Experimental vibrational Raman, vibrational Raman optical activity (VROA), and dimensionless circular intensity difference (CID) spectra are analyzed with quantum chemical (QC) predictions of the corresponding spectra using the B3LYP functional and the aug-cc-pVDZ basis set, for five bicyclic terpenes as test cases. The experimentally measured vibrational Raman and VROA spectra have arbitrary y-axis intensities, because of their dependence on instrumental parameters. As a result, the absolute magnitudes of intensities in experimental and calculated vibrational Raman or vibrational ROA spectra are not normally analyzed. However, the experimental dimensionless CID spectrum is independent of the instrumental parameters and can be evaluated quantitatively with corresponding QC predicted CID spectrum. The similarity overlaps between experimental and quantum chemical predictions of vibrational Raman, VROA, and dimensionless CID spectra are evaluated. The quantum chemical predictions of dimensionless CID spectral magnitudes at B3LYP/aug-ccpVDZ level match well with the corresponding experimental magnitudes. The individual anisotropic contributions to VROA and CID spectra are also presented. The anisotropic contribution involving electric dipole-electric quadrupole polarizability derivative tensor is relatively smaller than that involving electric dipole-magnetic dipole polarizability derivative tensor. A new format, which contains all of the information needed for the spectral analysis, has been advanced for presenting the vibrational Raman, VROA, and CID spectra and their similarity analysis with corresponding QC-predicted spectra. Copyright © 2016 John Wiley & Sons, Ltd.