Driven Quantum Dot Research Articles

On-Demand Single Photons with High Extraction Efficiency and Near-Unity Indistinguishability from a Resonantly Driven Quantum Dot in a Micropillar.

Scalable photonic quantum technologies require on-demand single-photon sources with simultaneously high levels of purity, indistinguishability, and efficiency. These key features, however, have only been demonstrated separately in previous experiments. Here, by s-shell pulsed resonant excitation of a Purcell-enhanced quantum dot-micropillar system, we deterministically generate resonance fluorescence single photons which, at π pulse excitation, have an extraction efficiency of 66%, single-photon purity of 99.1%, and photon indistinguishability of 98.5%. Such a single-photon source for the first time combines the features of high efficiency and near-perfect levels of purity and indistinguishabilty, and thus opens the way to multiphoton experiments with semiconductor quantum dots.

Sub-Poissonian phonon statistics in an acoustical resonator coupled to a pumped two-level emitter

The concept of an acoustical analog of the optical laser has been developed recently both in theoretical as well as experimental works. We discuss here a model of a coherent phonon generator with a direct signature of quantum properties of the sound vibrations. The considered setup is made of a laser driven quantum dot (QD) embedded in an acoustical nanocavity. The system's dynamics is solved for a single phonon mode in the steady-state and in the strong QD-phonon coupling regime beyond the secular approximation. We demonstrate that the phonon statistics exhibits quantum features, i.e. sub-Poissonian phonon statistics.

A Pulsed Nonclassical Light Source Driven by an Integrated Electrically Triggered Quantum Dot Microlaser

We present a novel compact nanophotonic device consisting of a nonclassical light source excited by a monolithically integrated and electrically driven quantum dot (QD) microlaser. Our device concept is based on self-assembled InAs QDs embedded in micropillar cavities and has many potential applications in the fields of quantum communication and quantum optics-based information processing. Electrically driven micropillars act as whispering gallery mode microlasers operable in both continuous and pulsed mode, with narrow pulse widths of 520 ps and decay constants as low as 160 ps observed. These microlasers are used as on-chip excitation sources to laterally excite individual QDs in nearby micropillars, which in turn act as vertically emitting nonclassical light sources. Our compact solid-state platform utilizes cavity-quantum electrodynamic effects to create antibunched light in continuous and pulsed operation with g (2)CW(0) = 0.76 ± 0.03 and g (2)Pulsed(0) = 0.78 ± 0.11, demonstrating its potential for the generation of triggered single photons in a highly integrated chip.

Behavior of Kinesin Driven Quantum Dots Trapped in a Microtubule Loop.

We report the observation of kinesin driven quantum dots (QDs) trapped in a microtubule loop, allowing the investigation of moving QDs for a long time and an unprecedented long distance. The QD conjugates did not depart from our observational field of view, enabling the tracking of specific conjugates for more than 5 min. The unusually long run length and the periodicity caused by the loop track allow comparing and studying the trajectory of the kinesin driven QDs for more than 2 full laps, i.e., about 70 μm, enabling a statistical analysis of interactions of the same kinesin driven object with the same obstacle. The trajectories were extracted and analyzed from kymographs with a newly developed algorithm. Despite dispersion, several repetitive trajectory patterns can be identified. A method evaluating the similarity is introduced allowing a quantitative comparison between the trajectories. The velocity variations appear strongly correlated to the presence of obstacles. We discuss the reasons making this long continuous travel distances on the loop track possible.

Floquet Majorana fermions in superconducting quantum dots

We consider different configurations of ac driven quantum dots coupled to superconductor leads where Majorana fermions can exist as collective quasiparticles. The main goal is to tune the existence, localization and properties of these zero energy quasiparticles by means of periodically driven external gates. In particular, we analyze the relevance of the system and driving symmetry. We predict the existence of different sweet spots with Floquet Majorana fermions in configurations where they are not present in the undriven system.

Scattering of two-dimensional Dirac fermions on gate-defined oscillating quantum dots

Within an effective Dirac-Weyl theory we solve the scattering problem for massless chiral fermions impinging on a cylindrical time-dependent potential barrier. The set-up we consider can be used to model the electron propagation in a monolayer of graphene with harmonically driven quantum dots. For static small-sized quantum dots scattering resonances enable particle confinement and interference effects may switch forward scattering on and off. An oscillating dot may cause inelastic scattering by excitation of states with energies shifted by integer multiples of the oscillation frequency, which significantly modifies the scattering characteristics of static dots. Exemplarily the scattering efficiency of a potential barrier with zero bias remains finite in the limit of low particle energies and small potential amplitudes. For an oscillating quantum dot with finite bias, the partial wave resonances at higher energies are smeared out for small frequencies or large oscillation amplitudes, thereby dissolving the quasi-bound states at the quantum dot.

Detuning-dependent narrowing of Mollow triplet lines of driven quantum dots

We study the two-time correlation function and the resonance fluorescence spectrum of a semi-conductor quantum dot excited by a strong off-resonant laser pulse. The obtained analytic expressions exhibit a specific detuning-dependent damping of Rabi oscillations of the dressed quantum dot as well as a detuning-dependent width of Mollow triplet lines. In the absence of pure dephasing, the central peak of the triplet is broadened upon increasing detuning, but the blue- and red-side peaks are narrowed. We demonstrate that the pure dephasing processes can invert these dependences. A crossover between the regimes of detuning-dependent narrowing and broadening of the side and central peaks is identified. The predicted effects are consistent with recent experimental results and numerical calculations.

Free space quantum key distribution over 500 meters using electrically driven quantum dot single-photon sources—a proof of principle experiment

Highly efficient single-photon sources (SPS) can increase the secure key rate of quantum key distribution (QKD) systems compared to conventional attenuated laser systems. Here we report on a free space QKD test using an electrically driven quantum dot single-photon source (QD SPS) that does not require a separate laser setup for optical pumping and thus allows for a simple and compact SPS QKD system. We describe its implementation in our 500 m free space QKD system in downtown Munich. Emulating a BB84 protocol operating at a repetition rate of 125 MHz, we could achieve sifted key rates of 5–17 kHz with error ratios of 6–9% and -values of 0.39–0.76.

Comment on “From fast light to slow light in resonantly driven quantum dot systems” [Opt. Commun. 298–299 (2013) 176–179

We show that the results and conclusions of the paper “From fast light to slow light in resonantly driven quantum dot systems” [Opt. Commun. 298–299 (2013) 176–179] are incorrect.

Phonon-mediated squeezing of the cavity field off-resonantly coupled with a coherently driven quantum dot

We theoretically propose a scheme for the quadrature squeezing of the cavity field via dissipative processes. The effects of the electron-phonon interaction (EPI) on the squeezing are investigated, where the cavity is off-resonantly coupled with a coherently driven quantum dot (QD) which is allowed to interact with an acoustic-phonon reservoir. Under certain conditions, the participation of the phonon induced by both the EPI and the off-resonant coupling of the cavity with the QD enables some dissipative processes to occur resonantly in the dressed-state basis of the QD. The cavity-mode photons emitted or absorbed during the phonon-mediated dissipative processes are correlated, thus leading to the squeezing of the cavity field. A squeezed vacuum reservoir for the cavity field is built up due to the EPI plus the off-resonant coupling between the cavity and the QD. The numerical results obtained with an effective polaron master equation derived using second-order perturbation theory indicate that, in low temperature limit, the degree of squeezing is maximal but the increasing temperature of the phonon reservoir could hinder the squeezing and degrade the degree of the squeezing of the cavity field. In addition, the presence of the photonic crystal could enhance the quadrature squeezing of the cavity field.

Complex band structure eigenvalue method adapted to Floquet systems: topological superconducting wires as a case study

For systems that can be modeled as a single-particle lattice extended along a privileged direction, such as, for example, quantum wires, the so-called eigenvalue method provides full information about the propagating and evanescent modes as a function of energy. This complex band structure method can be applied either to lattices consisting of an infinite succession of interconnected layers described by the same local Hamiltonian or to superlattices: systems in which the spatial periodicity involves more than one layer. Here, for time-dependent systems subject to a periodic driving, we present an adapted version of the superlattice scheme capable of obtaining the Floquet states and the Floquet quasienergy spectrum. Within this scheme the time periodicity is treated as existing along a spatial dimension added to the original system. The solutions at a single energy for the enlarged artificial system provide the solutions of the original Floquet problem. The method is suited for arbitrary periodic excitations, including strong and anharmonic drivings. We illustrate the capabilities of the methods for both time-independent and time-dependent systems by discussing: (a) topological superconductors in multimode quantum wires with spin–orbit interaction and (b) microwave driven quantum dots in contact with a topological superconductor.

Proposal for an on-demand source of polarized electrons into the edges of a topological insulator

We propose a device that allows for the emission of pairs of spin-polarized electrons into the edge-states of a two dimensional topological insulator. Charge and spin emission is achieved using a periodically driven quantum dot weakly coupled to the edge states of the host topological insulator. We present calculations of the emitted time-dependent charge and spin currents of such a dynamical scatterer using the Floquet scattering matrix approach. Experimental signatures of spin-polarized two-particle emission can be found in noise measurements. Here a new form of noise suppression, named $\mathbb{Z}_2$--antibunching, is introduced. Additionally, we propose a set-up in which entanglement of the emitted electrons is generated. This entanglement is based on a post-selection procedure and becomes manifest in a violation of a Clauser-Horne-Shimony-Holt inequality.

Dynamical Steady States in Driven Quantum Systems

We derive dynamical equations for a driven, dissipative quantum system in which the environment-induced relaxation rate is comparable to the Rabi frequency, avoiding assumptions on the frequency dependence of the environmental coupling. When the environmental coupling varies significantly on the scale of the Rabi frequency, secular or rotating wave approximations break down. We avoid these approximations, yielding dynamical steady states which account for the interaction between driven quantum dots and their phonon environment. The theory, which is motivated by recent experimental observations, qualitatively and quantitatively describes the transition from asymmetric unsaturated resonances at weak driving to population inversion at strong driving.

Mode selection in electrically driven quantum dot microring cavities

Within this paper a novel method for selecting certain lasing modes from a whispering gallery mode (WGM) spectrum of electrically pumped microrings is presented. Selection is achieved by introducing sub-wavelength sized notches of about 50 nm width and 500 nm depth to the sidewalls of ring shaped quantum dot micro cavities with 80 µm diameter and ridge widths below 2 µm. It is shown that the notches act as scattering centers, suppressing modes that have maxima in intensity at the notch position. By a variation of the angle between the notches, different repetitive patterns of lasing modes and suppressed modes are conceivable.

Model of the Optical Emission of a Driven Semiconductor Quantum Dot: Phonon-Enhanced Coherent Scattering and Off-Resonant Sideband Narrowing

We study the crucial role played by the solid-state environment in determining the photon emission characteristics of a driven quantum dot. For resonant driving, we predict a phonon enhancement of the coherently emitted radiation field with increasing driving strength, in stark contrast to the conventional expectation of a rapidly decreasing fraction of coherent emission with stronger driving. This surprising behavior results from thermalization of the dot with respect to the phonon bath and leads to a nonstandard regime of resonance fluorescence in which significant coherent scattering and the Mollow triplet coexist. Off resonance, we show that despite the phonon influence, narrowing of dot spectral sideband widths can occur in certain regimes, consistent with an experimental trend.

Accessing quantum nanoplasmonics in a hybrid quantum dot–metal nanosystem: Mollow triplet of a quantum dot near a metal nanoparticle

We present a theoretical study of the resonance fluorescence spectra of an optically driven quantum dot placed near a single metal nanoparticle. The metallic reservoir coupling is calculated for an 8-nm metal nanoparticle using a time-convolutionless master equation approach where the exact photon reservoir function is included using Green function theory. By exciting the system coherently near the nanoparticle dipole mode, we show that the driven Mollow spectrum becomes highly asymmetric due to internal coupling effects with higher-order plasmons. We also highlight regimes of resonance squeezing and broadening as well as spectral reshaping through light propagation. Our master equation technique can be applied to any arbitrary material system, including lossy inhomogeneous structures, where mode expansion techniques are known to break down.

Effects of pre-determined lateral separation on quantum dot size and dissolution

Placing quantum dots in precise arrays provides a unique environment in which to study the effects of surface energy driven quantum dot dissolution occurring during capping, which is difficult to study using randomly assembled dots. Quantum dot photoluminescence emission energy is shown to initially decrease with increasing pattern spacing, but then increases for separations greater than 1.0 μm. The shift in photoluminescence emission results from a competition between the effects of dot size and those of dissolution on the dot emission energy. These data also demonstrate the difference in the diffusion length of In on InAs and on GaAs.

Proposed robust and high-fidelity preparation of excitons and biexcitons in semiconductor quantum dots making active use of phonons.

It is demonstrated how the exciton and the biexciton state of a quantum dot can be prepared with high fidelity on a picosecond time scale by driving the dot with a strong laser pulse that is tuned above the exciton resonance for exciton preparation and in resonance with the exciton transition for biexciton preparation. The proposed protocols make use of the phonon-induced relaxation towards photon dressed states in optically driven quantum dots and combine the simplicity of traditional Rabi oscillation schemes with the robustness of adiabatic rapid passage schemes. Our protocols allow for an on-demand, fast, and almost perfect state preparation even at strong carrier-phonon interaction where other schemes fail. In fact, the performance of the presented protocols is shown to be better the stronger the carrier-phonon interaction is.

From fast light to slow light in resonantly driven quantum dot systems

In this article, we study the resonantly driven quantum dot systems. Based on the density matrix approach, we theoretically investigate the absorption and refractive index near the quantum dot resonance energy. We find that the systems show fast light effect at smaller incident light intensity due to the first order absorption, and show slow light effect at larger incident light intensity due to the third order absorption. It can be tuned by the incident light intensity, and be interpreted in terms of absorption saturation. It operates under normal environmental conditions and at telecommunication wavelengths, and may really be applied.

Electrically driven quantum dot single-photon source at 2 GHz excitation repetition rate with ultra-low emission time jitter

The influence of the bias voltage on emission properties of a red emitting InP/GaInP quantum dot based single-photon source was investigated. Under pulsed electrical excitation, we can influence the band bending of the p-i-n diode with the applied bias voltage and thus the charge carrier escape by quantum tunneling. This leads to control over the non-radiative decay channel and allows carrier escape times as low as 40 ps, effectively reducing the time jitter of the photon emission. We realized high excitation repetition rates of up to 2 GHz while autocorrelation measurements with g(2)(0)-values of 0.27 attest dominant single-photon emission.