Continuous wave (CW) and Q-switched diode-pumped laser operation of Yb3+:NaLa(MoO4)2 single crystal was to our knowledge, demonstrated for the first time. A CW output power of 220 mW and slope efficiency of 46% were obtained. Q-switched laser operation was achieved with a pulse duration of 60 ns average output power of 70 mW and slope efficiency of 22%.
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