Dissipative Phase Transition Research Articles

Probing a Dissipative Phase Transition via Dynamical Optical Hysteresis.

We experimentally explore the dynamical optical hysteresis of a semiconductor microcavity as a function of the sweep time. The hysteresis area exhibits a double power law decay due to the influence of fluctuations, which trigger switching between metastable states. Upon increasing the average photon number and approaching the thermodynamic limit, the double power law evolves into a single power law. This algebraic behavior characterizes a dissipative phase transition. Our findings are in good agreement with theoretical predictions for a single mode resonator influenced by quantum fluctuations, and the present experimental approach is promising for exploring critical phenomena in photonic lattices.

A dissipative quantum reservoir for microwave light using a mechanical oscillator

Isolation of a system from its environment is often desirable, from precision measurements to control of individual quantum systems; however, dissipation can also be a useful resource. Remarkably, engineered dissipation enables the preparation of quantum states of atoms, ions or superconducting qubits as well as their stabilization. This is achieved by a suitably engineered coupling to a dissipative cold reservoir formed by electromagnetic modes. Similarly, in the field of cavity electro- and optomechanics, the control over mechanical oscillators utilizes the inherently cold, dissipative nature of the electromagnetic degree of freedom. Breaking from this paradigm, recent theoretical work has considered the opposite regime in which the dissipation of the mechanical oscillator dominates and provides a cold, dissipative reservoir to an electromagnetic mode. Here we realize this reversed dissipation regime in a microwave cavity optomechanical system and realize a quasi-instantaneous, cold reservoir for microwave light. Coupling to this reservoir enables to manipulate the susceptibility of the microwave cavity, corresponding to dynamical backaction control of the microwave field. Additionally, we observe the onset of parametric instability, i.e. the stimulated emission of microwaves (masing). Equally important, the reservoir can function as a useful quantum resource. We evidence this by employing the engineered cold reservoir to implement a large gain (above 40 dB) phase preserving microwave amplifier that operates 0.87 quanta above the limit of added noise imposed by quantum mechanics. Such a dissipative cold reservoir forms the basis of microwave entanglement schemes, the study of dissipative quantum phase transitions, amplifiers with unlimited gain-bandwidth product and non-reciprocal devices, thereby extending the available toolbox of quantum-limited microwave manipulation techniques.

Observation of a Dissipative Phase Transition in a One-Dimensional Circuit QED Lattice

Condensed matter physics has been driven forward by significant experimental and theoretical progress in the study and understanding of equilibrium phase transitions based on symmetry and topology. However, nonequilibrium phase transitions have remained a challenge, in part due to their complexity in theoretical descriptions and the additional experimental difficulties in systematically controlling systems out of equilibrium. Here, we study a one-dimensional chain of 72 microwave cavities, each coupled to a superconducting qubit, and coherently drive the system into a nonequilibrium steady state. We find experimental evidence for a dissipative phase transition in the system in which the steady state changes dramatically as the mean photon number is increased. Near the boundary between the two observed phases, the system demonstrates bistability, with characteristic switching times as long as 60 ms -- far longer than any of the intrinsic rates known for the system. This experiment demonstrates the power of circuit QED systems for studying nonequilibrium condensed matter physics and paves the way for future experiments exploring nonequilbrium physics with many-body quantum optics.

Observation of the Photon-Blockade Breakdown Phase Transition

Non-equilibrium phase transitions exist in damped-driven open quantum systems, when the continuous tuning of an external parameter leads to a transition between two robust steady states. In second-order transitions this change is abrupt at a critical point, whereas in first-order transitions the two phases can co-exist in a critical hysteresis domain. Here we report the observation of a first-order dissipative quantum phase transition in a driven circuit quantum electrodynamics (QED) system. It takes place when the photon blockade of the driven cavity-atom system is broken by increasing the drive power. The observed experimental signature is a bimodal phase space distribution with varying weights controlled by the drive strength. Our measurements show an improved stabilization of the classical attractors up to the milli-second range when the size of the quantum system is increased from one to three artificial atoms. The formation of such robust pointer states could be used for new quantum measurement schemes or to investigate multi-photon quantum many-body phases.

Critical dynamical properties of a first-order dissipative phase transition

We theoretically investigate the critical properties of a single driven-dissipative nonlinear photon mode. In a well-defined thermodynamical limit of large excitation numbers, the exact quantum solution describes a first-order phase transition in the regime where semiclassical theory predicts optical bistability. We study the behavior of the complex spectral gap associated with the Liouvillian superoperator of the corresponding master equation. We show that in this limit the Liouvillian gap vanishes exponentially and that the bimodality of the photon Wigner function disappears. The connection between the considered thermodynamical limit of large photon numbers for the single-mode cavity and the thermodynamical limit of many cavities for a driven-dissipative Bose-Hubbard system is discussed.

Quantum phase transitions in the driven dissipative Jaynes-Cummings oscillator: From the dispersive regime to resonance

We follow the passage from complex amplitude bistability to phase bistability in the driven dissipative Jaynes-Cummings oscillator. Quasi-distribution functions in the steady state are employed, for varying qubit-cavity detuning and drive parameters, in order to track a first-order dissipative quantum phase transition up to the critical point marking a second-order transition and spontaneous symmetry breaking. We demonstrate the photon blockade breakdown in the dispersive regime, and find that the coexistence of cavity states in the regime of quantum bistability is accompanied by pronounced qubit-cavity entanglement. Focusing on the effect of quantum-activated switching for both coupled degrees of freedom, we move from a region of minimal entanglement in the dispersive regime, where we derive analytical perturbative results, to the threshold behaviour of spontaneous dressed-state polarization at resonance.

Non-equilibrium physics of Rydberg lattices in the presence of noise and dissipative processes

We study the non-equilibrium dynamics of driven spin lattices in the presence of decoherence caused by either laser phase noise or strong decay. In the first case, we discriminate between correlated and uncorrelated noise and explore their effect on the mean density of Rydberg states and the full counting statistics (FCS). We find that while the mean density is almost identical in both cases, the FCS differ considerably. The main method employed is the Langevin equation (LE) but for the sake of efficiency in certain regimes, we use a Markovian master equation and Monte Carlo rate equations, respectively. In the second case, we consider dissipative systems with more general power-law interactions. We determine the phase diagram in the steady state and analyse its generation dynamics using Monte Carlo rate equations. In contrast to nearest-neighbour models, there is no transition to long-range-ordered phases for realistic interactions and resonant driving. Yet, for finite laser detunings, we show that Rydberg lattices can undergo a dissipative phase transition to a long-range-ordered antiferromagnetic (AF) phase. We identify the advantages of Monte Carlo rate equations over mean field (MF) predictions.

Exact steady state of a Kerr resonator with one- and two-photon driving and dissipation: Controllable Wigner-function multimodality and dissipative phase transitions

We present exact results for the steady-state density matrix of a general class of driven-dissipative systems consisting of a nonlinear Kerr resonator in the presence of both coherent (one-photon) and parametric (two-photon) driving and dissipation. Thanks to the analytical solution, obtained via the complex P-representation formalism, we are able to explore any regime, including photon blockade, multiphoton resonant effects, and a mesoscopic regime with large photon density and quantum correlations. We show how the interplay between one- and two-photon driving provides a way to control the multimodality of the Wigner function in regimes where the semiclassical theory exhibits multistability. We also study the emergence of dissipative phase transitions in the thermodynamic limit of large photon numbers.

Quantum simulation with a boson sampling circuit

In this work we study a system that consists of $2M$ matter qubits that interact through a boson sampling circuit, i.e., an $M$-port interferometer, embedded in two different architectures. We prove that, under the conditions required to derive a master equation, the qubits evolve according to effective bipartite XY spin Hamiltonians, with or without local and collective dissipation terms. This opens the door to the simulation of any bipartite spin or hard-core boson models and exploring dissipative phase transitions as the competition between coherent and incoherent exchange of excitations. We also show that in the purely dissipative regime this model has a large number of exact and approximate dark states, whose structure and decay rates can be estimated analytically. We finally argue that this system may be used for the adiabatic preparation of boson sampling states encoded in the matter qubits.

Resummation for Nonequilibrium Perturbation Theory and Application to Open Quantum Lattices

Lattice models of fermions, bosons, and spins have long served to elucidate the essential physics of quantum phase transitions in a variety of systems. Generalizing such models to incorporate driving and dissipation has opened new vistas to investigate nonequilibrium phenomena and dissipative phase transitions in interacting many-body systems. We present a framework for the treatment of such open quantum lattices based on a resummation scheme for the Lindblad perturbation series. Employing a convenient diagrammatic representation, we utilize this method to obtain relevant observables for the open Jaynes-Cummings lattice, a model of special interest for open-system quantum simulation. We demonstrate that the resummation framework allows us to reliably predict observables for both finite and infinite Jaynes-Cummings lattices with different lattice geometries. The resummation of the Lindblad perturbation series can thus serve as a valuable tool in validating open quantum simulators, such as circuit-QED lattices, currently being investigated experimentally.

Universal energy transport law for dissipative and diffusive phase transitions

We present a scaling law for the energy and speed of transition waves in dissipative and diffusive media. By considering uniform discrete lattices and continuous solids, we show that---for arbitrary highly nonlinear many-body interactions and multistable on-site potentials---the kinetic energy per density transported by a planar transition wave front always exhibits linear scaling with wave speed and the ratio of energy difference to interface mobility between the two phases. We confirm that the resulting linear superposition applies to highly nonlinear examples from particle to continuum mechanics.

Degenerate parametric oscillation in quantum membrane optomechanics

The promise of innovative applications has triggered the development of many modern technologies capable of exploiting quantum effects. But in addition to future applications, such quantum technologies have already provided us with the possibility of accessing quantum-mechanical scenarios that seemed unreachable just a few decades ago. With this spirit, in this work we show that modern optomechanical setups are mature enough to implement one of the most elusive models in the field of open system dynamics: degenerate parametric oscillation. The possibility of implementing it in nonlinear optical resonators was the main motivation for introducing such model in the eighties, which rapidly became a paradigm for the study of dissipative phase transitions whose corresponding spontaneously broken symmetry is discrete. However, it was found that the intrinsic multimode nature of optical cavities makes it impossible to experimentally study the model all the way through its phase transition. In contrast, here we show that this long-awaited model can be implemented in the motion of a mechanical object dispersively coupled to the light contained in a cavity, when the latter is properly driven with multi-chromatic laser light. We focus on membranes as the mechanical element, showing that the main signatures of the degenerate parametric oscillation model can be studied in state-of-the-art setups, thus opening the possibility of studying spontaneous symmetry breaking and enhanced metrology in one of the cleanest dissipative phase transitions.

Quantum sweeps, synchronization, and Kibble-Zurek physics in dissipative quantum spin systems

We address dissipation effects on the non-equilibrium quantum dynamics of an ensemble of spins-1/2 coupled via an Ising interaction. Dissipation is modeled by a (ohmic) bath of harmonic oscillators at zero temperature and correspond either to the sound modes of a one-dimensional Bose-Einstein (quasi-)condensate or to the zero-point fluctuations of a long transmission line. We consider the dimer comprising two spins and the quantum Ising chain with long-range interactions, and develop a (mathematically and numerically) exact stochastic approach to address non-equilibrium protocols in the presence of an environment. For the two spin case, we first investigate the dissipative quantum phase transition induced by the environment through quantum quenches, and study the effect of the environment on the synchronization properties. Then, we address Landau-Zener-Stueckelberg-Majorana protocols for two spins, and for the spin array. In this latter case, we adopt a stochastic mean-field point of view and present a Kibble-Zurek type argument to account for interaction effects in the lattice. Such dissipative quantum spin arrays can be realized in ultra-cold atoms, trapped ions, mesoscopic systems, and are related to Kondo lattice models.

Macroscopic Self-Organized Electrochemical Patterns in Excitable Tissue and Irreversible Thermodynamics

In this paper we make the assertion that the key to understand the emergent properties of excitable tissue (brain and heart) lies in the application of irreversible thermodynamics. We support this assertion by pointing out where symmetry break, phase transitions both in structure of membranes as well as in the dynamic of interactions between membranes occur in excitable tissue and how they create emergent low dimensional electrochemical patterns. These patterns are expressed as physiological or physiopathological concomitants of the organ or organism behavior. We propose that a set of beliefs about the nature of biological membranes and their interactions are hampering progress in the physiology of excitable tissue. We will argue that while there is no direct evidence to justify the belief that quantum mechanics has anything to do with macroscopic patterns expressed in excitable tissue, there is plenty of evidence in favor of irreversible thermodynamics. Some key predictions have been fulfilled long time ago and they have been ignored by the mainstream literature. Dissipative structures and phase transitions appear to be a better conceptual context to discuss biological self-organization. The central role of time as a global coupling agent is emphasized in the interpretation of the presented results.

Self-consistent projection operator theory in nonlinear quantum optical systems: A case study on degenerate optical parametric oscillators

Nonlinear quantum optical systems are of paramount relevance for modern quantum technologies, as well as for the study of dissipative phase transitions. Their nonlinear nature makes their theoretical study very challenging and hence they have always served as great motivation to develop new techniques for the analysis of open quantum systems. In this article we apply the recently developed self-consistent projection operator theory to the degenerate optical parametric oscillator to exemplify its general applicability to quantum optical systems. We show that this theory provides an efficient method to calculate the full quantum state of each mode with high degree of accuracy, even at the critical point. It is equally successful in describing both the stationary limit and the dynamics, including regions of the parameter space where the numerical integration of the full problem is significantly less efficient. We further develop a Gaussian approach consistent with our theory, which yields sensibly better results than the previous Gaussian methods developed for this system, most notably standard linearization techniques.

Dissipative phase transitions: Independent versus collective decay and spin squeezing

We study the XY model with infinite-range interactions (Lipkin-Meshkov-Glick model) in the presence of dissipation from spontaneous decay. We show that independent and collective decay lead to qualitatively different phase transitions of the steady state, even though the phase boundary is the same. Independent decay leads to a second-order phase transition to a ferromagnet, while collective decay leads to a first-order transition to a time-dependent oscillatory phase. Then we show that the addition of a drive leads to infinite spin squeezing for collective decay in the thermodynamic limit. Our results can be experimentally seen in trapped-ion and cavity-QED experiments.

Stochastic projected Gross-Pitaevskii equation for spinor and multicomponent condensates

A stochastic Gross-Pitaevskii equation is derived for partially condensed Bose gas systems subject to binary contact interactions. The theory we present provides a classical-field theory suitable for describing dissipative dynamics and phase transitions of spinor and multi-component Bose gas systems comprised of an arbitrary number of distinct interacting Bose fields. A new class of dissipative processes involving distinguishable particle interchange between coherent and incoherent regions of phase-space is identified. The formalism and its implications are illustrated for two-component mixtures and spin-1 Bose-Einstein condensates. For systems comprised of atoms of equal mass, with thermal reservoirs that are close to equilibrium, the dissipation rates of the theory are reduced to analytical expressions that may be readily evaluated. The unified treatment of binary contact interactions presented here provides a theory with broad relevance for quasi-equilibrium and far-from-equilibrium Bose-Einstein condensates.

Antiferromagnetic long-range order in dissipative Rydberg lattices

We study the dynamics of dissipative spin lattices with power-law interactions, realized via few-level atoms driven by coherent laser-coupling and decoherence processes. Using Monte Carlo simulations, we determine the phase diagram in the steady state and analyze its generation dynamics. As opposed to mean-field predictions and nearest-neighbor models, there is no transition to long-range-ordered phases for realistic interactions and resonant driving. However, for finite laser detunings, we demonstrate the emergence of crystalline order. Although the static and dynamical critical exponents of the revealed dissipative phase transition fall into the two-dimensional Ising universality class, the found steady states differ considerably from those of an equilibrium Ising magnet. Two complementary schemes for an experimental implementation with cold Rydberg atoms are discussed.

Quantum information-geometry of dissipative quantum phase transitions.

A general framework for analyzing the recently discovered phase transitions in the steady state of dissipation-driven open quantum systems is still lacking. To fill this gap, we extend the so-called fidelity approach to quantum phase transitions to open systems whose steady state is a Gaussian fermionic state. We endow the manifold of correlation matrices of steady states with a metric tensor g measuring the distinguishability distance between solutions corresponding to a different set of control parameters. The phase diagram can then be mapped out in terms of the scaling behavior of g and connections with the Liouvillean gap and the model correlation functions unveiled. We argue that the fidelity approach, thanks to its differential-geometric and information-theoretic nature, provides insights into dissipative quantum critical phenomena as well as a general and powerful strategy to explore them.

Dissipative production of a maximally entangled steady state of two quantum bits

Entangled states are a key resource in fundamental quantum physics, quantum cryptography and quantum computation. Introduction of controlled unitary processes--quantum gates--to a quantum system has so far been the most widely used method to create entanglement deterministically. These processes require high-fidelity state preparation and minimization of the decoherence that inevitably arises from coupling between the system and the environment, and imperfect control of the system parameters. Here we combine unitary processes with engineered dissipation to deterministically produce and stabilize an approximate Bell state of two trapped-ion quantum bits (qubits), independent of their initial states. Compared with previous studies that involved dissipative entanglement of atomic ensembles or the application of sequences of multiple time-dependent gates to trapped ions, we implement our combined process using trapped-ion qubits in a continuous time-independent fashion (analogous to optical pumping of atomic states). By continuously driving the system towards the steady state, entanglement is stabilized even in the presence of experimental noise and decoherence. Our demonstration of an entangled steady state of two qubits represents a step towards dissipative state engineering, dissipative quantum computation and dissipative phase transitions. Following this approach, engineered coupling to the environment may be applied to a broad range of experimental systems to achieve desired quantum dynamics or steady states. Indeed, concurrently with this work, an entangled steady state of two superconducting qubits was demonstrated using dissipation.