Decay Constant Research Articles

Rapid predictive dosimetry for Second Strike prescription based on whole body radioiodine kinetics in differentiated thyroid cancer.

In systemic radionuclide therapy such as radioiodine (I-131) for differentiated thyroid cancer, post-therapy dosimetry is essential to verify pre-therapy predictions, which in turn informs the next treatment. However, post-therapy multi-time point dosimetry is resource intensive and unfeasible in many institutions. We devised a schema of rapid predictive dosimetry by circumventing post-First Strike multi-time point dosimetry with carefully assigned gestalt values of predicted kinetics to personalise the Second Strike prescription. Verification is performed after the First Strike. Patient-specific time-activity curve is plotted from serial measurements of whole body exposure rates to obtain its decay constant; its inverse is the whole body Time Integrated Activity Coefficient (TIAC). The percentage of whole body TIAC attributed to blood is carefully assigned by gestalt based on population kinetics tabulated in Part 1, adjusted by any metastasis on I-131 whole body scintigraphy. Marrow absorbed dose is calculated by EANM formularism. Lung safety threshold at 48h post-therapy is linearly scaled by height, where the patient's risk of lung radiotoxicity is revealed from the whole body time-activity curve value at 48h. Predictive prescription for the second I-131 fraction (Second Strike) is by careful gestalt assessment based on predicted kinetics, remaining marrow and lung tolerance, marrow dose rate constraint per fraction (0.265 Gy/h), local regulatory and facility requirements in relation to radiation protection. Tumour dosimetry is obviated under the assumption of severe tumour absorbed dose heterogeneity. The final prescription for the Second Strike is usually the lowest I-131 activity amongst all clinical, dosimetric and regulatory constraints. This schema is incorporated into a Predictive Calculator spreadsheet for rapid predictive dosimetry, and is freely available. Calculations may be completed within minutes to generate personalised predictive prescriptions, making it feasible for routine clinical implementation. Our innovative schema of rapid verification and predictive dosimetry bridges the technological gap between empiric vs theranostic prescription to help institutions modernise. Its expeditious design makes this schema feasible to be integrated into the routine clinical workflow. Its predictive estimates provide invaluable dosimetric insight to inform the next I-131 fraction, allowing every prescription to be scientifically rationalised and personalised according to individual circumstances.

Shallow conductance decay along the heme array of a single tetraheme protein wire.

Multiheme cytochromes (MHCs) are the building blocks of highly conductive micrometre-long supramolecular wires found in so-called electrical bacteria. Recent studies have revealed that these proteins possess a long supramolecular array of closely packed heme cofactors along the main molecular axis alternating between perpendicular and stacking configurations (TST = T-shaped, stacked, T-shaped). While TST arrays have been identified as the likely electron conduit, the mechanisms of outstanding long-range charge transport observed in these structures remain unknown. Here we study charge transport on individual small tetraheme cytochromes (STCs) containing a single TST heme array. Individual STCs are trapped in a controllable nanoscale tunnelling gap. By modulating the tunnelling gap separation, we are able to selectively probe four different electron pathways involving 1, 2, 3 and 4 heme cofactors, respectively, leading to the determination of the electron tunnelling decay constant along the TST heme motif. Conductance calculations of selected single-STC junctions are in excellent agreement with experiments and suggest a mechanism of electron tunnelling with shallow length decay constant through an individual STC. These results demonstrate that an individual TST motif supporting electron tunnelling might contribute to a tunnelling-assisted charge transport diffusion mechanism in larger TST associations.

Decay rate changes in radioactive gamma emission as affected by 18 MeV proton cyclotron

Previous efforts to investigate changes in the decay constants of radioactive nuclides discovered that solar flares can temporarily alter radioactive decay rates. Thus, discerning whether external factors affect radioactive decay rates is vital for understanding nuclear processes. This study sought to explore the effect of neutrinos on radioactive nuclei by constructing a gamma radiation detection system that employs a radioactive source in front of a neutrino emission system. Responding to cyclotron operations, each of the four detection systems registered gamma count rate decreases. The results of this study confirm that rises in neutrino flux affected the decay rates of the examined radioactive nuclides. Here we provide significant evidence that neutrinos affect the radioactive decay process. Neutrino detection is challenging due to the minuscule absorption in a stable nucleus. However, the study found a greater probability of radionuclides interaction with the neutrino.

Temperature-dependent excited states for detecting reversible phase transitions in 2D lead(II) iodide perovskites.

Significant interest exists in water-tolerant 2D lead iodide perovskites owing to their stability and proven potential in photovoltaic and photonic applications. These materials have solid-state phase transitions that are accessible below 100 °C. Here, the study witnesses the multiple phase transitions of the last members of a series of organic-inorganic hybrid materials, [(CnH2n+1NH3)2PbI4], with even n as n = 14, 16, and 18, once again. By employing temperature-dependent steady-state photoluminescence (PL) and temperature-dependent time-resolved photoluminescence (TRPL) spectroscopy in the temperature range of -18 to +90 °C and at -196 °C, we explore the thermal responses of these materials. The investigation reveals reversible phase transitions occurring between room temperature (RT) and elevated temperatures, impacting the optical properties and emitting colors of the perovskite compounds. The longer the alkyl chain, the higher the phase transition temperature, attributed to increased conformational disorder and enhanced perovskite symmetry. The decay constants for all compounds are very close in value, which confirms the underlying excited-state dynamics, pointing to contributions primarily from inorganic components across different phases. We anticipate that our results on the detection of phase transitions in 2D perovskites will not only motivate the use of these techniques for detecting phase transitions but also would help to understand their excited states in more details to selectively use them for solar cell and next-generation display technologies.

Delayed photodissociation of the tin cluster Sn22.

Millisecond-delayed photodissociation of gas-phase Sn22- clusters stored in a Penning trap is investigated as a function of excitation energy. Sn15- is the only significant charged fragment, indicative of the break-off of neutral heptamers. Fits of the time-resolved fragmentation require a distribution of decay constants, caused by the finite width of the internal energy distribution of the cluster ensemble prior to photoexcitation. A lower limit for the dissociation energy for the loss of Sn7 is determined to be 2.1(1) eV, a factor of two above literature quantum chemical calculations.

Tracking Li atoms in real-time with ultra-fast NMR simulations.

We present for the first time a multiscale machine learning approach to jointly simulate atomic structure and dynamics with the corresponding solid state Nuclear Magnetic Resonance (ssNMR) observables. We study the use-case of spin-alignment echo (SAE) NMR for exploring Li-ion diffusion within the solid state electrolyte material Li3PS4 (LPS) by calculating quadrupolar frequencies of 7Li. SAE NMR probes long-range dynamics down to microsecond-timescale hopping processes. Therefore only a few machine learning force field schemes are able to capture the time- and length scales required for accurate comparison with experimental results. By using a new class of machine learning interatomic potentials, known as ultra-fast potentials (UFPs), we are able to efficiently access timescales beyond the microsecond regime. In tandem, we have developed a machine learning model for predicting the full 7Li electric field gradient (EFG) tensors in LPS. By combining the long timescale trajectories from the UFP with our model for 7Li EFG tensors, we are able to extract the autocorrelation function (ACF) for 7Li quadrupolar frequencies during Li diffusion. We extract the decay constants from the ACF for both crystalline β-LPS and amorphous LPS, and find that the predicted Li hopping rates are on the same order of magnitude as those predicted from the Li dynamics. This demonstrates the potential for machine learning to finally make predictions on experimentally relevant timescales and temperatures, and opens a new avenue of NMR crystallography: using machine learning dynamical NMR simulations for accessing polycrystalline and glass ceramic materials.

Facilitation of motor adaptation using multiple gait rehabilitation interventions.

The rate of adjustment in a movement, driven by feedback error, is referred to as the adaptation rate, and the rate of recovery of a newly adapted movement to its unperturbed condition is called the de-adaptation rate. The rates of adaptation and de-adaptation are dependent on the training mechanism and intrinsic factors such as the participant's sensorimotor abilities. This study investigated the facilitation of the motor adaptation and de-adaptation processes for spatiotemporal features of an asymmetric gait pattern by sequentially applying split-belt treadmill (SBT) and asymmetric rhythmic auditory cueing (ARAC). Two sessions tested the individual gait characteristics of SBT and ARAC, and the remaining four sessions consisted of applying the two interventions sequentially during training. The adjustment process to the second intervention is referred to as "re-adaptation" and is driven by feedback error associated with the second intervention. Ten healthy individuals participated in the randomized six-session trial. Spatiotemporal asymmetries during the adaptation and post-adaptation (when intervention is removed) stages were fitted into a two-component exponential model that reflects the explicit and implicit adaptation processes. A double component was shown to fit better than a single-component model. The decay constants of the model were indicative of the corresponding timescales and compared between trials. Results revealed that the explicit (fast) component of adaptation to ARAC was reduced for step length and step time when applied after SBT. Contrarily, the explicit component of adaptation to SBT was increased when it was applied after ARAC for step length. Additionally, the implicit (slow) component of adaptation to SBT was inhibited when applied incongruently after ARAC for step time. These outcomes show that the role of working motor memory as a translational tool between different gait interventions is dependent on (i) the adaptation mechanisms associated with the interventions, (ii) the targeted motor outcome of the interventions; the effects of factors (i) and (ii) are specific to the explicit and implicit components of the adaptation processes; these effects are unique to spatial and temporal gait characteristics.

Dilute axion stars converting to photons in the Milky Way’s magnetic field

In this paper we examine the possibility of dilute axion stars converting to photons in the weak, large-scale magnetic field of the Milky Way and show that they can resonate with the surrounding plasma and produce a sizable signal. We consider two possibilities for the plasma: free electrons and HII regions. In the former case, we argue that the frequency of the photons will be too small to be observed even by space-based radio telescopes. In the latter case, their frequency is larger, safely above the solar wind cut-off. We provide an estimate of the flux as a function of the decay constant and show that for fa< 2 × 1011 GeV, the signal will be above the radio emission of the solar system’s planets and it could potentially be detected by the NCLE instrument which is on board the Chang’e-4 spacecraft. Finally, we calculate the time scale of decay of the axion star and demonstrate that back-reaction can be neglected for all physically interesting values of the decay constant, while the minimum time scale of decay is in the order of a few hours.

Feasibility of Kelvin probe force microscopy to measure the surface potential decay of polystyrene film due to relative humidity

AbstractThe feasibility of measuring the surface potential decay of polystyrene (PS) film is investigated at room temperature by using Kelvin probe force microscopy (KPFM). The PS film was charged by an ion injection method utilizing Bruker's atomic force microscope (AFM) Nanoman module with a pulse duration of 1 ms, SCM‐PIT electrically conductive probe, and a voltage pulse of −250 mV. The surface potential decayed linearly on a semi‐log scale with time, where the time decay constant was quantified for relative humidity (RH) = 5% by KPFM at room temperature. The surface potential decayed due to the interaction of the PS film with the hydronium ions available in the environment. Furthermore, the effect of the material forms (film vs. microspheres) on the time decay constant at RH = 5% was investigated. The time decay constants measured using different methods exhibited excellent correlation with the AFM‐KPFM. This also confirmed that the results are independent of the material form (microspheres vs. film form). As a result, the proposed method can be used to measure the effect of RH for any PS surface (i.e., particles of various sizes and films) exposed to these environmental conditions.

Polycyclic Aromatic Hydrocarbons (PAHs) in Wildfire Smoke Accumulate on Indoor Materials and Create Postsmoke Event Exposure Pathways.

Wildfire smoke contains PAHs that, after infiltrating indoors, accumulate on indoor materials through particle deposition and partitioning from air. We report the magnitude and persistence of select surface associated PAHs on three common indoor materials: glass, cotton, and mechanical air filter media. Materials were loaded with PAHs through both spiking with standards and exposure to a wildfire smoke proxy. Loaded materials were aged indoors over ∼4 months to determine PAH persistence. For materials spiked with standards, total PAH decay rates were 0.010 ± 0.002, 0.025 ± 0.005, and 0.051 ± 0.009 day-1, for mechanical air filter media, glass, and cotton, respectively. PAH decay on smoke-exposed samples is consistent with that predicated by decay constants from spiked materials. Decay curves of smoke loaded samples show that PAH surface concentrations are elevated above background for ∼40 days after the smoke clears. Cleaning processes efficiently remove PAHs, with reductions of 71% and 62% after cleaning smoke-exposed glass with ethanol and a commercial cleaner, respectively. Laundering smoke-exposed cotton in a washing machine and heated drying removed 48% of PAHs. An exposure assessment indicates that both inhalation and dermal PAH exposure pathways may be relevant following wildfire smoke events.

Nature of X(3872) from its radiative decay

We study the radiative decay of X(3872) based on the assumption that X(3872) is regarded as a cc‾ charmonium with quantum number JPC=1++ (J,P,C represent the spin, parity and charge conjugation, respectively). The form factors of X(3872) transitions to J/ψγ and ψ′γ (ψ′ denotes ψ(2S) throughout the paper) are calculated in the framework of the covariant light-front quark model. The phenomenological wave function of a meson depends on the parameter β, whose inverse essentially describes the confinement scale. In the present work, the parameters β for the vector J/ψ and ψ′ mesons will be determined through their decay constants, which are obtained from the experimental values of their partial decay widths to the electron-positron pair. For X(3872), we determined the value of β by the decay width of X(3872)→ψ′γ. Then, we examined the width of X(3872)→J/ψγ in a manner of parameter-free prediction and compared it with the experimental value. As a result, an inconsistency or contradiction occurs between the widths of X(3872)→J/ψγ and X(3872)→ψ′γ. We thus conclude that X(3872) cannot be a pure cc‾ resonance and that other components are necessary in its wave function.

Air Purification Study Based on the Adhesion Effect between Low-Curvature Liquid Surfaces and Air Convection Friction

Rapid urbanization and industrialization have heightened concerns about air quality worldwide. Conventional air purification methods, reliant on chemicals or energy-intensive processes, fall short in open spaces and in combating emerging pollutants. Addressing these limitations, this study presents a novel water-film air purification prototype leveraging the adhesion between low-curvature liquid surfaces and air convection friction. Uniquely designed, this prototype effectively targets toxic gases (e.g., formaldehyde, SO2, NO2) and particulate matter (such as PM2.5) while allowing continuous airflow. This research explores the adhesion and sedimentation capabilities of a low-curvature water solution surface under convection friction, reducing the surface energy to remove airborne pollutants efficiently. The prototype was able to reduce the initial concentration in a 30 m³ chamber within 180 min by 91% for formaldehyde, 78% for nitrogen dioxide (NO2), 99% for sulfur dioxide (SO2), and 96% for PM2.5. Experimentally validated indicators—decay constants, CADR, and purification efficiency—enable a comprehensive evaluation of the purification device, demonstrating its efficacy in mitigating air pollution. This innovative design, which is cost-effective due to its use of easily accessible components and water as the primary medium, indicates strong potential for large-scale deployment. This study points to an environmentally friendly and economical approach to air purification, shedding light on a promising direction for enhancing indoor air quality. Further optimization and exploration of diverse pollutants and environmental conditions will propel the practical applications of this pioneering technology.

Strong decay of in light cone sum rules* *Hao Sun is supported by the National Natural Science Foundation of China (12075043)

In this study, we assign the tetraquark state for the resonance and investigate the mass and decay constant of in the framework of SVZ sum rules through a different calculation technique. Then, we calculate the strong coupling by considering soft-meson approximation techniques within the framework of light cone sum rules, and we use the strong coupling to obtain the width of the decay . Our prediction for the mass agrees with the experimental measurement, and that for the decay width of is within the upper limit.

Heavy–Light meson spectroscopy with strong coupling at N2LO level in V-scheme

The quark–antiquark potential is one of the basic ingredients of QCD-inspired potential models. This work will report the results of the masses and decay constants of heavy-flavor pseudo-scalar mesons within a QCD-based potential model having both inverse distance Coulomb and the linear confinement pieces. To that end, we use the inverse piece incorporating two-loop effects as suggested in V-scheme. Quantum mechanical perturbative methods: Dalgarno’s method of perturbation theory and variationally improved perturbation theory are used for the investigation. We use the Coulombic piece as the parent which is allowed by both Dalgarno’s perturbation theory and variationally improved perturbation theory. The results are compared with the latest updated theoretical predictions and PDG data. The sensitivity of the input parameters of the model has been discussed.

Recombination dynamics and pronounced re-absorption effect in ZnO single crystals under two-photon excitation

Time-resolved photoluminescence measurements were conducted on ZnO single crystals using two-photon (2P) excitation at low temperatures ranging from 25 to 260 K. The decay constants of various emission peaks are determined and compared between one-photon and two-photon excitations using a recently modified localized-state ensemble model. The analysis is focused on the redshift of the phonon-assisted free exciton transition energy with increasing temperature. A significantly longer radiative recombination lifetime of approximately 840 ps is observed under 2P excitation. The extended lifetime of excitons during 2P excitation is achieved through the interplay of multiple mechanisms. Photon-recycling, enabled by high absorption coefficients and total internal reflection, facilitates re-absorption and new carrier generation. Phonon scattering lowers photon energy, allowing their escape from the crystal, while exciton–polariton interactions delay photon travel, collectively contributing to the extension of exciton lifetimes. The re-absorption effect and elongated carrier lifetime observed from our work could be beneficial for applications of ZnO materials in 2P imaging, particularly of biological samples.

Size- and Voltage-Dependent Electron Transport of C2N-Rings-Based Molecular Chains.

C2N-ring-based molecular chains were designed at the molecular level and theoretically demonstrated to show distinctive and valuable electron transport properties that were superior to the parent carbonaceous system and other similar nanoribbon-based molecular chains. This new -type molecular chain presented an exponential attenuation of the conductance and electron transmission with the length. Essentially, the molecular chain retained the electron-resonant tunneling within 7 nm and the dominant transport orbital was the LUMO. Shorter molecular chains with stronger conductance anomalously possessed a larger tunnel barrier energy, attributing to the compensation of a much smaller HOMO-LUMO gap, and these two internal factors codetermined the transport capacity. Some influencing factors were also studied. In contrast to the common O impurity with a tiny effect on electron transmission of the C2N rings chain, the common H impurity clearly improved it. When the temperature was less than 400 K, the electron transmission varied with temperature within a narrow range, and the structural disorder deriving from proper heating did not greatly modify the transmission possibility and the exponentially decreasing tendency with the length. In a non-equilibrium condition, the current increased overall with the bias but the growth rate varied with size. A valuable negative differential resistance (NDR) effect appeared in longer molecular chains with an even number of big carbon-nitrogen rings and strengthened with size. The emergence of such an effect originated from the reduction in transmission peaks. The conductance of longer molecular chains was enhanced with the voltage but the two shortest ones presented completely different trends. Applying the bias was demonstrated to be an effective way for C2N-ring-based molecular chains to slow down the conductance decay constant and affect the transport regime. C2N-ring-based molecular chains show a perfect application in tunneling diodes and controllable molecular devices.

A generic formation mechanism of ultralight dark matter solar halos

As-yet undiscovered light bosons may constitute all or part of the dark matter (DM) of our Universe, and are expected to have (weak) self-interactions. We show that the quartic self-interactions generically induce the capture of dark matter from the surrounding halo by external gravitational potentials such as those of stars, including the Sun. This leads to the subsequent formation of dark matter bound states supported by such external potentials, resembling gravitational atoms (e.g. a solar halo around our own Sun). Their growth is governed by the ratio ξ foc ≡ λdB/R ⋆ between the de Broglie wavelength of the incoming DM waves, λdB, and the radius of the ground state R ⋆.For ξ foc ≲ 1, the gravitational atom grows to an (underdense) steady state that balances the capture of particles and the inverse (stripping) process. For ξ foc ≳ 1, a significant gravitational-focusing effect leads to exponential accumulation of mass from the galactic DM halo into the gravitational atom. For instance, a dark matter axion with mass of the order of 10-14 eV and decay constant between 107 and 108 GeV would form a dense halo around the Sun on a timescale comparable to the lifetime of the Solar System, leading to a local DM density at the position of the Earth 𝒪(104) times larger than that expected in the standard halo model. For attractive self-interactions, after its formation, the gravitational atom is destabilized at a large density, which leads to its collapse; this is likely to be accompanied by emission of relativistic bosons (a `Bosenova').

Impact of Temperature and Moisture on the Decomposition of Peat-Forming Plants: Results of a Two-Year Incubation Experiment

The decomposition rate of plant residues is determined by both abiotic (temperature, moisture) and biotic factors (biochemical composition). To separate the contribution of each factor to the decomposition process, long-term incubation experiments under controlled conditions are required. Two-year incubation experiments were conducted with various types of peat-forming plants (Sphagnum fuscum, Chamaedaphne calyculata, Eriophorum vaginatum, and a mixed sample consisting of 60% Sphagnum fuscum and 40% Chamaedaphne calyculata). The experiments were carried out at temperatures of 2, 12, and 22 °C, with varying moisture levels (W = 30, 60, and 90% of their water-holding capacity). In all plant samples, the highest rates of C(CO2) emission (DecR) were observed in the initial stages of decomposition. The cumulative carbon loss (Ccum) during the experiment ranged from 45 to 196 mgC/g of plant material at 22 °C and 23 to 156 mgC/g of plant material at 2 °C. The decay constant (k) for all plant samples increased with rising temperature. The results of the three-way ANOVA showed that the influence of the examined factors on the cumulative losses of C(CO2) decreased in the following order: the type of plant &gt; temperature &gt; moisture. Throughout the experiment, the influence of the type of plant and moisture on DecR increased, while the effect of temperature decreased. The highest temperature sensitivity (Q10 = 0.71–6.19) was observed in the low-temperature range (2–12 °C) during months 4 to 6 of incubation. These results are relevant for modeling and predicting the rate of transformation of peat organic matter under changing climatic conditions.

Entanglement Negativity in de Sitter Biverse from Stringy Axionic Bell Pair: An Analysis Using Bunch‐Davies Vacuum

AbstractIn this work, signatures of quantum entanglement by computing entanglement negativity between two causally unrelated regions in 3 + 1 dimensional global de Sitter space are studied. A bipartite quantum field theoretic setup for this purpose, driven by an axionic Bell pair resulting from Type IIB string compactification on a Calabi‐Yau three fold is investigated. A spherical surface that divides the spatial slice of the global de Sitter space into exterior and interior causally unrelated sub regions is taken into account. For the computational purpose, the simplest possible initial choice of quantum vacuum, which is Bunch‐Davies state is used. The quantitative quantum information theoretic measure for entanglement negativity turns out be consistent with the results obtained for entanglement entropy, even it is better than that from quantum information theoretic point of view. The problem in a hyperbolic open chart where one of the causally unrelated observers remains constrained and the scale dependence enters to the corresponding quantum information theoretic entanglement measure for axionic Bell pair is designed. From the analysis it is found that in the large scales, initially maximally entangled Bunch‐Davies state turns out to be strongly entangled or weakly entangled depending on the axionic decay constant and the supersymmetry breaking scale. It is also found that at the small scales the initial entanglement can be perfectly recovered. The possibility of having a biverse picture, which is a mini version of the multiverse in the present theoretical set up is discussed. Last but not the least, the necessary criteria for generating non vanishing quantum entanglement measures within the framework of quantum field theory of global de Sitter space as well as well as in primordial cosmology due to the axion derived from string theory are provided.

Measurement of Isfahan heavy water zero-power reactor kinetic parameters using advanced pulsed neutron source method in a near critical state

The pulsed neutron source (PNS) technique was used to determine the prompt neutron decay constant for two different lattice pitches in the HWZPR heavy water zero power reactor. The results were compared to the variance-to-mean ratio (VTM) method. The neutron mean generation time was also calculated for both pitches, and the results were compared to previous Monte Carlo calculations. The findings of this research can be used as a benchmark nuclear codes to validate kinetic parameters.