The Coulomb excitation cross sections for the first excited state of 15 even-mass nuclei in the region of the rare earths have been determined from measurements on inelastically scattered protons and deuterons. From the cross sections, reduced E2-transition probabilities are obtained, in general in good agreement with those derived from the directly measured lifetimes of the nuclear states. The intrinsic quadrupole moments determined from the transition probabilities show, for each element, a regular variation with the mass number, but discontinuities occur when passing from one element to another. This behaviour appears to be correlated with the variation in the moment of inertia for the same nuclei. The individual intrinsic quadrupole moments of odd-mass nuclei in the same region often deviate from the moments of the neighbouring even isotopes, but on the average the quadrupole moments of odd-mass nuclei are almost the same as those for even nuclei.
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