wear scar diameter of 2.87 mm for g‐C3N4/MoS2‐MW and 3.45 mm for g‐C3N4/MoS2‐HT, indicating superior lubrication with the microwave‐assisted coating.