Degree Of Circular Polarization Research Articles

Interlayer exciton valley polarization dynamics in large magnetic fields

In van der Waals heterostructures (HS) consisting of stacked MoSe$_2$ and WSe$_2$ monolayers, optically bright interlayer excitons (ILE) can be observed when the constituent layers are crystallographically aligned. The symmetry of the monolayers allows for two different types of alignment, in which the momentum-direct interlayer transitions are either valley-conserving (R-type alignment) or changing the valley index (H-type anti-alignment). Here, we study the valley polarization dynamics of ILE in magnetic fields up to 30~Tesla by time-resolved photoluminescence (PL). For all ILE types, we find a finite initial PL circular degree of polarization ($DoP$) after unpolarized excitation in applied magnetic fields. For ILE in H-type HS, we observe a systematic increase of the PL $DoP$ with time in applied magnetic fields, which saturates at values close to unity for the largest fields. By contrast, for ILE in R-type HS, the PL $DoP$ shows a decrease and a zero crossing before saturating with opposite polarization. This unintuitive behavior can be explained by a model considering the different ILE states in H- and R-type HS and their selection rules coupling PL helicity and valley polarization.

Electrical control of orbital and vibrational interlayer coupling in bi- and trilayer 2H−MoS2

Manipulating electronic interlayer coupling in layered van der Waals (vdW) materials is essential for designing opto-electronic devices. Here, we control vibrational and electronic interlayer coupling in bi- and trilayer 2H-MoS$_2$ using large external electric fields in a micro-capacitor device. The electric field lifts Raman selection rules and activates phonon modes in excellent agreement with ab-initio calculations. Through polarization resolved photoluminescence spectroscopy in the same device, we observe a strongly tunable valley dichroism with maximum circular polarization degree of $\sim 60\%$ in bilayer and $\sim 35\%$ in trilayer MoS$_2$ that are fully consistent with a rate equation model which includes input from electronic band structure calculations. We identify the highly delocalized electron wave function between the layers close to the high symmetry $Q$ points as the origin of the tunable circular dichroism. Our results demonstrate the possibility of electric field tunable interlayer coupling for controlling emergent spin-valley physics and hybridization driven effects in vdW materials and their heterostructures.

One‐Interlayer‐Twisted Multilayer MoS2 Moiré Superlattices

AbstractTwist angle provides a new degree of freedom for 2D material modifications. In principle, the intrinsic properties of twisted multilayers can be regulated by twist angle between each adjacent layer and thus have greater tunability than widely studied bilayer structures. Considering its complexity, it is important to first investigate the simplest twisted multilayers with only one interface twisted. In this work, multilayer Moiré superlattices with only one twisted interface via paraffin‐assisted folding of non‐twisted stacked (highly symmetrically stacked) multilayer MoS2 are successfully fabricated, and their twist‐angle dependent optical properties are systematically studied. Compared to non‐twisted stacked multilayer MoS2, the one‐interface‐twisted multilayers show a 2–3.5 times higher PL intensity, and their interlayer coupling, indirect bandgap, and degree of circular polarization (DOCP) are tunable by twist angle. Notably, the DOCP for the one‐interface‐twisted four‐layer (folded bilayer) can reach 86%, which is the highest value ever reported for transition metal dichalcogenide homostructures above liquid nitrogen temperature. This work provides a solid base for understanding twist‐angle dependent properties of twisted multilayer 2D‐materials.

Design of a dielectric chiral micro-structured fiber applied in a fiber optic current sensor

During the process of drawing the screwed silicon-based fiber, there will be a uniform rotation rate in it, which results in a decrease of circular polarization degree of the fiber. In order to solve this problem, we presented a kind of dielectric chiral micro-structured fiber owing higher circular polarization degree. Meanwhile, the air holes of fiber will collapse during the progress of fiber drawing, which will change the position of air holes. As a result, the circular polarization degree of the fiber decreases. In order to reduce the change of circular polarization degree caused by the position fluctuation of the air holes, a highly symmetrical micro-structured dielectric chiral fiber was firstly designed in this paper. Then, we established a physical error model considering the fluctuation of the air holes’ position which was the design basis of the air holes’ position, size, and chiral parameters of the specific microstructure fiber. Next, comparing the circular polarization degree S3 of screwed silicon-based fiber and that of the dielectric chiral micro-structured fiber by simulation, it was proved that the dielectric chiral micro-structured fiber we designed has a higher circular polarization degree S3 than that of screwed silicon-based fiber. Finally, we applied the fiber designed in this paper as the fiber sensing coil in a fiber optic current sensor, and compared it with the fiber optic current sensor utilizing the original fiber sensing coil in ratio error. The simulation results proved that compared with the original system, dielectric chiral micro-structured fiber utilized as the fiber sensing coil in a fiber optic current sensor will decrease the ratio error by an order of magnitude in theory.

Machine Learning‐Based Optimization of Chiral Photonic Nanostructures: Evolution‐ and Neural Network‐Based Designs

Chiral photonics opens new pathways to manipulate light–matter interactions and tailor the optical response of metasurfaces and ‐materials by nanostructuring nontrivial patterns. Chirality of matter, such as that of molecules, and light, which in the simplest case is given by the handedness of circular polarization, have attracted much attention for applications in chemistry, nanophotonics and optical information processing. The design of chiral photonic structures using two machine learning methods, the evolutionary algorithm, and neural network approach, for rapid and efficient optimization of optical properties for dielectric metasurfaces, is reported. The design recipes obtained for visible light in the range of transition‐metal dichalcogenide exciton resonances show a frequency‐dependent modification in the reflected light's degree of circular polarization, that is represented by the difference between left‐ and right‐circularly polarized intensity. Our results suggest the facile fabrication and characterization of optical nanopatterned reflectors for chirality‐sensitive light–matter coupling scenarios employing tungsten disulfide as possible active material with features such as valley Hall effect and optical valley coherence.

Observation of the spin-Hall effect in Pt/GaAs by circular polarized photoconductivity

Electrically generated spin accumulation due to the spin Hall effect of Pt/GaAs is detected by circular polarized photoconductivity (CPPC), which shows electron spins with different polarizations accumulated around opposite sample boundaries. An optical absorption model incorporating spin is used to explain these features. The detailed analysis of the observed degree of circular polarization of the photocurrent strongly suggests that Pt and GaAs have the same spin accumulation length in the Pt/GaAs heterostructure.

Circularly Polarized Electroluminescence of InGaAs/GaAs/CoPt Spin Light Emitting Diodes Placed in a Strong and Weak Magnetic Field

A comparative study of the circular polarization degree dependences on external magnetic field was carried out in spin light-emitting diodes including semiconductor InGaAs/GaAs heterostructure and a magnetic CoPt contact and in control non-magnetic structures with an Au contact. In a weak magnetic field, the magnetic field dependence of electroluminescence circular polarization degree is similar to the magnetic field dependence of magnetization: it represents a hysteresis loop with saturation in a field of ~0.3 T. In a strong magnetic field, an additional linear contribution to the circular polarization degree is detected. This contribution is associated with the Zeeman splitting of energy levels. The magnitude of the linear contribution depends on the position of the quantum well relative to the ferromagnet/semiconductor interface. The obtained dependence is associated with the influence of the magnetic field of the inhomogeneously magnetized CoPt electrode on the spin relaxation time of carriers. Keywords: spin injection, quantum well, Zeeman splitting.

Циркулярно-поляризованная электролюминесценция спиновых светоизлучающих диодов InGaAs/GaAs/CoPt, помещенных в сильное и слабое магнитное поле

A comparative study of the circular polarization degree dependences on external magnetic field was carried out in spin light-emitting diodes including semiconductor InGaAs/GaAs heterostructure and a magnetic CoPt contact and in control non-magnetic structures with an Au contact. In a weak magnetic field, the magnetic field dependence of electroluminescence circular polarization degree is similar to the magnetic field dependence of magnetization: it represents a hysteresis loop with saturation in a field of ~ 0.3 T. In a strong magnetic field, an additional linear contribution to the circular polarization degree is detected. This contribution is associated with the Zeeman splitting of energy levels. The magnitude of the linear contribution depends on the position of the quantum well relative to the ferromagnet/semiconductor interface. The obtained dependence is associated with the influence of the magnetic field of the inhomogeneously magnetized CoPt electrode on the spin relaxation time of carriers.

Characterization of output circular polarization degree in lowcost asymmetric metasurfaces

Addition of asymmetry in plasmonic nanostructures can lead to chiro-optical phenomena, usually monitored as different absorption of left and right polarization, i.e. circular dichroism. Moreover, interesting features arise when the nanostructure changes the polarization state of the input beam. In this work, we perform extrinsic chirality characterization in a widely tuneable near-infrared range, by monitoring both polarization of the input and of the transmitted beam. We characterize low-cost metasurfaces based on polystyrene nanospheres asymmetrically covered by Ag, by exciting them at different angle of incidence with left, right and linear polarization. We then resolve the circular polarization degree of the transmitted beam, demonstrating resonance-governed circular polarization degree in the output, showing the interplay of both intrinsic and extrinsic chirality.

In situ tunable circular dichroism of flexible chiral metasurfaces composed of plasmonic nanorod trimers.

The circularly polarized light source is one of the keys to chiral photonic circuits and systems. However, it is difficult to integrate conventional light-emitting devices with circular polarization converters directly into compact chip-scale photonic systems partly because of their bulky structures. In this study, in situ optical chirality tunable nanorod trimer metasurfaces consisting of two types of nanorod dimers are demonstrated and integrated with a flexible polydimethylsiloxane (PDMS) substrate. The optical chirality variations originating from the tunable asymmetricity of nanorod trimers under different stretching scenarios are evaluated. Through the processes, the gap distances between nanorods are varied, and the degree of circular polarization of the transmitted wave is controlled through the manipulation of localized surface plasmon resonance (LSPR) coupling. The results reveal the circular dichroism tunability and durability of fabricated chiral metasurfaces which can be important elements for chip-scale flexible optoelectronic integrated circuits for sensing, display and communication applications.

Plasmonic nanobar-on-mirror antenna with giant local chirality: a new platform for ultrafast chiral single-photon emission.

Providing an additional degree of freedom for binary information encoding and nonreciprocal information transmission, chiral single photons have become a new research frontier in quantum optics. Without using complex external conditions (e.g., magnetic field, low temperature), coupling emitters to chiral optical antennas has become a promising strategy to efficiently convert single photons from linear to circular polarization states. For ideal chiral single-photon sources, essential properties such as giant Purcell factor, large degree of circular polarization (DCP), and high collection efficiency are highly demanded. Herein, to meet these combined requirements, we propose an emitter-coupled nanobar-on-mirror antenna platform with significant local chirality acquired from the broken symmetry, as well as the giant Purcell factor owing to its ultrasmall mode volume. An emitter embedded at the corner in the gap exhibits above 3 orders of magnitude enhancement of the chiral spontaneous emission with more than 80% collection efficiency, along with up to 70% DCP. Compatible with a myriad of nanoscale quantum emitters (e.g. transition metal dichalcogenides, color centers, quantum dots, etc.), this platform, not only manifests the potential for realizing ultrafast chiral single-photon generator towards GHz and THz operation speed but also provides versatile testbeds for investigating chiral light-matter interaction at the single-quantum level.

Experiments and simulations of chiro-optical response in lowcost nanohole arrays in silver

2D metasurfaces based on periodic nanoholes in metal have been proposed in various plasmonic platforms. Specifically, their resonant features have led to applications spanning in biosensing. Here we investigate additional degree of freedom in elliptical nanohole arrays with hexagonal geometry: chiro-optical effects. Namely, the in-plane asymmetry and a slightly elliptical shape of nanoholes were previously shown to differently extinct light of opposite handedness, even at normal incidence. We now fully characterize nanoholes in Ag, fabricated by low-cost nanosphere lithography. We first measure the dependence of the transmitted intensity for opposite handedness, in a broad spectral and angle of incidence range. We then resolve the circular polarization degree of the transmitted light when the nanohole array is excited with linear polarization. Finally, we numerically investigate the origin of the chiro-optical effect at the nanoscale. We believe that circular polarization resolving of the transmitted degree could be further adapted as a highly sensitive tool in chiral sensing.

Single charge control of localized excitons in heterostructures with ferroelectric thin films and two-dimensional transition metal dichalcogenides.

Single charge control of localized excitons (LXs) in two-dimensional transition metal dichalcogenides (TMDCs) is crucial for potential applications in quantum information processing and storage. However, traditional electrostatic doping method by applying metallic gates onto TMDCs may cause inhomogeneous charge distribution, optical quenching, and energy loss. Herein, by locally controlling the ferroelectric polarization of the ferroelectric thin film BiFeO3 (BFO) with a scanning probe, we can deterministically manipulate the doping type of monolayer WSe2 to achieve p-type and n-type doping. This nonvolatile approach can maintain the doping type and hold the localized excitonic charges for a long time without applied voltage. Our work demonstrated that the ferroelectric polarization of BFO can control the charges of LXs effectively. Neutral and charged LXs have been observed in different ferroelectric polarization regions, confirmed by magnetic optical measurement. Highly circular polarization degree with 90% photon emission from these quantum emitters was achieved in high magnetic fields. Controlling the single charge of LXs in a non-volatile way shows a great potential for deterministic photon emission with desired charge states for photonic long-term memory.

High-efficiency circularly polarized green light emission from GaN-based laser diodes integrated with GaN metasurface quarterwave plate

We demonstrated high efficient circularly polarized emission from the InGaN/GaN quantum well green laser diode (LD) integrated with GaN metasurface quarterwave plates. Optical properties of the nanoscale thin GaN nanograting metasurface were numerically studied and optimized for a quarter-wave plate. The fabricated nanogratings then were integrated on the emission facet of the LD. Both conversion efficiency and the polarization state of the device were measured, and the conversion efficiency is around 80% while the degree of circular polarization is maintained around 0.99. Our results of achieving a high degree of polarization and a high conversion efficiency at the integrated LD device pay the way for multi-functional applications in bio-imaging, submarine optical communication, quantum communication, and holographic display.

Accounting for light source angular distribution in backscattering Mueller matrix interpretation using double-planar small-angle scattering trajectory approximation

We extend the double-planar small-angle scattering trajectory approximation to account for the influence of the light source angular distribution on the polarization patterns of lidar backscattering returns from highly forward-peaked scattering medium. We formulate the lidar Mueller matrix return by introducing the azimuthal angle of emitting light relative to the meridian plane of receiving direction. The derived formulas have exactly the same forms as that for the vertical pencil-like light source. The essential difference is that the azimuthal angle of the emitting light can adjust the linear relation between the normalized Mueller matrix and single backscattering phase matrix as the dihedral angle between the outgoing and return forward scattering plane does too. The emitting azimuth effect can be significantly stronger than the effect of the dihedral angle of the two forward scattering planes when the receiving directions are within the cone of divergence. It can make the normalized elements of the Mueller matrix being zeros except those diagonal elements describing the linear and circular polarization degrees.

Toward the development of portable light emitting diode-based polarization spectroscopy tools for breast cancer diagnosis.

A robust, affordable and portable light emitting diode-based diagnostic tools (POLS-NIRDx) using a polarization-sensitive (linear as well as circular polarization) technique were designed and developed to quantify the degree of linear polarization (DOLP), degree of circular polarization (DOCP). The study was performed on malignant (invasive ductal carcinoma) and adjacent normal ex-vivo biopsy tissues excised from N=10 patients at the operating wavelengths of 850 and 940 nm. The average DOLP and DOCP values were lower for malignant than adjacent normal while operating at 850 and 940 nm. The highest accuracy was observed for DOLP (100%) and DOCP (80%) while operating at 850 nm, which reduced (80% for DOLP and 65% for DOCP) at 940 nm. This pilot study can be utilized as a differentiating factor to delineate malignant tissues from adjacent normal tissues.

Circular Dichroism in the Photoionization of Unpolarized Atoms by Two Crossing Photon Beams

The polarization dependence of the photoionization probability was analyzed in the case when a randomly oriented atom is irradiated by two crossing polarized monochromatic photon beams with the same frequency. It was found that the angular distributions of photoelectrons exhibit the effect of circular dichroism (CD), which consists of the dependence of the photoionization probability on the sign of the circular polarization degree of each beam. We demonstrate that the CD effect exists only for coherent crossing photon beams. It was shown that CD effects are strongly dependent on the phase difference between the electric field vectors of the photon beams and have a quite large magnitude. The possibilities of the experimental observation of CD effects are discussed.

Probing dark matter-cosmic ray electron interactions with circular polarisation of photons

Conventional indirect dark matter (DM) searches look for an excess in the electromagnetic emission from the sky that cannot be attributed to known astrophysical sources, but its polarisation has not been explored to date. In this proceeding, I argue that photon polarisation is an important feature to understand new physics interactions. Circular polarisation can be generated from Beyond the Standard Model interactions if they violate parity and there is an asymmetry in the number density of the initial state particles which participate in the interaction. I consider a simplified model for fermionic (Majorana) DM and study the circularly polarised gamma rays from DM cosmic ray electron interactions. I study the differential flux of positive and negative polarised photons from the Galactic Centre and show that the degree of circular polarization can reach up to 90%. Finally, I discuss the detection prospects of this signal in future experiments.

Circular polarisation of gamma rays as a probe of dark matter interactions with cosmic ray electrons

Conventional indirect dark matter (DM) searches look for an excess in the electromagnetic emission from the sky that cannot be attributed to known astrophysical sources. Here, we argue that the photon polarisation is an important feature to understand new physics interactions and can be exploited to improve our sensitivity to DM. In particular, circular polarisation can be generated from Beyond the Standard Model interactions if they violate parity and there is an asymmetry in the number of particles which participate in the interaction. In this work, we consider a simplified model for fermionic (Majorana) DM and study the circularly polarised gamma rays below 10 GeV from the scattering of cosmic ray electrons on DM. We calculate the differential flux of positive and negative polarised photons from the Galactic Center and show that the degree of circular polarisation can reach up to 90%. Finally, once collider and DM constraints have been taken into account, we estimate the required sensitivity from future experiments to detect this signal finding that, although a distinctive peak will be present in the photon flux spectrum, a near future observation is unlikely. However, different sources or models not considered in this work could provide higher intensity fluxes, leading to a possible detection by e-ASTROGAM. In the event of a discovery, we argue that the polarisation fraction is a valuable characterisation feature of the new sector.

Topological Control of 2D Perovskite Emission in the Strong Coupling Regime.

Momentum space topology can be exploited to manipulate radiation in real space. Here we demonstrate topological control of 2D perovskite emission in the strong coupling regime via polaritonic bound states in the continuum (BICs). Topological polarization singularities (polarization vortices and circularly polarized eigenstates) are observed at room temperature by measuring the Stokes parameters of photoluminescence in momentum space. Particularly, in symmetry-broken structures, a very large degree of circular polarization (DCP) of ∼0.835 is achieved in the perovskite emission, which is the largest in perovskite materials to our knowledge. In the strong coupling regime, lower polariton modes shift to the low-loss spectral region, resulting in strong emission enhancement and large DCP. Our reciprocity analysis reveals that DCP is limited by material absorption at the emission wavelength. Polaritonic BICs based on 2D perovskite materials combine unique topological features with exceptional material properties and may become a promising platform for active nanophotonic devices.