Direct Radiative Heating Research Articles

More Accurate Quantification of Direct Aerosol Radiative Effects Using Vertical Profiles of Single‐Scattering Albedo Derived From Tethered Balloon Observations

AbstractAerosol single‐scattering albedo (SSA) is the most critical factor for the accurately calculating of aerosol radiative effects, however, the observation of vertical profiles of SSA is difficult to realize. Current assessments of aerosol radiative effects remain uncertain because of the lack of long‐term, high‐resolution vertical profiles of SSA observations. High‐resolution SSA vertical profiles were observed in a semi‐arid region of Northwest China during winter using a tethered balloon. The observed SSA vertical profiles were used to calculate the aerosol direct radiative forcing and radiative heating rates. Significant differences in the calculated radiative forcing were found (e.g., a 48.3% relative difference for the heating effect in the atmosphere at 14:00) between the observed SSA profiles and the constant assumption with SSA = 0.90. Diurnal variations in the vertical distribution of SSA decisively influenced direct radiative forcing of aerosols. Furthermore, high‐resolution vertical profiles of absorbing aerosols and meteorological parameters provide robust observational evidence of the heating effect of an elevated absorbing aerosol layer. This study provides a more accurate calculation of aerosol radiative forcing using observed aerosol SSA profiles.

Accumulation of absorbing aerosols over the Indian Sector of Southern Ocean during the austral summer: Role of thermal inversions

Optical properties of aerosols and their direct radiative effect were analyzed from columnar Aerosol Optical Depth (AOD) and ambient Black Carbon (BC) mass concentration (MB) estimated during Indian Southern Ocean Expeditions (SOEs), conducted in the austral summers of 2016–17 (SOE-IX) and 2017–18 (SOE-X). The aforementioned observations were supplemented with concurrent vertical soundings of the lower atmosphere. Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) data aided in investigating the vertical distribution of aerosols up to 10 km altitude. The relative contribution of BC aerosols emanating from fossil fuel combustion and biomass burning showed the former to be predominant, as the latter is larger and preferentially scavenged during long-range transport to remote marine regions. The highest values of AOD at 500 nm (AOD500; 0.156 ± 0.026) and MB (90.78 ± 40.11 ng m−3) were encountered in the region between 50 and 60°S. Consequently, the atmospheric clear-sky Aerosol Direct Radiative Effect (ADRE; +3.10 ± 0.38 W m−2) and heating rate (HR; 0.087 ± 0.011 K day−1) were also observed to be the highest in the region. Multiple atmospheric inversions were detected between 40 and 69°S. Although a much lower AOD500 (0.070 ± 0.017) prevailed between 60 and 69°S, the average clear-sky ADRE (+1.56 ± 0.49 W m−2) and HR (0.044 ± 0.014 K day−1) were fairly high. The mean MB in the region was high (68.81 ± 28.40 ng m−3) for the pristine ice-covered region. Low-lying inversions prevented the vertical ventilation and dispersal of BC therein. Simulations of BC-induced atmospheric heating rates at three locations in the coastal Antarctic waters indicated a ≈ 3–5-fold increase, corresponding to an increase in ambient BC from 50 to 300 ng m−3.

Energy and economic aspects of efficient radiative heating for biodiesel production: Prospects and challenges of using solid magnetic CaO/CoFe2O4 nano-catalyst

Direct radiative heating using an infrared (IR) source is experimentally investigated in the production of biodiesel from waste edible oil using CaO and self-synthetized CaO/CoFe2O4 as heterogeneous solid catalysts. The nano-sized CaO/CoFe2O4 particles show 30 % lower specific energy (i.e. the required energy to produce 1-L biodiesel) than that of CaO for the case of radiative (IR) heating. Meanwhile, comparing the radiative and conventional heating methods shows that the specific energy and the reaction time are reduced by 75 % and up to 50 %. However, the specific cost (i.e. the cost required to produce 1-L biodiesel) corresponding to CaO/CoFe2O4 is higher than that of CaO by 36–56 %. The strong magnetic characteristic of CaO/CoFe2O4 makes the separation process easy and has a good potential for recycling purposes. Overall, CaO/CoFe2O4 under radiative heating showed the advantages of having a high yield efficiency, shorter reaction time, low specific energy, and ease of separation which make it a good candidate for large-scale productions, while the specific cost and cyclic performance are the present challenges and still require further studies.

Aerosol-boundary layer dynamics and its effect on aerosol radiative forcing and atmospheric heating rate in the Indian Ocean sector of Southern Ocean

The study examines the thermodynamic structure of the marine atmospheric boundary layer (MABL) and its effect on the aerosol dynamics in the Indian Ocean sector of Southern Ocean (ISSO) between 30°S-67°S and 57°E-77°E. It includes observations of aerosols and meteorology collected during the Xth Southern Ocean Expedition conducted in December 2017. The results revealed the effect of frontal-region-specific air-sea coupling on the thermodynamic structure of MABL and its role in regulating aerosols in ISSO. The MABL over the subtropical front was unstable and formed a well-evolved mixed layer (≈2400 m) capped by low-level inversions (≈660 m). Convective activities in the Sub-Antarctic Frontal region were associated with the Agulhas Retroflection Current, which supported the formation of a well-developed mixed layer (≈1860 m). The mean estimates of aerosol optical depth (AOD) and black carbon (BC) mass concentrations were 0.095 ± 0.006 and 50 ± 14 ng m−3, respectively, and the resultant clear sky direct shortwave radiative forcing (DARF) and atmospheric heating rate (HR) were 1.32 ± 0.11 W m−2 and 0.022 ± 0.002 K day−1, respectively. In the polar front (PF) region, frequent mid-latitude cyclones led to highly stabilized MABL, supported low-level multi-layered clouds (>3-layers) and multiple high-level inversions (strength > 0.5 K m−1 > 3000 m). The clouds were mixed-phased with temperatures less than −12 °C at 3000 m altitude. Interestingly, there was higher loading of dust and BC aerosols (276 ± 24 ng m−3), maximum AOD (0.109 ± 0.009), clear sky DARF (1.73 ± 0.02 W m−2), and HR (0.029 ± 0.005 K day−1). This showed an accumulation of long-range advected anthropogenic aerosols within baroclinic-boundaries formed over the PF region. Specifically, in the region south of PF, weak convection caused weakly-unstable MABL with a single low-level inversion followed by no clouds/single-layer clouds. Predominant clean maritime air holding a small fraction of dust and BC accounted for lower estimates of AOD (0.071 ± 0.004), BC concentrations (90 ± 55 ng m−3) and associated clear sky DARF and HR were 1.16 ± 0.06 W m−2 and 0.019 ± 0.001 K day−1, respectively.

Simulating Diurnal Variations of Water Temperature and Dissolved Oxygen in Shallow Minnesota Lakes

In shallow lakes, water quality is mostly affected by weather conditions and some ecological processes which vary throughout the day. To understand and model diurnal-nocturnal variations, a deterministic, one-dimensional hourly lake water quality model MINLAKE2018 was modified from daily MINLAKE2012, and applied to five shallow lakes in Minnesota to simulate water temperature and dissolved oxygen (DO) over multiple years. A maximum diurnal water temperature variation of 11.40 °C and DO variation of 5.63 mg/L were simulated. The root-mean-square errors (RMSEs) of simulated hourly surface temperatures in five lakes range from 1.19 to 1.95 °C when compared with hourly data over 4–8 years. The RMSEs of temperature and DO simulations from MINLAKE2018 decreased by 17.3% and 18.2%, respectively, and Nash-Sutcliffe efficiency increased by 10.3% and 66.7%, respectively; indicating the hourly model performs better in comparison to daily MINLAKE2012. The hourly model uses variable hourly wind speeds to determine the turbulent diffusion coefficient in the epilimnion and produces more hours of temperature and DO stratification including stratification that lasted several hours on some of the days. The hourly model includes direct solar radiation heating to the bottom sediment that decreases magnitude of heat flux from or to the sediment.

Design, Construction and Performance Evaluation of an Automated Mixed Mode Solar Tracking Cacao Dryer

This study designed, developed, and undertook performance evaluation of a mixed-mode solar dryer with solar tracking collector, which is integrated with electric heaters as a backup heat source for drying fermented cacao beans. The drying mechanism was based on the combination of direct radiation and convective heating with the incorporation of electric backup heaters to address the intermittent effect of drying. The solar tracking collector maximized thesolar reception during daytime by providing sufficient heat inside the chamber. The electric heaters also provided reliable heat sources during night time, preventing the occurrence of moisture re-absorption by the beans. The developed system maintained a drying temperature range of 40-600C by automatically switching the drying modes depending on the weather conditions. At the average drying rate of 0.17kg/h in 48 hours of continuous drying, it dehydrated the cacao beans from an initial moisture content in wet basis of 57.49% to 0.65%, against the ambient temperature of 200C-360C. Drying time was shortened by 50% against traditional open or natural sun-drying, which takes 4-6 days, reducing it to two days or 48 hours. The integrated design of the mixed mode solar dyer provided the ability to carry out the drying process continuously by optimizing heat sources while maintaining the drying requirements for cacao beans. This study validated that the solar dryer is suitable for drying cacao beans.

The Role of Radiation in Heating the Clear-Air Convective Boundary Layer: Revisiting CASES-97

Using data for 3 days in the Cooperative Atmosphere-Surface Exchange Study 1997 field experiment that are analyzed in LeMone et al. (Boundary-Layer Meteorol 104:1–52, 2002, hereafter L2002), it is shown that direct radiative heating can have a significant role in warming the nearly cloudless fair-weather convective boundary layer (CBL). Radiative heating becomes especially important in the presence of aerosols in the CBL, with a moist layer above the CBL also contributing. Not only does inclusion of radiative heating help “close” their potential-temperature budgets, but it affects entrainment estimates. Combined, radiative heating rates are of the order of 0.2 K h−1, based on calculations using the Rapid-Radiative Transfer Model for general circulation models (RRTMG) code in a single-column version of the Advanced Research Weather Research and Forecasting model and estimates of aerosol heating published in L2002. Our current estimates of clear-air direct radiative heating differ from the estimates in L2002 because the surface skin temperature was not included in the earlier calculations. Upwelling and downwelling longwave radiation computed using the RRTMG code agrees with aircraft measurements within 10–15 W m−2.

Unexpected Biomass Burning Aerosol Absorption Enhancement Explained by Black Carbon Mixing State

AbstractDirect and semi‐direct radiative effects of biomass burning aerosols (BBA) from southern and central African fires are still widely debated, in particular because climate models have been unsuccessful in reproducing the low single scattering albedo in BBA over the eastern Atlantic Ocean. Using state‐of‐the‐art airborne in situ measurements and Mie scattering simulations, we demonstrate that low single scattering albedo in well‐aged BBA plumes over southern West Africa results from the presence of strongly absorbing refractory black carbon (rBC), whereas the brown carbon contribution to the BBA absorption is negligible. Coatings enhance light absorption by rBC‐containing particles by up to 210%. Our results show that accounting for the diversity in black carbon mixing state by combining internal and external configurations is needed to accurately estimate the optical properties and henceforth the shortwave direct radiative effect and heating rate of BBA over southern West Africa.

The importance of cross-calibration and protecting water temperature sensors against direct solar radiation heating in hydrological studies

ABSTRACTWater temperature monitoring is important in many scientific studies. This study compares three models of water temperature sensors (Vemco Minilog II, HOBO TidbiT and HOBO Pendant) to test the importance of: (1) using cross-calibration to minimize relative errors, (2) using cross-calibration to improve on the accuracy of less accurate sensors, and (3) protecting sensors against direct solar radiation heating. The results show that when the same sensor models are cross-calibrated, the relative error can be reduced (Vemco: 0.01°C; HOBO TidbiT: 0.02°C; and HOBO Pendant: 0.07°C). Cross-calibration can also improve less accurate sensors (HOBO TidbiT and Pendant) to similar accuracies of Vemco (±0.1°C). Finally, no evidence of solar radiation heating was observed for Vemcos (unprotected); however, HOBO TidbiT and Pendant showed heating up to 2°C (maximum). When HOBO TidbiT and Pendant are shielded (flow-through system), heating is no longer an issue.

Separating the role of direct radiative heating and photolysis in modulating the atmospheric response to the amplitude of the 11-year solar cycle forcing

Abstract. The atmospheric response to the 11-year solar cycle is separated into the contributions from changes in direct radiative heating and photolysis rates using specially designed sensitivity simulations with the UM-UKCA (Unified Model coupled to the United Kingdom Chemistry and Aerosol model) chemistry–climate model. We perform a number of idealised time-slice experiments under perpetual solar maximum (SMAX) and minimum conditions (SMIN), and we find that contributions from changes in direct heating and photolysis rates are both important for determining the stratospheric shortwave heating, temperature and ozone responses to the amplitude of the 11-year solar cycle. The combined effects of the processes are found to be largely additive in the tropics but nonadditive in the Southern Hemisphere (SH) high latitudes during the dynamically active season. Our results indicate that, in contrast to the original mechanism proposed in the literature, the solar-induced changes in the horizontal shortwave heating rate gradients not only in autumn/early winter but throughout the dynamically active season are important for modulating the dynamical response to changes in solar forcing. In spring, these gradients are strongly influenced by the shortwave heating anomalies at higher southern latitudes, which are closely linked to the concurrent changes in ozone. In addition, our simulations indicate differences in the winter SH dynamical responses between the experiments. We suggest a couple of potential drivers of the simulated differences, i.e. the role of enhanced zonally asymmetric ozone heating brought about by the increased solar-induced ozone levels under SMAX and/or sensitivity of the polar dynamical response to the altitude of the anomalous radiative tendencies. All in all, our results suggest that solar-induced changes in ozone, both in the tropics/mid-latitudes and the polar regions, are important for modulating the SH dynamical response to the 11-year solar cycle. In addition, the markedly nonadditive character of the SH polar vortex response simulated in austral spring highlights the need for consistent model implementation of the solar cycle forcing in both the radiative heating and photolysis schemes.

High temperature expulsion of thermolabile groups for pore-space expansion in metal–organic frameworks

Direct radiative heating at 200 °C quantitatively converts sulfoxide-tags to desirable vinyl groups on a porous zinc(ii) metal–organic framework analogue of IRMOF-9.

Thermal stress during RTP processes and its possible effect on the light induced degradation in Cz-Si wafers

In this study, the carrier lifetime variation of p-type boron-doped Czochralski silicon (Cz-Si) wafers was investigated after a direct rapid thermal processing (RTP). Two wafers were passivated by silicon nitride (SiNx:H) layers, deposited by a PECVD system on both surfaces. Then the wafers were subjected to an RTP cycle at a peak temperature of 620 °C. The first wafer was protected (PW) from the direct radiative heating of the RTP furnace by placing the wafer between two as-cut Cz-Si shield wafers during the heat processing. The second wafer was not protected (NPW) and followed the same RTP cycle procedure. The carrier lifetime τeff was measured using the QSSPC technique before and after illumination for 5 h duration at 0.5 suns. The immediate results of the measured lifetime (τRTP) after the RTP process have shown a regeneration in the lifetime of the two wafers with the PW wafer exhibiting an important enhancement in τRTP as compared to the NPW wafer. The QSSPC measurements have indicated a good stable lifetime (τd) and a weak degradation effect was observed in the case of the PW wafer as compared to their initial lifetime value. Interferometry technique analyses have shown an enhancement in the surface roughness for the NPW wafer as compared to the protected one. Additionally, to improve the correlation between the RTP heat radiation stress and the carrier lifetime behavior, a simulation of the thermal stress and temperature profile using the finite element method on the wafers surface at RTP peak temperature of 620 °C was performed. The results confirm the reduction of the thermal stress with less heat losses for the PW wafer. Finally, the proposed method can lead to improving the lifetime of wafers by an RTP process at minimum energy costs.

The early summertime Saharan heat low: sensitivity of the radiation budget and atmospheric heating to water vapour and dust aerosol

Abstract. The Saharan heat low (SHL) is a key component of the west African climate system and an important driver of the west African monsoon across a range of timescales of variability. The physical mechanisms driving the variability in the SHL remain uncertain, although water vapour has been implicated as of primary importance. Here, we quantify the independent effects of variability in dust and water vapour on the radiation budget and atmospheric heating of the region using a radiative transfer model configured with observational input data from the Fennec field campaign at the location of Bordj Badji Mokhtar (BBM) in southern Algeria (21.4∘ N, 0.9∘ E), close to the SHL core for June 2011. Overall, we find dust aerosol and water vapour to be of similar importance in driving variability in the top-of-atmosphere (TOA) radiation budget and therefore the column-integrated heating over the SHL (∼ 7 W m−2 per standard deviation of dust aerosol optical depth – AOD). As such, we infer that SHL intensity is likely to be similarly enhanced by the effects of dust and water vapour surge events. However, the details of the processes differ. Dust generates substantial radiative cooling at the surface (∼ 11 W m−2 per standard deviation of dust AOD), presumably leading to reduced sensible heat flux in the boundary layer, which is more than compensated by direct radiative heating from shortwave (SW) absorption by dust in the dusty boundary layer. In contrast, water vapour invokes a radiative warming at the surface of ∼ 6 W m−2 per standard deviation of column-integrated water vapour in kg m−2. Net effects involve a pronounced net atmospheric radiative convergence with heating rates on average of 0.5 K day−1 and up to 6 K day−1 during synoptic/mesoscale dust events from monsoon surges and convective cold-pool outflows (“haboobs”). On this basis, we make inferences on the processes driving variability in the SHL associated with radiative and advective heating/cooling. Depending on the synoptic context over the region, processes driving variability involve both independent effects of water vapour and dust and compensating events in which dust and water vapour are co-varying. Forecast models typically have biases of up to 2 kg m−2 in column-integrated water vapour (equivalent to a change in 2.6 W m−2 TOA net flux) and typically lack variability in dust and thus are expected to poorly represent these couplings. An improved representation of dust and water vapour and quantification of associated radiative impact in models is thus imperative to further understand the SHL and related climate processes.

The evolution of zonally asymmetric austral ozone in a chemistry–climate model

Abstract. Asymmetry in the Southern Hemisphere stratospheric ozone hole is important due to both direct radiative heating and its effect on dynamics. It is also a strong indicator of the underlying quality of the stratospheric dynamics of a climate model. We investigate the simulation of the zonal asymmetry in ozone in the NIWA-UKCA atmosphere–ocean chemistry–climate model using elliptical diagnostics, a methodology used for the first time in this subject area. During spring, the region most depleted in ozone is displaced from the pole toward South America based on ERA-Interim and the model output. The model correctly simulates the direction of this displacement but significantly underestimates its magnitude. The model shows that as ozone becomes increasingly depleted over the late 20th century this asymmetry in the ozone distribution moves west, before moving east as polar ozone recovers over the course of the 21st century. Comparison with model runs in which ozone-depleting substances are held fixed at pre-ozone-hole levels shows that this shift is primarily a function of the magnitude of ozone depletion, although increases in greenhouse gases also have some effect.

B-ducted Heating of Black Widow Companions

Abstract The companions of evaporating binary pulsars (black widows and related systems) show optical emission suggesting strong heating. In a number of cases, large observed temperatures and asymmetries are inconsistent with direct radiative heating for the observed pulsar spindown power and expected distance. Here we describe a heating model in which the pulsar wind sets up an intrabinary shock (IBS) against the companion wind and magnetic field, and a portion of the shock particles duct along this field to the companion magnetic poles. We show that a variety of heating patterns, and improved fits to the observed light curves, can be obtained at expected pulsar distances and luminosities, at the expense of a handful of model parameters. We test this “IBS-B” model against three well-observed binaries and comment on the implications for system masses.

Physical Processes Controlling the Tide in the Tropical Lower Atmosphere Investigated Using a Comprehensive Numerical Model

Abstract The lower-atmospheric circulation in the tropics is strongly influenced by large-scale daily variations referred to as atmospheric solar tides. Most earlier studies have used simplified linear theory to explain daily variations in the tropics. The present study employs a comprehensive limited-area atmospheric model and revisits some longstanding issues related to atmospheric tidal dynamics. The tides in the tropical lower atmosphere are realistically simulated in the control experiment with a near-global (75°S–75°N) version of the model. Sensitivity experiments with different aspects of the solar heating suppressed showed that the semidiurnal (S2) tide near the surface can be attributed roughly equally to stratospheric and tropospheric direct solar heating and that the diurnal (S1) tide is excited almost entirely by tropospheric direct solar heating as well as solar heating of Earth’s surface. Linear theory with forcing only by direct radiative heating predicts the phase of the S2 barometric oscillation should be ~0910 LT versus the ~0945 LT phase seen in low-latitude observations. The roles of (i) convective and latent heating and (ii) mechanical dissipation, in determining the S2 phase, are assessed in the model. It is found that the former effect delays the phase by ~25 min and the latter by ~5 min; these two effects together explain the observed phase. When the model is run in limited-area domains comparable to those used in typical regional climate studies the S2, but not S1, tide is found to be significantly weaker than observed, even using atmospheric reanalysis data to drive the lateral boundaries.

A radiative transfer module for calculating photolysis rates and solar heating in climate models: Solar-J v7.5

Abstract. Solar-J is a comprehensive radiative transfer model for the solar spectrum that addresses the needs of both solar heating and photochemistry in Earth system models. Solar-J is a spectral extension of Cloud-J, a standard in many chemical models that calculates photolysis rates in the 0.18–0.8 µm region. The Cloud-J core consists of an eight-stream scattering, plane-parallel radiative transfer solver with corrections for sphericity. Cloud-J uses cloud quadrature to accurately average over correlated cloud layers. It uses the scattering phase function of aerosols and clouds expanded to eighth order and thus avoids isotropic-equivalent approximations prevalent in most solar heating codes. The spectral extension from 0.8 to 12 µm enables calculation of both scattered and absorbed sunlight and thus aerosol direct radiative effects and heating rates throughout the Earth's atmosphere.The Solar-J extension adopts the correlated-k gas absorption bins, primarily water vapor, from the shortwave Rapid Radiative Transfer Model for general circulation model (GCM) applications (RRTMG-SW). Solar-J successfully matches RRTMG-SW's tropospheric heating profile in a clear-sky, aerosol-free, tropical atmosphere. We compare both codes in cloudy atmospheres with a liquid-water stratus cloud and an ice-crystal cirrus cloud. For the stratus cloud, both models use the same physical properties, and we find a systematic low bias of about 3 % in planetary albedo across all solar zenith angles caused by RRTMG-SW's two-stream scattering. Discrepancies with the cirrus cloud using any of RRTMG-SW's three different parameterizations are as large as about 20–40 % depending on the solar zenith angles and occur throughout the atmosphere.Effectively, Solar-J has combined the best components of RRTMG-SW and Cloud-J to build a high-fidelity module for the scattering and absorption of sunlight in the Earth's atmosphere, for which the three major components – wavelength integration, scattering, and averaging over cloud fields – all have comparably small errors. More accurate solutions with Solar-J come with increased computational costs, about 5 times that of RRTMG-SW for a single atmosphere. There are options for reduced costs or computational acceleration that would bring costs down while maintaining improved fidelity and balanced errors.

The impact of seasonalities on direct radiative effects and radiative heating rates of absorbing aerosols above clouds

The impact of seasonalities on direct radiative effects (DREs) and radiative heating rates (RHRs) of absorbing aerosols above clouds in the southeast Atlantic is examined using radiative transfer calculations. For an aerosol optical thickness of 0.6 located between 0 and 4 km, a cloud optical thickness of 9.0 and a cloud effective radius of 12.8 µm at 0.55 µm located between 1 and 2 km, the diurnally averaged RHR at noon in the aerosol layer increases from ∼6.6 K day−1 in June to ∼8.9 K day−1 in October. In June (October), the RHR in the cloud layer at noon is 1.3 (1.7) K day−1 higher than the case of pristine clouds. However, an elevated aerosol layer (2–4 km) reduces the RHR by ∼0.2 K day−1 in the cloud layer relative to a pristine cloudy case. The DRE at top‐of‐atmosphere (TOA) reaches its peak when the solar zenith angle (SZA) is 54°. The DRE increases (decreases) with SZA for SZA less (greater) than 54°. The primary peak DRE is ∼29.5 W m−2 at 5.0°S 5.0°E, occurring at 0800 UTC. At noon, the DRE at TOA is ∼18.9, ∼20.5 and ∼23.1 W m−2 at 5.0°S, 15.0°S and 25.0°S along 5.0°E, respectively. This study provides data and theoretical understanding to help positioning science flights that target measurements of above‐cloud aerosol radiative effects.

The role of cloud radiative heating within the atmosphere on the high cloud amount and top‐of‐atmosphere cloud radiative effect

AbstractThe effect of cloud‐radiation interactions on cloud properties is examined in the context of a limited‐domain cloud‐resolving model. The atmospheric cloud radiative effect (ACRE) influences the areal extent of tropical high clouds in two distinct ways. The first is through direct radiative destabilization of the elevated cloud layers, mostly as a result of longwave radiation heating the cloud bottom and cooling the cloud top. The second effect is radiative stabilization, whereby cloud radiative heating of the atmospheric column stabilizes the atmosphere to deep convection. In limited area domain simulations, the stabilizing (or indirect) effect is the dominant role of the cloud radiative heating, thus reducing the cloud cover in simulations where ACRE is included compared to those where it is removed. Direct cloud radiative heating increases high cloud fraction, decreases mean cloud optical depth, and increases cloud top temperature. The indirect cloud radiative heating decreases high cloud fraction, but also decreases mean cloud optical depth and increases cloud top temperature. The combination of these effects increases the top‐of‐atmosphere cloud radiative effect. In mock‐Walker circulation experiments, the decrease in high cloud amount owing to radiative stabilization tends to cancel out the increase in high cloud amount owing to the destabilization within the cloud layer. The changes in cloud optical depth and cloud top pressure, however, are similar to those produced in the limited area domain simulations.

A Lagrangian view of longwave radiative fluxes for understanding the direct heating response to a CO2 increase

AbstractThis study puts forward a Lagrangian view of downward and upward longwave (LW) fluxes to improve our physical understanding of the influence of key factors on the downward and upward LW fluxes' response to an increase of CO2. To facilitate such a Lagrangian view, we introduce a new saturation‐level concept based on the LW radiative transfer theory. The Lagrangian view and the new saturation‐level concept enable us to provide, under a single framework, a general radiative transfer explanation of the spatial variation (e.g., stratospheric cooling and lower tropospheric warming) of the direct radiative heating response to an increase of the CO2 concentration. Following the saturation‐level concept, the radiatively unsaturated nature of the downward LW flux in the upper stratosphere, due to the lack of a LW source at the top of the atmosphere, is attributed as the root factor that leads to a cooling of the upper stratosphere in direct response to a CO2 increase. The upward LW flux perturbation further enhances the cooling as a result of the negative lapse rate in the stratosphere but is of secondary importance. Furthermore, this study indicates that ozone is not a necessary ingredient for stratospheric cooling to occur, and the stratospheric cooling is therefore a fundamental consequence of a CO2 increase. The unperturbed vertical profile of water vapor is important only in the lower troposphere, where the relatively large concentration of water vapor leads to a downward LW flux perturbation that warms the lower troposphere at the expense of the surface warming.