Dispersive Wave Emission Research Articles

Octave-wide broadening of ultraviolet dispersive wave driven by soliton-splitting dynamics

Coherent dispersive wave emission, as an important phenomenon of soliton dynamics, manifests itself in multiple platforms of nonlinear optics from fibre waveguides to integrated photonics. Limited by its resonance nature, efficient generation of coherent dispersive wave with ultra-broad bandwidth has, however, proved difficult to realize. Here, we unveil a new regime of soliton dynamics in which the dispersive wave emission process strongly couples with the splitting dynamics of the driving pulse. High-order dispersion and self-steepening effects, accumulated over soliton self-compression, break the system symmetry, giving rise to high-efficiency generation of coherent dispersive wave in the ultraviolet region. Simultaneously, asymmetric soliton splitting results in the appearance of a temporally-delayed ultrashort pulse with high intensity, overlapping and copropagating with the dispersive wave pulse. Intense cross-phase modulations lead to octave-wide broadening of the dispersive wave spectrum, covering 200–400 nm wavelengths. The highly-coherent, octave-wide ultraviolet spectrum, generated from the simple capillary fibre set-up, is in great demand for time-resolved spectroscopy, ultrafast electron microscopy and frequency metrology applications, and the critical role of the secondary pulse in this process reveals some new opportunities for all-optical control of versatile soliton dynamics.

Few-femtosecond soft X-ray transient absorption spectroscopy with tuneable DUV-Vis pump pulses

Achieving few-femtosecond resolution for a pump-probe experiment is crucial to measuring the fastest electron dynamics and for creating superpositions of valence states in quantum systems. However, traditional UV-Vis pump pulses cannot achieve few-fs durations and usually operate at fixed wavelengths. Here, we present, to our knowledge, an unprecedented temporal resolution and pump tuneability for UV-Vis-pumped soft X-ray transient absorption spectroscopy. We have combined few-fs deep-UV to visible tuneable pump pulses from resonant dispersive wave emission in hollow capillary fiber with attosecond soft X-ray probe pulses from high harmonic generation. We achieve sub-5-fs time resolution, sub-fs interferometric stability, and continuous tuneability of the pump pulses from 230 to 700 nm. We demonstrate that the pump can initiate an ultrafast photochemical reaction and that the dynamics at different atomic sites can be resolved simultaneously. These capabilities will allow studies of the fastest electronic dynamics in a large range of photochemical, photobiological and photovoltaic reactions.

Direct temporal characterization of sub-3-fs deep UV pulses generated by resonant dispersive wave emission: erratum

An erratum is presented to include the correct upper horizontal axis in Fig. 3 in our published manuscript [“Direct temporal characterization of sub-3-fs deep UV pulses generated by resonant dispersive wave emission” Opt. Express 31, 26854 (2023).10.1364/OE.494879

Ultra-low threshold deep ultraviolet generation in a hollow-core fiber.

Tunable ultrashort pulses in the ultraviolet spectral region are in great demand for a wide range of applications, including spectroscopy and pump-probe experiments. While laser sources capable of producing such pulses exist, they are typically very complex. Notably, resonant dispersive-wave (RDW) emission has emerged as a simple technique for generating such pulses. However, the required pulse energy used to drive the RDW emission, so far, is mostly at the microjoule level, requiring complicated and expensive pump sources. Here, we present our work on lowering the pump energy threshold for generating tuneable deep ultraviolet pulses to the level of tens of nanojoules. We fabricated a record small-core antiresonant fiber with a hollow-core diameter of just 6 μm. When filled with argon, the small mode area enables higher-order soliton propagation and deep ultraviolet (220 to 270 nm) RDW emission from 36 fs pump pulses at 515 nm with the lowest pump energy reported to date (tens of nanojoules). This approach will allow the use of low-cost and compact laser oscillators to drive nonlinear optics in gas-filled fibers for the first time to our knowledge.

HISOL: High-energy soliton dynamics enable ultrafast far-ultraviolet laser sources

Ultrafast laser sources in the far ultraviolet (100–300 nm) have been the subject of intense experimental efforts for several decades, driven primarily by the requirements of advanced experiments in ultrafast science. Resonant dispersive wave emission from high-energy laser pulses undergoing soliton self-compression in a gas-filled hollow capillary fiber promises to meet several of these requirements for the first time, most importantly by combining wide-ranging wavelength tuneability with the generation of extremely short pulses. In this Perspective, we give an overview of this approach to ultrafast far-ultraviolet sources, including its historical origin and underlying physical mechanism, the state of the art and current challenges, and our view of potential applications both within and beyond ultrafast science.

Emission of five OAM dispersive waves in dispersion-engineered double-ring core fiber

Beams carrying orbital angular momentum (OAM) have exhibited significant potential across various fields, such as metrology, image coding, and optical communications. High-performance broadband coherent OAM sources are critical to the operation of optical systems. The emission of dispersive waves facilitates the efficient transfer of energy to distant spectral domains while preserving the coherence among the generated frequency components. Light sources that maintain consistency over a wide range can increase the efficiency of optical communication systems and improve the measurement accuracy in imaging and metrology. In this work, we propose a germanium-doped double ring-core fiber for five OAM dispersive waves (DWs) generation. The OAM1,1 mode supported in the fiber exhibits three zero-dispersion wavelengths (ZDWs) located at 1275, 1720 and 2325 nm. When pumped under normal dispersion, the output spectrum undergoes broadening and exhibits five DWs, situated around 955, 1120, 1450, 2795 and 2965 nm, respectively. Concomitant with blue-shifted and red-shifted dispersive waves, the spectrum spans from 895 to 3050 nm with high coherence. The effect of the fiber and input pulse parameters on DWs generation, as well as the underlying dynamics of the dispersive wave generation process, are discussed. As expected, the number and location of DWs generated in the output spectrum have agreement with the prediction of the phase-matching condition. Overall, this multiple DWs generation method in the proposed fiber paves the way for developing efficient and coherent OAM light sources in fiber-based optical systems.

Applications of Microstructured Optical Fibers in Ultrafast Optics: A Review

With the development of laser technology, microstructured optical fibers (MOFs) have become an important part of ultrafast optics, providing excellent platforms for ultrafast laser pulse generation, amplification, and compression, promoting the development of fiber laser systems to generate high power, high pulse energy, and few-cycle duration pulses. MOFs extend the ultrafast laser spectrum to the vacuum ultraviolet (VUV) and even extreme ultraviolet (EUV) regions based on dispersive wave emission and high harmonic generation, as well as to the mid-infrared region based on soliton self-frequency shift (SSFS), contributing compact and low-cost light sources for precision microscopy and spectroscopy. In this paper, first several common types of MOFs are introduced, then the various applications of MOFs in ultrafast optics are discussed, mainly focusing on the aspects of ultrafast laser pulse scaling in pulse energy and spectral bandwidth, and finally the possible prospects of MOFs are given.

Vacuum-ultraviolet dispersive wave emission driven by phase-locked pulse pairs in a gas-filled hollow-core fiber: a numerical study

Vacuum-ultraviolet dispersive wave emission driven by phase-locked pulse pairs in a gas-filled hollow-core fiber: a numerical study

Nonlinear post-compression of a hybrid vortex mode in a gas-filled capillary.

We demonstrate nonlinear temporal compression of a vortex beam by propagation in a gas-filled capillary. Starting from an ytterbium-based laser delivering 700 μJ 640 fs pulses at a 100 kHz repetition rate, the vortex beam is generated using a spiral phase plate and coupled to a capillary where it excites a set of four modes that have an overlap integral of 97% with a Laguerre-Gauss LG10 mode. Nonlinear propagation of this hybrid, orbital angular momentum (OAM)-carrying mode results in temporal compression down to 74 fs at the output. Beam and pulse characterizations are carried out to determine the spatial profile and temporal duration of compressed pulses. This result in multimode nonlinear optics paves the way towards the generation of OAM-carrying few-cycle pulses, isolated attosecond XUV pulses, and tunable UV pulses through resonant dispersive wave emission.

Optical solitons in hollow-core fibres

I review the historical observation and subsequent research on optical soliton dynamics in gas-filled hollow-core optical fibres. I include both large-core hollow capillary fibres, and hollow-core photonic-crystal or microstructured fibres with smaller cores, in particular photonic bandgap and antiresonant guiding fibres. I discuss how the optical guidance properties of these different fibre structures influence the soliton dynamics that can be obtained. The dynamics I consider include: soliton propagation at peak power levels ranging from the megawatt to terawatt level, and pulse energies from sub-microjoule to millijoule range; pulse self-compression, leading to sub-cycle and sub-femtosecond pulse duration; soliton self-frequency shifting due to both the Raman effect, and the influence of photoionisation and plasma formation; and resonant dispersive wave emission, leading to the generation of tuneable few-femtosecond pulses across the vacuum and deep ultraviolet, visible, and near-infrared spectral regions.

Ultra-low time jitter transform-limited dissipative Kerr soliton microcomb.

Microresonator soliton frequency combs offer unique flexibility in synthesizing microwaves over a wide range of frequencies. Therefore, it is very important to study the time jitter of soliton microcombs. Here, we fabricate optical microresonators with perfect transmission spectrum that characterizes highly uniform extinction ratio and absence of mode interactions by laser machining high-purity silica fiber preforms. Based on such perfect whispering-gallery-mode cavity, We demonstrate that K-band microwave with ultra-low phase noise (-83 dBc/Hz@100 Hz; -112 dBc/Hz@1kHz; -133 dBc/Hz@10kHz) can be generated by photo-detecting the repetition rate of a soliton microcomb. Also, with the Raman scattering and dispersive wave emission largely restricted, we show that ultra-low time jitter soliton has a wide existence range. Our work illuminates a pathway toward low-noise photonic microwave generation as well as the quantum regime of soliton microcombs.

Enhanced spectral broadening via the optical rogue wave stimulated by spectral sinusoidal phase

We numerically investigate the extended spectral broadening via a spectral sinusoidal phase-modulated Gaussian pulse. The modulated pulse can create two predominant solitons that collide with each other to form a rogue wave (RW), resulting in an RW-induced dispersive wave emission. This leads to a further spectral broadening beyond the soliton-induced dispersive wave and can be manipulated by tuning the phase modulation parameters. Before the appearance of RW, the modulated pulse-propagation scenario is governed by the optical Newton’s cradles and the optical event horizons. These complex dynamics reveal a new method for controlling the RW generation as well as spectral broadening at relatively low power levels. Our results have potential implications for controllable excitation of RWs and broadband supercontinuum generation.

Interactions and Dynamics of One-Dimensional Droplets, Bubbles and Kinks

We explore the dynamics and interactions of multiple bright droplets and bubbles, as well as the interactions of kinks with droplets and with antikinks, in the extended one-dimensional Gross–Pitaevskii model including the Lee–Huang–Yang correction. Existence regions are identified for the one-dimensional droplets and bubbles in terms of their chemical potential, verifying the stability of the droplets and exposing the instability of the bubbles. The limiting case of the droplet family is a stable kink. The interactions between droplets demonstrate in-phase (out-of-phase) attraction (repulsion), with the so-called Manton’s method explicating the observed dynamical response, and mixed behavior for intermediate values of the phase shift. Droplets bearing different chemical potentials experience mass-exchange phenomena. Individual bubbles exhibit core expansion and mutual attraction prior to their destabilization. Droplets interacting with kinks are absorbed by them, a process accompanied by the emission of dispersive shock waves and gray solitons. Kink–antikink interactions are repulsive, generating counter-propagating shock waves. Our findings reveal dynamical features of droplets and kinks that can be detected in current experiments.

Direct temporal characterization of sub-3-fs deep UV pulses generated by resonant dispersive wave emission.

We report on the complete temporal characterization of ultrashort pulses, generated by resonant dispersive wave emission in gas-filled hollow-capillary fibers, with energy in the microjoule range and continuously tunable from the deep-ultraviolet to the ultraviolet. Temporal characterization of such ultrabroad pulses, particularly challenging in this spectral region, was performed using an all-in-vacuum setup for self-diffraction frequency resolved optical gating (SD-FROG). Sub-3-fs pulses were measured, tunable from 250 nm to 350 nm, with a minimum pulse duration of 2.4 ± 0.1 fs.

Optimization of mid-infrared dispersive wave generation at 3 µm in LiNbO3 waveguides

We propose an effective scheme to enhance mid-infrared dispersive wave (DW) emission, which includes dispersion engineering of the waveguide and the assistance of a CW trigger. Our suggested approach can help achieve better coherence and higher signal-to-noise ratio by adding a weak CW trigger with the femtosecond pulse pump in dispersion engineered lithium niobate (LiNbO3) waveguides. First, the integrated dispersion profile of LiNbO3 waveguides is designed based on dispersion engineering regarding the sidewall angle and slab thickness. Second, with the assistance of a weak CW trigger, the mid-infrared DW is enabled or further enhanced. The optimal CW-triggered wavelength and operating conditions are ascertained. Mid-infrared emission at around 3 µm with a sufficient power level is accessible after optimization, which is feasible for multi-species greenhouse gas detection through gas absorption spectroscopy.

Experimental Observation of the Spontaneous Emission of a Space–Time Wavepacket in a Multimode Optical Fiber

We provide a complete analysis, from theory to experiment, of the spontaneous emergence of a discretized conical wave of X-type (i.e., a localized 2D+1 space-time wavepacket) when an intense ultrashort pulse nonlinearly propagates in a multimode fiber. In particular, we reveal that this spatiotemporal phenomenon corresponds to broadband intermodal dispersive wave emission from an unsteady localized wave structure formed during nonlinear propagation. Theoretical phase-matching predictions are experimentally and numerically confirmed in a commercially available step-index multimode fiber. Our results provide a general understanding of phase-matched radiations emitted by nonlinear waves in multidimensional dispersive optical system.

Manipulating dispersive wave emission via temporal sinusoidal phase modulation.

We report the dispersive wave (DW) emission from the Gaussian pulse with temporal sinusoidal phase (TSP) modulation. The TSP-induced chirp can enhance or cancel the chirp generated by self-phase modulation by properly selecting the modulation parameters of TSP, which can influence the nonlinear propagation of the TSP-modulated pulse. It is shown that the TSP can effectively control the resonant frequency and energy conversion efficiency of the DW emission. We give a modified phase-matching condition to predict the resonant frequencies, which agree with the simulation results obtained by numerically solving the nonlinear Schrödinger equation. The enhanced conversion efficiency of the DWs can be increased up to 28% with only TSP modulation. Our results can extend the application of temporal phase modulation technology for wavelength conversion, and broadband supercontinuum generation.

Efficient and compact source of tuneable ultrafast deep ultraviolet laser pulses at 50 kHz repetition rate.

Deep ultraviolet (DUV) laser pulses with tuneable wavelength and very short duration are a key enabling technology for next-generation technology and ultrafast science. Their generation has been the subject of extensive experimental effort, but no technique demonstrated thus far has been able to meet all requirements in one light source. Here we demonstrate a bright, efficient, and compact source of tuneable DUV ultrafast laser pulses based on resonant dispersive wave emission in hollow capillary fiber. In a total footprint of only 120cm×75cm, including the ytterbium-based drive laser, we generate pulses between 208nm and 363nm at 50kHz repetition rate with a total efficiency of up to 3.6%. Down-scaling of the DUV generation reduces the required energy sufficiently to enable the generation of two-color few-femtosecond DUV pulses.

Soliton dynamics in a piecewise gas-filled hollow-core fiber for efficient dispersive wave emission in the vacuum-ultraviolet range

Table-top coherent vacuum-ultraviolet (VUV) sources are important in many researches. Dispersive wave (DW) emission in a gas-filled hollow-core fiber (HCF) is an efficient way to obtain tunable VUV source with microjoule-level pulse energy. However, the shortest VUV wavelength is limited above 110 nm. This work investigated a method using a piecewise HCF in order to push the shortest VUV DW emission below 110 nm efficiently. The rich and complex spatiotemporal soliton dynamics in the HCF is revealed through rigorous numerical simulations and quantitative analysis. It is found that both the generation of VUV light below 110 nm and the overall conversion efficiencies below 150 nm can be significantly improved if the piecewise gas-filled HCF system is properly designed. As a result, the whole VUV spectrum (200--100 nm) can now be accessed efficiently, with single pulse energy of microjoule level. Different from other widely used intense VUV sources, this source has broad spectrum along with femtosecond time width. These unique characteristics in the VUV spectrum can lead to new research opportunities in various areas.

Mid-Infrared Highly Efficient, Broadband, and Flattened Dispersive Wave Generation via Dual-Coupled Thin-Film Lithium-Niobate-on-Insulator Waveguide

We designed a structure of dual-coupled ridge waveguide in thin-film lithium-niobate-on-insulator (LNOI) and numerically studied the highly efficient, broadband, and flattened dispersive wave-enhanced supercontinuum generation in the mid-infrared region. By leveraging the mode coupling of the proposed dual-coupled waveguide structure, one of the supermodes, namely the anti-symmetric mode, can produce additional zero-dispersion wavelengths in the mid-infrared region, and consequently multiple normal dispersion regions for dispersive wave emission. Given the rich geometrical degrees of freedom powered by this dual-coupled LNOI waveguide structure, we can tailor the dispersion profile so that a well-established mode-locked fiber laser in the telecommunication band can serve as the pump. Thus, the whole system can potentially be fiber-to-chip integrated and packaged, enabling a compact, cost-effective, and low system-complexity platform. We numerically show that the broadband dispersive wave covering the wavelength range of 1.92~3.55 μm (−20 dB level, near octave-spanning) with spectral flatness of 6.31 dB can be achieved using a 1550 nm, 190 pJ femtosecond pump seed. When the dual hump-shaped spectrum is obtained, the conversion efficiency of the mid-infrared dispersive wave can be up to 19.31%. The influence of the pumping conditions on the performance of mid-infrared dispersive wave generation was also studied. This work provides a competitive candidate for efficient, broadband, and flattened mid-infrared spectrum generation, which can find important applications in spectroscopy, metrology, and communication.